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Revaporization behavior of cesium and iodine compounds from their deposits in the steam-boron atmosphere

Rizaal, M.; 三輪 周平; 鈴木 恵理子; 井元 純平; 逢坂 正彦; Gou$"e$llo, M.*

ACS Omega (Internet), 6(48), p.32695 - 32708, 2021/12

This paper presents our investigation on cesium and iodine compounds revaporization from cesium iodide (CsI) deposits on the surface of stainless steel type 304L, which were initiated by boron and/or steam flow. A dedicated basic experimental facility with a thermal gradient tube (TGT) was used for simulating the phenomena. The number of deposits, the formed chemical compounds, and elemental distribution were analyzed from samples located at temperature range 1000-400 K. In the absence of boron in the gas flow, it was found that the initial deposited CsI at 850 K could be directly re-vaporized as CsI vapor/aerosol or reacted with the carrier gas and stainless steel (Cr$$_{2}$$O$$_{2}$$ layer) to form Cs$$_{2}$$CrO$$_{4}$$ on the former deposited surface. The latter mechanism consequently gave a release of gaseous iodine that was accumulated downstream. After introducing boron to the steam flow, a severe revaporization of iodine deposit at 850 K occurred (more than 70% initial deposit). This was found as a result of the formation of two kinds of cesium borates (Cs$$_{2}$$B$$_{4}$$O$$_{7}$$$$cdot$$5H$$_{2}$$O and CsB$$_{5}$$O$$_{8}$$$$cdot$$4H$$_{2}$$O) which contributed to a large release of gaseous iodine that was capable of reaching outlet of TGT ($$<$$ 400 K). In the case of nuclear severe accident, our study have demonstrated that gaseous iodine could be expected to increase in the colder region of a reactor after late release of boron or a subsequent steam flow after refloods of the reactor, thus posing its near-term risk once leaked to the environment.


動作不能からの復帰を可能とする多連結移動ロボットの半自律遠隔操作技術の確立(委託研究); 令和2年度英知を結集した原子力科学技術・人材育成推進事業

廃炉環境国際共同研究センター; 電気通信大学*

JAEA-Review 2021-025, 33 Pages, 2021/11




The Impact of cement on argillaceous rocks in radioactive waste disposal systems; A Review focusing on key processes and remaining issues

Wilson, J.*; Bateman, K.; 舘 幸男

Applied Geochemistry, 130, p.104979_1 - 104979_19, 2021/07

 被引用回数:1 パーセンタイル:0.56(Geochemistry & Geophysics)



Surface complexation of Ca and competitive sorption of divalent cations on montmorillonite under alkaline conditions

杉浦 佑樹; 石寺 孝充; 舘 幸男

Applied Clay Science, 200, p.105910_1 - 105910_10, 2021/01

 被引用回数:2 パーセンタイル:0.03(Chemistry, Physical)

In the geological disposal system, increase of Ca concentration with the alteration of cementitious materials would affect the retention of other radionuclides by competitive sorption. Batch sorption experiments were performed to investigate sorption behavior of Ca and competition with other divalent cations (Sr and Ni) on the edge site of montmorillonite under alkaline conditions. Ca and Sr formed surface complexation with the edge site at higher pH region compared to Ni. Sr sorption decreased with Ca concentration in alkaline pH region, whereas Ni sorption was not affected by Ca concentration. These results indicate that Ca and Sr sorb onto the same site while Ca and Ni sorb onto different sites, and competitive sorption depends on the chemical similarity such as hydrolysis behavior. Sorption model parameters obtained from the single element batch sorption experiments successfully reproduced the results of competitive sorption experiments.



岡野 蒼*; 木本 和志*; 松井 裕哉

第15回岩の力学国内シンポジウム講演論文集(インターネット), p.633 - 636, 2021/01



Chapter 18, Moving particle semi-implicit method

Wang, Z.; Duan, G.*; 越塚 誠一*; 山路 哲史*

Nuclear Power Plant Design and Analysis Codes, p.439 - 461, 2021/00

The Moving Particle Semi-implicit (MPS) method is one kind of particles methods which are based on Lagrangian approach. It has been developed to analyze complex thermal-hydraulic problems, including those in nuclear engineering. Since meshes are no longer used, large deformation of free surfaces or interfaces can be simulated without the problems of mesh distortion. This approach is effective in solving multiphase fluid dynamics which is subject to complex motion of free surfaces or interfaces. Since its development, MPS method has been extensively utilized for wide range of applications in nuclear engineering. In this chapter, the basic theory of the MPS method is firstly explained. Then, some examples of its application in nuclear engineering, including bubble dynamic, vapor explosion, jet breakup, multiphase flow instability, in-vessel phenomenon, molten spreading, molten core concrete interaction (MCCI) and flooding, are presented.


