Fujita, Shunya*; Abe, Yutaka*; Kaneko, Akiko*; Yuasa, Tomohisa*; Segawa, Tomoomi; Yamada, Yoshikazu; Kato, Yoshiyuki; Ishii, Katsunori
Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 8 Pages, 2018/07
Mixed uranium oxide and plutonium oxide powder is produced from uranyl nitrate and plutonium nitrate mixed solution by the microwave heating denitration method in the spent fuel reprocessing process. Since the microwave heating method is accompanied by a boiling phenomenon, it is necessary to fully grasp the operating conditions in order to avoid flashing and spilling in the mass production of denitrification technology for the future. In this research, it was confirmed that a potassium chloride aqueous solution as a simulant of uranyl nitrate aqueous solution with high dielectric loss cause loss of microwave at the solution surface as the dielectric loss increased with the increase of KCl concentration by experimental and electromagnetic field analysis, and revealed that the change in the heating condition affects the generation of flushing.
Suda, Kazunori; Shimizu, Ryo; Tazaki, Makiko; Tamai, Hiroshi; Kitade, Yuta
Nihon Kaku Busshitsu Kanri Gakkai Dai-38-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2018/04
Since India's nuclear explosion in 1974, there has been continued discussion on nuclear non-proliferation. At first, to prevent proliferation of nuclear weapons, the International Nuclear Fuel Cycle Evaluation (INFCE) was established to discuss reprocessing, plutonium handling, and so on. After that, to respond to the threat of proliferation posed by DPRK, the international community desired to further enhance nuclear non-proliferation by strengthening the IAEA safeguards system. In recent years, some researchers at universities and national laboratories are studying proliferation resistance from the standpoint of nuclear materials that may be inherently self-protecting. This paper discusses minimization of proliferation risk and future prospects based on alternative measures for reprocessing, plutonium handling, and recycling described in INFCE-WG4.
Tsujimoto, Kazufumi; Arai, Yasuo; Minato, Kazuo
Nippon Genshiryoku Gakkai-Shi, 59(11), p.644 - 648, 2017/11
no abstracts in English
Fujita, Shunya*; Abe, Yutaka*; Kaneko, Akiko*; Chonan, Fuminori*; Yuasa, Tomohisa*; Yamaki, Tatsunori*; Segawa, Tomoomi; Yamada, Yoshikazu
Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 8 Pages, 2017/07
From the observation results, in the process of flushing, the behaviors leading to flushing were classified divided into three types. First type is that first generation bubble from heating leads to flushing. Second type is that nucleate boiling continues during heating and stop, finally single bubble generates and leads to flushing. Third type is defined that gradual evaporation occurs without bubbles. It was revealed that the total quantities of heat released by flushing are approximately equal when assuming the flushing mechanism, it can be triggered that a large amount of micro bubbles are instantaneously generated and grew.
Tamai, Hiroshi; Okubo, Ayako; Kimura, Yoshiki; Shinohara, Nobuo; Tazaki, Makiko; Shimizu, Ryo; Suda, Kazunori; Tomikawa, Hirofumi
Proceedings of INMM 58th Annual Meeting (Internet), 6 Pages, 2017/07
Nuclear forensics is a technical measure to analyse and collate samples of illegally used nuclear materials, etc., to clarify their origins, routes, etc. and contribute to criminal identifications. Close collaboration with police and judicial organizations is essential. The national response framework is being built up with international cooperation. Discussions on promoting technical capability and regional cooperation are presented.
Nakayama, Shinichi; Okumura, Masahiko*; Nagasaki, Shinya*; Enokida, Yoichi*; Umeki, Hiroyuki*; Takase, Hiroyasu*; Kawasaki, Daisuke*; Hasegawa, Shuichi*; Furuta, Kazuo*
Genshiryoku Bakkuendo Kenkyu (CD-ROM), 23(2), p.131 - 148, 2016/12
A symposium "Science of nuclear fuel cycle and backend - Research and education -" was held at the Univer-sity of Tokyo in June 25, 2016. This aimed at developing the research on nuclear fuel cycle and backend. The time and the number of participants of the symposium were limited, but the active discussion was conducted, and the common perception for the future was shared among the experienced participants in those fields. This paper provides the discussions made in the symposium, and also, as a memory to Professor Ahn, the University of California, Berkeley, his prominent achievements in academic research and education.
