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Journal Articles

Evaluation of materials for developing a new individual dosemeter using electron spin resonance spectroscopy

Kitamura, Yoshimasa; Oka, Toshitaka; Seito, Hajime*; Yokozuka, Eri*; Nagasawa, Naotsugu*; Kitatsuji, Yoshihiro

Radiation Protection Dosimetry, 200(16-18), p.1660 - 1665, 2024/11

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

In this work, we evaluated the applicability of hydroxyapatite, which is a main component of tooth enamel, as individual dosimeters that can detect from less than 1 Gy to several tens Gy. Commercially available hydroxyapatite was irradiated by $$^{60}$$Co gamma-ray up to 75 Gy and ESR spectrum of the irradiated sample was observed. The relationship between the intensity of produced carbonated radical and the absorbed dose shows a good linearity ($$mathrm{R}^{2}=1$$) from 0 to 75 Gy. The detection limit of this samples was estimated to be 99.7 mGy, and the radical intensity do not change for eight month from the irradiation. These results suggest that this sample can be used as a candidate of the individual dosimeter.

Journal Articles

Attempt to re-estimate organ doses of victims in non-homogeneous exposure accident by means of the state-of-the-art Mesh-type Reference Computational Phantom; A Case study of an IR-192 source accident

Kowatari, Munehiko*; Yoshitomi, Hiroshi; Tani, Kotaro*; Tanimura, Yoshihiko; Kurihara, Osamu*

Radiation Protection Dosimetry, 200(16-18), p.1574 - 1579, 2024/11

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Comparison of codes for calculation of projocted radiation-induced cancer risks

Kujiraoka, Ikuo; Noguchi, Yoshihiro*; Shimada, Kazumasa; Hirouchi, Jun; Takahara, Shogo

Radiation Protection Dosimetry, 200(16-18), p.1561 - 1567, 2024/11

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Lifetime Attributable Risk (LAR) of cancer induced by radiation exposures is one of the important factors for deciding about radiological protection measures or protective actions for nuclear emergency preparedness and response. In Japan, while a model for estimating LAR for the Japanese population has been developed based on epidemiological data from A-bomb survivors, a flexible projection code implementing this model needs to be developed. This study investigated the existing codes to contribute to the development of the projection code. Based on these investigations, we compared their LAR calculation results, and explored the cause of their differences.

Journal Articles

ESR measurement of carbonated hydroxyapatite for dosemeter

Seito, Hajime*; Yokozuka, Eri*; Oka, Toshitaka; Kitatsuji, Yoshihiro; Nagasawa, Naotsugu*

Radiation Protection Dosimetry, 200(16-18), p.1656 - 1659, 2024/11

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

We have examined dosimetric characteristics of bio-inspired carbonated hydroxyapatite (CO$$_{3}$$HAp), which is a main component of calcified tissues like tooth enamel. CO$$_{3}$$HAp powder samples were exposed to gamma-ray with radiation doses ranging from 1 Gy to 1000 Gy at room temperature, and ESR spectra were measured immediately after irradiation and subsequently measured each 1 day during 90 days. The post-irradiation fading resulted in significant 20% decay of the signal amplitude, which stabilised within 7 days after irradiation, and the intensity approached a constant. The sample has good linear dose response in the experiment range of 10 Gy - 1000 Gy. Our results indicate that the CO$$_{3}$$HAp materials is suitable for chemical dosimetry.

Journal Articles

Development of $$alpha$$-ray visualization survey meter in high gamma and neutron background environment

Tsubota, Yoichi; Kobayashi, Kenji; Ishii, Tatsuya; Hirato, Misaki; Shioya, Satoshi; Nakagawa, Takahiro

