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Journal Articles

Fabrication of low-O/M fast reactor MOX fuel and analysis on its oxygen potential behaviors

Hirooka, Shun; Vauchy, R.; Horii, Yuta; Sunaoshi, Takeo*; Saito, Kosuke

Proceedings of TopFuel 2025; Nuclear Reactor Fuel Performance Conference (Internet), 10 Pages, 2025/10

Reducing the oxygen-to-metal (O/M) ratio in MOX fuels plays an important role in suppressing the corrosion depth in the cladding due to fuel-cladding chemical interaction (FCCI), which is the key to determining the lifetime of fast reactor MOX fuels. Owing to a number of irradiation and post-irradiation experiments, a clear decreasing trend in the corrosion depth with lower O/M ratio in the as-fabricated MOX pellet was reported, whereas a significant redistribution of the O/M ratio in a pellet driven by the radial temperature gradient during irradiation could supply a higher oxygen potential near the pellet periphery where the FCCI should occur. The reduction of the O/M ratio in the MOX pellet fabrication processes can be achieved by heat treatment by taking high temperature, longer time, and lower oxygen partial pressure in the gas into account; the properties governing the reduction are not sufficiently studied. This study demonstrated the variation of O/M ratio in MOX pellets and the in-situ O/M ratio during the heat treatment was analyzed by using a thermogravimeter, which revealed a decreasing behavior during heating and dwell as well as an increasing behavior in the O/M ratio during the cooling step. Furthermore, the redistribution of O/M ratio, analyzed by Sari's model, was discussed to investigate the O/M ratio and the oxygen potential near the pellet periphery which is likely to have a more direct influence on the FCCI than the as-fabricated O/M ratio. By using the recent oxygen potential data on MOX, it is found that the oxygen potential profile in the radial direction is especially drastic near the pellet periphery and is sensitive to the as-fabricated O/M ratio.

JAEA Reports

Annual report of Engineering Services Department on JFY2023

Engineering Services Department, Nuclear Science Research Institute

JAEA-Review 2025-018, 83 Pages, 2025/09

JAEA-Review-2025-018.pdf:4.99MB

The Engineering Services Department is in charge of operation and maintenance of utility facilities (water distribution systems, electricity supply systems, steam generation systems and drain water systems etc.) in whole of the institute. And also is in charge of operation and maintenance of specific systems (power receiving and transforming facilities, an emergency electric power supply system, an air/liquid waste treatment system, a compressed air supply system) in nuclear reactor facilities, nuclear fuel material usage facilities and usual facilities or buildings. In addition, the department is in charge of maintenance of buildings, design and repair of electrical/mechanical equipment. This annual report describes summary of activities, operation and maintenance data and technical developments of the department carried out in JFY 2023. We hope that this report may help to future work.

Journal Articles

Control and irradiation behaviors of oxygen potential of MOX fuel

Hirooka, Shun; Vauchy, R.; Horii, Yuta; Sunaoshi, Takeo*; Saito, Kosuke; Ozawa, Takayuki

Proceedings of Workshop on Fuel Performance Assessment and Behaviour for Liquid Metal Cooled Fast Reactors (Internet), 8 Pages, 2025/07

no abstracts in English

Journal Articles

Multi-dimensional characteristics of upward bubbly flows in a vertical large-size square channel

Sun, Haomin; Kunugi, Tomoaki*; Yokomine, Takehiko*; Shen, X.*; Hibiki, Takashi*

International Journal of Heat and Mass Transfer, 211, p.124214_1 - 124214_17, 2023/09

 Times Cited Count:7 Percentile:51.27(Thermodynamics)

Journal Articles

The Development of a Multiphysics Coupled Solver for Studying the Effect of Dynamic Heterogeneous Configuration on Particulate Debris Bed Criticality and Cooling Characteristics

Li, C.-Y.; Wang, K.*; Uchibori, Akihiro; Okano, Yasushi; Pellegrini, M.*; Erkan, N.*; Takata, Takashi*; Okamoto, Koji*

Applied Sciences (Internet), 13(13), p.7705_1 - 7705_29, 2023/07

 Times Cited Count:2 Percentile:24.15(Chemistry, Multidisciplinary)

Journal Articles

Recent studies on fuel properties and irradiation behaviors of Am/Np-bearing MOX

Hirooka, Shun; Yokoyama, Keisuke; Kato, Masato

Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Sustainable Clean Energy for the Future (FR22) (Internet), 8 Pages, 2022/04

Property studies on Am/Np-bearing MOX were carried out and how the properties influences on the irradiation behaviors was discussed. Both Am and Np inclusions increase the oxygen potential of MOX. Inter-diffusion coefficients obtained by using diffusion couple technique indicate that the inter-diffusion coefficient is larger in the order of U-Am, U-Pu and U-Np. Also, the inter-diffusion coefficients were evaluated to be larger at the O/M = 2 than those of O/M $$<$$ 2 by several orders. The increase of oxygen potential with Am/Np leads to higher vapor pressure of UO$$_{3}$$ and the acceleration of the pore migration along temperature gradient during irradiation. The redistributions of actinide elements were also considered with the relationship of the pore migration and diffusion in solid state. Thus, the obtained inter-diffusion coefficients directly influence on the redistribution rate. The obtained properties were modelled and can be installed in a fuel irradiation simulation code.

