Kinetic and thermodynamic controls on CsI-Mo gas-phase reactions under varying oxygen potentials

Shiotsu, Hiroyuki

Progress in Nuclear Energy, 195, p.106300_1 - 106300_11, 2026/05

https://doi.org/10.1016/j.pnucene.2026.106300

Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2025-048, 56 Pages, 2026/02

JAEA-Review-2025-048.pdf:2.89MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor" conducted in FY2023. The present study aims to develop a high-resolution imaging camera for alpha dust and a high-dose rate monitor. To realize the high-resolution imaging camera for alpha dust, we have developed novel scintillation materials with emission bands of 500-800 nm. Moreover, we have prepared several materials for the camera and software. We have also developed novel scintillation materials with emission bands of 650-1,000 nm, and simulation studies have been conducted for the high-dose-rate monitor system consisting of optical fiber. In addition, we demonstrated this monitoring system, and the dose-rate dynamic range was found to be 20 mSv/h to 1 kSv/h.

Development of an innovative n/ scintillation detection system for simple non-destructive measurements (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2025-046, 70 Pages, 2026/01

JAEA-Review-2025-046.pdf:5.46MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Development of an innovative n/ scintillation detection system for simple non-destructive measurements" conducted in FY2023. At 1F, removal of fuel debris from the primary containment vessel (PCV) is scheduled for FY2023, and a phased expansion of the removal scale is being considered in the future. As a solution to the above problem, this study will develop an innovative scintillation radiation detection system for screening and continuous monitoring during target sample removal. To develop a remote measurement system that contributes to in-vessel investigations for decommissioning of nuclear facilities such as 1F. More specifically, we will develop vertically integrated research into the following elemental technologies: (1) development of innovative high-performance scintillation materials for thermal neutron / gamma-ray discrimination (Tohoku University), (2) downsizing of censer and signal processing system (the University of Tokyo), (3) construction and characterization of various radiation fields (National Institute of Advanced Industrial Science and Technology), and (4) development of a simple non-destructive measurement system and hot cell demonstration test (JAEA). By vertically integrating elemental technologies, R&D on each research item planned in FY2023 was conducted to develop a detector that can discriminate gamma-ray and neutron radiation in environments exceeding 10 Gy/h and simultaneously identify the dose rate and nuclide of each in PCVs and in each acceptance cell.

Mutual separation of Ru, Rh, and Pd via reflux-assisted extraction and reverse-extraction using ion-pair and solvation with S- and amino-N-donor reagents

Sasaki, Yuji; Kaneko, Masashi; Matsumiya, Masahiko*; Kumagai, Yuta

Journal of Molecular Liquids, 441, p.129013_1 - 129013_10, 2026/01

https://doi.org/10.1016/j.molliq.2025.129013

This study determined extraction and back-extraction conditions for the mutual separation of three light PGMs, Ru, Rh, and Pd. Results revealed that reagents containing soft N and S donor atoms efficiently extract and strip Pd through solvation. In comparison, Ru and Rh undergo ion-pair extraction, requiring both anionic metal species and cationic extractants. These essential chlorinated PGM anions and protonated extractants having amino N atoms are present in HCl media. D(Ru) and D(Rh) values of approximately 100 and 10, respectively, were obtained using nitrilo-triacet-amide (NTAamide), which exhibits tetradentate coordination. Refluxing in 3-6 M HCl at 250 C, a condition that promotes the formation of highly chlorinated PGM anionic species, increased D(Ru) and D(Rh). Based on these findings, a flow diagram for the mutual separation of three PGMs was developed.

Research and development of remote optical measurement technology for PCV gas-phase leakage location and leakage volume estimation (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Chiba University*

JAEA-Review 2025-038, 84 Pages, 2025/12

JAEA-Review-2025-038.pdf:6.08MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Research and development of remote optical measurement technology for PCV gas-phase leakage location and leakage volume estimation" conducted in FY2023. The present study aims to locate leakage points using a remote optical measurement system including Lidar, and to develop a visualization method for leakage at those points. The Lidar can be distance-resolved in the line-of-sight direction and can separate and observe signals from walls and pipes in the building and surrounding gas-phase molecules (nitrogen N, water vapor HO, etc.) and suspended particles (aerosols). In addition, flash Lidar, which combines a laser beam with a high-sensitivity imaging sensor, and high-sensitivity shearography, which uses interference of light waves, are used to image and visualize the leakage location and to estimate the amount of leakage. Through comparison of these methods, we will clarify the positional resolution in locating the leakage point and the lower detection limit of the leakage amount that can be visualized.

