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Journal Articles

J-PARC proton beam irradiation facility plan

Meigo, Shinichiro

Kasokuki, 21(4), p.333 - 344, 2025/01

For the study of material damage under the beam irradiation circumstance of accelerator-driven systems (ADS), the JAEA had planned to construct a TEF-T using J-PARC Linac 400-MeV proton beams and the LBE spallation target. The task force for evaluating partitioning and transmutation technology in the MEXT recommended that the facility be considered to maximize the advantages of using Linac to meet users' various needs. The proton irradiation facility, a successor of TEF-T, is planned to be constructed for 1) Material irradiation examinations, 2) Semiconductor soft-error examinations using spallation neutrons, 3) Medical RI production, and 4) Proton beam applications for space use. A user community was established in 2022 to incorporate user input as a more attractive facility. In this paper, the present design status of the facility is described.

Journal Articles

Breakdown of linear spin-wave theory and existence of spinon bound states in the frustrated kagome-lattice antiferromagnet

Mattan, K.*; Ono, Toshio*; Kawamura, Seiko; Nakajima, Kenji; Nambu, Yusuke*; Sato, Taku*

Physical Review B, 105(13), p.134403_1 - 134403_8, 2022/04

 Times Cited Count:4 Percentile:33.23(Materials Science, Multidisciplinary)

Spin dynamics of the spin-1/2 kagome-lattice antiferromagnet Cs$$_{2}$$Cu$$_{3}$$SnF$$_{12}$$ was studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving rise to continuum scattering.

Journal Articles

Development of proton beam control technology for transmutation characteristic test

Takei, Hayanori

Isotope News, (779), p.11 - 15, 2022/02

The Japan Atomic Energy Agency (JAEA) has designed a Transmutation Physics Experimental Facility (TEF-P) as an experimental facility in the Japan Proton Accelerator Research Complex (J-PARC). The TEF-P is a critical assembly driven by a low-power proton beam, a maximum of 10 W, which is extracted from a high-power beam source, such as 250 kW of 400 MeV proton beam of the J-PARC Linac. To extract such a low-power proton beam from the high-power proton beam, we developed a laser charge exchange (LCE) device and employed its technique, which is one of the non-contact beam extraction techniques. For the proof of performance of the LCE device to the TEF-P, a low-power proton beam was extracted using a negative-hydrogen Linac having an energy of 3 MeV, and a bright laser. This paper summarizes the experimental results.

Journal Articles

Low-power proton beam extraction by the bright continuous laser using the 3-MeV negative-hydrogen linac in Japan Proton Accelerator Research Complex

Takei, Hayanori; Tsutsumi, Kazuyoshi*; Meigo, Shinichiro

Journal of Nuclear Science and Technology, 58(5), p.588 - 603, 2021/05

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The Japan Atomic Energy Agency (JAEA) has designed a Transmutation Physics Experimental Facility (TEF-P) as an experimental facility in the Japan Proton Accelerator Research Complex (J-PARC). The TEF-P is a critical assembly driven by a low-power proton beam, a maximum of 10 W, which is extracted from a high-power beam source, such as 250 kW of 400 MeV proton beam of the J-PARC Linac. To extract such a low-power proton beam from the high-power proton beam, we developed a laser charge exchange (LCE) device and employed its technique, which is one of the non-contact beam extraction techniques. For the proof of performance of the LCE device to the TEF-P, a low-power proton beam was extracted using a negative-hydrogen (H$$^{-}$$) Linac having an energy of 3 MeV, and a bright continuous laser. Proton beam with the power of 0.57 mW was successfully extracted with a laser stripping efficiency of $$2.3times10^{-5}$$. These experimental values are in good agreement with the estimated ones.

Journal Articles

Strong lattice anharmonicity exhibited by the high-energy optical phonons in thermoelectric material

Wu, P.*; Fan, F.-R.*; Hagihara, Masato*; Kofu, Maiko; Peng, K.*; Ishikawa, Yoshihisa*; Lee, S.*; Honda, Takashi*; Yonemura, Masao*; Ikeda, Kazutaka*; et al.

