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Li, X.; Yamaji, Akifumi*; Sato, Ikken*; Yamashita, Takuya
Annals of Nuclear Energy, 214, p.111217_1 - 111217_13, 2025/05
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Fukuda, Kodai; Obara, Toru*; Suyama, Kenya
Nuclear Technology, 211(5), p.963 - 973, 2025/05
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Sayato, Natsuki; Otsuka, Kaoru; Fuyushima, Takumi; Endo, Yasuichi; Otsuka, Noriaki; Kitagishi, Shigeru; Tobita, Masahiro*; Isozaki, Futoshi*; Matsumoto, Satoshi*; Takemoto, Noriyuki
JAEA-Technology 2024-016, 247 Pages, 2025/02
Japan Materials Testing Reactor (JMTR, 50MW) was selected as a project to be subsidized by the Ministry of Education, Culture, Sports, Science and Technology (MEXT) for the "Establishment of an International Research and Development Center through Advanced Utilization of the World's Most Advanced Research Reactor". As part of this project, JMTR has installed "LWR Water Environment Simulation Tests" since 2010. This facility can control temperature, pressure, and water quality (dissolved oxygen, dissolved hydrogen, etc.) to simulate the water environment of light water reactors (BWR and PWR) and perform neutron irradiation of in-core structural materials, etc. In addition, this facility is also designed for PWR conditions. Chemical injection system for adding boron and lithium was added to the facility for PWR conditions. After the equipment was installed, test operation was carried out to confirm the performance of the facility. This report summarizes the establishment and test operation of LWR Water Environment Simulation Tests after the establishment.
Uchida, Shunsuke; Hata, Kuniki; Hanawa, Satoshi
JAEA-Data/Code 2024-003, 119 Pages, 2025/01
The calculation code for determining corrosive circumstance in light water reactors, WRAC-JAEA, has been developed based on water radiolysis calculation codes for BWR. The code has involved several new calculation functions to apply it for PWR, i.e., (1) high temperature pH (pH), (2) pH
effects on water radiolysis, (3) electrochemical corrosion potential (ECP) based on the mixed potential theory, and (4) ECP based on the water radiolysis calculation results. Moderation of corrosive conditions in the primary cooling systems is one of the promising procedures to mitigate the loss of reliabilities of major components in the systems, especially in aging plants. However, water chemistry control for corrosive environment mitigation procedures are much different in BWRs and PWRs. In BWRs, intergranular stress corrosion cracking (IGSCC) of stainless steel is the dominant causes for determining plant reliability. It is difficult to increase pH and injected hydrogen amounts due to direct power cycle operation. So, precise control of hydrogen injection with supported by water radiolysis and ECP analyses has been carried out to keep material reliability. In PWRs, it is possible to maintain stable control of corrosive circumstances with higher pH and sufficiently large hydrogen concentration. Recently, it was pointed out that one of the major causes of primary water stress corrosion cracking (PWSCC) of nickel alloys was hydrogen. The optimal hydrogen concentration should be evaluated to mitigate ECP without increasing hydrogen concentration. For this, a combined water radiolysis and ECP analysis code is required to determine the suitable hydrogen concentration and ECP. WRAC-JAEA can contribute not only to evaluation of corrosive conditions each of BWR and PWR, but also to prepare for suitable countermeasures for both BWR and PWR by cross-talking the knowledge and experience with assistance of the code results.
Fukuda, Kodai; Obara, Toru*
Nuclear Technology, 12 Pages, 2025/00
Li, X.; Yamaji, Akifumi*; Sato, Ikken*; Yamashita, Takuya; Nagae, Yuji
Proceedings of 11th European Review Meeting on Severe Accident Research Conference (ERMSAR 2024) (Internet), 12 Pages, 2024/05
Hata, Kuniki; Uchida, Shunsuke; Hanawa, Satoshi; Chimi, Yasuhiro; Sato, Tomonori
Proceedings of 21st International Conference on Environmental Degradation of Materials in Nuclear Power Systems - Water Reactors (Internet), 14 Pages, 2023/08
Sato, Ikken; Arai, Yuta*; Yoshikawa, Shinji
Journal of Nuclear Science and Technology, 58(4), p.434 - 460, 2021/04
Times Cited Count:7 Percentile:62.34(Nuclear Science & Technology)Udagawa, Yutaka; Mihara, Takeshi; Taniguchi, Yoshinori; Kakiuchi, Kazuo; Amaya, Masaki
Annals of Nuclear Energy, 139, p.107268_1 - 107268_9, 2020/05
Times Cited Count:3 Percentile:27.12(Nuclear Science & Technology)Udagawa, Yutaka; Sugiyama, Tomoyuki; Amaya, Masaki
Journal of Nuclear Science and Technology, 56(12), p.1063 - 1072, 2019/12
Times Cited Count:8 Percentile:58.81(Nuclear Science & Technology)no abstracts in English
Li, X.; Sato, Ikken; Yamaji, Akifumi*
Annals of Nuclear Energy, 133, p.21 - 34, 2019/11
Times Cited Count:6 Percentile:47.74(Nuclear Science & Technology)Kasahara, Shigeki; Chimi, Yasuhiro; Hata, Kuniki; Fukuya, Koji*; Fujii, Katsuhiko*
Proceedings of 19th International Conference on Environmental Degradation of Materials in Nuclear Power Systems - Water Reactors (Internet), p.1345 - 1355, 2019/08
This paper describes empirical equation development of crack growth rates (CGR) in consideration of IASCC of neutron irradiated stainless steel to contribute to structural integrity assessment of BWR reactor internals. Empirical equations of CGR (da/dt) were developed based on a formula of da/dt = MK
, assuming that "M" and "n" tend to be saturated with increasing neutron fluence. To obtain the empirical equations for normal water chemistry (NWC) and hydrogen water chemistry (HWC) of BWR, a data fitting with least square method was applied to the datasets consisting of F, K and CGR from post irradiation examinations of neutron irradiated stainless steel under simulated NWC and HWC conditions from open literature. As a result, calculated results by the equation for NWC showed good agreement with measured CGR data, meanwhile those for HWC did not. The above difference was seemed to be attributed that CGR data obtained under HWC conditions were scattered extensively.
