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Journal Articles

Synergistic effect of aluminum lactate and sodium molybdate on freshwater corrosion of carbon steel under irradiation

Otani, Kyohei; Kato, Chiaki; Igarashi, Takahiro

Corrosion, 79(11), p.1277 - 1286, 2023/11

JAEA Reports

Application of satellite remote sensing in geological environment investigation; Development of a geobotanical remote sensing method for estimating high water table areas in a humid warm-temperate region

Koide, Kaoru

JAEA-Research 2023-003, 101 Pages, 2023/06

JAEA-Research-2023-003.pdf:14.08MB

This study developed a geobotanical remote sensing method for estimating high water table areas such as groundwater discharge points using differences in the growth conditions of forest trees induced by moisture supply from groundwater in a humid warm-temperate forest area. A new vegetation index (VI) termed AgbNDVI (Added green band NDVI) was proposed to discriminate the differences. The AgbNDVI proved to be more sensitive to water stress on green vegetation than existing VIs: SAVI and EVI2, and possessed a strong linear correlation with the vegetation fraction. To validate the proposed method, a 23 km$$^{2}$$ study area was selected in the Tono region of Gifu Prefecture, central Japan. The AgbNDVI values were calculated from atmospheric corrected SPOT HRV data. To correctly detect high VI points, the influence factors on tree growth were identified using the AgbNDVI values, DEM and forest type data; the study area was then divided into 555 segments according to combinations of the influence factors: elevation, slope gradient, slope aspect and forest type. Thresholds for detecting high VI points were defined for each segment based on a histogram of AgbNDVI values. By superimposing the high VI points on topographic and geologic maps, most of the high VI points are clearly located on the concave/convex slopes and near the geologic boundaries prone to groundwater runoff. In addition, field investigations support the correctness of the high VI points, because the growth increments and biomass of trees (${it Pinus densiflora}$) are greater than at points other than the high VI points, and they are located around known groundwater seeps and in a high water table area. Consequently, the proposed method can be expected to provide useful information for characterizing hydrogeological structures by combining with conventional photo-geological interpretation.

Journal Articles

Treatment of U contaminated waste generated from nuclear fuel fabrication process, 1; Ce(IV) recovery by temperature swing extraction with monoamides

Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 4 Pages, 2023/05

Applicability of temperature swing extraction technology employing monoamides was examined for uranium contaminated waste treatment procedure. Separation experiments on simulated target solution with three kinds of monoamides with different structure showed that Ce(IV) in the solution was selectively recovered by the temperature swing extraction operation. Based on the experiments, an appropriate monoamide for the procedure was selected.

Journal Articles

Possible pathway of zeolite formation through alkali activation chemistry of metakaolin for geopolymer-zeolite composite materials; ATR-FTIR study

Onutai, S.; Sato, Junya; Osugi, Takeshi

Journal of Solid State Chemistry, 319, p.123808_1 - 123808_10, 2023/03

 Times Cited Count:24 Percentile:97.55(Chemistry, Inorganic & Nuclear)

Journal Articles

Alumino-silicate structural formation during alkali-activation of metakaolin; In-situ and ex-situ ATR-FTIR studies

Onutai, S.; Osugi, Takeshi; Sone, Tomoyuki

Materials, 16(3), p.985_1 - 985_14, 2023/02

 Times Cited Count:18 Percentile:91.81(Chemistry, Physical)

Journal Articles

Emulsification of low viscosity oil in alkali-activated materials

Reeb, C.*; Davy, C. A.*; Pierlot, C.*; Bertin, M.*; Cantarel, V.; Lambertin, D.*

Cement and Concrete Research, 162, p.106963_1 - 106963_16, 2022/12

 Times Cited Count:9 Percentile:56.43(Construction & Building Technology)

Journal Articles

Acid dissociation constant of bis(2-ethylhexyl) hydrogen phosphate impregnated in a polymer layer coated on silica microparticles

Miyagawa, Akihisa*; Takeuchi, Masayuki; Arai, Tsuyoshi*; Watanabe, So; Sano, Yuichi; Nakatani, Kiyoharu*

Bulletin of the Chemical Society of Japan, 95(4), p.566 - 568, 2022/04

 Times Cited Count:3 Percentile:22.15(Chemistry, Multidisciplinary)

We demonstrate that pKa of extractant impregnated in a polymer phase varies with the cross-linking degree and the coexistence of other extractants, which induces a change in the hydrophobicity of the polymer phase. The results presented herein will be beneficial for the development of novel solid-extraction adsorbents.

