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Yildirim, A. C.*; Mei, H.*; Toda, Kanako*; Aoyagi, Noboru; Saito, Takumi*
Applied Clay Science, 274, p.107853_1 - 107853_9, 2025/09
Times Cited Count：0Soma, Yasutaka; Komatsu, Atsushi; Kaji, Yoshiyuki; Yamamoto, Masahiro*; Igarashi, Takahiro
Corrosion Science, 251, p.112897_1 - 112897_15, 2025/07
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)Experimental and modeling studies of the oxygen ingression at the crevices of stainless steels were conducted in high-temperature water (288
C). The limiting distance of oxygen ingression, 
, was defined as the point beyond which the primary surface oxide changed (hematite 
magnetite), regardless of crevice gap, oxygen concentration, and time. In situ measurements revealed increased electrical conductivity around the position indicating ion enrichment due to a differential oxygen concentration cell. increased with increasing crevice gap, oxygen concentration, and immersion time. Modeling study suggested that oxide layer growth reduced anodic dissolution and slowed oxygen consumption, allowing oxygen ingression with time.
Gu, G. H.*; Jeong, S. G.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Cho, J.*; Kim, H. S.*; 4 of others*
Journal of Materials Science & Technology, 223, p.308 - 324, 2025/07
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)Kondo, Ryoichi; Yamamoto, Akio*; Endo, Tomohiro*
EPJ Nuclear Sciences & Technologies (Internet), 11, p.21_1 - 21_9, 2025/06
The flux distribution tallies using the proper orthogonal decomposition (POD) called "the POD tallies" have been developed in our previous study. The POD tallies can achieve dimensionality and statistical uncertainty reduction for a finely discretized flux distribution. Some characteristics of the POD tallies, which are left by our previous work, are revealed in the present study. Firstly, the POD tallies with the track length estimator are newly implemented. Since the statistical uncertainty of the POD tallies is reduced compared with the cell tallies, the POD tallies with the track length estimator can obtain the most precise result among the present implantations. Secondly, the basis vectors obtained by the deterministic and the stochastic methods are compared. The statistical uncertainty of the snapshot data invokes the degradation of the extracted basis vectors. This result indicates that the deterministic method might be more efficient for the snapshot calculation. Finally, the impact of the covariances of expansion coefficients on the statistical uncertainty of expanded flux distribution is investigated. The reconstructed statistical uncertainty considering only the variances of the expansion coefficients differs from the reference. This result reveals that the covariances of the expansion coefficients are important to estimate the statistical uncertainty of the local flux in the flux distribution.
Uesawa, Shinichiro; Yamashita, Susumu; Sano, Yoshihiko*; Yoshida, Hiroyuki
Journal of Nuclear Science and Technology, 62(6), p.523 - 541, 2025/06
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Japan Atomic Energy Agency (JAEA) has developed a numerical method with the JUPITER code with a porous medium model to calculate the thermal behavior in PCVs of 1F. In this study, we performed an experiment and numerical simulation of the natural convective heat transfer with the porous medium to validate JUPITER with the porous medium model. In comparison of the temperature and velocity distributions between the experiment and simulation, the temperature distribution in the simulation was in good agreement with the distribution in the experiment except the temperature near the top surface of the porous medium. The velocity distribution also agreed qualitatively with the experimental result. In addition, we also performed the numerical simulations with various effective thermal conductivity models to discuss the effect of the conductivity based on the internal structure of porous media on the natural convective heat transfer. The result indicated that the temperature distribution in the porous medium and the velocity distribution of the natural convection were significantly different for each model, and thus the conductivity of the fuel debris was one of the key parameters of in the thermal behavior analysis in 1F.
Wilson, J.*; Sasamoto, Hiroshi; Tachi, Yukio; Kawama, Daisuke*
Applied Clay Science, 275, p.107862_1 - 107862_15, 2025/05
Times Cited Count：0High-Level Radioactive Waste (HLW) repositories include iron or steel-based containers/overpack and bentonite buffers. Over the last 25 years or so, research efforts have attempted to elucidate the nature of iron-bentonite interactions, especially the potential for the deleterious alteration of the swelling clay component (smectite), to iron-rich layer silicates, some of which lack the capacity for intracrystalline swelling. This could result in a reduction or loss in swelling pressure in the bentonite buffer which is designed to protect waste containers from shear forces and also acts to restrict water and solute transport, as part of an engineered barrier system. Most data on iron-bentonite interactions come from experimental and geochemical modelling studies, as natural analogue data are lacking. The data suggests that there is the potential for the development of an iron-rich bentonite alteration zone with smectite (generally present as the aluminous montmorillonite type) undergoing alteration to iron-rich solids, including layer silicates and steel corrosion products such as green rust or magnetite. The evidence available is complex, arguably incomplete, with many potential complex couplings. Many uncertainties remain despite efforts taken over the last 25 years, but plausible scenarios for iron-bentonite interactions have been identified and possible implications for buffer properties have been suggested.
