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Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki
Progress in Nuclear Science and Technology (Internet), 7, p.195 - 198, 2025/05
Extraction chromatgraphy technology for trivalent minor actinide (MA(III) ; Am(III) and Cm(III)) recovery from the solution generated by an extraction process in reprocessing of spent nuclear fuel has been developed. A fine particle is generated in the solution. The fine particle must be removed before MA recovery operation, because that leads clogging of the extraction chlomatography column. In order to prevent clogging the column, filtration system utilizing porous silica beads packed column has been designed. In this study, a fine particle trapping system was developed and particle removal performance of the system was experimentally evaluated using alumina particles as simulated fine particle. Column experiments revealed that the fine particle with the particle size from 0.12 to 15 m is cause of clogging of the filtration column. Since simulated fine particles were trapped on filtration experiments, a filtration system using the porous silica beads column is practical,
Abe, Takumi; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*
Progress in Nuclear Science and Technology (Internet), 7, p.299 - 304, 2025/05
Currently, much research continues on stable energy sources that do not emit CO in order to achieve a carbon-neutral and sustainable society. Nuclear energy is one of the such sources, and various new reactors and reprocessing technologies are being developed. In order to implement the nuclear fuel cycle with these technologies, a nuclear fuel cycle simulator is required to quantitatively evaluate various quantities, such as the distribution of nuclear fuel materials and the scale of waste loading. For this purpose, NMB4.0 was developed in collaboration with Tokyo Institute of Technology and Japan Atomic Energy Agency. This code calculates the material balance of 179 nuclides including actinides and fission products (FPs) from the front-end to the back-end and simulates the nuclear fuel cycle in an integrated manner. Unlike other nuclear fuel cycle simulators, the code is capable of performing precise back-end analyses such as the number of radioactive wastes and the scale of the geological repository considering heat generation of waste package under diverse nuclear energy scenario, and is an open source code that runs on Microsoft Excel. By these features, it is possible to quantitatively study nuclear energy utilization strategies with various stakeholders. The presentation will detail the numerical model used in NMB4.0.
Nagatani, Taketeru; Kosuge, Yoshihiro*; Sagara, Hiroshi*; Nakaguki, Sho; Nomi, Takayoshi; Okumura, Keisuke
Progress in Nuclear Science and Technology (Internet), 7, p.41 - 46, 2025/05
Myagmarjav, O.; Tanaka, Nobuyuki; Noguchi, Hiroki; Kamiji, Yu; Ono, Masato; Nomura, Mikihiro*; Takegami, Hiroaki
Progress in Nuclear Science and Technology (Internet), 7, p.235 - 242, 2025/05
Sato, Hiroyuki; Yan, X.
Progress in Nuclear Science and Technology (Internet), 7, p.293 - 298, 2025/05
Arai, Yoichi; Watanabe, So; Nakahara, Masaumi; Funakoshi, Tomomasa; Hoshino, Takanori; Takahatake, Yoko; Sakamoto, Atsushi; Aihara, Haruka; Hasegawa, Kenta; Yoshida, Toshiki; et al.
Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/05
The Japan Atomic Energy Agency (JAEA) has been conducting a project named "Systematic Treatment of RAdioactive liquid waste for Decommissioning (STRAD)" project since 2018 for fundamental and practical studies for treating radioactive liquid wastes with complicated compositions. Fundamental studies have been conducted using genuine liquid wastes accumulated in a hot laboratory of the JAEA called the Chemical Processing Facility (CPF), and treatment procedures for all liquid wastes in CPF were successfully designed on the results obtained. As the next phase of the project, new fundamental and practical studies on primarily organic liquid wastes accumulated in different facilities of JAEA are in progress. This paper reviews the representative achievements of the STRAD project and introduces an overview of ongoing studies.