Development of importance measures reflecting the risk triplet in dynamic probabilistic risk assessment; The Concept and measures of risk importance

Narukawa, Takafumi*; Takata, Takashi*; Zheng, X.; Tamaki, Hitoshi; Shibamoto, Yasuteru; Maruyama, Yu; Takada, Tsuyoshi

Journal of Nuclear Engineering (Internet), 6(4), p.49_1 - 49_14, 2025/12

https://doi.org/10.3390/jne6040049

Separation test of heat generating nuclides from high-level liquid waste

Hotoku, Shinobu; Ban, Yasutoshi; Konda, Miki; Kitatsuji, Yoshihiro

JAEA-Technology 2025-009, 33 Pages, 2025/11

JAEA-Technology-2025-009.pdf:1.9MB

High-level liquid waste (HLLW) produced from reprocessing of spent nuclear fuels contains heat generating nuclides such as Sr-90, Y-90, Cs-137, Ba-137m, and Am-241. Separation and recovery of these nuclides lead to reduce the volume and toxicity of high-level waste. Furthermore, the recovered nuclides and elements could be utilized as resources after purification. In this test, Sr separation by extraction chromatography using Sr resin and Pb resin, Cs separation by co-precipitation using ammonium phosphomolybdate (AMP), and Am separation by solvent extraction using alkyl diamideamine (ADAAM) were carried out, cold tests were performed for the separation of Cs and Sr in a nitric acid solution. Based on the results, hot tests were performed using dissolution solutions of spent fuel at the Nuclear Fuel Cycle Safety Engineering Research Facility (NUCEF), and each component contained in the separated solution was analyzed. In the Sr separation by extraction chromatography, most of Sr was separated from other elements using 8 mol/L nitric acid for absorption and 0.02 mol/L nitric acid for elution. In the separation of Cs, more than 99.9% of Cs was selectively co-precipitated by adding AMP to the HLLW, in which nitric acid concentration was adjusted to 3.1 mol/L. In solvent extraction of Am by ADAAM, 81.4% of Am-241 was recovered by a single stage batch experiment. Since Sr, Cs, and Am were properly separated and recovered from HLLW, the effectiveness of the present separation method was successfully demonstrated.

Development of inspection technology for pipes in high background radiation environments (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; University of Fukui*

JAEA-Review 2025-036, 88 Pages, 2025/11

JAEA-Review-2025-036.pdf:6.36MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Development of inspection technology for pipes in high background radiation environments" conducted in FY2023. The following two studies are being conducted with the aim of comprehensively developing technologies to address the three needs indicated in the hearing with TEPCO regarding observation of the inside of piping: (1) Hydrogen content, (2) Presence of precipitates, (3) Presence or absence of / radiation emitting nuclides. First, by downsizing existing nondestructive inspection equipment and developing a dedicated radiation detector capable of nondestructively imaging the inside of piping, we aim to obtain information on the inside of piping by nondestructive inspection using lasers, etc., and to clarify the presence or absence of -nuclides in piping and the internal conditions of piping, etc. In addition, we will develop equipment to visualize -nuclides and discriminate -nuclides in high dose rate environments, as well as technology to investigate the contents of the piping. Deployment of the developed technology is expected to be put into practical use by TEPCO and private companies.

Development and evaluation of a real-time 3D positioning embedded system combining wireless UWB and camera image analysis (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokai National Higher Education and Research System*

JAEA-Review 2025-023, 63 Pages, 2025/11

JAEA-Review-2025-023.pdf:5.74MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development and evaluation of a real-time 3D positioning embedded system combining wireless UWB and camera image analysis" conducted in FY2023. The present study aims to realize an embedded system that combines two of the latest popular technologies, "wireless UWB (Ultra Width Band)" and "multi-camera object recognition" with the goal of simple real-time 3D positioning with less than 10 cm accuracy by a human or robot for measuring air doses in nuclear reactor buildings. In this research, Gifu Univ. and National Institute of Technology, Fukushima College have developed an embedded system with camera shooting function, camera analysis function, and wireless communication function, in order to realize real-time 3D positioning based on the analysis of camera images by using these multiple devices. The Univ. of Tokyo and LocationMind Inc. will apply UWB real-time positioning technology to the inside of nuclear reactor buildings and attempt to develop technology to improve stability. Nagoya Univ. will be in charge of verifying wireless UWB stability from the hardware side by using electromagnetic wave absorbing materials. The radiation resistance evaluation will be conducted in cooperation with the JAEA and National Institute of Technology, Fukushima College.

Estimation of the beam trip frequency of a proton linear accelerator for an accelerator-driven nuclear transmutation system and comparison with the allowable beam trip frequency

Takei, Hayanori

Journal of Nuclear Science and Technology, 62(11), p.1051 - 1070, 2025/11

https://doi.org/10.1080/00223131.2025.2523023

The Japan Atomic Energy Agency is working on the research and development of an accelerator-driven nuclear transmutation system (ADS) for transmuting minor actinides. This system combines a subcritical nuclear reactor with a high-power superconducting proton linear accelerator (JADS-linac). One of the factors limiting the advancement of the JADS-linac is beam trips, which often induce thermal cycle fatigue, thereby damaging the components in the subcritical core. The average beam current of the JADS-linac is 32 times higher than that of the linear accelerator (linac) of the Japan Proton Accelerator Research Complex (J-PARC). Therefore, according to the development stage, comparing the beam trip frequency of the JADS-linac with the allowable beam trip frequency (ABTF) is necessary. Herein the beam trip frequency of the JADS-linac was estimated through a Monte Carlo program using the reliability functions based on the operational data of the J-PARC linac. The Monte Carlo program afforded the distribution of the beam trip duration, which cannot be obtained using traditional analytical methods. Results show that the frequency of the beam trips with a duration exceeding 5 min must be reduced to 27% of the current J-PARC linac level to be below the ABTF.