Fablet, L.*; P
drot, M.*; Choueikani, F.*; Kieffer, I.*; Proux, O.*; Pierson-Wickmann, A.-C.*; Cagniart, V.*; Yomogida, Takumi; Marsac, R.*
Environmental Science; Nano, 12(5), p.2815 - 2827, 2025/05
Times Cited Count：0 Percentile：0.00(Chemistry, Multidisciplinary)Nickel is an omnipresent trace element in the environment. Due to its high affinity for iron oxide nanoparticles, its elimination from soils and water by these nanoparticles represents an interesting strategy, specially by magnetites, which is naturally present in the environment. However, the interactions between Ni and magnetite are poorly understood, because of the difficulty to control the stoichiometry (Fe(II)-to-Fe(III) ratio) of magnetite. The behavior of Ni in the presence of magnetite nanoparticles with different stoichiometries, in aqueous solution and inert atmosphere, are probed by adsorption experiments and X-ray Absorption Spectroscopy. This study helps predicting the interactions between Ni and magnetite in environmental conditions, which can be used for the development of efficient remediation strategies.
Uesawa, Shinichiro; Ono, Ayako; Nagatake, Taku; Yamashita, Susumu; Yoshida, Hiroyuki
Journal of Nuclear Science and Technology, 62(5), p.432 - 456, 2025/05
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)We performed electrostatic simulations of a wire-mesh sensor (WMS) for a single spherical bubble and bubbly flow to clarify the accuracy of the WMS. The electrostatic simulation for the single bubble showed the electric current density distribution and the electric current path from the excited transmitter to receivers for various bubble locations. It indicated systematic errors based on the nonuniform current density distribution around the WMS. The electrostatic simulation for the bubbly flow calculated by the computational fluid dynamics code, JAEA Utility Program for Interdisciplinary Thermal-hydraulics Engineering and Research (JUPITER), indicated that the WMS had difficulty in quantitatively measuring the intermediate values of the instantaneous void fraction between 0 and 1 because they cannot be estimated by previous transformation methods from the WMS signal to the void fraction, such as linear approximation or Maxwell's equation, and have a significant deviation of the void fraction of 
0.2 for the WMS signal. However, the electrostatic simulation indicated that the time-averaged void fractions around the center of the flow channel can be estimated using linear approximation, and the time-averaged void fraction near the wall of the flow channel can be estimated using Maxwell's equation.
Abe, Takumi; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*
Progress in Nuclear Science and Technology (Internet), 7, p.299 - 304, 2025/05
Currently, much research continues on stable energy sources that do not emit CO
in order to achieve a carbon-neutral and sustainable society. Nuclear energy is one of the such sources, and various new reactors and reprocessing technologies are being developed. In order to implement the nuclear fuel cycle with these technologies, a nuclear fuel cycle simulator is required to quantitatively evaluate various quantities, such as the distribution of nuclear fuel materials and the scale of waste loading. For this purpose, NMB4.0 was developed in collaboration with Tokyo Institute of Technology and Japan Atomic Energy Agency. This code calculates the material balance of 179 nuclides including actinides and fission products (FPs) from the front-end to the back-end and simulates the nuclear fuel cycle in an integrated manner. Unlike other nuclear fuel cycle simulators, the code is capable of performing precise back-end analyses such as the number of radioactive wastes and the scale of the geological repository considering heat generation of waste package under diverse nuclear energy scenario, and is an open source code that runs on Microsoft Excel. By these features, it is possible to quantitatively study nuclear energy utilization strategies with various stakeholders. The presentation will detail the numerical model used in NMB4.0.
Myagmarjav, O.; Tanaka, Nobuyuki; Noguchi, Hiroki; Kamiji, Yu; Ono, Masato; Nomura, Mikihiro*; Takegami, Hiroaki
Progress in Nuclear Science and Technology (Internet), 7, p.235 - 242, 2025/05
Nagatani, Taketeru; Kosuge, Yoshihiro*; Sagara, Hiroshi*; Nakaguki, Sho; Nomi, Takayoshi; Okumura, Keisuke
Progress in Nuclear Science and Technology (Internet), 7, p.41 - 46, 2025/05
Sato, Hiroyuki; Yan, X.
Progress in Nuclear Science and Technology (Internet), 7, p.293 - 298, 2025/05
Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki
Progress in Nuclear Science and Technology (Internet), 7, p.195 - 198, 2025/05
Extraction chromatgraphy technology for trivalent minor actinide (MA(III) ; Am(III) and Cm(III)) recovery from the solution generated by an extraction process in reprocessing of spent nuclear fuel has been developed. A fine particle is generated in the solution. The fine particle must be removed before MA recovery operation, because that leads clogging of the extraction chlomatography column. In order to prevent clogging the column, filtration system utilizing porous silica beads packed column has been designed. In this study, a fine particle trapping system was developed and particle removal performance of the system was experimentally evaluated using alumina particles as simulated fine particle. Column experiments revealed that the fine particle with the particle size from 0.12 to 15 
m is cause of clogging of the filtration column. Since simulated fine particles were trapped on filtration experiments, a filtration system using the porous silica beads column is practical,
Arai, Yoichi; Watanabe, So; Nakahara, Masaumi; Funakoshi, Tomomasa; Hoshino, Takanori; Takahatake, Yoko; Sakamoto, Atsushi; Aihara, Haruka; Hasegawa, Kenta; Yoshida, Toshiki; et al.
Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/05
The Japan Atomic Energy Agency (JAEA) has been conducting a project named "Systematic Treatment of RAdioactive liquid waste for Decommissioning (STRAD)" project since 2018 for fundamental and practical studies for treating radioactive liquid wastes with complicated compositions. Fundamental studies have been conducted using genuine liquid wastes accumulated in a hot laboratory of the JAEA called the Chemical Processing Facility (CPF), and treatment procedures for all liquid wastes in CPF were successfully designed on the results obtained. As the next phase of the project, new fundamental and practical studies on primarily organic liquid wastes accumulated in different facilities of JAEA are in progress. This paper reviews the representative achievements of the STRAD project and introduces an overview of ongoing studies.
Wada, Yuki*; Morimoto, Takeshi*; Wu, T.*; Wang, D.*; Kikuchi, Hiroshi*; Nakamura, Yoshitaka*; Yoshikawa, Eiichi*; Ushio, Tomoo*; Tsuchiya, Harufumi
Science Advances (Internet), 11(21), p.eads6906_1 - eads6906_10, 2025/05
Times Cited Count：0
C alloy measured in the electrostatic levitation furnace onboard the international space stationIshikawa, Takehiko*; Oda, Hirohisa*; Koyama, Chihiro*; Shimonishi, Rina*; Ikeuchi, Rumiko*; Paradis, P.-F.*; Okada, Jumpei*; Fukuyama, Hiroyuki*; Yamano, Hidemasa
International Journal of Microgravity Science and Application, 42(2), p.420202_1 - 420202_10, 2025/04
Sato, Yuki; Terasaka, Yuta; Ichiba, Yuta*
Journal of Nuclear Science and Technology, 62(4), p.389 - 400, 2025/04
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Watanabe, Tomoaki; Tada, Kenichi; Endo, Tomohiro*; Yamamoto, Akio*
Journal of Nuclear Science and Technology, 16 Pages, 2025/04
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)This study investigated the impact of nuclear data updates from JENDL-4.0 (J4) to JENDL-5 (J5) on the light-water reactor fuel burnup calculations. Burnup calculations were conducted with J4 and J5 for PWR pin-cell and BWR fuel assembly geometries. The calculation results revealed significant burnup-dependent differences in the neutron multiplication factor (k
). Across the burnup range of 0-50 GWd/t, k
values of J5 were consistently smaller than those of J4 and the difference gradually increased as burnup progressed. Direct sensitivity calculations, in which each nuclide data was replaced from J4 to J5, indicated that updates to the cross-sections of 
U, 
U, and 
Pu and the thermal scattering law data of H in HO notably impacted the k differences. For the BWR assembly geometry containing Gd fuels, large k differences were observed in the burnup range of 10-15 GWd/t. This difference was primarily attributed to updates in the U, 
Gd, and 
Gd cross-sections, and thermal scattering law data of H in HO. Furthermore, we investigated how the nuclear data updates affected the k differences by examining nuclide number densities, the energy-dependent sensitivities, and the neutron spectra.
Watanabe, Tomoaki; Aizawa, Naoto*; Chiba, Go*; Tada, Kenichi; Yamamoto, Akio*
Proceedings of International Conference on Mathematics and Computational Methods Applied to Nuclear Science and Engineering (M&C 2025) (Internet), 10 Pages, 2025/04
Currently, a major burnup calculation method for the nuclide composition of nuclear fuel conducts neutron transport calculations at each burnup step to account for changes in the neutron spectrum. While this method is highly accurate, the large computational cost of neutron transport calculations can be problematic. Therefore, a fast burnup calculation method based on neutron spectrum reconstruction with the proper orthogonal decomposition (POD) and regression model is investigated. In this method, dimensionality reduction by POD is applied to many neutron fluxes obtained from detailed burnup calculations for various input parameter sets, and regression models are constructed to connect the dimensionality-reduced neutron fluxes and parameters. By substituting arbitrary input parameters to the regression models, the neutron flux is reconstructed and the burnup calculation is performed. This method performs burnup calculations that consider changes in the neutron spectrum based on input conditions without neutron transport calculations. The present method was applied to a PWR UO fuel pin cell model. The results show the nuclide inventory can be calculated with a prediction accuracy within a few percent. In addition, it is found that the calculation error is dominated by the regression models, which implies the further improvement of the regression models leads to improving the accuracy.
Sweet, M.*; Mishima, Kenji*; Harada, Masahide; Kurita, Keisuke; Iikura, Hiroshi; Tasaki, Seiji*; Kikuchi, Norio*
Quantum Beam Science (Internet), 9(2), p.11_1 - 11_17, 2025/04
Neutron beam, being electrically neutral and highly penetrating, offers unique advantages for irradiation of biological species such as plants, seeds, and microorganisms. We comprehensively investigated the potential of neutron irradiation for inducing genetic mutations using simulations of J-PARC BL10, JRR-3 TNRF, and KUANS for spallation, reactor, and compact neutron sources.
