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Journal Articles

Regional distribution and isotope ratios of radiocesium from the Fukushima Daiichi Nuclear Power Station and global fallout in Tokai-mura

Shimada, Asako; Tsukahara, Takehiko*; Nomura, Masao*; Shimada, Taro; Takeda, Seiji; Takahashi, Hiroaki*

Scientific Reports (Internet), 15(1), p.39024_1 - 39024_10, 2025/11

 Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)

Due to the accident at the Fukushima Daiichi Nuclear Power Station (FDNPS), radiocesium such as $$^{134}$$Cs, $$^{135}$$Cs, and $$^{137}$$Cs was dispersed over a wide area of eastern Japan and mixed with radiocesium from global fallout. The depth profiles of $$^{137}$$Cs for samples taken in 2003 before the FDNPS accident and in 2017 after the FDNPS accident in Tokai-mura (about 115 km NE of Tokyo) were both described by exponential equations from the surface up to a depth of 15 cm. Systematic grid sampling of surface soil at a depth of 5 cm was conducted at 3 sites in Tokai-mura in 2019, and distributions of the $$^{137}$$Cs concentration, $$^{134}$$Cs/$$^{137}$$Cs radioactivity ratio, and $$^{135}$$Cs/$$^{137}$$Cs isotope ratio were measured. It was found that the $$^{137}$$Cs concentration varied among sites and within individual sites, while the $$^{134}$$Cs/$$^{137}$$Cs radioactivity ratio was constant for all samples collected at 3 sites, 1.01$$pm$$0.04 (2$$sigma$$). The $$^{135}$$Cs/$$^{137}$$Cs isotope ratio for the two sites was constant and comparable to that obtained for soil sampled near FDNPS. On the other hand, the $$^{135}$$Cs/$$^{137}$$Cs isotope ratio. For the other site varied and showed higher values (0.355-0.446), suggesting the influence of global fallout. Based on the results, the mixture percentages of radiocesium originating from global fallout and the FDNPS accident were estimated.

JAEA Reports

Sampling of radioactive materials remaining in JMTR Reactor Facility

Ouchi, Takuya; Nagata, Hiroshi; Shinoda, Yuya; Yoshida, Hayato; Inoue, Shuichi; Chinone, Marina; Abe, Kazuyuki; Ide, Hiroshi; Watahiki, Shunsuke

JAEA-Technology 2025-006, 25 Pages, 2025/10

JAEA-Technology-2025-006.pdf:1.59MB

In the future, radioactive waste which generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried for the near surface disposal. It is necessary to establish the method to evaluate the radioactivity concentrations of the radioactive wastes. Therefore, at the Oarai Nuclear Engineering Institute, in order to contribute to the study of methods for evaluating radioactivity concentrations of the radioactive wastes from nuclear research facilities, samples were taken from radioactive waste that are expected to be buried in the future and radiochemical analysis is used to obtain data on the radioactivity concentration of each nuclide contained in the radioactive waste. This report presents the concept of selecting sample collection targets and summarizes the sampling of radioactive materials conducted at the JMTR reactor facility in fiscal years 2023 and 2024 to obtain data on radioactivity concentrations.

Journal Articles

High-temperature oxidation failure in reactivity-initiated accidents; An Evaluation of failure criteria based on oxygen concentration from the previous NSRR experiments

Luu, V. N.; Taniguchi, Yoshinori; Udagawa, Yutaka; Katsuyama, Jinya

Nuclear Engineering and Design, 442, p.114222_1 - 114222_15, 2025/10

 Times Cited Count:2 Percentile:83.88(Nuclear Science & Technology)

Journal Articles

Measurement of transient fission gas release from high-burnup MOX fuel under a simulated reactivity-initiated accident condition using fission gas dynamics testing technique

Taniguchi, Yoshinori; Urano, Kenta; Mihara, Takeshi; Udagawa, Yutaka; Kakiuchi, Kazuo; Katsuyama, Jinya

Proceedings of TopFuel 2025; Nuclear Reactor Fuel Performance Conference (Internet), p.1292 - 1301, 2025/10

Journal Articles

Preliminary study of diffusion and SP3 calculations in unstructured mesh geometry for core deformation reactivity evaluation on SFR

