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Journal Articles

$$^{239}$$Pu nuclear magnetic resonance in the candidate topological insulator PuB$$_4$$

Dioguardi, A. P.*; Yasuoka, Hiroshi*; Thomas, S. M.*; Sakai, Hironori; Cary, S. K.*; Kozimor, S. A.*; Albrecht-Schmitt, T. E.*; Choi, H. C.*; Zhu, J.-X.*; Thompson, J. D.*; et al.

Physical Review B, 99(3), p.035104_1 - 035104_6, 2019/01

 Times Cited Count:5 Percentile:30.83(Materials Science, Multidisciplinary)

We present a detailed nuclear magnetic resonance (NMR) study of $$^{239}$$Pu in bulk and powdered single-crystal plutonium tetraboride (PuB$$_4$$), which has recently been investigated as a potential correlated topological insulator. The $$^{239}$$Pu NMR spectra are consistent with axial symmetry of the shift tensor showing for the first time that $$^{239}$$Pu NMR can be observed in an anisotropic environment and up to room temperature. The temperature dependence of the $$^{239}$$Pu shift, combined with a relatively long spin-lattice relaxation time ($$T_1$$), indicate that PuB$$_4$$ adopts a nonmagnetic state with gaplike behavior consistent with our density functional theory calculations. The temperature dependencies of the NMR Knight shift and $$T^{-1}$$ imply bulk gaplike behavior confirming that PuB$$_4$$ is a good candidate topological insulator.

JAEA Reports

Nuclear data evaluation for $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Pu and $$^{242}$$Pu irradiated by neutrons and protons at the energies up to 250 MeV

Konobeyev, A. Y.; Fukahori, Tokio; Iwamoto, Osamu

JAERI-Research 2002-029, 48 Pages, 2002/12


The evaluation of nuclear data for plutonium isotopes with atomic mass number from 238 to 242 has been performed. Neutron data were obtained at the energies from 20 to 250 MeV and combined with JENDL-3.3 data at 20 MeV. Evaluation of the proton data has been done from 1 to 250 MeV. The coupled channel optical model was used to obtain angular distributions for elastic and inelastic scattering and transmission coefficients. Pre-equilibrium exciton model and Hauser-Feshbach statistical model were used to describe neutron and charged particles emission from the excited nuclei. These evaluation is the first work for producing the full set of evaluated file up to 250 MeV for plutonium isotopes.

Oral presentation

Preparation of mixed spike with $$^{239}$$Pu and $$^{235}$$U for MOX analysis by isotope dilution mass spectrometry and application to actual sample

Horigome, Kazushi; Taguchi, Shigeo; Yamamoto, Masahiko; Inada, Satoshi; Kuno, Takehiko

no journal, , 

no abstracts in English

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