Journal Articles

Separation of light and middle lanthanides using multistage extraction with diglycolamide extractant

Matsutani, Takafumi; Sasaki, Yuji; Katsuta, Shoichi*

Analytical Sciences, 37(11), p.1603 - 1609, 2021/11

 Times Cited Count:7 Percentile:39.31(Chemistry, Analytical)

We investigated the chemical behavior of lanthanides (Ln) using diglycolamide extractant with multistage extraction. We obtained the breakthrough curves for light and middle Ln. Our study reveals that the metal extraction limit depends on their $$D$$ values and metal concentrations used in the experiments. From the multistage extractions of 15 aqueous phases and 15 organic phases, three curves (extraction curves, back-extraction curves, and separation curves) were obtained by changing the nitric acid concentration. As an example, under a condition of the separation curve experiment (aqueous phase: 0.5 M HNO$$_{3}$$, organic phase: 0.1 M TDDGA ($$N,N,N',N'$$-tetradecyl-diglycolamide) in $$n$$-dodecane), a recovery of more than 99% of Sm in the organic phase with less than 1% Nd can be obtained.

Journal Articles

Effects of pressure and heat loss on the unstable motion of cellular-flame fronts caused by intrinsic instability in hydrogen-air lean premixed flames

Kadowaki, Satoshi; Thwe Thwe, A.; Furuyama, Taisei*; Kawata, Kazumasa*; Katsumi, Toshiyuki; Kobayashi, Hideaki*

Journal of Thermal Science and Technology (Internet), 16(2), p.20-00491_1 - 20-00491_12, 2021/00

 Times Cited Count:9 Percentile:42.27(Thermodynamics)

Effects of pressure and heat loss on the unstable motion of cellular-flame fronts in hydrogen-air lean premixed flames were numerically investigated. The reaction mechanism for hydrogen-oxygen combustion was modeled with seventeen reversible reactions of eight reactive species and a diluent. Two-dimensional unsteady reactive flow was treated, and the compressibility, viscosity, heat conduction, molecular diffusion and heat loss were taken into account. As the pressure became higher, the maximum growth rate increased and the unstable range widened. These were due mainly to the decrease of flame thickness. The burning velocity of a cellular flame normalized by that of a planar flame increased as the pressure became higher and the heat loss became larger. This indicated that the pressure and heat loss affected strongly the unstable motion of cellular-flame fronts. In addition, the fractal dimension became larger, which denoted that the flame shape became more complicated.

Journal Articles

Development of Short-Term Emergency Assessment system of Marine Environmental Radioactivity

Kobayashi, Takuya; Kawamura, Hideyuki; Kamidaira, Yuki

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 62(11), p.635 - 639, 2020/11

It is important to predict the dispersion of radioactive materials released into the ocean due to nuclear accidents in the surrounding ocean of the east Asian countries. The Japan Atomic Energy Agency developed a Short-Term Emergency Assessment system of Marine Environmental Radioactivity (STEAMER) based on an oceanic dispersion model. STEAMER quickly predicts the oceanic dispersion of radioactive materials in the surrounding ocean of the east Asian countries using the online prediction data of oceanic condition. We validated the predictability of the oceanic dispersion and demonstrated the improvement of the predictability using an ensemble prediction method. Moreover, we developed a high resolution model in the coastal region using a Regional Ocean Modeling System (ROMS).