Kato, Shinya; Doda, Norihiro; Yokoyama, Kenji; Tanaka, Masaaki; Endo, Tomohiro*

Proceedings of 2025 International Congress on Advances in Nuclear Power Plants (ICAPP 2025) (Internet), 11 Pages, 2025/09

During a reactor power increase in ULOF and UTOP events in sodium-cooled fast reactors, core deformation due to thermal expansion of core elements is expected to cause a negative feed-back effect to suppress this power increase. An analytical evaluation method of core deformation reactivity for design is being developed in JAEA. However, the neutronics calculation module uses several approximations. This study aims to develop the detailed evaluation method as a reference neutron transport calculation code for confirmation of the validity of the calculated core deformation reactivity. Here, the two-dimensional finite volume method (FVM) code based on simplified P3 (SP3) approximation with unstructured mesh have been developed as the first step of the development. This paper describes the calculation theory of the FVM code, the procedure of introducing SP3 approximation into the code and the verification results of the functions developed.

JAEA Reports

Achievement of safety demonstration tests using HTTR; Loss of forced cooling test at 100% reactor power (30 MW)

Nagasumi, Satoru; Hasegawa, Toshinari; Nakagawa, Shigeaki; Kubo, Shinji; Iigaki, Kazuhiko; Shinohara, Masanori; Saikusa, Akio; Nojiri, Naoki; Saito, Kenji; Furusawa, Takayuki; et al.

JAEA-Research 2025-005, 23 Pages, 2025/07

JAEA-Research-2025-005.pdf:2.68MB

A safety demonstration test under abnormal operating conditions using the HTTR (High Temperature Engineering Test Reactor) was conducted to demonstrate safety features of the HTGRs (High Temperature Gas-cooled Reactors). Under a simulation of a control rod shutdown failure, all primary helium gas circulators were intentionally stopped during a steady-state operation at 100% reactor thermal power (30 MW), temporal changes of the reactor power and temperatures around the reactor pressure vessel (RPV) were obtained after the complete loss of forced heat removal from the reactor core. After the event (primary coolant flow stopped), the reactor power quickly decreased due to the negative reactivity feedback associated with the core temperature rise, and then the reactor power spontaneously shifted to a stable state of low power (about 1.2%) even after a recriticality. Heat dissipation from RPV surface to a surrounding vessel cooling system (water-cooled panels) ensured the amount of heat removal required to maintain the reactor temperature constant in the low power state. In this way, the transition from the event occurrence to the stable and safety state, i.e., inherent safety features of HTGRs, were demonstrated in the case of core forced cooling loss without active shutdown operations.

JAEA Reports

Detailed computational models for nuclear criticality analyses on the first startup cores of NSRR: A TRIGA annular core pulse reactor

Yanagisawa, Hiroshi; Motome, Yuiko

JAEA-Research 2025-001, 99 Pages, 2025/06

JAEA-Research-2025-001.pdf:1.98MB

The detailed computational models for nuclear criticality analyses on the first startup cores of NSRR (Nuclear Safety Research Reactor), which is categorized as a TRIGA-ACPR (Annular Core Pulse Reactor), were created for the purposes of deeper understandings of safety inspection data on the neutron absorber rod worths of reactivity and improvement of determination technique of the reactivity worths. The uncertainties in effective neutron multiplication factor (k$$_{rm eff}$$) propagated from errors in the geometry, material, and operation data for the present models were evaluated in detail by using the MVP version 3 code with the latest Japanese nuclear data library, JENDL-5, and the previous versions of JENDL libraries. As a result, the overall uncertainties in k$$_{rm eff}$$ for the present models were evaluated to be in the range of 0.0027 to 0.0029 $$Delta$$k$$_{rm eff}$$. It is expected that the present models will be utilized as the benchmark on k$$_{rm eff}$$ for TRIGA-ACPR. Moreover, it is confirmed that the overall uncertainties were sufficiently smaller than the values of absorber rod worths determined in NSRR. Thus, it is also considered that the present models are applicable to further analyses on the absorber rod worths in NSRR.

