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Journal Articles

Swift heavy ion irradiation effects in nanocrystalline gold

Chimi, Yasuhiro; Iwase, Akihiro*; Ishikawa, Norito; Kobiyama, Mamoru*; Inami, Takashi*; Kambara, Tadashi*; Okuda, Shigeo*

Nuclear Instruments and Methods in Physics Research B, 245(1), p.171 - 175, 2006/04

 Times Cited Count:13 Percentile:30.44(Instruments & Instrumentation)

We have studied effects of irradiation with energetic particles on defect accumulation in nanocrystalline gold (nano-Au). The specimens of nano-Au foil (3-5 $$mu$$m thickness) with various grain sizes (23-156 nm) are prepared by the gas deposition method and subsequent thermal annealings. Irradiations of the specimens with 60-MeV $$^{12}$$C ions, 3.54-GeV $$^{136}$$Xe ions or 2.0-MeV electrons are performed at low temperature. The defect accumulation behavior is observed by measuring the electrical resistivity change during irradiation. Through an analysis of defect accumulation behavior, cross-sections for defect production, $$sigma$$$$_{d}$$, and annihilation, $$sigma$$$$_{r}$$, in nano-Au increase monotonically as the grain size decreases. These results are considered to be caused by the existence of a large volume fraction of the regions near grain boundaries in nano-Au where the threshold energy for atomic displacements, E$$_{d}$$, becomes lower than in polycrystalline gold. The possibility of electronic excitation effects in nano-Au is also discussed.

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