動作不能からの復帰を可能とする多連結移動ロボットの半自律遠隔操作技術の確立(委託研究); 令和元年度英知を結集した原子力科学技術・人材育成推進事業

廃炉環境国際共同研究センター; 電気通信大学*

JAEA-Review 2020-025, 34 Pages, 2020/12




Water distribution in Nafion thin films on hydrophilic and hydrophobic carbon substrates

伊藤 華苗; 原田 雅史*; 山田 悟史*; 工藤 憲治*; 青木 裕之; 金谷 利治*

Langmuir, 36(43), p.12830 - 12837, 2020/11

 被引用回数:2 パーセンタイル:21.55(Chemistry, Multidisciplinary)

We performed H$$_{2}$$O and D$$_{2}$$O double contrast neutron reflectivity measurements on $$sim$$25-nm-thick Nafion thin films on hydrophilic and hydrophobic carbon in water and 80% relative humidity vapor to investigate the depth profile of the water and Nafion distribution. We found a dense Nafion layer at the air or water interface regardless of the carbon hydrophilicity. On the other hand, a water-rich Nafion dense layer was observed at the carbon interface only for hydrophilic carbon. The double contrast measurements provided quantitative information about the depth profile but simultaneously indicated that the sum of the volume occupancies of water and Nafion in the film was less than unity. We assessed the problem based on two possibilities: voids in the film or "residual water", which cannot be exchanged or is difficult to exchange with water outside.


Acceleration of fusion plasma turbulence simulations using the mixed-precision communication-avoiding Krylov method

井戸村 泰宏; 伊奈 拓也*; Ali, Y.*; 今村 俊幸*

Proceedings of International Conference for High Performance Computing, Networking, Storage, and Analysis (SC 2020) (Internet), p.1318 - 1330, 2020/11

5次元ジャイロ運動論モデルに基づく次世代核融合実験炉ITERのマルチスケールfull-$$f$$シミュレーションは核融合科学において最も計算コストが大きい問題の一つである。本研究では、新しい混合精度省通信クリロフ法を用いてジャイロ運動論的トロイダル5次元オイラーコードGT5Dを高速化した。演算加速環境における大域的集団通信のボトルネックを省通信クリロフ法によって解決した。これに加えて、A64FXにおいて新たにサポートされたFP16SIMD演算を用いて設計された新しいFP16前処理により、反復(袖通信)の回数と計算コストの両方を削減した。富岳とSummitにおける1,440CPU/GPUを用いた1,000億格子のITER規模シミュレーションに対して、提案手法の処理性能は従来の非省通信クリロフ法に比べてそれぞれ2.8倍, 1.9倍高速化され、5,760CPU/GPUまで良好な強スケーリングを示した。


高レベル放射性廃液ガラス固化体の表面積の増加に関する調査及び評価; 地層処分性能評価のための割れによる表面積増加比及びその根拠等

五十嵐 寛

JAEA-Review 2020-006, 261 Pages, 2020/09


本調査報告では、公開情報を対象に我が国の地層処分研究開発第2次取りまとめ(H12レポート)以降の諸外国の包括的性能評価報告書を中心として、ソースタームとしての核種溶出モデルにおけるガラス固化体の割れによる表面積増加比の設定値及びその根拠・背景の視点から調査した。また、海外の知見を参考に表面積増加に関する試験の日本の報告例に対する評価を試行した。調査文献から得られた知見に基づき、ガラス固化体の直径、ガラス固化体製造時の冷却条件、ガラス固化体への衝撃、地層処分場閉鎖後の水との接触等の環境条件等が、割れによる表面積増加比(又は割れ係数)に及ぼす影響について検討した。多くの国において、ガラス固化体の割れの要因はガラス固化体の製造, 輸送, 保管, 貯蔵など処分前管理の段階及び処分後の現象又は事象に起因するとされている。その影響は地層処分の性能評価における核種溶出モデルでも考慮されている。各国の核種溶出モデルにおける表面積増加比とその根拠等を概観し、各国の間の相違点及び共通点を整理するとともに、これまでに報告された表面積増加比の測定値と測定方法との関係及び測定方法の特性について考察した。また、各国の核種溶出モデルで設定されている表面積増加比の根拠としての表面積増加比の測定に用いられた測定方法を整理した。さらに、廃棄物管理工程の流れの中でのガラス固化体の割れによる表面積増加比に影響する要因、表面積増加比の特徴等の各工程との関わりを検討した。これらの調査及び検討により、性能評価における保守的かつ現実的な表面積増加比の適用に向けた知見を拡充し、我が国の地層処分のシステムのセーフティケースの作成・更新に資することができる。


Continuous and discontinuous yielding behaviors in ferrite-cementite steels

Wang, Y.*; 友田 陽*; 大村 孝仁*; Gong, W.*; Harjo, S.; 田中 雅彦*

Acta Materialia, 196, p.565 - 575, 2020/09

 被引用回数:6 パーセンタイル:69.06(Materials Science, Multidisciplinary)

The continuous and discontinuous yielding behaviors in ferrite-cementite steels were complementarily investigated via nano- and macroscale deformation examinations. The results obtained by electron microscopy, synchrotron X-ray, and neutron diffractions indicate that the ferrite-cementite interface of the heat-treated specimen is semi-coherent with a high internal stress field, whereas that of the recrystallized one is incoherent with a low internal stress field. Moreover, coherency strain, which depends on the total area of the ferrite-cementite interface, and thermal strain, which is governed by temperature, are the two factors that influence peak broadening. The nanoindentation tests revealed that the critical loads are significantly lower near the semi-coherent interface than those near the incoherent interface and the ferrite grain boundary; this suggests that dislocations are easily emitted from the semi-coherent interface.


