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Saito, Tatsuo; Yamazawa, Hiromi*; Mochizuki, Akihito
Journal of Environmental Radioactivity, 255, p.107035_1 - 107035_14, 2022/12
Times Cited Count：0 Percentile：0.00(Environmental Sciences)The seasonal variation of dissolved U (DU) in Lake Biwa was reproduced by the following model and parameter research. The introduced models are the water-DU mass balance, and the ion exchange between UO
and H
on the lakeshore soil. The optimized parameters were the CEC of the lakeshore, TU as the sum of DU and AU (soil adsorbed U), kads and kdes as the first order reaction rate coefficients during rapid soil adsorption and desorption of U, respectively. Tabulated by the chemical equilibria constituting DU and analyzed the contribution of each chemical species, it is shown that the seasonal variation of DU is caused by the seasonal variation of pH. A correction to the ion-exchange equilibrium to shift to first order rate reaction only when the daily AU ratio increased above kads or decreased below kdes, improved the reproducibility of DU measurements and reproduced the delay of the DU peak from the pH peak.
Kumamaru, Hiroshige; ; Murata, Hideo; Kukita, Yutaka; Akiyama, Mamoru*; ; ; ; ; ; et al.
Proc. of ASME
JSME 4th Int. Conf. on Nuclear Engineering 1996 (ICONE-4), 1(PART B), p.669 - 674, 1996/00
no abstracts in English
Nagao, Seiya*;
Science of the Total Environment, 117-118, p.439 - 447, 1992/00
no abstracts in English