Hamdani, A.; Soma, Shu; Abe, Satoshi; Shibamoto, Yasuteru
Progress in Nuclear Science and Technology (Internet), 7, p.53 - 59, 2025/03
Oizumi, Akito; Sagara, Hiroshi*
Progress in Nuclear Science and Technology (Internet), 7, p.331 - 337, 2025/03
Research and development of transuranium (TRU) fuel cycle with accelerator-drive systems (ADSs) transmuting minor actinides separated from the commercial cycles has been continuously conducted to reduce the high-level radioactive waste contained in spent fuel discharged from nuclear power plants. Since the chemical form and composition of the ADS fuels are different from those of the current commercial cycles, it is necessary to examine the inspection goal of the safeguards which are required for the ADS cycle. In this study, the of Pu was evaluated assuming the diversion of any items in the ADS cycle in terms of nuclear non-proliferation. They were compared with the
of the MOX fuel assemblies (fresh and spent fuels) for a conventional boiling water reactor (BWR). The all items in the ADS cycle, regardless of whether they are fresh or spent fuel, were found to have the same
of Pu as the spent fuel assembly of BWR-MOX. Additionally, in order to design and evaluate accounting systems for safeguards, the assumed uncertainty (
) values of measurements by operators and verification by regulators for the Pu flow rate in the ADS cycle were derived with reference to the accuracy targets for Pu measurement technology. The derived
values were compared with the 1 significant quantity (1SQ), which was generally used as a target value, and the spent fuel standard (equivalent to 5%) set based on the
evaluation, respectively. As a result, it was clarified that the both
values of Pu measurements by the operator and the regulator exceeded 1SQ but the spent fuel standard was generally achievable.
Tsujimura, Norio; Takahashi, Fumiaki; Takada, Chie
Progress in Nuclear Science and Technology (Internet), 6, p.148 - 151, 2019/01
Shimada, Taro; Miwa, Kazuji; Takeda, Seiji
Progress in Nuclear Science and Technology (Internet), 6, p.203 - 207, 2019/01
Rubbles less than 5 Sv/h of surface dose rate, which are stored outdoor in the Fukushima Daiichi NPS (1F) site, will be recycled and applied in a restricted reuse only within 1F site in the future. In this study, we suggested a concept for establishing the reference radioactive concentration of recycling material for the restricted use in the 1F site. Reference radiocesium concentration is calculated so that increased dose rate by restricted reuse does not exceed 1
Sv/h which is the minimum value of dose rate map in the 1F entire site. In order to justify the restricted reuse under the reference concentration calculated, additional occupational dose, dose rate at the site boundary and groundwater concentration at the outlet to the ocean are evaluated and confirmed that the values are below 2 mSv/y, 1 mSv/y and 1 Bq/cm
of
Cs and
Cs, respectively. And then calculated the reference radiocesium concentrations of the recycling material used for paved roads and the bases of concrete building.
Miwa, Kazuji; Shimada, Taro; Takeda, Seiji
Progress in Nuclear Science and Technology (Internet), 6, p.166 - 170, 2019/01
In this study, in order to validate the restricted use of recycling material at the reference radiocesium concentration (determined in series report (1)), we evaluated worker annual doses, air dose rate at the site boundary and impact of migrated radiocesium into groundwater. Firstly, we evaluated the additional annual dose for workers, on the assumption that typical workers coming in contact with the source after construction (Road: 1.2 mSv/y, Building: 1.3 mSv/y). Secondly, we evaluated the air dose rates by distance from road and building including recycling material, and investigated the distance for not exceeding 1 mSv/y (including additional dose rate by recycling and background dose rate of 0.6 mSv/y) at the site boundary (Road: 25 m, Building: 1 m). Thirdly, we evaluated the Cs migration in groundwater, and investigated the distance required for satisfying the operation target value (Cs: 1 Bq/L,
Cs: 1 Bq/L) at the boundary (coastal line) (Road: 10 m, Building: 10 m).
Kamada, So*; Kato, Michio*; Nishimura, Kazuya*; Nancekievill, M.*; Watson, S.*; Lennox, B.*; Jones, A.*; Joyce, M. J.*; Okumura, Keisuke; Katakura, Junichi*
Progress in Nuclear Science and Technology (Internet), 6, p.199 - 202, 2019/01
As a technology development to investigate the distribution of submerged fuel debris in the primary containment vessel (PCV) of the Fukushima Daiichi Nuclear Power Station, we are conducting development experiments of sonar system to be mounted in a compact ROV. The experiments were conducted in two types of water tanks with different depths, simulating the PCV, using sonar with different sizes, ultrasonic frequencies, and beam scanning method, and simulated fuel debris. As a result, we characterized the shape discrimination performance of the simulated debris, and the noise due to multi-path in narrow closed space.
