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Takai, Toshihide; Furukawa, Tomohiro; Watanabe, Shigeki*; Ishioka, Noriko*
Mechanical Engineering Journal (Internet), 9(4), p.21-00397_1 - 21-00397_11, 2022/08
For the mass production of astatine-211, a promising radiopharmaceutical for cancer treatment, the National Institute for Quantum and Radiological Science and Technology has proposed the innovative "Liquid Bismuth Target System." The target window in this system must be made from a material that resists the highly corrosive liquid bismuth environment. To meet this requirement, a promising target window material was selected in corrosion experiments performed in stagnant liquid bismuth. Based on knowledge of corrosion in liquid lead-bismuth eutectic gained during the development of fast reactors and accelerator-driven subcritical systems, experiments were carried out under saturated dissolved oxygen and low oxygen conditions, and the corrosion behaviors of the specimens were evaluated. The FeCrAl-alloy exhibited the most excellent corrosion resistance, followed by FeCrMo-alloy. Both materials are suitable candidates for the target window.
Kawakita, Yukinobu; Kikuchi, Tatsuya*
Hamon, 29(2), p.91 - 94, 2019/05
Bismuth (Bi) has a double-layered structure based on Peierls distortion in crystalline phase. Complicated static structure in liquid phase which cannot be interpreted by a simple packing model has been conjectured that Peierls distortion may remain even in liquid phase. We measured quasi-elastic neutron scattering (QENS) of liquid Bi by using AMATERAS installed at BL14 beamport of Materials and Life Science Experimental Facility (MLF) in J-PARC and analyzed coherent QENS spectra. A time-space correlation function revealed that the nearest neighboring shell followed by a shoulder-like structure at longer side consists of four contributions of short and long correlations with relatively long relaxation time of a few tens pico second and medium-ranged and the longest correlations with a short relaxation time of sub-pico second, which is a direct observation of the existing layered structure in liquid Bi. In this article, we report the above scientific results and the method to analyze coherent QENS by the time-space correlation function.
Yamana, Hajimu*; Moriyama, Hirotake*; Asano, Hideki*; Shiokawa, Yoshinobu*; Yamamura, Tomoo*; Hasegawa, Kazuki*; Kimura, Akihiro*; Umekita, Satoshi*
JAERI-Tech 2002-018, 33 Pages, 2002/03
JAERI-Tech-2002-018.pdf:1.95MB
no abstracts in English
Takai, Toshihide; Furukawa, Tomohiro; Watanabe, Shigeki*; Ishioka, Noriko*
no journal, ,
For the mass production of astatine-211, a promising radiopharmaceutical for cancer treatment, the National Institute for Quantum and Radiological Science and Technology has proposed the innovative "Liquid Bismuth Target System." The target window in this system must be made from a material that resists the highly corrosive liquid bismuth environment. To meet this requirement, a promising target window material was selected in corrosion experiments performed in stagnant liquid bismuth. Based on knowledge of corrosion in liquid lead-bismuth eutectic gained during the development of fast reactors and accelerator-driven subcritical systems, experiments were carried out under saturated dissolved oxygen and low oxygen conditions, and the corrosion behaviors of the specimens were evaluated. The FeCrAl-alloy exhibited the most excellent corrosion resistance, followed by FeCrMo-alloy. Both materials are suitable candidates for the target window.
