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Journal Articles

Nested antiferromagnetic spin fluctuations and non-Fermi-liquid behavior in electron-doped CeCo$$_{1-x}$$Ni$$_{x}$$In$$_5$$

Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Kotegawa, Hisashi*; To, Hideki*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.

Physical Review B, 106(23), p.235152_1 - 235152_8, 2022/12

 Times Cited Count:1 Percentile:9.28(Materials Science, Multidisciplinary)

We investigate the electronic state of Ni-substituted CeCo$$_{1-x}$$Ni$$_x$$In$$_5$$ by nuclear quadrupole and magnetic resonance (NQR/NMR) techniques. The heavy fermion superconductivity below $$T_{rm c} = 2.3$$ K for $$x = 0$$ is suppressed by Ni substitutions, and $$T_{rm c}$$ reaches zero for $$x = 0.25$$. The $$^{115}$$In NQR spectra for $$x = 0.125$$ and 0.25 can be explained by simulating the electrical field gradient that is calculated for a virtual supercell with density functional theory. The spin-lattice relaxation rate $$1/T_1$$ indicates that Ni substitution weakens antiferromagnetic correlations that are not localized near the substituent but instead are uniform in space. The temperature ($$T$$) dependence of $$(T_1T)^{-1}$$ for $$x = 0.25$$ shows a maximum around $$T_{rm g} = 2$$ K and $$(T_1T)^{-1}$$ decreases toward almost zero when temperature is further reduced as if a gap might be opening in the magnetic excitation spectrum; however, the magnetic specific heat and the static magnetic susceptibility evolve smoothly through $$T_{rm g}$$ with a $$-ln T$$ dependence. The peculiar T dependence of $$(T_1T)^{-1}$$ and non-Fermi-liquid specific heat and susceptibility can be interpreted in a unified way by assuming nested antiferromagnetic spin fluctuations in a quasi-two-dimensional electronic system.

Journal Articles

Progress of neutron-capture cross-section measurements promoted by ImPACT project at ANNRI in MLF of J-PARC

Nakamura, Shoji; Kimura, Atsushi; Hales, B. P.; Iwamoto, Osamu; Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*

JAEA-Conf 2018-001, p.199 - 203, 2018/12

Study on cross-section measurements has been promoted for $$^{135}$$Cs among long-lived fission products in ImPACT Project. The feasibility study on $$^{79}$$Se sample preparation also has been conducted to measure its cross sections in future. During the feasibility study, we started the neutron-capture cross-section measurements of stable Se isotopes. This paper reports research progresses on preparation of a radioactive $$^{135}$$Cs sample, neutron irradiation experiments with the Cs sample, and cross-section measurements of stable Se isotopes.

Journal Articles

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai-Nakata, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09

AA2018-0352.pdf:1.16MB

 Times Cited Count:5 Percentile:23.50(Materials Science, Multidisciplinary)

Journal Articles

Research on neutron capture cross sections at J-PARC in ImPACT Project

Nakamura, Shoji; Kimura, Atsushi; Hales, B. P.; Iwamoto, Osamu; Tsubata, Yasuhiro; Matsumura, Tatsuro; Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*

JAEA-Conf 2017-001, p.15 - 22, 2018/01

Neutron nuclear data of long lived fission products (LLFPs) have been required as basic data for the technology of reduce environmental impact involved in high level radioactive wastes (HLW). The innovative large project called by "Impusing Paradigm Change through Disruptive Technologies Program: ImPACT" have been started from October, 2014. In the ImPACT project, some research groups of JAEA engaged in the Project No.2 (Nuclear Reaction Data Measurements), and have started measurements of neutron capture cross-section at J-PARC/MLF/ANNRI. In our research, we selected cesium-135 ($$^{135}$$Cs) nuclide (half life: 2.3$$times$$10$$^{6}$$ yr.) among LLFPs in the HLW, and decided to measure the neutron capture cross-sections of $$^{135}$$Cs. When measurement, the $$^{135}$$Cs sample might contained cecium-137 ($$^{137}$$Cs) as impurities because it's impossible to chemically separate each other. To measure the cross-sections of $$^{135}$$Cs, there should be also needed to know the cross-sections of $$^{137}$$Cs. In this work, sample maintenance also has been examined especially for selen-79 ($$^{79}$$Se) nuclide among LLFPs having difficulty in sample preparations. In this oral session, the outline of our research project will be presented together with a research motivation, situations of past reported data, total schedules, progress, future plans, and some of high light data for neutron capture cross-section measurements.

