Evaluation of the distribution accuracy of radioactivity from a gamma-ray source using an omnidirectional detector for radiation imaging with fractal geometry

Sasaki, Miyuki; Abe, Yuki*; Sanada, Yukihisa; Torii, Tatsuo*

Nuclear Instruments and Methods in Physics Research A, 1072, p.170207_1 - 170207_12, 2025/03

https://doi.org/10.1016/j.nima.2025.170207

We have developed an omnidirectional radiation imager with fractal geometry named the FRIE system. This paper presents the development and evaluation of the FRIE system, designed to accurately estimate radioactivity distribution within decommissioning environments, such as the Fukushima Daiichi Nuclear Power Station. The FRIE system is a unit of tetrahedral radiation sensors; 16 sensors are arranged in a Sierpinski tetrahedron shape, and the space between the sensors is filled with tungsten-based alloy for radiation shielding. This study assessed the performance of the FRIE system in estimating radiation distribution through simulations and actual measurement tests. From the results of the simulations and experimental data, it was confirmed that by maintaining a measurement density of at least 2 points/m, limiting the positional error to within 10 cm, and the angular error to within 10 degrees, it is possible to estimate the source location with an angular resolution of approximately 30 degrees. Future improvements in the arrangement of the FRIE system's crystals and shielding should enhance the performance metrics. This research signifies a pioneering implementation of fractal-based radiation imaging technology, offering a new direction in radiation measurement.

Measurements of displacement cross sections of metals for 120-GeV proton beam irradiation

Iwamoto, Yosuke; Matsuda, Hiroki*; Meigo, Shinichiro; Yonehara, Katsuya*; Pellemoine, F.*; Liu, Z.*; Lynch, K.*; Yoshida, Makoto*; Yabuuchi, Atsushi*; Yoshiie, Toshimasa*; et al.

Nuclear Instruments and Methods in Physics Research B, 557, p.165543_1 - 165543_8, 2024/12

https://doi.org/10.1016/j.nimb.2024.165543

The number of displacements per atom is widely used as an indicator of irradiation damage to materials in proton accelerator facilities. Experiments have been carried out on protons below 3 GeV to verify the dpa of metallic materials. However, the dpa for high-energy protons above 3 GeV has not been measured. In order to validate the displacement cross sections of metals in the high-energy region, the electrical resistivity changes of aluminium, copper and tungsten wires at a temperature of 8 K were measured using protons with energy of 120 GeV. The results show that the conventional irradiation damage model of PHITS overestimates the experimental data. On the other hand, the calculation results using the athermal recombination correction model were in agreement with the experimental data.

Development of a forward Monte Carlo based weight-window generator using the history-counter function in PHITS

Sato, Tatsuhiko; Hashimoto, Shintaro; Mrquez Damin, J. I.*; Niita, Koji*

Nuclear Instruments and Methods in Physics Research B, 557, p.165535_1 - 165535_8, 2024/12

https://doi.org/10.1016/j.nimb.2024.165535

Characterization of mineral composition using PIXE and EXAFS analyses to elucidate the Barium adsorption mechanism

Oguri, Kaori; Hagura, Naoto*; Yamaguchi, Akiko; Okumura, Masahiko; Matsuura, Haruaki*; Tsunashima, Yasumichi; Aoki, Katsumi; Arai, Yoichi; Watanabe, So

Nuclear Instruments and Methods in Physics Research B, 556, p.165516_1 - 165516_8, 2024/11

https://doi.org/10.1016/j.nimb.2024.165516

Ningyo-toge is the uranium mine that has been operated in Japan. Various radioactive elements such as Uranium (U), and Radium (Ra) are still present in the mine ground water with very small amount, and behavior of those elements is not fully understood. In this study, we investigated the composition of metal oxides and clay minerals in a soil of slag deposit at the mine, and systematics of adsorption structure of various ions were examined. Identifying the composition and chemical forms of minerals present in the soil of slag can provide useful information for the safety assessment and evaluation of influence on the surrounding environment.

Ion beam induced luminescence of lanthanide complexes in organic solvents irradiated by hydrogen and argon ion beams

Nakahara, Masaumi; Watanabe, So; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yuri, Yosuke*; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Koka, Masashi*; Yamada, Naoto*; Hagura, Naoto*

Nuclear Instruments and Methods in Physics Research B, 554, p.165449_1 - 165449_5, 2024/09

https://doi.org/10.1016/j.nimb.2024.165449

Ion beam induced luminescence analysis of lanthanide complexes in the organic solvents for minor actinides recovery process was carried out to investigate the structures of complexes. In this study, hydrogen ion beam obtained from the single-ended accelerator and argon ion beam obtained from the azimuthally varying field cyclotron were used in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In the experiments, ion beam induced luminescence spectra of lanthanide complexes in the organic solvents were measured, and the relationship between the obtained spectra and the structures of complexes was studied.