J-PARC 3-GeV RCS; 1-MW beam operation and beyond

發知 英明; 原田 寛之; 林 直樹; 金正 倫計; 岡部 晃大; Saha, P. K.; 菖蒲田 義博; 田村 文彦; 山本 風海; 山本 昌亘; et al.

Journal of Instrumentation (Internet), 15(7), p.P07022_1 - P07022_16, 2020/07

 被引用回数:1 パーセンタイル:27.17(Instruments & Instrumentation)




青柳 和平; 櫻井 彰孝; 宮良 信勝; 杉田 裕

JAEA-Research 2020-004, 68 Pages, 2020/06





青木 智幸*; 谷 卓也*; 坂井 一雄*; 古賀 快尚*; 青柳 和平; 石井 英一

JAEA-Research 2020-002, 83 Pages, 2020/06




Development of a user-friendly interface IRONS for atmospheric dispersion database for nuclear emergency preparedness based on the Fukushima database

El-Asaad, H.*; 永井 晴康; 相楽 洋*; Han, C. Y.*

Annals of Nuclear Energy, 141, p.107292_1 - 107292_9, 2020/06

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)



Vertical and horizontal distributions of $$^{137}$$Cs on paved surfaces affected by the Fukushima Dai-ichi Nuclear Power Plant accident

吉村 和也; 渡辺 貴善; 操上 広志

Journal of Environmental Radioactivity, 217, p.106213_1 - 106213_6, 2020/06

 被引用回数:3 パーセンタイル:39.03(Environmental Sciences)

To obtain the important information and parameter for the measurement of $$^{137}$$Cs activity per unit area on paved ground, this study evaluated their vertical and horizontal distributions. This study showed that $$^{137}$$Cs was retained in extremely surface layer with mass depth less than 0.5 cm$$^{-2}$$. This study also demonstrated the horizontal variations of $$^{137}$$Cs activity and the relation of the variation with grid size.


Numerical simulation of two-phase flow in 4$$times$$4 simulated bundle

小野 綾子; 山下 晋; 鈴木 貴行*; 吉田 啓之

Mechanical Engineering Journal (Internet), 7(3), p.19-00583_1 - 19-00583_12, 2020/06



Observation of aerosol particle capturing behavior near gas-liquid interface

上澤 伸一郎; 吉田 啓之

Mechanical Engineering Journal (Internet), 7(3), p.19-00539_1 - 19-00539_9, 2020/06

Air pollution control equipment with spraying liquid in aerosol is used in severe accidents of nuclear power plants to remove radioactive aerosol particles. The removal performance of the equipment has been confirmed based on actual-scale tests. However, unexpected situations may happen in severe accidents due to large-scale disasters. We have developed a numerical analysis method for evaluating radioactive aerosol particle removal performance to optimize the performance and the design. As a part of the development of the numerical analysis, in order to grasp the capturing behavior of the aerosol particle deposition on a gas-liquid interface, we performed a direct observation of aerosol particle behavior near the gas-liquid interface of a droplet. As the capturing behavior near the gas-liquid interface, the particle penetration into liquid, the deposition on the gas-liquid interface and the deposition on the interface after moving to slide on the interface were confirmed in the experiment. The observation result indicated that the penetration was observed with the higher Stokes number and the deposition was observed with the lower Stokes number. However, for the lower Stokes number, the case where particles were not captured on the gas-liquid interface was also confirmed. Thus, the Stokes number is one of the important parameters for the aerosol particle capturing by gas-liquid interface.


Development of FRENDY nuclear data processing code; Generation capability of multi-group cross sections from ACE file

山本 章夫*; 遠藤 知弘*; 多田 健一

Transactions of the American Nuclear Society, 122(1), p.714 - 717, 2020/06



Effects of the Montague resonance on the formation of the beam distribution during multiturn injection painting in a high-intensity proton ring

發知 英明

Physical Review Accelerators and Beams (Internet), 23(5), p.050401_1 - 050401_13, 2020/05

 被引用回数:3 パーセンタイル:71.11(Physics, Nuclear)

J-PARC RCSのベータトロン振動数は2Qx-2Qy=0共鳴(モンタギュー共鳴)の近傍に設定されている。この共鳴は、ビーム自身が作る非線形な空間電場によって励起され、水平・鉛直間のエミッタンス交換を通して付加的な分布変動を引き起こす。そのため、この共鳴は、ペイント入射後のビームの分布形状に大きな影響を及ぼすことになる。数値シミュレーションと実験結果との詳細比較から、2Qx-2Qy=0共鳴がペイント範囲やペイント経路の取り方に依存して複数の異なった効果をビームに及ぼしていることが明らかとなった。本論文では、2Qx-2Qy=0共鳴によって生じる特徴的なビーム粒子の振る舞いを議論すると共に、その検討結果に基づいて、新たなペイント入射方式を提案する。

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