Kubo, Kotaro; Jang, S.*; Takata, Takashi*; Yamaguchi, Akira*
Journal of Nuclear Science and Technology, 59(3), p.357 - 367, 2022/03
Dynamic probabilistic risk assessment (PRA), which handles epistemic and aleatory uncertainties by coupling the thermal-hydraulics simulation and probabilistic sampling, enables a more realistic and detailed analysis than conventional PRA. However, enormous calculation costs are incurred by these improvements. One solution is to select an appropriate sampling method. In this paper, we applied the Monte Carlo, Latin hypercube, grid-point, and quasi-Monte Carlo sampling methods to the dynamic PRA of a station blackout sequence in a boiling water reactor and compared each method. The result indicated that quasi-Monte Carlo sampling method handles the uncertainties most effectively in the assumed scenario.
Yoshida, Kazuo; Tamaki, Hitoshi; Hiyama, Mina*
JAEA-Research 2021-013, 20 Pages, 2022/01
An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. An idea has been proposed to implement a steam condenser as an accident countermeasure. This measure is expected to prevent nitric acid steam diffusing in facility building and to increase gaseous Ru trapping ratio into condensed water. A simulation study has been carried out with a hypothetical typical facility building to analyze the efficiency of steam condenser. In this study, SCHERN computer code simulates chemical behaviors of Ru in nitrogen oxide, nitric acid and water mixed vapor based on the conditions obtained from simulation with thermal-hydraulic computer code MELCOR. The effectiveness of steam condenser has been analyzed quantitively in preventing mixed vapor diffusion and gaseous Ru trapping effect. Some issues to be solved in analytical model has been also clarified in this study.
Yoshida, Naoki; Ono, Takuya; Yoshida, Ryoichiro; Amano, Yuki; Abe, Hitoshi
JAEA-Research 2021-011, 12 Pages, 2022/01
In boiling and drying accidents involving high-level liquid waste in fuel reprocessing plants, emphasis is placed on the behavior of ruthenium (Ru). Ru would form volatile species, such as ruthenium tetroxide (RuO), and could be released to the environment with coexisting gases, including nitric acid, water, or nitrogen oxides. In this study, to contribute toward safety evaluations of these types of accidents, the migration behavior of gaseous Ru into the liquid phase has been experimentally measured by simulating the condensate during an accident. The gas absorption of RuO was enhanced by increasing the nitrous acid (HNO) concentration in the liquid phase, indicating the occurrence of chemical absorption. In control experiments without HNO, the lower the temperature, the greater was the Ru recovery ratio in the liquid phase. Conversely, in experiments with HNO, the higher the temperature, the higher the recovery ratio, suggesting that the reaction involved in chemical absorption was activated at higher temperatures.
Okawa, Tomio*; Mori, Shoji*; Liu, W.*; Ose, Yasuo*; Yoshida, Hiroyuki; Ono, Ayako
Nihon Genshiryoku Gakkai-Shi ATOMO, 63(12), p.820 - 824, 2021/12
The evaluation method of the critical heat flux based on the mechanism is needed for the efficient design and development of fuel in reactors and the appropriate safety evaluation. In this paper, the current researches relating to the mechanism of the critical heat flux are reviewed, and the issue to be considered in the future are discussed.
Yoshida, Kazuo; Tamaki, Hitoshi; Hiyama, Mina*
JAEA-Research 2021-005, 25 Pages, 2021/08
An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. Accurate quantitative estimation of released Ru is one of the important issues for risk assessment of those facilities. To resolve this issue, an empirical correlation equation of Ru mass transfer coefficient across the vapor-liquid surface, which can be useful for quantitative simulation of Ru mitigating behavior, has been obtained from data analyses of small-scale experiments conducted to clarify gaseous Ru migrating behavior under steam-condensing condition. A simulation study has been also carried out with a hypothetical typical facility building successfully to demonstrate the feasibility of quantitative estimation of amount of Ru migrating in the facility using the obtained correlation equation implemented in SCHERN computer code which simulates chemical behaviors of nitrogen oxide based on the condition also simulated thermal-hydraulic computer code.
Yoshida, Kazuo; Tamaki, Hitoshi; Hiyama, Mina*
JAEA-Data/Code 2021-008, 35 Pages, 2021/08
An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. In addition to this, nitrogen oxides (NO) are also released formed by the thermal decomposition of metal nitrates of fission products (FP) in HLLW. It has been observed experimentally that NOx affects to the migration behavior of Ru at the anticipated atmosphere condition in cells and/or compartments of the facility building. Chemical reactions of NO with water and nitric acid are also recognized as the complex phenomena to undergo simultaneously in the vapor and liquid phases. The analysis program, SCHERN has been under developed to simulate chemical behavior including Ru coupled with the thermo-hydraulic condition in the flow paths in the facility building. This technical guide for SCHERN-V2 presents the overview of covered accident, analytical models including newly developed models, differential equations for numerical solution, and user instructions.