JAEA Reports

Investigation of measurement accuracy of burnup reactivity of accelerator-driven system during normal operation

Katano, Ryota; Abe, Takumi; Cibert, H.*

JAEA-Research 2024-019, 22 Pages, 2025/05

JAEA-Research-2024-019.pdf:1.03MB

An accelerator-driven system (ADS) dedicated to transmutation of minor actinides (MAs) is driven in subcritical states. It is important for establishment of the subcriticality control of ADS to predict the burnup reactivity. To validate the prediction accuracy, the burnup reactivity, especially at the first cycle, must be measured with sufficient accuracy. In this study, we focus on Current-To-Flux (CTF) method. We have simulated the burnup reactivity monitoring during the ADS normal operation with the CTF method by performing fixed-source-burnup calculations using a continuous energy Monte Carlo code SERPENT2 with some tallies that models in-core fission chambers and have estimated its measurement uncertainty. We have clarified that the 10% biases of measure burnup reactivities appear independently of the burnup duration and their detector position dependence is particularly small in the outer region of the system.

Journal Articles

Three-dimensional localization and radioactivity quantification of radiation sources through inverse estimation based on Compton camera measurements

Sato, Yuki

Radiation Protection Dosimetry, 201(7), p.490 - 500, 2025/05

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Large disequilibrium of $$^{234}$$U/$$^{238}$$U isotope ratios in deep groundwater and its potential application as a groundwater mixing indicator

Kuribayashi, Chika*; Miyakawa, Kazuya; Ito, Akane*; Tanimizu, Masaharu*

Geochemical Journal, 59(2), p.35 - 44, 2025/00

 Times Cited Count:2 Percentile:76.37(Geochemistry & Geophysics)

no abstracts in English

Journal Articles

Radioactivity estimation of radioactive hotspots using a Compton camera and derivation of dose rates in the surrounding environment

Sato, Yuki

Applied Radiation and Isotopes, 212, p.111421_1 - 111421_8, 2024/10

 Times Cited Count:2 Percentile:47.49(Chemistry, Inorganic & Nuclear)

Journal Articles

Impact of uncertainty reduction on lead-bismuth coolant in accelerator-driven system using sample reactivity experiments

Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro; Pyeon, C. H.*; Yamamoto, Akio*; Endo, Tomohiro*

Nuclear Science and Engineering, 198(6), p.1215 - 1234, 2024/06

 Times Cited Count:1 Percentile:14.77(Nuclear Science & Technology)

In this study, we have demonstrated that data assimilation using lead and bismuth sample reactivities measured in the Kyoto University Critical Assembly A-core can successfully reduce the uncertainty of the coolant void reactivity in accelerator-driven systems derived from inelastic-scattering cross-sections of lead and bismuth. We re-evaluated and highlighted the experimental uncertainties and correlations of the sample reactivities for the data assimilation formula. We used the MCNP6.2 code to evaluate the sample reactivities and their uncertainties, and performed data assimilation using the reactor analysis code system MARBLE. The high-sensitivity coefficients of the sample reactivities to lead and bismuth allowed us to reduce the cross-section-induced uncertainty of the void reactivity of the accelerator-driven system from 6.3% to 4.8%, achieving a provisional target accuracy of 5% in this study. Furthermore, we demonstrated that the uncertainties arising from other dominant factors, such as minor actinides and steel, can be effectively reduced by using integral experimental data sets for the unified cross-section dataset ADJ2017.

Journal Articles

Numerical study of initiating phase of core disruptive accident in small sodium-cooled fast reactors with negative void reactivity

Ishida, Shinya; Fukano, Yoshitaka; Tobita, Yoshiharu; Okano, Yasushi

Journal of Nuclear Science and Technology, 61(5), p.582 - 594, 2024/05

 Times Cited Count:1 Percentile:14.77(Nuclear Science & Technology)

Journal Articles

TRU oxide sample reactivity worths measured in the FCA-IX assemblies with systematically changed neutron energy spectra

Fukushima, Masahiro; Okajima, Shigeaki*; Mukaiyama, Takehiko*

Journal of Nuclear Science and Technology, 61(4), p.478 - 497, 2024/04

 Times Cited Count:4 Percentile:55.39(Nuclear Science & Technology)