Corrigendum to "Development of 0.5 mm gauge size radial collimators for high-pressure neutron diffraction experiments at PLANET in J-PARC" [Nucl. Instrum. Methods Phys. Res. A 1059 (2024) 168956]

Hattori, Takanori; Suzuki, Koji*; Miyo, Tatsuya*; Ito, Takayoshi*; Machida, Shinichi*

Nuclear Instruments and Methods in Physics Research A, 1064, p.169448_1 - 169448_9, 2024/07

https://doi.org/10.1016/j.nima.2024.169448

The authors regret that the abstract and summary explain that the cup diameter of a standard double-toroidal anvils is 1.5 mm. This is incorrect; the standard diameter is 4.0 mm. The authors would like to apologise for any inconvenience caused.

Measurement of the response of a Li-glass detector to gamma rays by a coincidence method

Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Mochimaru, Takanori*; Hori, Junichi*; Terada, Kazushi*; Koizumi, Mitsuo

Nuclear Instruments and Methods in Physics Research A, 1064, p.169465_1 - 169465_9, 2024/07

https://doi.org/10.1016/j.nima.2024.169465

Development of a practical tritiated water monitor to supervise the discharge of treated water from Fukushima Daiichi Nuclear Power Plant

Sanada, Yukihisa; Oshikiri, Keisuke*; Kanno, Marina*; Abe, Tomohisa

Nuclear Instruments and Methods in Physics Research A, 1062, p.169208_1 - 169208_7, 2024/05

https://doi.org/10.1016/j.nima.2024.169208

As part of the decommissioning work at the Fukushima Daiichi Nuclear Power Plant (FDNPP), the release of stored treated water began in 2023. In this study, we developed a practical tritium monitor to continuously monitor the concentration of tritiated water, as confirmed by batch sampling measurements at the FDNPP. The monitor is arranged with a flow cell detector comprising inexpensive plastic scintillator pellets and incorporating simultaneous measurements by three detectors, a veto detector, and lead shielding to reduce the influence of environmental -rays. The system reached a detection limit of 911 Bq L-1 with a measurement time of 30 min, which is lower than the discharge standard for tritiated water of 1,500 Bq L-1. The system can also qualitatively distinguish the presence of disturbances due to interfering radionuclides other than tritium or background radiation using the -ray spectrum.

Defect formation simulated by track structure calculation model

Ogawa, Tatsuhiko; Iwamoto, Yosuke

Nuclear Instruments and Methods in Physics Research B, 549, p.165255_1 - 165255_4, 2024/04

https://doi.org/10.1016/j.nimb.2024.165255

Atomic defect is one of the critical factors that determines the irradiation effects in materials. The atoms are recoiled by the impulse of incoming radiation, which changes the mechanical, electrical and chemical properties of the target materials. Methods to calculate atomic displacement based on nuclear reaction cross sections and Rutherford scattering cross sections were proposed but they were dedicated to calculation of the defect density in macroscopic scale whereas some phenomena are attributed to the topological arrangements of defects in microscopic scale. Application of a track-structure calculation model, ITSART implemented to a general-purpose radiation transport code PHITS for calculation of the topological arrangement of radiation-induced defects is proposed in this study. To verify the defect production calculated by ITSART, DPA (Displacement Per Atom) cross section in Cu was calculated and compared with literature data. The agreement indicates the accuracy of ITSART for calculating atomic displacement. By using the same methodology to a smaller volume, the defects in SiO exposed to 600 MeV proton beam was calculated. PHITS users can make use of the outputs by forwarding them to other tools, such as molecular dynamics codes, to analyse the further evolution of the defects.

Development of wide range photon detection system for muonic X-ray spectroscopy

Mizuno, Rurie*; Niikura, Megumi*; Saito, Takeshi*; Matsuzaki, Teiichiro*; Sakurai, Hiroyoshi*; Amato, A.*; Asari, Shunsuke*; Biswas, S.*; Chiu, I.-H.; Gianluca, J.*; et al.

Nuclear Instruments and Methods in Physics Research A, 1060, p.169029_1 - 169029_14, 2024/03

https://doi.org/10.1016/j.nima.2023.169029