Saito, Shimpei*; De Rosis, A.*; Fei, L.*; Luo, K. H.*; Ebihara, Kenichi; Kaneko, Akiko*; Abe, Yutaka*
Physics of Fluids, 33(2), p.023307_1 - 023307_21, 2021/02
A Boiling phenomenon in a liquid flow field is known as forced-convection boiling. We numerically investigated the boiling system on a cylinder in a flow at a saturated condition. To deal with such a phenomenon, we developed a numerical scheme based on the pseudopotential lattice Boltzmann method. The collision was performed in the space of central moments (CMs) to enhance stability for high Reynolds numbers. Furthermore, additional terms for thermodynamic consistency were derived in a CMs framework. The effectiveness of the model was tested against some boiling processes, including nucleation, growth, and departure of a vapor bubble for high Reynolds numbers. Our model can reproduce all the boiling regimes without the artificial initial vapor phase. We found that the Nukiyama curve appears even though the focused system is the forced-convection system. Also, our simulations support experimental observations of intermittent direct solid-liquid contact even in the film-boiling regime.
Ono, Ayako; Sakashita, Hiroto*; Yoshida, Hiroyuki
Heat Transfer Engineering, 42(21), p.1775 - 1788, 2021/00
In this study, the macrolayer formation model is proposed to predict the critical heat flux in the saturated and subcooled pool boiling based on the macrolayer dryout model. This model concept is based on the results of the previous experiments. In the model, the nucleation site is assumed to distribute based on the Poisson distribution. Combining the proposed macrolayer formation model and macrolayer dryout model, the CHFs up to subcooling 40K were predicted and they are successfully good agreement with the experimental data. Moreover, the concept of the model was confirmed by the numerical simulation using the TPFIT.
Yoshida, Naoki; Amano, Yuki; Ono, Takuya; Yoshida, Ryoichiro; Abe, Hitoshi
JAEA-Research 2020-014, 33 Pages, 2020/12
Considering the boiling and drying accident of high-level liquid waste in fuel reprocessing plant, Ruthenium (Ru) is an important element. It is because Ru would form volatile compounds such as ruthenium tetroxide (RuO) and could be released into the environment with other coexisting gasses such as nitric oxides (NOx) such as nitric oxide (NO) and nitrogen dioxide (NO). To contribute to the safety evaluation of this accident, we experimentally evaluated the effect of NOx on the decomposition and chemical change behavior of the gaseous RuO (RuO(g)). As a result, the RuO(g) decomposed over time under the atmospheric gasses with NO or NO, however, the decomposition rate was slower than the results of experiments without NOx. These results showed that the NOx stabilized RuO(g).
Ioka, Ikuo; Kuriki, Yoshiro*; Iwatsuki, Jin; Kawai, Daisuke*; Yokota, Hiroki*; Inagaki, Yoshiyuki; Kubo, Shinji
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 5 Pages, 2020/08
A thermochemical water-splitting iodine-sulfur processes (IS process) is one of candidates for the large-scale production of hydrogen using heat from solar power. Severe corrosive environment which is thermal decomposition of sulfuric acid exists in the IS process. A hybrid material with the corrosion-resistance and the ductility was made by a plasma spraying and laser treatment. The specimen had excellent corrosion resistance in the condition of 95 mass% boiling sulfuric acid. This was attributed to the formation of SiO on the surface. The container using the hybrid material was experimentally made. The pre-oxidized container using hybrid technique was prepared for the corrosion test in boiling sulfuric acid to evaluate the corrosion characteristics of the container. There was no detaching of the surface with the weld part and the R processing. We proposed the calculation method of corrosion rate from the ions dissolved in the sulfuric acid solution after the corrosion test.
Lu, K.; Katsuyama, Jinya; Li, Y.
Proceedings of ASME 2020 Pressure Vessels and Piping Conference (PVP 2020) (Internet), 10 Pages, 2020/08
Miwa, Shuhei; Takase, Gaku; Imoto, Jumpei; Nishioka, Shunichiro; Miyahara, Naoya; Osaka, Masahiko
Journal of Nuclear Science and Technology, 57(3), p.291 - 300, 2020/03
For the evaluation of transport behavior of control material boron in a severe accident of BWR from the viewpoint of chemical effects on cesium and iodine behavior, boron chemistry during transportation in the high temperature region above 400 K was experimentally investigated. The heating tests of boron oxide specimen were conducted using the dedicated experimental apparatus reproducing fission product release and transport in steam atmosphere. Released boron oxide vapor was deposited above 1,000 K by the condensation onto stainless steel. The boron deposits and/or vapors significantly reacted with stainless steel above 1,000 K and formed the stable iron-boron mixed oxide (FeO)BO. These results indicate that released boron from degraded BWR control blade in a severe accident could remain in the high temperature region such as a Reactor Pressure Vessel. Based on these results, it can be said that the existence of boron deposits in the high temperature region would decrease the amount of transported cesium vapors from a Reactor Pressure Vessel due to possible formation of low volatile cesium borate compounds by the reaction of boron deposits with cesium vapors.