Journal Articles

Predictability of a short-term emergency assessment system of the marine environmental radioactivity

Kawamura, Hideyuki; Kamidaira, Yuki; Kobayashi, Takuya

Journal of Nuclear Science and Technology, 57(4), p.472 - 485, 2020/04

 Times Cited Count:3 Percentile:26.48(Nuclear Science & Technology)

The Japan Atomic Energy Agency developed a Short-Term Emergency Assessment system of the Marine Environmental Radioactivity (STEAMER) to predict the oceanic dispersion of radionuclides in the ocean around Japan. The purpose of this study is to validate the predictability of STEAMER using oceanographic forecast and reanalysis data, which were saved for past several years. Results of oceanic dispersion simulations that are driven by oceanographic reanalysis data are assumed to be true solutions. Oceanic dispersion simulations are conducted for Cs-137 released hypothetically from the Fukushima Daiichi Nuclear Power Plant. The predictability of STEAMER is quantitatively examined for the length of the forecast period. Ensemble forecast simulations are also conducted to successfully improve the predictability of STEAMER.

Journal Articles

Rheo-SANS study on relationship between micellar structures and rheological behavior of cationic gemini surfactants in solution

Iwase, Hiroki*; Kawai, Risa*; Morishima, Ken*; Takata, Shinichi; Yoshimura, Tomokazu*; Shibayama, Mitsuhiro*

Journal of Colloid and Interface Science, 538, p.357 - 366, 2019/03

 Times Cited Count:17 Percentile:42.74(Chemistry, Physical)

Journal Articles

Numerical investigation on unstable behaviors of cellular premixed flames at low Lewis numbers based on the diffusive-thermal model and compressible Navier-Stokes equations

Thwe Thwe, A.; Kadowaki, Satoshi; Hino, Ryutaro

Journal of Thermal Science and Technology (Internet), 13(2), p.18-00457_1 - 18-00457_12, 2018/12

 Times Cited Count:0 Percentile:0.00(Thermodynamics)

Two dimensional unsteady calculations of reactive flows were performed in large domain to investigate the unstable behaviors of cellular premixed flames at low Lewis numbers based on the diffusive-thermal (D-T) model and compressible Navier-Stokes (N-S) equations. The growth rates obtained by the compressible N-S equations were large and the unstable ranges were wide compared with those obtained by the D-T model equations. When the length of computational domain increased, the number of small cells separated from large cells of the cellular flame increased drastically. The stronger unstable behaviors and the larger average burning velocities were observed especially in the numerical results based on the compressible N-S equations. In addition, the fractal dimension obtained by the compressible N-S equations was larger than that by the D-T model equations. Moreover, we confirmed that the radiative heat loss promoted the instability of premixed flames at low Lewis numbers.

Journal Articles

Measurements of neutronic characteristics of rectangular and cylindrical coupled hydrogen moderators

Kai, Tetsuya; Kamiyama, Takashi*; Hiraga, Fujio*; Oi, Motoki; Hirota, Katsuya*; Kiyanagi, Yoshiaki*

Journal of Nuclear Science and Technology, 55(3), p.283 - 289, 2018/03

 Times Cited Count:1 Percentile:9.99(Nuclear Science & Technology)

Journal Articles

Conductance of a long rectangular channel; Pressure dependence

Ogiwara, Norio; Hikichi, Yusuke*; Kamiya, Junichiro; Kinsho, Michikazu; Yoshida, Hajime*; Arai, Kenta*

Journal of the Vacuum Society of Japan, 60(12), p.475 - 480, 2017/12

Journal Articles

Minor actinides recovery from irradiated fuel for SmART cycle test

Takeuchi, Masayuki; Sano, Yuichi; Watanabe, So; Nakahara, Masaumi; Aihara, Haruka; Kofuji, Hirohide; Koizumi, Tsutomu; Mizuno, Tomoyasu

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 6 Pages, 2017/04

Journal Articles

Highly practical and simple ligand for separation of Am(III) and Eu(III) from highly acidic media

Suzuki, Hideya; Tsubata, Yasuhiro; Kurosawa, Tatsuya; Shibata, Mitsunobu; Kawasaki, Tomohiro; Urabe, Shunichi*; Matsumura, Tatsuro

Analytical Sciences, 32(4), p.477 - 479, 2016/04

 Times Cited Count:29 Percentile:71.77(Chemistry, Analytical)

An impeccable, high-performance new reagent called alkyl diamide amine (ADAAM) was examined from the viewpoint of mutual separation of Am(III) and Eu(III). ADAAM has three donor atoms, one soft N-donor atom and two hard O-donor atoms, in the central frame. The combination of soft and hard atoms affords a tridentate donor set of atoms that ensures remarkable extractability and selectivity of Am(III) and Eu(III) in highly acidic media.