Segawa, Tomoomi; Fukasawa, Tomonori*; Huang, A.-N.*; Yamada, Yoshikazu; Suzuki, Masahiro; Fukui, Kunihiro*
Chemical Engineering Science, 153, p.108 - 116, 2016/10
The influence of the heating method and rate on the morphology of CuO powders synthesized from Cu(NO)3HO aqueous solutions by denitration was investigated. The median diameter of the obtained powder was found to decrease as the heating rate increased, independent of the heating method. The microwave heating method remarkably reduced the particle size and enhanced the irregularity and disorder of the shape and surface of the particles, which were found to be more widely distributed. In contrast, the microwave hybrid heating method yielded the most spherical particles with the smoothest surface. It was also found that this heating method sharpened the particle size distribution and had higher energy efficiency than the MW method. Numerical simulations also indicated a difference in the energy efficiency between these two methods. The simulations also revealed that the hybrid method could heat the whole reactor more uniformly with a lower microwave output.
Segawa, Tomoomi; Kawaguchi, Koichi; Ishii, Katsunori; Suzuki, Masahiro; Arimitsu, Naoki*; Yoshida, Hideto*; Fukui, Kunihiro*
Advanced Powder Technology, 26(3), p.983 - 990, 2015/05
Denitration of the aqueous solution of nickel nitrate hexahydrate (Ni(NO)6HO) by a microwave heating method was investigated. Since Ni(NO)6HO aqueous solution cannot be heated to over 300 C by microwave irradiation owing to the low microwave absorptivity of its intermediate, NiO could not previously be obtained by microwave heating. We propose a novel NiO synthesis method that uses microwave heating without the risk of chemical contamination. A NiO powder reagent was added to the solution as a microwave acceptor. The denitration efficiency to NiO could be improved by an adiabator around the reactor to increase the temperature homogeneity in the reactor. Numerical simulations also reveal that the use of the adiabator results in remarkable changes in the electromagnetic field distribution in the reactor, temperature inhomogeneity decreases.
Sakamoto, Atsushi; Sano, Yuichi; Takeuchi, Masayuki; Okamura, Nobuo; Koizumi, Kenji
Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 5 Pages, 2015/05
Fukui, Kunihiro*; Igawa, Yusuke*; Arimitsu, Naoki*; Suzuki, Masahiro; Segawa, Tomoomi; Fujii, Kanichi*; Yamamoto, Tetsuya*; Yoshida, Hideto*
Chemical Engineering Journal, 211-212, p.1 - 8, 2012/11
The process for synthesizing metallic oxide powders by the microwave denitration method was investigated using hexahydrated nickel nitrate and trihydrated copper nitrate aqueous solutions, and the electrical field and the temperature distributions in the reactor were numerically simulated. Although CuO powder can be obtained from a trihydrated copper nitrate aqueous solution by the microwave denitration method, a hexahydrated nickel nitrate aqueous solution cannot be heated up to over 270 C by microwave irradiation. It was also found that the reaction routes for microwave heating are the same as those for conventional external heating. This finding indicates that the success of producing oxide particles by microwave denitration depends not only on the microwave absorptivity of the intermediate and the metallic oxide, but also on the temperature difference.
Oigawa, Hiroyuki; Nishihara, Kenji; Minato, Kazuo; Kimura, Takaumi; Arai, Yasuo; Morita, Yasuji; Nakayama, Shinichi; Katakura, Junichi
JAERI-Review 2005-043, 193 Pages, 2005/09
JAERI has been conducting research and development on partitioning and transmutation (P&T) technology for long-lived nuclides to develop the double-strata fuel cycle concept, in accordance with the Atomic Energy Commission's "Research and Development of Technologies for Partitioning and Transmutation of Long-lived Nuclides - Status and Evaluation Report" issued in 2000. The double-strata fuel cycle concept consists of four major processes: partitioning, fuel fabrication, transmutation, and fuel processing. The five-year achievement and future perspectives for the technology on these processes are presented in this report. It also provides an analytical study on impacts of introducing P&T technology on waste management, and on deployment of P&T for the future nuclear energy system.