Fukuya, Koji*; Fujii, Katsuhiko*; Chimi, Yasuhiro; Hata, Kuniki
Proceedings of 19th International Conference on Environmental Degradation of Materials in Nuclear Power Systems - Water Reactors (Internet), p.523 - 531, 2019/08
For structural integrity assessment on reactor internals of light water reactors, empirical equations of tensile properties as a function of neutron dose, and trend curves of stress-strain relations of neutron-irradiated austenitic stainless steels was proposed by fitting to recently developed database. The data in the database were obtained from reports of national projects in Japan and open literature, which was summarized in the form of data sheets. The empirical equations for tensile properties were formulated by using a saturation-type formulae. The equations were for CW 316 and SA 304/316 stainless steels in the temperature range of 280-350C and the dose range up to 80 dpa. Stress-strain relation curves were reproduced based on the Swift model. Obtained calculated results by the empirical equations and stress-strain relations were reasonably well fitted to experimental data. The effects of composition and cold-working, etc. on tensile properties were discussed.
Sato, Ikken
Journal of Nuclear Science and Technology, 56(5), p.394 - 411, 2019/05
Times Cited Count:12 Percentile:73.30(Nuclear Science & Technology)Water columns were adopted in the pressure measurement system of Fukushima-Daiichi Unit-3. Part of these water columns evaporated during the accident condition jeopardizing correct understanding on actual pressure. Through comparison of RPV (Reactor Pressure Vessel) and S/C pressures with D/W pressure, such water-column effect was evaluated. Correction for this effect was developed enabling clarification of slight pressure difference among RPV, S/C and D/W. This information was then integrated with other available data such as, water level, CAMS and environmental dose rate, into an interpretation of accident focusing on RPV and PCV pressurization/depressurization and radioactive material release to environment. It is suggested that dryout of in-vessel and ex-vessel debris was likely causing pressure decrease. S/C water poured into pedestal heated by relocated debris was the likely cause of pressurization. Cyclic reflooding of pedestal debris and dryout was likely.
Ueno, Fumiyoshi
Zairyo To Kankyo, 68(1), p.2 - 8, 2019/01
It is important to control the cooling water of light water reactors (boiling water reactor and pressurized water reactor) to suitable quality in order to reduce corrosion of structural materials and generation of radioactive corrosion products. For that purpose, monitoring of water quality using electrochemical measurement method is necessary. In this article, the application of ECP measurement to BWR is mainly focused, I describe the water quality of light water reactors and the necessity of electrochemical measurement.
Yamamoto, Masahiro; Soma, Yasutaka; Igarashi, Takahiro; Ueno, Fumiyoshi
Proceedings of Annual Congress of the European Federation of Corrosion (EUROCORR 2018) (USB Flash Drive), 7 Pages, 2018/09
In order to clarify the SCC behavior of SUS316L under BWR environment, mass transfer inside crevice of SUS316L in high temperature water using various crevice gap samples was investigated. The samples were prepared by put together two SUS316L sheets. Crevice gap differs from 0.005 mm to 0.1 mm. Corrosion tests were conducted in 8 ppm dissolved oxygen (DO) conditions. Surface oxide film was analysed by laser Raman spectroscopy (LRS) after immersion. Numerical simulations were also conducted by using COMSOL Maltiphysics. Diffusion process of DO and the other chemical species were calculated with connected to electrochemical process. Electrical conductivities inside the crevice were 100 times larger than these of outer water. The reason of high conductivity is existence of Fe ions at the DO depletion crevice.
