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capture and release at high pressures on a unique large-pore mesoporous carbonSzab
, L.*; Inoue, Mizuki*; Sekine, Yurina; Motokawa, Ryuhei; Matsumoto, Yusuke*; Nge, T. T.*; Ismail, E.*; Ichinose, Izumi*; Yamada, Tatsuhiko*
ChemSusChem, p.e202402034_1 - e202402034_13, 2025/00
Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)Here, we developed a large-pore mesoporous carbon with pore sizes centered around 20-30 nm using a templated technical lignin. During the soft-templating process, unique cylindrical supramolecular assemblies form from the copolymer template, distinct from other systems reported thus far. This peculiar nanostructuring takes place due to the presence of polyethylene glycol (PEG) segments on both the Pluronic template and the PEG- grafted lignin derivative (glycol lignin). A large increase in CO
uptake occurs on the resulting large-pore mesoporous carbon at 270 K close to the saturation pressure, owing to capillary condensation.
-edge EXAFS and magnetic EXAFS studies on the halfmetallic ferromagnet Co
MnSiKogo, Junya*; Fujiwara, Hidenori*; Sekiyama, Akira*; Saito, Yuji; Umetsu, Rie*; Niki, Kaori*
Journal of the Physical Society of Japan, 91(3), p.034702_1 - 034702_12, 2022/03
Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)
emission reduction goal in 2050Kamiji, Yu; Suzuki, Koichi*; Yan, X.
JAEA-Technology 2016-010, 24 Pages, 2016/07
Japanese government has set the goal of reducing CO
emission by 26% in 2030 below the 2013 level, in longer term, by 80% below the 1990 level. To achieve the goals, various measures should be taken. The GTHTR300, a commercial High Temperature Gas-cooled Reactor (HTGR) design being developed by JAEA offers spectrum of heat applications by using its high temperature heat up to 950
C. The potential contribution of CO
emission reduction by HTGR is estimated considering domestic and overseas deployment of the GTHTR300. The best estimate for domestic CO
reduction is 2.07
10
ton- CO
/yr and that from oversea is 2.25
10
ton- CO
/yr. The sum of these is about 47% of 9.13
10
ton- CO
/yr which is CO
reduction target in 2050, for which deployment of 52 plants in Japan and 113 plants abroad, with each plant containing four 600 MWt reactor units, is required.

Rouillard, F.*; Furukawa, Tomohiro
Corrosion Science, 105, p.120 - 132, 2016/04
Times Cited Count:117 Percentile:97.47(Materials Science, Multidisciplinary)The high temperature corrosion behavior of two 9Cr and 12Cr ferritic-martensitic steel grades was studied under CO
pressure varying from 1 to 250 bar for exposure times up to 8000 h. No breakaway oxidation was observed. 9Cr steel grades suffered from fast parabolic uniform oxidation and fast carburisation. Increasing CO
pressure had very little effect on the oxidation rate but increased the carburisation rate. The corrosion behavior of both 12Cr steel grades differed and might be influenced by gas composition, minor elements or surface finish. A corrosion mechanism coupling oxidation and carburisation is proposed.
laser interferometer/polarimeter system in JT-60SASasao, Hajime; Kawano, Yasunori*; Arakawa, Hiroyuki; Sakuma, Takeshi; Imazawa, Ryota; Kubo, Hirotaka; Itami, Kiyoshi
Journal of Instrumentation (Internet), 11, p.C02082_1 - C0208_11, 2016/02
Development of CO
laser interferometer/polarimeter system for JT-60SA has progressed. The CO
laser interferometer/polarimeter system consists of a two color heterodyne interferometer and a polarimeter based on dual PEMs. In JT-60SA, the laser interferometer/ polarimeter system is located in a diagnostic room apart from the tokamak hall, and the laser transmission length is about 200 m. Therefore, it is a key issue for the reliable measurement to transmit the laser light with high stability for the long distance. To realize the stable long-distance transmission, new technologies are developed including a laser spectral beam profile monitor for two color lasers and a laser axis stabilizing system. In addition, a new method for expansion of polarization angle is developed to improve measurement resolution of the polarimeter.
