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JAEA Reports

Investigation of measurement accuracy of burnup reactivity of accelerator-driven system during normal operation

Katano, Ryota; Abe, Takumi; Cibert, H.*

JAEA-Research 2024-019, 22 Pages, 2025/05

JAEA-Research-2024-019.pdf:1.03MB

An accelerator-driven system (ADS) dedicated to transmutation of minor actinides (MAs) is driven in subcritical states. It is important for establishment of the subcriticality control of ADS to predict the burnup reactivity. To validate the prediction accuracy, the burnup reactivity, especially at the first cycle, must be measured with sufficient accuracy. In this study, we focus on Current-To-Flux (CTF) method. We have simulated the burnup reactivity monitoring during the ADS normal operation with the CTF method by performing fixed-source-burnup calculations using a continuous energy Monte Carlo code SERPENT2 with some tallies that models in-core fission chambers and have estimated its measurement uncertainty. We have clarified that the 10% biases of measure burnup reactivities appear independently of the burnup duration and their detector position dependence is particularly small in the outer region of the system.

Journal Articles

Large disequilibrium of $$^{234}$$U/$$^{238}$$U isotope ratios in deep groundwater and its potential application as a groundwater mixing indicator

Kuribayashi, Chika*; Miyakawa, Kazuya; Ito, Akane*; Tanimizu, Masaharu*

Geochemical Journal, 59(2), p.35 - 44, 2025/00

 Times Cited Count:0 Percentile:0.00(Geochemistry & Geophysics)

no abstracts in English

Journal Articles

Radioactivity estimation of radioactive hotspots using a Compton camera and derivation of dose rates in the surrounding environment

Sato, Yuki

Applied Radiation and Isotopes, 212, p.111421_1 - 111421_8, 2024/10

 Times Cited Count:0 Percentile:0.00(Chemistry, Inorganic & Nuclear)

Journal Articles

Impact of uncertainty reduction on lead-bismuth coolant in accelerator-driven system using sample reactivity experiments

Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro; Pyeon, C. H.*; Yamamoto, Akio*; Endo, Tomohiro*

Nuclear Science and Engineering, 198(6), p.1215 - 1234, 2024/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

In this study, we have demonstrated that data assimilation using lead and bismuth sample reactivities measured in the Kyoto University Critical Assembly A-core can successfully reduce the uncertainty of the coolant void reactivity in accelerator-driven systems derived from inelastic-scattering cross-sections of lead and bismuth. We re-evaluated and highlighted the experimental uncertainties and correlations of the sample reactivities for the data assimilation formula. We used the MCNP6.2 code to evaluate the sample reactivities and their uncertainties, and performed data assimilation using the reactor analysis code system MARBLE. The high-sensitivity coefficients of the sample reactivities to lead and bismuth allowed us to reduce the cross-section-induced uncertainty of the void reactivity of the accelerator-driven system from 6.3% to 4.8%, achieving a provisional target accuracy of 5% in this study. Furthermore, we demonstrated that the uncertainties arising from other dominant factors, such as minor actinides and steel, can be effectively reduced by using integral experimental data sets for the unified cross-section dataset ADJ2017.

Journal Articles

Numerical study of initiating phase of core disruptive accident in small sodium-cooled fast reactors with negative void reactivity

Ishida, Shinya; Fukano, Yoshitaka; Tobita, Yoshiharu; Okano, Yasushi

Journal of Nuclear Science and Technology, 61(5), p.582 - 594, 2024/05

 Times Cited Count:1 Percentile:27.70(Nuclear Science & Technology)

Journal Articles

TRU oxide sample reactivity worths measured in the FCA-IX assemblies with systematically changed neutron energy spectra

Fukushima, Masahiro; Okajima, Shigeaki*; Mukaiyama, Takehiko*

Journal of Nuclear Science and Technology, 61(4), p.478 - 497, 2024/04

 Times Cited Count:3 Percentile:65.16(Nuclear Science & Technology)