Journal Articles

Local moments in the heterogeneous electronic state of Cd-substituted CeCoIn$$_5$$; NQR relaxation rates

Sakai, Hironori; Ronning, F.*; Hattori, Takanori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Wakeham, N.*; Yasuoka, Hiroshi; Bauer, E. D.*; Thompson, J. D.*

Journal of Physics; Conference Series, 807(3), p.032001_1 - 032001_6, 2017/04

 Times Cited Count:3 Percentile:66.52(Physics, Condensed Matter)

We have used nuclear quadrupole resonance (NQR) to probe microscopically the response of a prototypical quantum critical metal CeCoIn$$_5$$ to substitutions of small amounts of Cd for In. Approximately half of the Cd substituents induce local Ce moments in their close proximity, as observed by site-dependent longitudinal nuclear spin relaxation rates $$1/T_1$$. To reaffirm that localized $$f$$ moments are induced around the Cd substituents, we find a Gaussian spin-echo decay rate $$1/T_{rm 2G}$$ of transverse nuclear spin relaxation. Further, $$T_1T/T_{rm 2G}^2$$ for the NQR subpeak is found to be proportional to temperatures, again indicating local moments fluctuations around the Cd substituents, while that for the NQR main peak shows a $$T^{0.7}$$-dependence. The latter temperature dependence is close to 0.75 in pure CeCoIn$$_5$$ and indicates that the bulk electronic state is located close to a two dimensional quantum critical instability.

Journal Articles

Relativistic band-structure calculations for CeTIn$$_5$$(T=Ir and Co) and analysis of the energy bands by using tight-binding method

Maehira, Takahiro; Hotta, Takashi; Ueda, Kazuo; Hasegawa, Akira*

Journal of the Physical Society of Japan, 72(4), p.854 - 864, 2003/04

 Times Cited Count:75 Percentile:90.01(Physics, Multidisciplinary)

In order to investigate electronic properties of recently discovered heavy fermion superconductors CeTIn$$_5$$ (T=Ir and Co), we employ the relativistic linear augmented-plane-wave (RLAPW) method to clarify the energy band structures and Fermi surfaces of those materials.The obtained energy bands mainly due to the large hybridization between Ce $$4f$$ and In 5$$p$$ states well reproduce the Fermi surfaces consistent with the de Haas-van Alphen experimental results. For the purpose, we construct a tight-binding model for CeTIn$$_5$$ by including $$f$$-$$f$$ and $$p$$-$$p$$ hoppings as well as $$f$$-$$p$$ hybridization, which are expressed by the Slater-Koster integrals, determined by the direct comparison with the band-calculation result. Similarity and difference between CeIrIn$$_5$$ and CeCoIn$$_5$$ are discussed based on the obtained tight-binding model, suggesting a significant importance of the effect of crystalline electric field to understand the difference in electronic properties among CeTIn$$_5$$.

Journal Articles

The Water detritiation system of the ITER tritium plant

Iwai, Yasunori; Misaki, Yonosuke*; Hayashi, Takumi; Yamanishi, Toshihiko; Konishi, Satoshi; Nishi, Masataka; Ninomiya, R.*; Yanagimachi, S.*; Senrui, S.*; Yoshida, Hiroshi

Fusion Science and Technology, 41(3), p.1126 - 1130, 2002/05

no abstracts in English

Journal Articles

Sorption behavior of radium and actinium on soils

Sakamoto, Yoshiaki; Takebe, Shinichi; Ogawa, Hiromichi; Muraoka, Susumu; Ishii, Tomoaki*; Inagawa, Satoshi*; Gunji, Yasuyoshi*

Materials Research Society Symposium Proceedings, Vol.663, p.1207 - 1214, 2001/00

no abstracts in English

Journal Articles

A Design study of water detritation and hydrogen isotope separation systems for ITER

