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JAEA Reports

Development of Environmental Mitigation Technology with Novel Water Purification Agents (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Shinshu University*

JAEA-Review 2021-051, 81 Pages, 2022/01


The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of environmental mitigation technology with novel water purification agents" conducted in FY2020. The present study aims to develop a reusable adsorbent for strontium ions through joint research between Japan and the United Kingdom, and to reduce the amount of used adsorbent generated through the decontamination process. The basic strategy of this research is to produce adsorbents and examine their Sr adsorption performance at Shinshu University. The structural analyses of the adsorbents are conducted by the Institute for Molecular Science (IMS) and the UK teams. The adsorption data and structural information are theoretically analyzed at Tohoku University with data science, leading to a new synthetic guid

Journal Articles

Direct quantitation of $$^{135}$$Cs in spent Cs adsorbent used for the decontamination of radiocesium-containing water by laser ablation inductively coupled plasma mass spectrometry

Asai, Shiho*; Ohata, Masaki*; Hanzawa, Yukiko; Horita, Takuma; Yomogida, Takumi; Kitatsuji, Yoshihiro

Analytical Chemistry, 92(4), p.3276 - 3284, 2020/02

 Times Cited Count:2 Percentile:41.67(Chemistry, Analytical)

The long-term safety assessment of spent Cs adsorbents produced during the decontamination of radiocesium-containing water at the Fukushima Daiichi Nuclear Power Plant requires one to estimate their $$^{135}$$Cs content prior to final disposal. $$^{135}$$Cs is usually quantified by inductively coupled plasma mass spectrometry (ICP-MS), which necessitates the elution of Cs from Cs adsorbents. However, this approach suffers from the high radiation dose from $$^{137}$$Cs. To address this challenge, we herein employed laser ablation ICP-MS for direct quantitation of $$^{135}$$Cs in Cs adsorbents and used a model Cs adsorbent prepared by immersion of a commercially available Cs adsorbent into radiocesium-containing liquid waste to verify the developed technique. The use of the $$^{135}$$Cs/$$^{137}$$Cs ratio and $$^{137}$$Cs radioactivity obtained by gamma spectrometry achieved simple and precise quantitation of $$^{135}$$Cs and the resulting $$^{135}$$Cs activity of 0.36 Bq agreed well with that in the original radiocesium-containing liquid waste.

Journal Articles

Characteristics of TPDN/SiO$$_{2}$$-P adsorbent for MA(III) recovery

Kofuji, Hirohide; Watanabe, So; Takeuchi, Masayuki; Suzuki, Hideya; Matsumura, Tatsuro; Shiwaku, Hideaki; Yaita, Tsuyoshi

Progress in Nuclear Science and Technology (Internet), 5, p.61 - 65, 2018/11

Journal Articles

Encapsulation of cesium from contaminated water with highly selective facial organic-inorganic mesoporous hybrid adsorbent

Awual, M. R.; Miyazaki, Yuji; Taguchi, Tomitsugu; Shiwaku, Hideaki; Yaita, Tsuyoshi

Chemical Engineering Journal, 291, p.128 - 137, 2016/05

 Times Cited Count:166 Percentile:99.43(Engineering, Environmental)

Journal Articles

A Reliable hybrid adsorbent for efficient radioactive cesium accumulation from contaminated wastewater

Awual, M. R.; Yaita, Tsuyoshi; Miyazaki, Yuji; Matsumura, Daiju; Shiwaku, Hideaki; Taguchi, Tomitsugu

Scientific Reports (Internet), 6, p.19937_1 - 19937_10, 2016/01


 Times Cited Count:132 Percentile:98.16(Multidisciplinary Sciences)

Journal Articles

Schiff based ligand containing nano-composite adsorbent for optical copper(II) ions removal from aqueous solutions

Awual, M. R.; Eldesoky, G. E.*; Yaita, Tsuyoshi; Naushad, M.*; Shiwaku, Hideaki; Alothman, Z. A.*; Suzuki, Shinichi

Chemical Engineering Journal, 279, p.639 - 647, 2015/11

 Times Cited Count:185 Percentile:99.32(Engineering, Environmental)

Journal Articles

A Sensitive ligand embedded nano-conjugate adsorbent for effective cobalt(II) ions capturing from contaminated water

Awual, M. R.; Yaita, Tsuyoshi; Shiwaku, Hideaki; Suzuki, Shinichi

Chemical Engineering Journal, 276, p.1 - 10, 2015/09

 Times Cited Count:126 Percentile:98.44(Engineering, Environmental)

Journal Articles

Comparative study of Sr adsorbents for radioactive contaminated water on severe accident

