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Cs behavior in the ocean around Fukushima considering multiphase interaction processesIkenoue, Tsubasa; Nakanishi, Takahiro; Kawamura, Hideyuki
Marine Pollution Bulletin, 232, p.120110_1 - 120110_9, 2026/11
Times Cited Count：0The accident at the Fukushima Daiichi Nuclear Power Plant caused a large-scale migration of radionuclides, including cesium-137 (Cs), into the marine environment. Cesium-137 in the ocean exists in four phases (dissolved, suspended, seabed sediment, and biota), and the interactions between these phases have a great impact on its long-term behavior. Therefore, this study developed an oceanic dispersion model considering multiphase behavior and evaluated the impact of interphase interactions on the long-term behavior of Cs during the decade after the accident. The model sufficiently reproduced the oceanographic conditions and the behavior of planktons, suspended particles, and Cs. The results were consistent with previous studies, suggesting that the dissolved phase and seabed sediment phase played a central role in the Cs behavior within the first three months after the accident and thereafter, respectively. Within 10 years after the accident, the concentrations of all phases in offshore waters (deeper than 25 m) returned to pre-accident levels, but those in coastal waters (shallower than 25 m) were still at high levels due to the long-term source from seabed sediment to other phases, which is attributed to the retention of high concentrations in the seabed sediment phase. The quantitative analysis of interphase interactions made it possible to confirm that this retention was caused by a large proportion of fine-grained particles (bay area), riverine inputs (northern Fukushima), and high accumulation in the surface layers in the early stage of the accident and vigorous vertical mixing (southern Fukushima).
CsKobayashi, Hikaru*; Ma, X.*; Suto, Masahito*; Yamamori, Ryo*; Furuta, Takuya
Radiation Measurements, 197, p.107743_1 - 107743_13, 2026/09
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Monte Carlo photon transport simulations are widely used to predict indoor dose distributions from Cs-137 ground deposition, but their computational cost can be high. To improve efficiency, we propose the fluence boundary method (FBM), which accounts for contributions from distant sources by applying analyzed photon fluence profiles at near-site boundaries surrounding a building. These profiles are defined according to the land-cover type adjacent to each boundary. The method was validated by comparing FBM results with full simulations, demonstrating that FBM achieved a maximum absolute percentage error below 5% across indoor dose distributions. The feasibility of representing fluence boundaries using land-cover types was further examined by evaluating the impact of uncertainties in relaxation mass depth (
) for paved and soil surfaces. The normalized indoor dose distributions showed weak dependence on within a reasonable range, indicating that indoor dose distributions can be reliably predicted using representative values when doses are normalized to measurements.
Furuno, Akiko; Omori, Ryuta*; Tateoka, Hisanori*; Minakawa, Yuya*; Kurihara, Toshiyuki; Yamamoto, Yoichi; Tomita, Yutaka
Pure and Applied Geophysics, 182(12), p.5175 - 5188, 2025/12
Times Cited Count：2 Percentile：25.54(Geochemistry & Geophysics)The Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) Okinawa radionuclide monitoring station (JPP37) is located on a hill facing the East China Sea at the center of the main island of Okinawa. It occasionally detects Cs-137, although no nuclear facilities are located on the island. This study focused on the detection of Cs-137 at JPP37 and examined the ratio of simultaneous detections at nearby stations of the International Monitoring System (IMS) of the CTBTO and the relationship with Asian dust from inland East Asia. The detection of Cs-137 in JPP37 from 2020 to 2023, which motivated this study, was high in spring. Among the nine IMS radionuclide stations in East Asia, the detections in Beijing, Lanzhou, and Ulaanbaatar, Mongolia, were also high in spring. This suggested a high association with the detection of Asian dust in East Asia. Thus, we confirmed the detection of Cs-137 at nine nearby IMS stations when Asian dust was observed at any of the sites in Japan. In addition, we observed that the detection rates were high in Takasaki, Beijing, Lanzhou, and Ulaanbaatar. It can be inferred that the Cs-137 observed mainly in spring at the IMS particulate radionuclide stations in the East Asian region around Japan were likely to pick up the effects of global fallout conveyed by Asian dust. Thereafter, we conducted a preliminary source estimation analysis for Asian dust arrival near Japan. Atmospheric dispersion simulations explained the detection of Cs-137 at nearby IMS particulate radionuclide stations, assuming that Cs-137 was emitted from the desert, the source of the Asian dust.