A series of integral experiments was conducted to evaluate the fission and the capture cross- sections of transuranic (TRU) nuclides at the fast critical facility FCA of the Japan Atomic Energy Agency (JAEA). The experiments were carried out using seven uranium-fueled assemblies of the FCA. The neutron energy spectra of the core regions were adjusted so as to change from an intermediate neutron spectrum to a fast neutron spectrum on an assembly-by-assembly basis. The integral data measured with these experimental configurations provide some neutron energy characteristics: 1) fission rate ratios (FRRs) of $$^{237}$$Np, $$^{238}$$Pu, $$^{242}$$Pu, $$^{241}$$Am, $$^{243}$$Am, and $$^{244}$$Cm relative to $$^{239}$$Pu by using absolutely calibrated fission chambers, 2) small sample reactivity worths (SRWs) of $$^{237}$$Np, $$^{238}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, and $$^{243}$$Am where oxide powders of around 15 to 20 grams were used, 3) criticalities, and 4) spectral indices such as fission rate ratios of $$^{238}$$U relative to $$^{235}$$U. In this paper, details of the SRW measurements are reported, and the latest Japanese Evaluated Nuclear Data Library JENDL-5 is tested by using the integral data obtained in systematically varied neutron energy spectra.

Journal Articles

Preliminary study of the criticality monitoring method based on the simulation for the activity ratio of short half-life noble-gas fission products from fuel debris

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi; Kanno, Ikuo

Journal of Nuclear Science and Technology, 61(2), p.269 - 276, 2024/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

High-temperature rupture failure of high-burnup LWR-MOX fuel under a reactivity-initiated accident condition

Taniguchi, Yoshinori; Mihara, Takeshi; Kakiuchi, Kazuo; Udagawa, Yutaka

Annals of Nuclear Energy, 195, p.110144_1 - 110144_11, 2024/01

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Radioactivity estimation of multiple radiation sources using a Compton camera to investigate radioactively contaminated objects

Sato, Yuki

Applied Radiation and Isotopes, 203, p.111083_1 - 111083_9, 2024/01

 Times Cited Count:2 Percentile:49.11(Chemistry, Inorganic & Nuclear)

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities, 2

Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro

JAEA-Data/Code 2023-011, 32 Pages, 2023/11

JAEA-Data-Code-2023-011.pdf:0.93MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{235}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.

Journal Articles

Void reactivity in lead and bismuth sample reactivity experiments at Kyoto University Critical Assembly

Pyeon, C. H.*; Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro

Nuclear Science and Engineering, 197(11), p.2902 - 2919, 2023/11

 Times Cited Count:2 Percentile:49.11(Nuclear Science & Technology)

Sample reactivity and void reactivity experiments are carried out in the solid-moderated and solid-reflected cores at the Kyoto University Critical Assembly (KUCA) with the combined use of aluminum (Al), lead (Pb) and bismuth (Bi) samples, and Al spacers simulating the void. MCNP6.2 eigenvalue calculations together with JENDL-4.0 provide good accuracy of sample reactivity with the comparison of experimental results; also experimental void reactivity is attained by using MCNP6.2 together with JENDL-4.0 and ENDF/B-VII.1 with a marked accuracy of relative difference between experiments and calculations. Uncertainty quantification of sample reactivity and void reactivity is acquired by using the sensitivity coefficients based on MCNP6.2/ksen and covariance library data of SCALE6.2 together with ENDF/B-VII.1, arising from the impact of uncertainty induced by Al, Pb and Bi cross sections. A series of reactivity analyses with the Al spacer simulating the void demonstrates the means of analyzing the void in the solid-moderated and solid-reflected cores at KUCA

Journal Articles

Evaluation of thermal expansion reactivity feedback effect in water-moderated fuel-particle-dispersion system

Fukuda, Kodai

Proceedings of 4th Reactor Physics Asia Conference (RPHA2023) (Internet), 4 Pages, 2023/10

Brief evaluations were performed using the N-F model to quantitatively clarify the effect of thermal expansion on the consequences of criticality accidents in the water-moderated fuel-particle-dispersion system. The analysis clarified that ignoring thermal expansion can lead to underestimation or overestimation of the consequences by several tens of percent. It is concluded that evaluators can ignore the thermal expansion when they evaluate the consequences of the prompt supercritical transient in water-moderated solid fuel-dispersion systems, such as fuel debris systems. Only the Doppler effect can be considered when the fuel-temperature-feedback coefficient is prepared. However, depending on the required accuracy, the evaluators should take care of the error caused by ignoring thermal expansion.