Soma, Yasutaka; Komatsu, Atsushi; Ueno, Fumiyoshi
Zairyo To Kankyo, 67(9), p.381 - 385, 2018/09
In-situ measurement of electrical conductivity of solution within crevice of SUS316L stainless steel in 288C water has been conducted with newly developed electrochemical sensor system. The sensor measures local electrical conductivity of crevice solution beneath the electrode (
) with electrochemical impedance method. The sensors were installed at different positions within tapered crevice of SUS316L stainless steel. The crevice specimen with the sensors were immerged into 288
C, 8 MPa, pure oxygen saturated high purity water for 100 h.
at a position with crevice gap of
59.3
m was 8-11
S/cm, least deviate from conductivity of 288
C pure water (4.4
S/cm) and no localized corrosion occurred. On the contrary,
at a position with crevice gap of
4.4
m increased with time and showed maximum value of
1600
S/cm at 70 h. Localized corrosion occurred in the vicinity of this position. Thermodynamic equilibrium calculation showed
of 1600
S/cm being equivalent to pH of 3 to 3.7. It can be concluded that acidification occurred in tight crevice even under high purity bulk water and resulted in localized corrosion.
Kurata, Masaki; Barrachin, M.*; Haste, T.*; Steinbrueck, M.*
Journal of Nuclear Materials, 500, p.119 - 140, 2018/03
Times Cited Count:33 Percentile:62.98(Materials Science, Multidisciplinary)Severe accidents occurred at the Fukushima-Daiichi Nuclear Power Station (FDNPS) required an immediate re-examination of fuel degradation phenomenology. The present paper reviews the updated knowledge on the phenomenology of the fuel degradation, focusing mainly on the BWR fuel assembly degradation at the macroscopic scale and that of the individual interactions at the meso-scale. Oxidation of boron carbide (BC) control rods potentially generate far larger amounts of heat and hydrogen under BWR accident conditions. All integral tests with B
C control rods or control blades have shown early failure, liquefaction, relocation and oxidation of B
C starting at temperatures around 1250
C, well below the significant interaction temperatures of UO
-Zry. These interactions or reactions potentially influence the progress of fuel degradation in the early phase. The steam-starved conditions, which are being discussed as a likely scenario at the FDNPS accident, highly influence the individual interactions and potentially lead the fuel degradation in non-prototypical directions. The detailed phenomenology of individual interactions and their influence on the transient and on the late phase of the severe accidents are also discussed.
Tada, Kenichi; Kikuchi, Takeo*; Sakino, Takao; Suyama, Kenya
Journal of Nuclear Science and Technology, 55(2), p.138 - 150, 2018/02
Times Cited Count:3 Percentile:25.74(Nuclear Science & Technology)The criticality safety of the fuel debris in Fukushima Daiichi Nuclear Power Plant is one of the most important issues and the adoption of the burnup credit is desired for the criticality analysis. The assay data of used nuclear fuel irradiated in 2F2 is evaluated to validate SWAT4.0 for BWR fuel burnup problem. The calculation results revealed that number density of many heavy nuclides and FPs showed good agreement with the experimental data except for U,
Np,
Pu and Sm isotopes. The cause of the difference is assumption of the initial number density and void ratio and overestimation of the capture cross section of
Np. The C/E-1 values do not depend on the types of fuel rods (UO
or UO
-Gd
O
) and it is similar to that for the PWR fuel. These results indicate that SWAT4.0 appropriately analyzes the isotopic composition of the BWR fuel and it has sufficient accuracy to be adopted in the burnup credit evaluation of the fuel debris.
Chimi, Yasuhiro; Kasahara, Shigeki; Seto, Hitoshi*; Kitsunai, Yuji*; Koshiishi, Masato*; Nishiyama, Yutaka
Proceedings of the 18th International Conference on Environmental Degradation of Materials in Nuclear Power Systems - Water Reactors, Vol.2, p.1039 - 1054, 2018/00
Times Cited Count:2 Percentile:53.34(Materials Science, Multidisciplinary)In order to understand irradiation-assisted stress corrosion cracking (IASCC) growth behavior, crack growth rate (CGR) tests have been performed in simulated Boiling Water Reactor water conditions at 288
C on neutron-irradiated 316L stainless steels (SSs) at
12-14 dpa. After the tests, the microstructures near the crack tip of the specimens are examined with scanning transmission electron microscope (FE-STEM). In comparison with a previous study at
2 dpa, this result shows a less benefit of low electrochemical corrosion potential (ECP) conditions on CGR. A crack tip immersed over 1000 hours was filled with oxides, while almost no oxide film was observed near the crack front in the low-ECP conditions. In addition, a high density of deformation twins and dislocations were found near the fracture surface of the crack front. It is considered that both localized deformation and oxidation are possible dominant factors for the SCC growth in highly irradiated SSs.