I in riverbank sediment after the Fukushima accidentNakanishi, Takahiro; Sakuma, Kazuyuki; Oyama, Takuya; Hagiwara, Hiroki; Suzuki, Takashi
Environmental Pollution, 355, p.124213_1 - 124213_7, 2024/08
Times Cited Count：8 Percentile：61.99(Environmental Sciences)This study investigated the transport behavior of I by riverbank surveys conducted from 2013 to 2015 in a watershed where the I/Cs activity ratio is low in the mountainous area and high in the plain as of 2011. Until 2015, the I/Cs activity ratio of the levee crown in the studied watershed was similar to that of the surrounding area in 2011. However, the I/Cs ratios of the surface riverbank sediments were all low, indicating that radionuclides transported from the mountainous area were deposited on the riverbank in the plain. The vertical distribution of the I/Cs ratio in the riverbank sediments indicated that some I and Cs deposited during the accident remained in the lower layers, but most were eroded immediately after the accident. Based on the I/Cs ratios of sediments deposited on the riverbank, which remained constant until 2015 after the accident, the amount of I discharged to the ocean was determined from the previously evaluated Cs discharge. It was calculated that 1.8
10
Bq and 1.210
Bq of I were discharged with sediment from the studied watershed and the contaminated river watersheds (Abukuma River and Fukushima coastal rivers, including the study river), respectively. The results of this study indicate that the continuous I discharge from the river contribute little to their amount in the seafloor sediments along the Fukushima coast.
Cs in river waterEnomoto, Kazuyuki*; Hoshina, Hiroyuki*; Kasai, Noboru*; Kurita, Keisuke; Ueki, Yuji*; Nagao, Yuto*; Yin, Y.-G.*; Suzui, Nobuo*; Kawachi, Naoki*; Seko, Noriaki*
Chemical Engineering Journal, 460, p.141696_1 - 141696_9, 2023/03
Times Cited Count：3 Percentile：13.35(Engineering, Environmental)This study develops a method that combines a radiation-grafting fibrous Cs-adsorbent filter of ammonium molybdophosphate (AMP) and a Ce:Gd
Al
GaO
scintillator based 
-ray detector for in situ measurements of the activity concentrations of Cs in a continuous water flow.
Sr and Cs into wild animals after the Fukushima Daiichi Nuclear Power Plant accident using hard tissue as an indicatorKoarai, Kazuma
Hosha Kagaku, (47), p.24 - 27, 2023/03
Ca-based tissues, such as teeth and bones, are called hard tissues. Sr is incorporated into the tooth during calcification. Once incorporated, it remains until the tooth falls out. Therefore, Sr in teeth recorded Sr contamination by the 1F accident in the environment during the formation period. The article presents current research findings.
Moriguchi, Yuichi*; Sato, Yosuke*; Morino, Yu*; Goto, Daisuke*; Sekiyama, Tsuyoshi*; Terada, Hiroaki; Takigawa, Masayuki*; Tsuruta, Haruo*; Yamazawa, Hiromi*
KEK Proceedings 2021-2, p.21 - 27, 2021/12
no abstracts in English
Nakanishi, Takahiro; Oyama, Takuya; Hagiwara, Hiroki; Sakuma, Kazuyuki
Journal of Coastal Research, 114(SI), p.310 - 314, 2021/10
Times Cited Count：7 Percentile：29.64(Environmental Sciences)The two huge typhoons in 2019, Hagibis and Bualoi, caused enormous flood damage to Fukushima. On the basis of field observations over 6 years in Ukedo River near the Fukushima Nuclear Power Plant, sediment and Cs discharges from the river catchment were quantitatively evaluated. Approximately 90% of annual sediment and Cs discharges in 2019 was occupied during the typhoons Hagibis and Bualoi events. This sediment discharge was almost twice than the discharge during the largest ever flood event since the Fukushima nuclear accident, caused by typhoon Etau in September 2015. However, Cs discharge during Hagibis and Bualoi events was two-thirds that of Etau event, because the particulate Cs concentration in river water decreased during the observation period. Moreover, Cs discharge during two typhoon events in 2019 accounted for only 0.1% of the catchment Cs deposition and the impact of radiocesium to the coastal area was extremely limited.