Journal Articles

Elemental analysis and radioactivity evaluation of aerosols generated during heating of simulated fuel debris; The Urasol project in the framework of Fukushima Daiichi fuel debris removal

Tsubota, Yoichi; Porcheron, E.*; Journeau, C.*; Delacroix, J.*; Suteau, C.*; Lallot, Y.*; Bouland, A.*; Roulet, D.*; Mitsugi, Takeshi

Proceedings of International Conference on Environmental Remediation and Radioactive Waste Management (ICEM2023) (Internet), 6 Pages, 2023/10

In order to safely remove fuel debris from the Fukushima Daiichi Nuclear Power Station (1F), it is necessary to quantitatively evaluate radioactive airborne particulate generated by the cutting of nuclear fuel debris. We fabricated Uranium-bearing simulated fuel debris (SFD) with In/Ex-Vessel compositions and evaluated the physical and chemical properties of aerosols generated by heating the SFDs. Based on these results, we estimated the isotopic composition and radioactivity of aerosols produced when 1F-Unit2 fuel debris is laser cut, which is a typical example of a heating method. Plutonium, mainly $$^{238}$$Pu,$$^{241}$$Am, and $$^{244}$$Cm were found to be the alpha nuclide, and $$^{241}$$Pu, $$^{137}$$Cs-Ba, and $$^{90}$$Sr-Y were found to be the beta nuclide of interest.

Journal Articles

Radiation imaging of a highly contaminated filter train inside Fukushima Daiichi Nuclear Power Station Unit 2 using an integrated Radiation Imaging System based on a Compton camera

Sato, Yuki; Terasaka, Yuta

Journal of Nuclear Science and Technology, 60(8), p.1013 - 1026, 2023/08

 Times Cited Count:12 Percentile:97.39(Nuclear Science & Technology)

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-2, JRR-3 and Hot laboratory

Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; Konda, Miki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2023-002, 81 Pages, 2023/05

JAEA-Data-Code-2023-002.pdf:3.0MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2, JRR-3 and Hot laboratory facilities. In this report, we summarized the radioactivity concentrations of 20 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{99}$$Tc, $$^{rm 108m}$$Ag, $$^{129}$$I, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2020.

Journal Articles

Development of transient behavior analysis code for metal fuel fast reactor during initiating phase of core disruptive accident

Ota, Hirokazu*; Ogata, Takanari*; Yamano, Hidemasa; Futagami, Satoshi; Shimada, Sadae*; Yamada, Yumi*

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 8 Pages, 2023/05

Journal Articles

JAEA-JRC collaborative development of delayed gamma-ray spectroscopy for nuclear safeguards nuclear material accountancy

Rodriguez, D.; Abbas, K.*; Bertolotti, D.*; Bonaldi, C.*; Fontana, C.*; Fujimoto, Masami*; Geerts, W.*; Koizumi, Mitsuo; Macias, M.*; Nonneman, S.*; et al.

Proceedings of INMM & ESARDA Joint Annual Meeting 2023 (Internet), 8 Pages, 2023/05

Journal Articles

JAEA/ISCN delayed gamma-ray spectroscopy inverse Monte Carlo development status

Rodriguez, D.; Rossi, F.

Proceedings of INMM & ESARDA Joint Annual Meeting 2023 (Internet), 9 Pages, 2023/05

Journal Articles

Validation of feedback reactivity evaluation models for plant dynamics analysis code during unprotected loss of heat sink event in sodium-cooled fast reactors

Yoshimura, Kazuo; Doda, Norihiro; Igawa, Kenichi*; Tanaka, Masaaki; Yamano, Hidemasa

Journal of Nuclear Engineering and Radiation Science, 9(2), p.021601_1 - 021601_9, 2023/04

Feedback reactivity automatically caused by radial expansion of the core is known as one of the inherent safety features in a sodium-cooled fast reactor (SFR). In order to validate the evaluation models of the reactivity feedback equipped in the in-house plant dynamics analysis code named Super-COPD, the benchmark analyses for the unprotected loss of heat sink (ULOHS) tests of BOP-302R and BOP-301 in an experimental SFR, EBR-II were conducted and the applicability of the evaluation method for the reactivity feedback was indicated during the ULOHS even, by comparing the numerical results and the experimental data.

Journal Articles

Iron-induced association between selenium and humic substances in groundwater from deep sedimentary formations

Terashima, Motoki; Endo, Takashi*; Kimuro, Shingo; Beppu, Hikari*; Nemoto, Kazuaki*; Amano, Yuki

Journal of Nuclear Science and Technology, 60(4), p.374 - 384, 2023/04

 Times Cited Count:2 Percentile:30.61(Nuclear Science & Technology)

451 (Records 1-20 displayed on this page)