Iwai, Yasunori; Yoshida, Hiroshi; Yamanishi, Toshihiko; Senrui, S.*; Nishi, Masataka

Fusion Engineering and Design, 49-50, p.847 - 853, 2000/11

 Times Cited Count:17 Percentile:71.54(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Design of neutron monitor for wide energy range from thermal to 100MeV

Kim, E.; Endo, Akira; Yamaguchi, Yasuhiro; Yoshizawa, Michio; Nakamura, Takashi*; Shiomi, T.*

Proceedings of 10th International Congress of the International Radiation Protection Association (IRPA-10) (CD-ROM), 6 Pages, 2000/05

no abstracts in English

Journal Articles

Measurements of the response function and the detection efficiency of an NE213 scintillator for neutrons between 20 and 65 MeV

Meigo, Shinichiro

Nuclear Instruments and Methods in Physics Research A, 401, p.365 - 378, 1997/00

 Times Cited Count:61 Percentile:95.83(Instruments & Instrumentation)

no abstracts in English

Journal Articles

A Tritium recovery system from waste water of fusion reactor using CECE and cryogenic-wall thermal diffusion column

Arita, Tadaaki; Yamanishi, Toshihiko; Iwai, Yasunori; Okuno, Kenji; Kobayashi, Noboru*; Yamamoto, Ichiro*

Fusion Technology, 30(3), p.864 - 868, 1996/12

no abstracts in English

Journal Articles

Design study of feasible water detritiation systems for fusion reactor of ITER scale

Iwai, Yasunori; Yamanishi, Toshihiko; Okuno, Kenji; Yokogawa, Nobuhisa*; ; Yoshida, Hiroshi; O.K.Kveton*

Journal of Nuclear Science and Technology, 33(12), p.981 - 992, 1996/12

 Times Cited Count:28 Percentile:89.28(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Tritiated water processing using liquid phase catalytic exchange and solid oxide electrolyte cell

Yamai, Hideki*; Konishi, Satoshi; Hara, Masahide*; Okuno, Kenji; Yamamoto, Ichiro*

Fusion Technology, 28(3), p.1591 - 1596, 1995/10

no abstracts in English

Journal Articles

Measurement of capacity coefficient of inclined liquid phase catalytic exchange column for tritiated water processing

Yamai, Hideki*; Konishi, Satoshi; Yamanishi, Toshihiko; Okuno, Kenji

Fusion Technology, 26(3), p.654 - 658, 1994/11

no abstracts in English

Journal Articles

Oral presentation

NQR/NMR study on Zn-doped CeCoIn$$_5$$

Sakai, Hironori; Hattori, Taisuke; Tokunaga, Yo; Kambe, Shinsaku; Ronning, F.*; Zhu, J.-X.*; Suzuki, Kohei*; Oshima, Yoshiki*; Yokoyama, Makoto*

no journal, , 

Dilute substitutions of non-magnetic dopants Zn can induce a long-ranged antiferromagnetic ordering to a heavy fermion superconductor CeCoIn$$_5$$. We have microscopically investigated the Zn-doped CeCoIn$$_5$$ by means of the nuclear quadrupole/magnetic resonance (NQR/NMR) techniques.

Oral presentation

Heterogeneous electronic state by Zn-substitutions in heavy fermion superconductor CeCoIn$$_5$$

Sakai, Hironori; Tokunaga, Yo; Haga, Yoshinori; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Ramakrishna, S. K.*; Reyes, A. P.*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.

no journal, , 

Substitutions of In sites by Zn atoms in heavy fermion superconductor CeCoIn$$_5$$ is reported to induce an antiferromagnetic order by Yokoyama et al. in Ibaraki University. Near the critical region, non-Fermi-liquid behavior has been observed in magnetization and specific heat. We have performed NMR measurements to reveal the spin fluctuations near the critical region.

Oral presentation

NMR/NQR study for substitution effect in a antiferromagnetic quantum critical metal CeCoIn$$_5$$

Sakai, Hironori

no journal, , 

We have performed NMR/NQR experiments for slightly substituted CeCoIn$$_5$$ by several substituents of Cd, Zn and Ni. In this presentation, the microscopic electronic states will be discussed.

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