Hayashi, Kentaro*; Kasahara, Seiji; Kurihara, Kohei*; Nakagaki, Takao*; Yan, X.; Inagaki, Yoshiyuki; Ogawa, Masuro
ISIJ International, 55(2), p.348 - 358, 2015/02
Times Cited Count:11 Percentile:44.17(Metallurgy & Metallurgical Engineering)Reducing coking coal consumption and CO
emissions by application of iACRES (ironmaking system based on active carbon recycling energy system) was investigated using process flow modeling to show effectiveness of HTGRs (high temperature gas-cooled reactors) adoption to iACRES. Two systems were evaluated: a SOEC (solid oxide electrolysis cell) system using CO
electrolysis and a RWGS (reverse water-gas shift reaction) system using RWGS reaction with H
produced by IS (iodine-sulfur) process. Both the effects on saving of the coking coal and reduction of CO
emissions were greater in the RWGS system. It was the reason of the result that excess H
which was not consumed in the RWGS reaction was used as reducing agent in the BF as well as CO. Heat balance in the HTGR, SOEC and RWGS modules were evaluated to clarify process components to be improved. Optimization of the SOEC temperature was desired to reduce Joule heat input for high efficiency operation of the SOEC system. Higher H
production thermal efficiency in the IS process for the RWGS system is effective for more efficient HTGR heat utilization. The SOEC system was able to utilize HTGR heat to reduce CO
emissions more efficiently by comparing CO
emissions reduction per unit heat of HTGR.
C]CO
Matsuhashi, Shimpei; Fujimaki, Shu; Uchida, Hiroshi*; Ishioka, Noriko; Kume, Tamikazu
Applied Radiation and Isotopes, 64(4), p.435 - 440, 2006/04
Times Cited Count:19 Percentile:75.96(Chemistry, Inorganic & Nuclear)no abstracts in English
exchange processes into a multilayer atmosphere-soil-vegetation modelNagai, Haruyasu
Journal of Applied Meteorology, 44(10), p.1574 - 1592, 2005/10
This paper describes the incorporation of CO
exchange processes into an atmosphere-soil-vegetation model SOLVEG and examination of its sensitivity and impact of its stomatal resistance calculation on the latent heat flux over a winter wheat field. The model framework for the heat and water exchanges between the atmosphere and ground surface was validated in the previous papers (Nagai 2002, 2003). In this study, CO
exchange processes are incorporated in the model and the performance is examined. In the test calculation, the model simulated the CO
flux at 2 m above the ground well as a whole. A sensitivity test to clarify uncertainties for the model settings and parameters showed that the CO
production in the soil is the most important factor for the CO
calculation. Also, the impact of the CO
processes on the latent heat flux is discussed. The results indicate that the new model is effective and preferable to study surface exchanges of heat and water as well as CO
.
Kawano, Yasunori; Nakano, Tomohide; Asakura, Nobuyuki; Tamai, Hiroshi; Isayama, Akihiko; Kondoh, Takashi; Hatae, Takaki; Takenaga, Hidenobu; Ide, Shunsuke
Purazuma, Kaku Yugo Gakkai-Shi, 81(10), p.743 - 744, 2005/10
Electron density of post-disruption runaway plasmas in JT-60U has been measured by the tangential CO
laser interferometer. Increases in electron density after the first drop of runaway plasma current have been observed during a fast termination phase of the runaway plasma. At the second current drop, an increase in electron density with multiple spikes or oscillation with the period of 1 ms has been found. It is suggested that the increased electron density seems to take part in the shorter current decay time after the second current drop.
Hatae, Takaki; Kondoh, Takashi; Naito, Osamu; Nakatsuka, Masahiro*; Yoshida, Hidetsugu*
Proceedings of 12th International Symposium on Laser-Aided Plasma Diagnostics (LAPD-12) (CD-ROM), 6 Pages, 2005/09
no abstracts in English

Kobayashi, Kazuhiro; Terada, Osamu*; Miura, Hidenori*; Hayashi, Takumi; Nishi, Masataka
Fusion Science and Technology, 48(1), p.476 - 479, 2005/07
Times Cited Count:10 Percentile:55.21(Nuclear Science & Technology)To construct the ITER with high safety and acceptability, it is necessary to establish and to ensure the tritium safe handling technology. The performance of the detritiation system at the off-normal events has not been confirmed well. To obtain performance data of detritiation system at the off normal events, the detritiation experiment was performed at TPL/JAERI using a scaled detritiation system for the oxidation performance test. The detritiation system consists of two oxidation catalyst beds (473K and 773K) and a molecular sieve drying absorber. Basic performance of the detritiation system for hydrogen and methane in air was evaluated under maximum ventilation flow rate. Obtained oxidation efficiency was more than 99.99% for hydrogen in the catalyst bed of 473K and more than 99.9% for methane in the 773K one, respectively. It was confirmed that these performances were maintained even under carbon dioxide , carbon monoxide if oxygen remained in the process gas.
exchange processes; SOLVEG2Nagai, Haruyasu
JAERI-Data/Code 2004-014, 92 Pages, 2004/11
A new atmosphere-soil-vegetation model named SOLVEG2 (SOLVEG version 2) was developed to study the heat, water, and CO
exchanges between the atmosphere and land-surface. The model consists of one-dimensional multilayer sub-models for the atmosphere, soil, and vegetation. It also includes sophisticated processes for solar and long-wave radiation transmission in vegetation canopy and CO
exchanges among the atmosphere, soil, and vegetation. The model can be also used by coupling with a three-dimensional atmosphere model. In this paper, details of SOLVEG2, which includes the function of coupling with atmosphere model MM5, are described.