New Journal of Physics (Internet), 22(8), p.083083_1 - 083083_9, 2020/08

 Times Cited Count:13 Percentile:64.36(Physics, Multidisciplinary)

Thermoelectric material SnSe has aroused world-wide interests in the past years, and its inherent strong lattice anharmonicity is regarded as a crucial factor for its outstanding thermoelectric performance. However, the understanding of lattice anharmonicity in SnSe system remains inadequate, especially regarding how phonon dynamics are affected by this behavior. In this work, we present a comprehensive study of lattice dynamics on Na$$_{0.003}$$Sn$$_{0.997}$$Se$$_{0.9}$$S$$_{0.1}$$ by means of neutron total scattering, inelastic neutron scattering, Raman spectroscopy as well as frozen-phonon calculations. Lattice anharmonicity is evidenced by pair distribution function, inelastic neutron scattering and Raman measurements. By separating the effects of thermal expansion and multi-phonon scattering, we found that the latter is very significant in high-energy optical phonon modes. The strong temperature-dependence of these phonon modes indicate the anharmonicity in this system. Moreover, our data reveals that the linewidths of high-energy optical phonons become broadened with mild doping of sulfur. Our studies suggest that the thermoelectric performance of SnSe could be further enhanced by reducing the contributions of high-energy optical phonon modes to the lattice thermal conductivity via phonon engineering.

Journal Articles

$$q$$=0 long-range magnetic order in centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O; A Spin-$$frac{1}{2}$$ perfect kagome antiferromagnet with $$J_{1}$$-$$J_{2}$$-$$J_{d}$$

Iida, Kazuki*; Yoshida, Hiroyuki*; Nakao, Akiko*; Jeschke, H. O.*; Iqbal, Y.*; Nakajima, Kenji; Kawamura, Seiko; Munakata, Koji*; Inamura, Yasuhiro; Murai, Naoki; et al.

Physical Review B, 101(22), p.220408_1 - 220408_6, 2020/06

 Times Cited Count:28 Percentile:79.78(Materials Science, Multidisciplinary)

Crystal and magnetic structures of the mineral centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O are investigated by means of synchrotron X-ray diffraction and neutron diffraction measurements complemented by density functional theory (DFT) and pseudofermion functional renormalization group (PFFRG) calculations. In CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O, Cu$$^{2+}$$ ions form a geometrically perfect kagome network with antiferromagnetic $$J_{1}$$. No intersite disorder between Cu$$^{2+}$$ and Ca$$^{2+}$$ ions is detected. CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O enters a magnetic long-range ordered state below $$T_{rm N}$$ = 7.2 K, and the $$q$$=0 magnetic structure with negative vector spin chirality is obtained. The ordered moment at 0.3 K is suppressed to 0.58(2)$$mu$$B. Our DFT calculations indicate the presence of antiferromagnetic $$J_{2}$$ and ferromagnetic $$J_{d}$$ superexchange couplings of a strength which places the system at the crossroads of three magnetic orders (at the classical level) and a spin-$$frac{1}{2}$$ PFFRG analysis shows a dominance of $$q$$=0 type magnetic correlations, consistent with and indicating proximity to the observed $$q$$=0 spin structure. The results suggest that this material is located close to a quantum critical point and is a good realization of a $$J_{1}$$-$$J_{2}$$-$$J_{d}$$ kagome antiferromagnet.