Radiation Protection Dosimetry, 200(16-18), p.1676 - 1680, 2024/11

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

In the decommissioning of the Fukushima Daiichi Nuclear Power Station (FDNPS, 1F), workers are removing structures from inside the buildings, monitoring radioactive contamination, and decontaminating inside the buildings. For the measurement of contamination of suit surfaces of workers, we have developed a hand-held survey meter that can measure and visualize surface radioactive contamination of $$alpha$$-nuclides in a high $$beta$$/ $$gamma$$-ray background environment. In order to selectively measure $$alpha$$-nuclides, we designed and built a prototype hand-held survey meter for $$alpha$$-rays, which consists of a thin-film ZnS:Ag scintillator, a multi-anode photomultiplier tube (MA-PMT), individual amplification and counting circuits for each channel of the MA-PMT. Based on the result of $$alpha$$-ray counting, the developed device is capable of counting the $$alpha$$-radiation beyond 2.1$$times$$10$$^{7}$$ cpm. In the $$gamma$$-ray response test, there was no $$gamma$$-ray response even when the detector was in close proximity to a high intensity source; The dose rate was estimated to be more than 1 Sv/h. In the future, we plan to reduce the weight and size of the device, as well as improve the usability of the device through actual testing in contaminated environments.

Journal Articles

Establishment of a $$^{241}$$Am gamma calibration field based on international standards and its conversion coefficients

Tsuji, Tomoya; Yoshitomi, Hiroshi; Kowatari, Munehiko*; Tanimura, Yoshihiko

Radiation Protection Dosimetry, 200(15), p.1416 - 1424, 2024/09

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Analysis of the relationship between ambient dose, ambient dose equivalent and effective dose in operational neutron spectra

Endo, Akira

Radiation Protection Dosimetry, 200(13), p.1266 - 1273, 2024/08

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

This study examines the relationship between ambient dose $$H^*$$, ambient dose equivalent $$H^*(10)$$, and effective dose for external neutron irradiation over 163 operational spectra from different workplaces. The results show that $$H^*$$ provides a reasonable estimate with a controlled margin, even if overestimated, to assess effective dose compared with $$H^*(10)$$, which can lead to a significant overestimation or underestimation of effective dose depending on the neutron spectra. The results highlight the limitations of $$H^*(10)$$ and the superiority of $$H^*$$ in estimating effective dose according to the requirements of the operational quantity, especially in environments with high-energy neutrons.

Journal Articles

Development of DynamicMC for PHITS Monte Carlo package

Watabe, Hiroshi*; Sato, Tatsuhiko; Yu, K. N.*; Zivkovic, M.*; Krstic, D.*; Nikezic, D.*; Kim, K. M.*; Yamaya, Taiga*; Kawachi, Naoki*; Tanaka, Hiroki*; et al.

Radiation Protection Dosimetry, 200(2), p.130 - 142, 2024/02

 Times Cited Count:2 Percentile:27.70(Environmental Sciences)

Previously, we have developed DynamicMC for modelling relative movement of ORNL phantom in a radiation field for MCNP. Using this software, 3-dimensional dose distributions in a phantom irradiated by a certain mono-energetic source can be deduced through its graphical user interface (GUI). In this study, we extended DynamicMC to be used in combination with the PHITS by providing it with a higher flexibility for dynamic movement for a less sophisticated anthropomorphic phantom. We anticipate that the present work and the developed open-source tools will be in the interest of nuclear radiation physics community for research and teaching purposes.

Journal Articles

Characterization of small radiophotoluminescence dosemeter in terms of $$H_{P}$$(0.07) for extremity dose monitoring of medical personnel

Kowatari, Munehiko*; Yoshitomi, Hiroshi; Nagamoto, Keisuke*; Nakagami, Koichi*; Moritake, Takashi*; Kunugita, Naoki*

Radiation Protection Dosimetry, 199(15-16), p.1807 - 1812, 2023/10

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Interlaboratory comparison of electron paramagnetic resonance tooth enamel dosimetry with investigations of the dose responses of the standard samples

Toyoda, Shin*; Inoue, Kazuhiko*; Yamaguchi, Ichiro*; Hoshi, Masaharu*; Hirota, Seiko*; Oka, Toshitaka; Shimazaki, Tatsuya*; Mizuno, Hideyuki*; Tani, Atsushi*; Yasuda, Hiroshi*; et al.

Radiation Protection Dosimetry, 199(14), p.1557 - 1564, 2023/09

 Times Cited Count:1 Percentile:27.70(Environmental Sciences)

Interlaboratory comparison studies are important for radiation dosimetry in order to demonstrate how the technique is universally available. The set of standard samples are examined in each participating laboratory in the present study. After a set of standard samples together with the samples with unknown doses, which were prepared in the same laboratory as the standard samples, are measured at a participating laboratory, those samples are sent to another participating laboratory for next measurement. There is some small difference observed in the sensitivity (the slope of the dose response line) of the standard samples while the differences in the obtained doses for the samples with unknown doses are rather systematic, implying that the difference is mostly due to the samples but not to measurements.