JAEA Reports

Fabrication and test results of testing equipment for remote-handling of MA fuel, 2; Evaluation of heat transfer parameter crossing rectangular lattice matrix

Eguchi, Yuta; Sugawara, Takanori; Nishihara, Kenji; Tazawa, Yujiro; Inoue, Akira; Tsujimoto, Kazufumi

JAEA-Technology 2015-052, 34 Pages, 2016/03

JAEA-Technology-2015-052.pdf:5.02MB

Transmutation Physics Experimental Facility (TEF-P) planned in the J-PARC project uses minor actinide (MA) fuel which has large decay heat. So it is necessary to consider the increase of the core temperature when the core cooling system is stopped. This change of the core temperature was evaluated by thermal conduction analysis. It was found that the impact of thermal insulation in the empty rectangular lattice matrix area was large. So it is necessary to verify reliability and accuracy of heat transfer effect used in this area. Testing equipment was fabricated to verify the accuracy of calculation model for the empty lattice matrix which was the free convection model of sealed fluid. By using this equipment, thermal distribution and one dimensional heat flow through the lattice were measured. It was observed that the actual equivalent thermal conductivity in the lattice was larger than the free convection model. It was also confirmed that the insertion of the aluminum block into the empty lattice could achieve the higher equivalent thermal conductivity. These results could be the useful data for the thermal conduction analysis.

Journal Articles

Fabrication of hard-coated optical absorbers with microstructured surfaces using etched ion tracks; Toward broadband ultra-low reflectance

Amemiya, Kuniaki*; Koshikawa, Hiroshi; Yamaki, Tetsuya; Maekawa, Yasunari; Shitomi, Hiroshi*; Numata, Takayuki*; Kinoshita, Kenichi*; Tanabe, Minoru*; Fukuda, Daiji*

Nuclear Instruments and Methods in Physics Research B, 356-357, p.154 - 159, 2015/08

 Times Cited Count:10 Percentile:60.88(Instruments & Instrumentation)

Broadband low reflectance materials have various applications in the field of optical energy management; however, materials with ultra-low reflectance (below 0.1%) have been considered as mechanically delicate. We have developed a novel hard-surface optical absorber with microstructured, diamond-like carbon coated ion tracks on CR-39 plastic substrate. The spectral reflectance of the first prototype was below 2% for wavelengths ranging from 400 nm to 1400 nm; moreover, the optical absorber had mechanically hard surface and exhibited temporal durability. Choosing the appropriate design of the surface structure and coating layer is likely to reduce the reflectance to the order of 0.1%. This technique yields easy-to-handle broadband ultra-low reflectance absorbers.

Journal Articles

Neutron capture cross section and capture $$gamma$$-ray spectra of $$^{138}$$Ba in the keV-neutron energy region

Katabuchi, Tatsuya*; Yanagida, Shotaro*; Terada, Kazushi; Iwamoto, Nobuyuki; Igashira, Masayuki*

EPJ Web of Conferences, 93, p.02008_1 - 02008_2, 2015/05

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

$$^{138}$$Ba has the smallest neutron capture cross section among the stable Ba isotopes. The neutron capture reaction of $$^{138}$$Ba is dominated by resolved resonances in the astrophysically relevant energy region. Thus, reliable experimental data of the capture cross section are necessary. In the present work, we measured the neutron capture cross section of $$^{138}$$Ba in the energy region from 15 to 100 keV by the time-of-flight method at the Tokyo Institute of Technology. The capture cross sections were obtained from the pulse height spectra by the pulse-height weighting technique. A comparison of the present results with previous experimental data and evaluated data was made. We also derived $$gamma$$-ray spectra by unfolding the pulse height spectra. It was revealed that the shape of $$gamma$$-ray spectra strongly depends on neutron energy.

126 (Records 1-20 displayed on this page)