Journal Articles

Long beam pulse extraction by the laser charge exchange method using the 3-MeV linac in J-PARC

Takei, Hayanori; Hirano, Koichiro; Meigo, Shinichiro; Tsutsumi, Kazuyoshi*

Proceedings of 8th International Beam Instrumentation Conference (IBIC 2019) (Internet), p.595 - 599, 2020/06

Japan Proton Accelerator Research Complex (J-PARC) has a plan to build the Transmutation Physics Experimental Facility (TEF-P), in which a 400-MeV proton beam will be delivered from negative hydrogen (H$$^{-}$$) accelerated by the linac. Since the TEF-P requires a stable proton beam with a power of less than 10 W, a steady and meticulous beam extraction method is required to extract a small amount of the proton beam from the high power beam using 250 kW. To fulfill this requirement, we have developed beam extraction based on the Laser Charge Exchange (LCE) method. For the demonstration present beam extraction technique, an experiment was conducted using H$$^{-}$$ beam accelerated by the 3-MeV linac at RFQ test-stand in J-PARC. As a result of the experiment with continuous wave (CW) of the Laser, a charge-exchanged long-pulsed H$$^{+}$$ beam with a power of about 0.70 W equivalent was successfully obtained under the TEF-P beam condition.

Journal Articles

Research and development of low activation neutron absorber Au-In-Cd alloy at J-PARC Material and Life Science Experimental Facility

Oi, Motoki

Shiki, 43, P. 3, 2019/06

At the J-PARC Materials and Life Science Facility (MLF), we developed an Au-In-Cd alloy as a low activation neutron absorber for reducing the activity of moderator assembly, and put it to practical use in the reflector and moderator. As a method to confirm the distribution of indium in the alloy, pulse neutron imaging method is adopted, and the individual element distribution is measured by focusing on the resonance peak of indium, and the uniformity of the alloy is confirmed.

Journal Articles

Target test facility for ADS and cross-section experiment in J-PARC

Meigo, Shinichiro; Iwamoto, Hiroki; Matsuda, Hiroki; Takei, Hayanori

Journal of Physics; Conference Series, 1021(1), p.012072_1 - 012072_4, 2018/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Cross section measurement in J-PARC for neutronics of the ADS

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Hiroki

Proceedings of 13th International Topical Meeting on Nuclear Applications of Accelerators (AccApp '17) (Internet), p.396 - 402, 2018/05

no abstracts in English

Journal Articles

Beam extraction by the laser charge exchange method using the 3-MeV LINAC in J-PARC

Takei, Hayanori; Hirano, Koichiro; Tsutsumi, Kazuyoshi; Meigo, Shinichiro

Plasma and Fusion Research (Internet), 13(Sp.1), p.2406012_1 - 2406012_6, 2018/03

The Japan Proton Accelerator Research Complex (J-PARC) has a plan to build the Transmutation Physics Experimental Facility (TEF-P), in which a 400-MeV negative proton (H$$^{-}$$) beam will be delivered from the J-PARC linac. Since the TEF-P requires a stable proton beam with a power of less than 10 W, a stable and meticulous beam extraction method is required to extract a small amount of the proton beam from the high power beam using 250 kW. To fulfil this requirement, the Laser Charge Exchange (LCE) method has been developed. To demonstrate the charge exchange of the H$$^{-}$$, a preliminary LCE experiment was conducted using a linac with energy of 3 MeV in J-PARC. As a result of the experiment, a charge-exchanged H$$^{+}$$ beam with a power of about 8 W equivalent and an accuracy of about 2% was obtained under the J-PARC linac beam condition.

Journal Articles

Beam extraction by the laser charge exchange method using the 3-MeV linac in J-PARC

Takei, Hayanori; Hirano, Koichiro; Meigo, Shinichiro; Tsutsumi, Kazuyoshi*

Proceedings of 6th International Beam Instrumentation Conference (IBIC 2017) (Internet), p.435 - 439, 2018/03

The Japan Proton Accelerator Research Complex (J-PARC) has a plan to build the Transmutation Physics Experimental Facility (TEF-P), in which a 400-MeV negative proton (H$$^{-}$$) beam will be delivered from the J-PARC linac. Since the TEF-P requires a stable proton beam with a power of less than 10 W, a stable and meticulous beam extraction method is required to extract a small amount of the proton beam from the high power beam using 250 kW. To fulfil this requirement, the Laser Charge Exchange (LCE) method has been developed. To demonstrate the charge exchange of the H$$^{-}$$, a preliminary LCE experiment was conducted using a linac with energy of 3 MeV in J-PARC. As a result of the experiment, a charge-exchanged H$$^{+}$$ beam with a power of about 8 W equivalent and an accuracy of about 2% was obtained under the J-PARC linac beam condition.