Journal Articles

Estimation of external dose for wild Japanese macaques captured in Fukushima prefecture; Decomposition of electron spin resonance spectrum

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.

Radiation Protection Dosimetry, 199(14), p.1620 - 1625, 2023/09

 Times Cited Count:1 Percentile:27.70(Environmental Sciences)

We have been conducting dose assessments for Japanese macaques captured in Fukushima to reveal radiobiological effects on the low-dose expose animals. To accurately determine the external exposure dose, it is desirable to examine the analysis of the CO$$_{2}^{-}$$ radical intensity. We examined ESR spectra of teeth of 10 macaques captured in Fukushima by two spectrum-decomposition algorithms.

Journal Articles

Development of a method of evaluating PuO$$_{2}$$ particle diameters using an alpha-particle imaging detector

Morishita, Yuki; Sagawa, Naoki; Takada, Chie; Momose, Takumaro; Takasaki, Koji

Radiation Protection Dosimetry, 199(13), p.1376 - 1383, 2023/08

 Times Cited Count:2 Percentile:49.11(Environmental Sciences)

It is very important to evaluate the diameters (activity median aerodynamic diameter) of Plutonium dioxide (PuO$$_{2}$$) particles for internal exposure dose evaluation. In this study, a method of evaluating PuO$$_{2}$$ particle diameters using an alpha-particle imaging detector was developed. PuO$$_{2}$$ particles with different diameters were modeled by Monte Carlo simulation, and the change in the shape of the energy spectrum for each particle diameter was evaluated. Two different patterns were modeled, namely, the case of $$^{239}$$PuO$$_{2}$$ and the case of PuO$$_{2}$$ (including isotopic composition of Pu). Multiple regression analysis was performed to determine the PuO$$_{2}$$ particle diameter from the obtained parameters. The simulated diameters and the diameters obtained with the regression model were in good agreement. The advantage of using the alpha-particle imaging detector is to measure the alpha energy spectrum for individual particle, and this allows accurate measurement of particle diameter distribution.

Journal Articles

Estimation of inhomogeneous occupational exposure to the lens of the eyes and the extremities of radiation workers in a research accelerator facility

Kowatari, Munehiko*; Kubota, Takumi*; Yoshitomi, Hiroshi; Kunugita, Naoki*

Radiation Protection Dosimetry, 199(11), p.1239 - 1247, 2023/07

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Visualization software for radioactive contamination based on Compton camera: COMRIS

Sato, Yuki; Minemoto, Kojiro*; Nemoto, Makoto*

Radiation Protection Dosimetry, 199(8-9), p.1021 - 1028, 2023/06

 Times Cited Count:3 Percentile:65.16(Environmental Sciences)

Journal Articles

Dose measurement precision of an RPLD-based eye lens dosemeter applicable to the medical sector

Kowatari, Munehiko*; Nagamoto, Keisuke*; Nakagami, Koichi*; Yoshitomi, Hiroshi; Moritake, Takashi*; Kunugita, Naoki*

Radiation Protection Dosimetry, 198(17), p.1303 - 1312, 2022/10

 Times Cited Count:2 Percentile:30.61(Environmental Sciences)

Journal Articles

Crystal configuration dependence of CsI(Tl) scintillation detectors on environmental dose rate measurement

Tsuda, Shuichi; Saito, Kimiaki

Radiation Protection Dosimetry, 198(17), p.1283 - 1291, 2022/10

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Spherical or cylindrical detectors superior to directional characteristic are commonly used to monitor dose rates in the environment to detect scattering gamma-rays emitted from radionuclides in soil or air. The authors have performed environmental dose rates measurements using various kinds of detectors to investigate the directional characteristics, and experimentally verified the variations in dose rates due to directional characteristics unique to each detector. Furthermore, a dose rate measured by a CsI(Tl) scintillation detector with cuboidal crystal agreed with that by a CsI(Tl) scintillation detector with cylindrical crystal. Simulations by PHITS under various CsI(Tl) crystal configurations revealed that there are certain aspect ratios of cuboidal CsI(Tl) crystal with less directional dependence. Since cubes are advantageous in terms of production cost, this result indicates the potential of CsI(Tl) scintillation detectors with cuboidal crystal for use in the environmental dose rate monitoring.