Akie, Hiroshi; Nabeshima, Kunihiko; Uchikawa, Sadao
JAERI-Conf 2005-009, 153 Pages, 2005/08
As a research on the future innovative water reactor, the development of Reduced-Moderation Water Reactors (RMWRs) has been performed in JAERI. The workshop on RMWRs is aiming at information exchange between JAERI and other organizations, and has been held every year since 1998. The program of the 7th workshop was composed of 5 lectures and an overall discussion time. This report includes the original papers presented at the workshop and summaries of the questions and answers for each lecture as well as of the discussion time. In addition in Appendix, there are included presentation handouts of each lecture.
Fujita, Mitsutane*; Xu, Y.*; Kaji, Yoshiyuki; Tsukada, Takashi; Mashiko, Shinichi*; Onose, Shoji*
RIST News, (38), p.3 - 14, 2004/11
The distributed materials database system named "Data-Free-Way(DFW)" has been developed with the collaboration of three organizations: the National Institute for Materials Science, the Japan Atomic Energy Research Institute, and the Japan Nuclear Cycle Development Institute over the Internet since 1990. At present, the development of a distributed knowledge based system, in which knowledge extracted from DFW is expressed, is planned with the collaboration of three organizations as we add data into DFW and make DFW open for the public use. Network technique and presentation and acquisition technique of the information developed rapidly and these techniques brought about a revolution in the society and our daily life changed. This paper describe the present status of DFW and future direction of the material databases with the transition of information technology.
7th NUCEF Seminar Working Group
JAERI-Conf 2004-011, 166 Pages, 2004/07
no abstracts in English
Okamoto, Yoshihiro; Minato, Kazuo
JAERI-Conf 2004-008, 228 Pages, 2004/04
Applications of molten salts technology to separation and synthesis of materials have a potential to give us a civilized life, for example aluminium refinement. Recently, much attention is given to the pyrochemical reprocessing of spent nuclear fuels in the molten salt research field. On the other hand, computer simulation technique is expected to play an important role for supporting experimental works and predicting unknown physical properties in the molten salts application studies. Research group for Actinides Science, Department of Materials Science, Japan Atomic Energy Research Institute(JAERI), together with Reprocessing and Recycle Technology Division, Atomic Energy Society of Japan, organized the 3rd Workshop on Molten Salts Technology and Computer Simulation at Tokai Research Establishment, JAERI on December 16, 2003. Many molten salts researchers in Japan participated in the workshop and many useful presentations and discussions were performed.
6th NUCEF Seminar Working Group
JAERI-Conf 2003-018, 132 Pages, 2003/10
no abstracts in English
Sakurai, Kiyoshi; Nojiri, Ichiro*
JAERI-Conf 2003-019, p.855 - 857, 2003/10
This paper provides overview of sub-criticality safety analysis seminar (July 2000-July 2003, JAERI, total 40 engineers from universities, research institutes and enterprises) for nuclear fuel cycle facility with the Monte Carlo method in Japan. MCNP-4C2 system (MS-DOS version) was installed in each note-type personal computer. Fundamental theory of reactor physics and Monte Carlo simulation including MCNP-4C manual was lectured. Effective neutron multiplication factor and neutron spectrum were calculated for JCO deposit tank, JNC uranium solution storage tank, JNC plutonium solution storage tank and JAERI TCA core. In the seminar, methodology of safety management for nuclear fuel cycle facility was discussed in order to prevent criticality accident.
; Sato, Haruo
JNC-TN8410 2001-028, 36 Pages, 2002/03
For a safety assessment of the high-level radioactive waste disposal, effective diffusion coefficients (D) of radionuclides in bentonite have been accumulated by the through-diffusion method. It has been found recently that experimental results on Ds for several cations (cesium and strontium) by the fairly standard experimental method in JNC differ from those previously reported in several papers. Discrepancy can be considered to be due to different design of diffusion cell and system. In order to confirm influences of the experimental design on cation diffusivities in bentonite, a flow-through diffusion system was developed and several diffusion experiments were conducted.As a result, magnitude of D and its salinity dependence were relatively different between the standard and flow-through diffusion system. Since the latter system can control boundary conditions of the experiment more strictly than the standard method, we can conclude that the flow-through diffusion system provide correct results. In addition, we apply this flow-through diffusion system to a modification of controlling boundary condition during the experiment and to the diffusion experiment under controlled temperature.