Hidaka, Akihide
Fission Product Behavior under Severe Accident, p.85 - 88, 2021/05
no abstracts in English
Cs concentrations from the Fukushima Daiichi Nuclear Power Plant accident, phase III; Simulation with an identical source term and meteorological field at 1-km resolutionSato, Yosuke*; Sekiyama, Tsuyoshi*; Fang, S.*; Kajino, Mizuo*; Qu
rel, A.*; Qulo, D.*; Kondo, Hiroaki*; Terada, Hiroaki; Kadowaki, Masanao; Takigawa, Masayuki*; et al.
Atmospheric Environment; X (Internet), 7, p.100086_1 - 100086_12, 2020/10
The third model intercomparison project for investigating the atmospheric behavior of Cs emitted during the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident (FDNPP-MIP) was conducted. A finer horizontal grid spacing (1 km) was used than in the previous FDNPP-MIP. Nine of the models used in the previous FDNPP-MIP were also used, and all models used identical source terms and meteorological fields. Our analyses indicated that most of the observed high atmospheric Cs concentrations were well simulated, and the good performance of some models improved the performance of the multi-model ensemble. The analyses also confirmed that the use of a finer grid resolution resulted in the meteorological field near FDNPP being better reproduced. The good representation of the wind field resulted in the reasonable simulation of the narrow distribution of high deposition amount to the northwest of FDNPP and the reduction of the overestimation over the area to the south of FDNPP. In contrast, the performance of the models in simulating plumes observed over the Nakadori area, the northern part of Gunma, and the Tokyo metropolitan area was slightly worse.
Sr and Cs in soils near the Fukushima Daiichi Nuclear Power StationSasaki, Takayuki*; Matoba, Daisuke*; Dohi, Terumi; Fujiwara, Kenso; Kobayashi, Taishi*; Iijima, Kazuki
Journal of Radioanalytical and Nuclear Chemistry, 326(1), p.303 - 314, 2020/10
Times Cited Count：11 Percentile：64.92(Chemistry, Analytical)Machida, Masahiko; Yamada, Susumu; Iwata, Ayako; Otosaka, Shigeyoshi; Kobayashi, Takuya; Watanabe, Masahisa; Funasaka, Hideyuki; Morita, Takami*
Journal of Nuclear Science and Technology, 57(8), p.939 - 950, 2020/08
Times Cited Count：16 Percentile：77.81(Nuclear Science & Technology)After direct discharges of highly contaminated water of the Fukushima Daiichi Nuclear Power Plant (1F) from April to May 2011, Kanda suggested that relatively small amounts of run-off of radionuclides from the 1F port into the Fukushima coastal region subsequently continued by his estimation method. However, the estimation period was limited to up to September 2012. Therefore, this paper estimates the discharge inventory up to June 2018. In the missing period, the Japanese government and Tokyo Electric Power Company Holdings have continued efforts to stop the discharge, and consequently, the radionuclide concentration in seawater inside the 1F port has gradually diminished. We show the monthly discharge inventory of Cs up to June 2018 by two methods, i.e., Kanda method partially improved by the authors and a more sophisticated method using Voronoi tessellation reflecting the increase in the number of monitoring points inside the 1 F port. The results show that the former always yields overestimated results compared with the latter, but the ratio of the former to the latter is less than one order of magnitude. Using these results, we evaluate the impact of the discharge inventory from the 1F port into the coastal area and radiation dose upon fish ingestion.