Journal Articles

Cesium-rich microparticles runoff during rainfall; A Case study in the Takase River

Tatsuno, Takahiro*; Waki, Hiromichi*; Kakuma, Minato*; Nihei, Naoto*; Wada, Toshihiro*; Yoshimura, Kazuya; Nakanishi, Takahiro; Ote, Nobuhito*

Radiation Protection Dosimetry, 198(13-15), p.1052 - 1057, 2022/09

 Times Cited Count:2 Percentile:30.61(Environmental Sciences)

Journal Articles

Performance evaluation of commercial scintillation cocktails for low-level tritium counting by high-capacity liquid scintillation counter

Kuwata, Haruka*; Tazoe, Hirofumi*; Kranrod, C.*; Fujiwara, Kenso; Terashima, Motoki; Matsueda, Makoto; Hirao, Shigekazu*; Akata, Naofumi*

Radiation Protection Dosimetry, 198(13-15), p.1014 - 1018, 2022/09

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Development of emergency monitoring system for alpha-particle-emitting radionuclides in the air

Hokama, Tomonori; Fujita, Hiroki; Nakano, Masanao; Iimoto, Takeshi*

Radiation Protection Dosimetry, 196(3-4), p.136 - 140, 2021/11

 Times Cited Count:2 Percentile:10.40(Environmental Sciences)

During the early phase of a nuclear accident, major radioactive materials are released into the environment, necessitating the prompt deployment of various protective actions to avoid or reduce radiation exposure. To implement these actions, the levels of radioactivity in the environment should be determined. However, the radioactivity concentrations of artificial alpha-particle-emitting radionuclides such as plutonium are difficult to measure in airborne samples, because they are interfered with natural radionuclides such as uranium decay products. Therefore, chemical separation is required to measure the concentrations. This study presents a new emergency monitoring system for airborne samples, which performs multiple-pulse time-interval analysis (MTA) without chemical separation. The system is used in conjunction with an alpha/beta-particle survey meter and adopted an analysis method focusing on the detected time interval of each particle. Its features are that a short time to output measurement result, easy handling and nondestructive. The estimated detection limit of the system was 9.5$$times$$10$$^{-2}$$ Bq m$$^{-3}$$. The MTA-based monitoring system could be useful in situations requiring prompt measurement and screening of samples.

Journal Articles

Analyses of $$H$$*(10) dose rates measured in environment contaminated by radioactive caesium; Correction of directional dependence of scintillation detectors

Tsuda, Shuichi; Tanigaki, Minoru*; Yoshida, Tadayoshi; Okumura, Ryo*; Saito, Kimiaki

Radiation Protection Dosimetry, 193(3-4), p.228 - 236, 2021/03

AA2020-0760.pdf:0.87MB

 Times Cited Count:6 Percentile:41.66(Environmental Sciences)

Environmental dose rate monitoring has been performed with various scintillation detectors since the Fukushima Dai-ichi Nuclear Power Plant accident. Gamma-rays from caesium isotopes deposited in soil enter radiation detectors in any direction, but directional dependence of the detectors used for dose rate measurements are not always uniform and the dose rates vary even if measurement takes place at the same place. To investigate the influence of crystal configurations on dose rate, dose rate measurements using several scintillation detectors with different crystal configurations were conducted. By measuring pulse height spectra and multiplying them with spectrum - dose conversion operators (G(E) function), dose rates were deduced and compared. It was found that the dose rates varied within approximately 25% among six detectors. To reduce the differences, the dose rate using G(E) functions determined in rotational geometry were obtained and applied instead. The revised dose rates agreed with one another within uncertainties, but this was not the case of scintillation detector with flat crystal shape, and it means this method could not compensate its strong directional dependence. These experimental results reveal that detectors with superior directional characteristics should be used for environmental dose rate measurement since the compensation of directional dependence using a G(E) function determined in rotational geometry is not always available.

177 (Records 1-20 displayed on this page)