Koizumi, Yasuo*; Uesawa, Shinichiro; Ono, Ayako; Shibata, Mitsuhiko; Yoshida, Hiroyuki
Nihon Kikai Gakkai Netsu Kogaku Konfarensu 2019 Koen Rombunshu (USB Flash Drive), 1 Pages, 2019/10
no abstracts in English
Hiyama, Mina*; Tamaki, Hitoshi; Yoshida, Kazuo
JAEA-Data/Code 2019-006, 17 Pages, 2019/07
An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. In addition to this, nitrogen oxides (NOx) are also released formed by the thermal decomposition of metal nitrates of fission products (FP) in HLLW. It has been observed experimentally that NOx affects strongly to the transport behavior of Ru at the anticipated atmosphere condition in cells and/or compartments of the facility building. Chemical reactions of NOx with water and nitric acid are also recognized as the complex phenomena to undergo simultaneously in the vapor and liquid phases. An analysis program has been developed to simulate chemical reaction coupled with the thermo-hydraulic condition in the flow paths in the facility building.
Yoshida, Kazuo; Tamaki, Hitoshi; Yoshida, Naoki; Amano, Yuki; Abe, Hitoshi
JAEA-Research 2017-015, 18 Pages, 2018/01
An accident of evaporation to dryness by boiling of high level liquid waste is postulated as one of the severe accidents at a fuel reprocessing facility. It was observed at the experiments that a large amount of ruthenium (Ru) is volatilized and transfer to the vapor phase in the tank. The nitric acid and water mixed vapor released from the tank is condensed. Volatilized Ru is expected to transfer into the condensed water at the compartments in the building. Quantitative estimation of the amount of Ru transferred condensed water is key issues to evaluate the reduction the amount of Ru through leak path in the facility building. This report presents that a correlation has been developed for Ru transfer rate to condensed water with vapor condensing rate based on the experimental results and additional thermal-hydraulic simulation of the experiments. Applicability of the correlation has been also demonstrated with the accident simulation of typical facilities in full-scale.
Uesawa, Shinichiro; Koizumi, Yasuo; Shibata, Mitsuhiko; Yoshida, Hiroyuki
Journal of Nuclear Engineering and Radiation Science, 3(4), p.041002_1 - 041002_13, 2017/10
Hoshasen Kagaku (Internet), (103), P. 65, 2017/04
no abstracts in English
Yonomoto, Taisuke; Shibamoto, Yasuteru; Satou, Akira; Okagaki, Yuria
Journal of Nuclear Science and Technology, 53(9), p.1342 - 1352, 2016/09
Our previous study investigated the rewetting behavior of dryout fuel surface during transients beyond anticipated operational occurrences (AOOs) for BWRs, which indicated the rewetting velocity was significantly affected by the precursory cooling defined as cooling immediately before rewetting. The present study further investigated the previous experiments by conducting additional experimental and numerical heat conduction analyses to characterize the precursory cooling. For the characterization, the precursory cooling was firstly defined quantitatively based on evaluated heat transfer rates; the rewetting velocity was investigated as a function of the cladding temperature immediately before the onset of the precursory cooling. The results indicated that the propagation velocity appeared to be limited by the maximum heat transfer rate near the rewetting front. This limitation was consistent with results of the heat conduction analysis.
JAEA-Research 2016-012, 24 Pages, 2016/08
An accident of evaporation to dryness by boiling of high level liquid waste is postulated as one of the severe accidents. In this case, Ru volatilization increases in liquid waste temperature over 120 centigrade at later boiling and dry out phases. It has been observed at the experiments with actual and synthetic liquid waste that some amount of Ru volatilizes and transfers into condensed nitric acid solution at those phases. The nitric acid and water vapor from waste tank condenses at compartments of actual facilities building. The volatilized Ru could transfer into condensed liquid. It is key issues for quantifying the amount of transferred Ru through the facility building to simulate these thermodynamic and chemical behaviors. An analytical model has been proposed in this report based on the condensation mechanisms of nitric acid and water in vapor-liquid equilibria. It has been also carried out to review the thermodynamic properties of nitric acid solution.
JAEA-Research 2016-004, 15 Pages, 2016/06
An accident of evaporation to dryness by boiling of high level liquid waste is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, some amount of fission products (FPs) will be transferred to the vapor phase in the tank, and could be released to the environment. Two mitigative accident measures have been proposed by the licensee. One of them is injecting cold water to waste tanks to prevent dryness and another is leading generated vapor through temporary duct to huge spaces in the facility to condense to liquid. Thermal-hydraulics and aerosol transport behaviors in compartments of a typical facility building have been analyzed based on the scenario with these accident measures. The effects of measures are discussed form a view point of the reduction of radioactive material release to environment.