F
irradiated with two-frequency CO
laser lightsYokoyama, Atsushi; Oba, Hironori; Hashimoto, Masashi; Katsumata, Keiichi; Akagi, Hiroshi; Ishii, Takeshi*; Oya, Akio*; Arai, Shigeyoshi*
Applied Physics B, 79(7), p.883 - 889, 2004/11
Times Cited Count:10 Percentile:43.89(Optics)Silicon isotope separation has been done utilizing the Infrared Multiphoton Dissociation of Si
F
irradiated with two-frequency CO
laser lights. The two-frequency excitation method improved the separation efficiency with keeping the high enrichment factors. For example, Si
F
with the
Si fraction of 99.4 % was obtained at 40.0 % dissociation of Si
F
after the simultaneous irradiation of 100 pulses with 966.23 cm
photons (0.089 J/cm
) and 954.55 cm
photons (0.92 J/cm
), while 1000 pulses were needed to obtain 99.0 % of
Si at 27.2 % dissociation in the case of single frequency irradiation at 954.55 cm
(0.92 J/cm
). The single-step enrichment factors of
Si and
Si increased with increasing Si
F
pressure. The reason for this enhancement has been discussed in terms of the rotational and vibrational relaxations by collisions with ambient gases.
Kondoh, Takashi; Costley, A. E.*; Sugie, Tatsuo; Kawano, Yasunori; Malaquias, A.*; Walker, C. I.*
Review of Scientific Instruments, 75(10), p.3420 - 3422, 2004/10
Times Cited Count:23 Percentile:71.16(Instruments & Instrumentation)In order to measure the line average electron density on ITER, a CO
laser interferometer/polarimeter system is being developed. The design of the interferometer/polarimeter is improved from the previous design, which uses CO
and CO laser, on the basis of experience gained with a dual CO
system on JT-60U in which good reliability was confirmed for both interferometry and polarimetry operation. The performance of the dual CO
laser meets requirements for ITER (accuracy; 1%, time resolution; 1 ms).
O
Soda, Minoru*; Yasui, Yukio*; Ito, Masafumi*; Iikubo, Satoshi*; Sato, Masatoshi*; Kakurai, Kazuhisa
Journal of the Physical Society of Japan, 73(2), p.464 - 468, 2004/02
Times Cited Count:42 Percentile:80.95(Physics, Multidisciplinary)no abstracts in English
O
Soda, Minoru*; Yasui, Yukio*; Fujita, Toshiaki*; Miyashita, Takeshi*; Sato, Masatoshi*; Kakurai, Kazuhisa
Journal of the Physical Society of Japan, 72(7), p.1729 - 1734, 2003/07
Times Cited Count:76 Percentile:89.88(Physics, Multidisciplinary)no abstracts in English
hydrate; Synthesis, composition, structure, dissociation behavior, and a comparison to structure I CH
hydrateCircone, S.*; Stern, L. A.*; Kirby, S. H.*; Durham, W. B.*; Chakoumakos, B. C.*; Rawn, C. J.*; Rondinone, A. J.*; Ishii, Yoshinobu
Journal of Physical Chemistry B, 107(23), p.5529 - 5539, 2003/06
Times Cited Count:201 Percentile:96.33(Chemistry, Physical)no abstracts in English
CO
flux at soil-atmosphere interface and distribution of
C in forest ecosystemKoarashi, Jun; Amano, Hikaru; Atarashi-Andoh, Mariko; Iida, Takao*; Moriizumi, Jun*
Journal of Environmental Radioactivity, 60(3), p.249 - 261, 2002/06
Times Cited Count:16 Percentile:34.86(Environmental Sciences)no abstracts in English
Si by infrared multiple photon decomposition of Si
F
Yokoyama, Atsushi; Oba, Hironori; Shibata, Takemasa; Kawanishi, Shunichi*; Sugimoto, Shunichi*; Ishii, Takeshi*; Oya, Akio*; Miyamoto, Yoshiki*; Isomura, Shohei*; Arai, Shigeyoshi*
Journal of Nuclear Science and Technology, 39(4), p.457 - 462, 2002/04
Times Cited Count:3 Percentile:22.51(Nuclear Science & Technology)no abstracts in English
Ogiyanagi, Jin; Meguro, Yoshihiro; Yoshida, Zenko; Ohashi, Kozaburo*
Analytical Sciences (CD-ROM), 17(Suppl.), p.717 - 720, 2002/03
no abstracts in English