Kawamura, Hideyuki; Kamidaira, Yuki; Kobayashi, Takuya
Journal of Nuclear Science and Technology, 57(4), p.472 - 485, 2020/04
Times Cited Count：3 Percentile：22.02(Nuclear Science & Technology)The Japan Atomic Energy Agency developed a Short-Term Emergency Assessment system of the Marine Environmental Radioactivity (STEAMER) to predict the oceanic dispersion of radionuclides in the ocean around Japan. The purpose of this study is to validate the predictability of STEAMER using oceanographic forecast and reanalysis data, which were saved for past several years. Results of oceanic dispersion simulations that are driven by oceanographic reanalysis data are assumed to be true solutions. Oceanic dispersion simulations are conducted for Cs-137 released hypothetically from the Fukushima Daiichi Nuclear Power Plant. The predictability of STEAMER is quantitatively examined for the length of the forecast period. Ensemble forecast simulations are also conducted to successfully improve the predictability of STEAMER.
Machida, Masahiko; Yamada, Susumu; Iwata, Ayako; Otosaka, Shigeyoshi; Kobayashi, Takuya; Watanabe, Masahisa; Funasaka, Hideyuki; Morita, Takami*
Nihon Genshiryoku Gakkai Wabun Rombunshi, 18(4), p.226 - 236, 2019/12
After direct discharges of highly-contaminated water from Unit 2 and 3 in Fukushima Daiichi Nuclear Power Plant (1F) in April to May 2011, Kanda suggested that relatively small run-off of radionuclides from 1F port into Fukushima coastal region has subsequently continued by using his estimation scheme. However, the estimation period was limited until September 2012, and there has been no report on the issue since the work. Therefore, this paper focuses on discharge inventory from 1F port until June 2018. In the missing period, the central government and Tokyo Electric Power Company Holdings have done continuous efforts to stop the discharge, and consequently sea water concentration inside 1F port has diminished gradually. We show monthly discharge inventory of Cs-137 until June 2018 by two schemes, i.e., Kanda's scheme partially improved by authors and more sophisticated one using Voronoi tessellation reflecting the increment of the number of monitoring points inside 1F port. The results show that the former always presents overestimated results compared to the latter but the ratio of former to latter is less than one order. Based on these results, we evaluate impact of discharge inventory from 1F port into the coastal area and radiation does via fish digestion.
Cs plumes from the Fukushima Daiichi Nuclear Power Plant; Evaluation of the model intercomparison data of the Science Council of JapanKitayama, Kyo*; Morino, Yu*; Takigawa, Masayuki*; Nakajima, Teruyuki*; Hayami, Hiroshi*; Nagai, Haruyasu; Terada, Hiroaki; Saito, Kazuo*; Shimbori, Toshiki*; Kajino, Mizuo*; et al.
Journal of Geophysical Research; Atmospheres, 123(14), p.7754 - 7770, 2018/07
Times Cited Count：29 Percentile：64.65(Meteorology & Atmospheric Sciences)We compared seven atmospheric transport model results for Cs released during the Fukushima Daiichi Nuclear Power Plant accident. All the results had been submitted for a model intercomparison project of the Science Council of Japan in 2014. We assessed model performance by comparing model results with observed hourly atmospheric concentrations of Cs, focusing on nine plumes over the Tohoku and Kanto regions. The results showed that model performance for Cs concentrations was highly variable among models and plumes. We also assessed model performance for accumulated Cs deposition. Simulated areas of high deposition were consistent with the plume pathways, though the models that best simulated Cs concentrations were different from those that best simulated deposition. The ensemble mean of all models consistently reproduced Cs concentrations and deposition well, suggesting that use of a multimodel ensemble results in more effective and consistent model performance.
Kawamura, Hideyuki; Furuno, Akiko; Kobayashi, Takuya; In, Teiji*; Nakayama, Tomoharu*; Ishikawa, Yoichi*; Miyazawa, Yasumasa*; Usui, Norihisa*
Journal of Environmental Radioactivity, 180, p.36 - 58, 2017/12
Times Cited Count：17 Percentile：37.48(Environmental Sciences)This study simulates the oceanic dispersion of Fukushima-derived Cs-137 by an oceanic dispersion model and multiple oceanic general circulation models. The models relatively well reproduced the observed Cs-137 concentrations in the coastal, offshore, and open oceans. Multiple simulations in the coastal, offshore, and open oceans consistently suggested that Cs-137 dispersed along the coast in the north-south direction during the first few months post-disaster, and were subsequently dispersed offshore by the Kuroshio Current and Kuroshio Extension. Quantification of the Cs-137 amounts suggested that Cs-137 actively dispersed from the coastal and offshore oceans to the open ocean, and from the surface layer to the deeper layers in the North Pacific.