Journal Articles

Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12

The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.

Journal Articles

Sample environment at the J-PARC MLF

Kawamura, Seiko; Oku, Takayuki; Watanabe, Masao; Takahashi, Ryuta; Munakata, Koji*; Takata, Shinichi; Sakaguchi, Yoshifumi*; Ishikado, Motoyuki*; Ouchi, Keiichi*; Hattori, Takanori; et al.

Journal of Neutron Research, 19(1-2), p.15 - 22, 2017/11

Sample environment (SE) team at the Materials and Life Science Experimental Facility (MLF) in J-PARC has worked on development and operation of SE equipment and devices. All the members belong to one sub-team at least, such as Cryogenic and magnet, High temperature, High pressure, Soft matter and special environment including Pulse magnet, Hydrogen environment, Light irradiation and $$^3$$He spin filter. Cryostats, a magnet, furnaces, a VX-6-type Paris-Edinburgh press and a prototype of a Spin-Exchange Optical Pumping (SEOP) based $$^3$$He spin filter for polarized neutron beam experiments are in operation. Furthermore, a prototype of compact power supply for a pulsed magnet system is currently developed. In the J-PARC Research Building, several pieces of equipment for softmatter research such as a rheometer and a gas and vapor adsorption measurement instrument have been prepared.

Journal Articles

Measurement of aluminum activation cross section and gas production cross section for 0.4 and 3-GeV protons

Meigo, Shinichiro; Nishikawa, Masaaki; Iwamoto, Hiroki; Matsuda, Hiroki

EPJ Web of Conferences, 146, p.11039_1 - 11039_4, 2017/09

BB2016-1181.pdf:0.4MB

 Times Cited Count:2 Percentile:75.05(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Materials and Life Science Experimental Facility at the Japan Proton Accelerator Research Complex, 3; Neutron devices and computational and sample environments

Sakasai, Kaoru; Sato, Setsuo*; Seya, Tomohiro*; Nakamura, Tatsuya; To, Kentaro; Yamagishi, Hideshi*; Soyama, Kazuhiko; Yamazaki, Dai; Maruyama, Ryuji; Oku, Takayuki; et al.

Quantum Beam Science (Internet), 1(2), p.10_1 - 10_35, 2017/09

Neutron devices such as neutron detectors, optical devices including supermirror devices and $$^{3}$$He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF.

JAEA Reports

Investigation and measures of abnormal events of helium refrigerator for cryogenic hydrogen system at J-PARC

Aso, Tomokazu; Teshigawara, Makoto; Hasegawa, Shoichi; Aoyagi, Katsuhiro*; Muto, Hideki*; Nomura, Kazutaka*; Takada, Hiroshi; Ikeda, Yujiro

JAEA-Technology 2017-021, 75 Pages, 2017/08

JAEA-Technology-2017-021.pdf:33.03MB

Liquid hydrogen is employed as a cold neutron moderator material at the spallation neutron source of Materials and Life science experimental Facility of Japan Proton Accelerator Research Complex (J-PARC). From January 2015, it became observable that the differential pressure between heat exchangers and an 80 K adsorber (ADS) in a helium refrigerator system increased with operating time. In November 2015, the differential pressure rise became more significant, leading to degrade the refrigerating performance in cooling liquid hydrogen. In order to investigate the cause of the abnormal differential pressure rise between the heat exchangers and the ADS, we carried out visual inspection inside the heat exchangers and analyzed the impurities contained in the helium gas. Unfortunately, we could not identify the impurities causing the performance degradation, but observed a trace of oil in the inlet piping of the heat exchanger. Based on investigations of the abnormal events occurred in the refrigerators with similar refrigerating capacity at other facilities, we took measures that cleaning the heat exchangers with Freon and replacing the ADS with new one. As a result, the differential pressure rise phenomenon was removed to recover the performance. We have detected oil from the Freon used for cleaning the heat exchangers and at a felt supporting charcoal packed in the ADS. In particular, oil was accumulated in membranous form onto the felt at the entrance side in the ADS. The amount of oil contained in the helium gas was about 10 ppb or so, less than the design value, in the helium refrigerator. However, the oil accumulated onto the felt in the ADS through long operating period may cause abnormal differential pressure rise, leading to the performance degradation of the helium refrigerator. Further study is needed to specify the cause more clearly.