Kowatari, Munehiko; Tanimura, Yoshihiko; Kessler, P.*; Neumaier, S.*; Roettger, A.*
Progress in Nuclear Science and Technology (Internet), 6, p.81 - 85, 2019/01
Kowatari, Munehiko; Yoshitomi, Hiroshi; Oishi, Tetsuya; Yoshizawa, Michio
Progress in Nuclear Science and Technology (Internet), 6, p.86 - 90, 2019/01
Okumura, Keisuke; Riyana, E. S.; Sato, Wakaei*; Maeda, Hirobumi*; Katakura, Junichi*; Kamada, So*; Joyce, M. J.*; Lennox, B.*
Progress in Nuclear Science and Technology (Internet), 6, p.108 - 112, 2019/01
In order to establish the prediction method of the dose rate distribution in the primary containment vessel (PCV) of the Fukushima Daiichi Nuclear Power Station, a series of calculations were carried out in the following way; (1) burnup calculation to obtain fuel composition at the time of accident, (2) activation calculation for the structural materials including impurities, (3) estimation of Cs contamination in PCV based on the result of severe accident analysis by IRID, (4) decay calculation of radioactive nuclides, (5) photon transport calculation to obtain dose rate distribution. After that, Cs concentration around the dry-well of 1F was modified to be consistent with locally measured dose rates in the PCV-investigation by IRID.
Kim, B.-J.*; Sasaki, Miyuki; Sanada, Yukihisa
Progress in Nuclear Science and Technology (Internet), 6, p.130 - 133, 2019/01
Sasaki, Miyuki; Ishizaki, Azusa; Sanada, Yukihisa
Progress in Nuclear Science and Technology (Internet), 6, p.63 - 67, 2019/01
Since the accident at Fukushima Daiichi Nuclear Power Station (FDNPS), some unmanned vehicles (UAVs) are applied to airborne radiation measurement in around FDNPS. In conventional analysis methods, count rate that is obtained in the sky is converted to air dose rate at 1 m above the ground (agl.) under following premises. (1) Topography under the UAV is a plane (plane source model). (2) The air dose rate at 1 m agl. under the UAV is constant inside approximately 10 m radius. (3) Relationship of altitude and count rate is exponential correlation. Therefore, it is difficult that dose rate by airborne radiation measurement is precisely measured at the mountains and uneven place of dose rate by the conventional method. In this study, Maximum Likelihood-Expectation Maximization (ML-EM) method which is used in the medical radiation such as Positron Emission Tomography (PET) is attempted to apply to environmental radiation measurement using UAV.
Matsuda, Norihiro; Kunieda, Satoshi; Okamoto, Tsutomu*; Tada, Kenichi; Konno, Chikara
Progress in Nuclear Science and Technology (Internet), 6, p.225 - 229, 2019/01
Ochi, Kotaro; Sasaki, Miyuki; Ishida, Mutsushi*; Sanada, Yukihisa
Progress in Nuclear Science and Technology (Internet), 6, p.103 - 107, 2019/01
After the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, a large amount of radionuclides was spread out all over the world. In our previous study, we developed the aerial radiation monitoring technique using unmanned helicopter for investigating the dose rate derived deposited radionuclides over wide area. In addition, many monitoring techniques were developed for investigating the local distribution of radionuclides using unmanned aerial vehicle, handheld instrument and car within small area. Distinction of these methods depends on desirable position resolution of dose rate. However, the comparison method of the measurement result between different methods is not established. In this study, we attempted to evaluate the some methods of airborne and ground radiation measurement in same extended farm.
Matsuda, Hiroki; Meigo, Shinichiro; Iwamoto, Hiroki
Progress in Nuclear Science and Technology (Internet), 6, p.171 - 174, 2019/01
Activation cross sections of various materials are strongly required for the improvement of the accuracy of nuclear design and the reduction of the construction costs for spallation neutron sources and transmutation systems. Activation cross sections have been measured in several facilities. However, they have low accuracy and precision. Especially, there are merely experimental data with 3 GeV protons which are used for spallation neutron source (MLF) in J-PARC, the experimental data is required for the improvement of the target materials. Thus, we measured cross sections of tungsten, gold, indium, and beryllium with 0.4 GeV to 3.0 GeV protons. Moreover, ones of aluminium that are set with materials were also measured for a variation of this experiment. It was found that more accurate data than current ones would be measured by using precise beam controls and highly accurate beam monitoring. We compared the experimental data, the evaluated data (JENDL-HE/2007), and the calculations with several intra-nuclear cascade models by PHITS code. Although the experimental data agreed with JENDL-HE/2007, the calculations underestimated about 40%. This could come from the evaporation model (GEM) being included in PHITS code. We found that the calculations agreed with the experimental data by upgrading PHITS code. The cross sections for the other materials have been analysed so far.