Saito, Kyoichi*; Kojima, Takashi*; Asai, Shiho
Bunseki Kagaku, 66(4), p.233 - 242, 2017/04
Times Cited Count：1 Percentile：2.86(Chemistry, Analytical)Insoluble cobalt ferrocyanide and sodium titanate specifically capture cesium and strontium ions, respectively, in water contaminated with radionuclides which is found in Fukushima Daiichi NPP. The inorganic compounds used in this study were formed as precipitates in the polymer chain grafted onto a commercially available 6-nylon fiber using radiation-induced graft polymerization. An impregnation structure with the precipitates entangled by the grafted polymer chain through an electrostatic interaction via multipoints was indicated. The resultant insoluble cobalt ferrocyanide- or sodium titanate-impregnated fiber exhibited a higher adsorption rate and adsorption capacity per gram of the inorganic compound for cesium or strontium ions in seawater than conventional granular adsorbents.
CsWatanabe, Ritsuko; Hattori, Yuya; Kai, Takeshi
International Journal of Radiation Biology, 92(11), p.660 - 664, 2016/11
Times Cited Count：3 Percentile：23.64(Biology)To understand the effect of internal exposure of Cs, we focus on estimation of microscopic energy deposition pattern and DNA damage induced by directly emitted electrons (beta-rays, internal conversion electrons, Auger electrons) from Cs. Monte Carlo track simulation method was used to calculate the microscopic energy deposition pattern. To simulate the energy deposition by directly emitted electrons, we considered the multiple ejections of electrons after internal conversion. Induction process of DNA strand breaks and base lesions was modeled and simulated using Monte Carlo methods for cell mimetic condition. The yield and spatial distribution of simple and complex DNA damage were calculated for the cases of -rays and electrons from Cs. The simulation showed that significant difference of DNA damage spectrum was not caused by the difference between secondary electron spectrum by -rays and directly ejected electron spectrum. The result support that the existing evaluation that internal exposure and external exposure are almost equivalent.
Cs in forest surface environments; Application to a contaminated forest site near Fukushima and assessment of potential impacts of soil organic matter interactionsOta, Masakazu; Nagai, Haruyasu; Koarashi, Jun
Science of the Total Environment, 551-552, p.590 - 604, 2016/05
Times Cited Count：38 Percentile：69.30(Environmental Sciences)A model for Cs transfer in forest was developed to assess behavior of Fukushima-derived Cs. The model simulation well reproduced observed 3 year migration of Cs in organic layer and mineral soil. Long-term predictions indicated that more than 90% of the deposited Cs remains in the top 5 cm soil till 30 years, suggesting that forest acts as a long-term reservoir of Cs with limited loss via groundwater pathway. Impacts of soil organic matter (SOM) on Cs dynamics were investigated by modifying parameters of Cs turnover. The results showed that SOM-induced reduction of Cs adsorption, slower fixation of Cs by clay and enhanced mobilization of the fixed Cs elevate soil-to-plant transfer of Cs by increasing fraction of dissolved Cs. A substantial proportion (27% 
73%) of Cs in these soils was delivered to horizons deeper than 5 cm decades later. These results suggested that SOM significantly influences behavior of Cs over long-term.
Yamasaki, Shinya*; Imoto, Jumpei*; Furuki, Genki*; Ochiai, Asumi*; Onuki, Toshihiko; Sueki, Keisuke*; Namba, Kenji*; Ewing, R. C.*; Utsunomiya, Satoshi*
Science of the Total Environment, 551-552, p.155 - 162, 2016/05
Times Cited Count：38 Percentile：68.42(Environmental Sciences)Cesium-137 (Cs) of estuary sediment impacted by the FDNPP was measured. Increasing radioactivity was observed from surface to bottom. 90% of the Cs was strongly bound to clay minerals in the estuary sediments. These results suggest that Cs is being transported from contaminated paddy fields to the estuary.