Takahatake, Yoko; Shibata, Atsuhiro; Nomura, Kazunori

Proceedings of 21st International Conference & Exhibition; Nuclear Fuel Cycle for a Low-Carbon Future (GLOBAL 2015) (USB Flash Drive), p.2099 - 2104, 2015/09

Journal Articles

Large-pore diameter nano-adsorbent and its application for rapid lead(II) detection and removal from aqueous media

Shahat, A.*; Awual, M. R.; Khaleque, M. A.*; Alam, M. Z.*; Naushad, M.*; Chowdhury, A. M. S*

Chemical Engineering Journal, 273, p.286 - 295, 2015/08

 Times Cited Count:221 Percentile:99.61(Engineering, Environmental)

Journal Articles

Functional ligand anchored nanomaterial based facial adsorbent for cobalt(II) detection and removal from water samples

Shahat, A.*; Awual, M. R.; Naushad, M.*

Chemical Engineering Journal, 271, p.155 - 163, 2015/07

 Times Cited Count:187 Percentile:99.39(Engineering, Environmental)

Journal Articles

Ultimate selenium(IV) monitoring and removal from water using a new class of organic ligand based composite adsorbent

Awual, M. R.; Yaita, Tsuyoshi; Suzuki, Shinichi; Shiwaku, Hideaki

Journal of Hazardous Materials, 291, p.111 - 119, 2015/06

 Times Cited Count:152 Percentile:98.7(Engineering, Environmental)

Journal Articles

A Novel facial composite adsorbent for enhanced copper(II) detection and removal from wastewater

Awual, M. R.

Chemical Engineering Journal, 266, p.368 - 375, 2015/04

 Times Cited Count:311 Percentile:99.8(Engineering, Environmental)

Journal Articles

Investigation of ligand immobilized nano-composite adsorbent for efficient cerium(III) detection and recovery

Awual, M. R.; Hasan, M. M.*; Shahat, A.*; Naushad, M.*; Shiwaku, Hideaki; Yaita, Tsuyoshi

Chemical Engineering Journal, 265, p.210 - 218, 2015/04

 Times Cited Count:179 Percentile:99.3(Engineering, Environmental)

Journal Articles

Organic-inorganic based nano-conjugate adsorbent for selective palladium(II) detection, separation and recovery

Awual, M. R.; Hasan, M. M.*; Znad, H.*

Chemical Engineering Journal, 259, p.611 - 619, 2015/01

 Times Cited Count:158 Percentile:99.03(Engineering, Environmental)

Journal Articles

Colorimetric detection and removal of copper(II) ions from wastewater samples using tailor-made composite adsorbent

Awual, M. R.; Hasan, M. M.*

Sensors and Actuators B; Chemical, 206, p.692 - 700, 2015/01

 Times Cited Count:178 Percentile:99.77(Chemistry, Analytical)

Journal Articles

Adsorption properties of styrenesulfonate-grafted fibrous metal adsorbent

Ueki, Yuji; Saiki, Seiichi; Seko, Noriaki

Nihon Ion Kokan Gakkai-Shi, 25(4), p.99 - 104, 2014/11

Journal Articles

Functionalized novel mesoporous adsorbent for selective lead(II) ions monitoring and removal from wastewater

Awual, M. R.; Hasan, M. M.*; Shahat, A.*

Sensors and Actuators B; Chemical, 203, p.854 - 863, 2014/11

 Times Cited Count:133 Percentile:99.17(Chemistry, Analytical)

Journal Articles

A Novel ligand based dual conjugate adsorbent for cobalt(II) and copper(II) ions capturing from water

Awual, M. R.; Yaita, Tsuyoshi; Okamoto, Yoshihiro

Sensors and Actuators B; Chemical, 203, p.71 - 80, 2014/11

 Times Cited Count:136 Percentile:99.2(Chemistry, Analytical)

Journal Articles

Mesoporous silica based novel conjugate adsorbent for efficient selenium(IV) detection and removal from water

Awual, M. R.; Hasan, M. M.*; Ihara, Toshihiro*; Yaita, Tsuyoshi

Microporous and Mesoporous Materials, 197, p.331 - 338, 2014/10

 Times Cited Count:133 Percentile:99.19(Chemistry, Applied)

Journal Articles

Novel conjugate adsorbent for visual detection and removal of toxic lead(II) ions from water

Awual, M. R.; Hasan, M. M.*

Microporous and Mesoporous Materials, 196, p.261 - 269, 2014/09

 Times Cited Count:177 Percentile:99.7(Chemistry, Applied)

33 (Records 1-20 displayed on this page)