A series of integral experiments was conducted to evaluate the fission and the capture cross- sections of transuranic (TRU) nuclides at the fast critical facility FCA of the Japan Atomic Energy Agency (JAEA). The experiments were carried out using seven uranium-fueled assemblies of the FCA. The neutron energy spectra of the core regions were adjusted so as to change from an intermediate neutron spectrum to a fast neutron spectrum on an assembly-by-assembly basis. The integral data measured with these experimental configurations provide some neutron energy characteristics: 1) fission rate ratios (FRRs) of $$^{237}$$Np, $$^{238}$$Pu, $$^{242}$$Pu, $$^{241}$$Am, $$^{243}$$Am, and $$^{244}$$Cm relative to $$^{239}$$Pu by using absolutely calibrated fission chambers, 2) small sample reactivity worths (SRWs) of $$^{237}$$Np, $$^{238}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, and $$^{243}$$Am where oxide powders of around 15 to 20 grams were used, 3) criticalities, and 4) spectral indices such as fission rate ratios of $$^{238}$$U relative to $$^{235}$$U. In this paper, details of the SRW measurements are reported, and the latest Japanese Evaluated Nuclear Data Library JENDL-5 is tested by using the integral data obtained in systematically varied neutron energy spectra.

Journal Articles

Preliminary study of the criticality monitoring method based on the simulation for the activity ratio of short half-life noble-gas fission products from fuel debris

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi; Kanno, Ikuo

Journal of Nuclear Science and Technology, 61(2), p.269 - 276, 2024/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

High-temperature rupture failure of high-burnup LWR-MOX fuel under a reactivity-initiated accident condition

Taniguchi, Yoshinori; Mihara, Takeshi; Kakiuchi, Kazuo; Udagawa, Yutaka

Annals of Nuclear Energy, 195, p.110144_1 - 110144_11, 2024/01

 Times Cited Count:2 Percentile:30.64(Nuclear Science & Technology)

Journal Articles

Radioactivity estimation of multiple radiation sources using a Compton camera to investigate radioactively contaminated objects

Sato, Yuki

Applied Radiation and Isotopes, 203, p.111083_1 - 111083_9, 2024/01

 Times Cited Count:7 Percentile:77.55(Chemistry, Inorganic & Nuclear)

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities, 2

Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro

JAEA-Data/Code 2023-011, 32 Pages, 2023/11

JAEA-Data-Code-2023-011.pdf:0.93MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{235}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.

Journal Articles

Void reactivity in lead and bismuth sample reactivity experiments at Kyoto University Critical Assembly

Pyeon, C. H.*; Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro

Nuclear Science and Engineering, 197(11), p.2902 - 2919, 2023/11

 Times Cited Count:3 Percentile:44.12(Nuclear Science & Technology)

Sample reactivity and void reactivity experiments are carried out in the solid-moderated and solid-reflected cores at the Kyoto University Critical Assembly (KUCA) with the combined use of aluminum (Al), lead (Pb) and bismuth (Bi) samples, and Al spacers simulating the void. MCNP6.2 eigenvalue calculations together with JENDL-4.0 provide good accuracy of sample reactivity with the comparison of experimental results; also experimental void reactivity is attained by using MCNP6.2 together with JENDL-4.0 and ENDF/B-VII.1 with a marked accuracy of relative difference between experiments and calculations. Uncertainty quantification of sample reactivity and void reactivity is acquired by using the sensitivity coefficients based on MCNP6.2/ksen and covariance library data of SCALE6.2 together with ENDF/B-VII.1, arising from the impact of uncertainty induced by Al, Pb and Bi cross sections. A series of reactivity analyses with the Al spacer simulating the void demonstrates the means of analyzing the void in the solid-moderated and solid-reflected cores at KUCA

Journal Articles

Evaluation of thermal expansion reactivity feedback effect in water-moderated fuel-particle-dispersion system

Fukuda, Kodai

Proceedings of 4th Reactor Physics Asia Conference (RPHA2023) (Internet), 4 Pages, 2023/10

Brief evaluations were performed using the N-F model to quantitatively clarify the effect of thermal expansion on the consequences of criticality accidents in the water-moderated fuel-particle-dispersion system. The analysis clarified that ignoring thermal expansion can lead to underestimation or overestimation of the consequences by several tens of percent. It is concluded that evaluators can ignore the thermal expansion when they evaluate the consequences of the prompt supercritical transient in water-moderated solid fuel-dispersion systems, such as fuel debris systems. Only the Doppler effect can be considered when the fuel-temperature-feedback coefficient is prepared. However, depending on the required accuracy, the evaluators should take care of the error caused by ignoring thermal expansion.

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