Journal Articles

Present status of the laser charge exchange test using the 3-MeV linac in J-PARC

Takei, Hayanori; Chishiro, Etsuji; Hirano, Koichiro; Kondo, Yasuhiro; Meigo, Shinichiro; Miura, Akihiko; Morishita, Takatoshi; Oguri, Hidetomo; Tsutsumi, Kazuyoshi

Proceedings of 5th International Beam Instrumentation Conference (IBIC 2016) (Internet), p.736 - 739, 2017/03

The Accelerator-driven System (ADS) is one of the candidates for transmuting long-lived nuclides, such as minor actinide (MA), produced by nuclear reactors. For efficient transmutation of the MA, a precise pre-diction of neutronics of ADS is required. In order to obtain the neutronics data for the ADS, the Japan Pro-ton Accelerator Research Complex (J-PARC) has a plan to build the Transmutation Physics Experimental Facility (TEF-P), in which a 400-MeV negative proton (H$$^{-}$$) beam will be delivered from the J-PARC linac. Since the TEF-P requires a stable proton beam with a power of less than 10W, a stable and meticulous beam extraction method is required to extract a small amount of the proton beam from the high power beam using 250kW. To fulfil this requirement, the Laser Charge Exchange (LCE) method has been developed. The LCE strips the electron of the H$$^{-}$$ beam and neutral protons will separate at the bending magnet in the proton beam transport. To demonstrate the charge exchange of the H$$^{-}$$, a preliminary LCE experiment was conducted using a linac with energy of 3MeV in J-PARC. As a result of the experiment, a charge-exchanged H$$^{+}$$ beam with a power of about 5W equivalent was obtained under the J-PARC linac beam condition, and this value almost satisfied the power requirement of the proton beam for the TEF-P.

Journal Articles

Preliminary results of the laser charge exchange test using the 3-MeV linac in J-PARC

Takei, Hayanori; Hirano, Koichiro; Tsutsumi, Kazuyoshi; Chishiro, Etsuji; Miura, Akihiko; Kondo, Yasuhiro; Morishita, Takatoshi; Oguri, Hidetomo; Meigo, Shinichiro

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.987 - 991, 2016/11

Accelerator-driven system (ADS) is one of candidates to transmute long-lived nuclides such as minor actinide (MA) produced at nuclear reactor. For efficient transmutation of the MA, precise prediction of neutronics of ADS is indispensable. In order to obtain the neutronics data for the ADS, J-PARC has a plan to build the Transmutation Physics Experimental Facility (TEF-P). Since the TEF-P requires stable power of the beam and will operate with thermal power less than 500 W and the proton beam power of 10 W so that a stable and meticulous beam extraction method is required to extract small amount of the beam from the high power LINAC beam with 250 kW. To fulfill requirement, Laser charge exchange method (LCE) has been developed for delivery of 400-MeV proton beam with 25Hz to the TEF-P. The LCE strips the electron of H$$^{-}$$ beam and H$$^{0}$$ will separate at the bending magnet at the proton beam transport. The LCE device consists of YAG-laser with high power as 1.6 J/shot and 25 Hz and transport control system with high accuracy of the beam position. For the demonstration of the charge exchange of the H$$^{-}$$, the further LCE tests is conducted using H$$^{-}$$ beam with energy of 3-MeV at RFQ test stand in J-PARC. In this paper, present status of LCE tests is presented.

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