JAEA Reports

Annual report of Engineering Services Department on JFY2020

Engineering Services Department, Nuclear Science Research Institute

JAEA-Review 2021-054, 85 Pages, 2022/01

JAEA-Review-2021-054.pdf:95.12MB

The Engineering Services Department is in charge of operation and maintenance of utility facilities (water distribution systems, electricity supply systems, steam generation systems and drain water systems etc.) in whole of the institute. And also is in charge of operation and maintenance of specific systems (power receiving and transforming facilities, an emergency electric power supply system, an air/liquid waste treatment system, a compressed air supply system) in nuclear reactor facilities, nuclear fuel treatment facilities and usual facilities or buildings. In addition, the department is in charge of maintenance of buildings, design and repair of electrical/mechanical equipments. This annual report describes summary of activities, operation and maintenance data and technical developments of the department carried out in JFY 2020. We hope that this report may help to future work.

Journal Articles

An Investigation on the control rod homogenization method for next-generation fast reactor cores

Takino, Kazuo; Sugino, Kazuteru; Oki, Shigeo

Annals of Nuclear Energy, 162, p.108454_1 - 108454_7, 2021/11

 Times Cited Count:1 Percentile:7.55(Nuclear Science & Technology)

JAEA Reports

Annual report of Engineering Services Department on JFY2019

Engineering Services Department, Nuclear Science Research Institute

JAEA-Review 2021-011, 86 Pages, 2021/08

JAEA-Review-2021-011.pdf:5.35MB

The Engineering Services Department is in charge of operation and maintenance of utility facilities (water distribution systems, electricity supply systems, steam generation systems and drain water systems etc.) in whole of the institute. And also is in charge of operation and maintenance of specific systems (power receiving and transforming facilities, an emergency electric power supply system, an air/liquid waste treatment system, a compressed air supply system) in nuclear reactor facilities, nuclear fuel treatment facilities and usual facilities or buildings. In addition, the department is in charge of maintenance of buildings, design and repair of electrical/mechanical equipments. This annual report describes summary of activities, operation and maintenance data and technical developments of the department carried out in JFY 2019. We hope that this report may help to future work.

Journal Articles

Analytical study on removal mechanisms of cesium aerosol from a noble gas bubble rising through liquid sodium pool, 2; Effects of particle size distribution and agglomeration in aerosols

Miyahara, Shinya*; Kawaguchi, Munemichi; Seino, Hiroshi; Atsumi, Takuto*; Uno, Masayoshi*

Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 6 Pages, 2021/08

In a postulated accident of fuel pin failure of sodium cooled fast reactor, a fission product cesium will be released from the failed pin as an aerosol such as cesium iodide and/or cesium oxide together with a fission product noble gas such as xenon and krypton. As the result, the xenon and krypton released with cesium aerosol into the sodium coolant as bubbles have an influence on the removal of cesium aerosol by the sodium pool in a period of bubble rising to the pool surface. In this study, cesium aerosol removal behavior due to inertial deposition, sedimentation and diffusion from a noble gas bubble rising through liquid sodium pool was analyzed by a computer program which deals with the expansion and the deformation of the bubble together with the aerosol absorption considering the effects of particle size distribution and agglomeration in aerosols. In the analysis, initial bubble diameter, sodium pool depth and temperature, aerosol particle diameter and density, initial aerosol concentration in the bubble were changed as parameter, and the results for the sensitivities of these parameters on decontamination factor (DF) of cesium aerosol were compared with the results of the previous study in which the effects of particle size distribution and agglomeration in aerosols were not considered. From the results, it was concluded that the sensitivities of initial bubble diameter, the aerosol particle diameter and density to the DF became significant due to the inertial deposition of agglomerated aerosols. To validate these analysis results, the simulation experiments have been conducted using a simulant particles of cesium aerosol under the condition of room temperature in water pool and air bubble systems. The experimental results were compared with the analysis results calculated under the same condition.

Journal Articles

Derivation of ideal power distribution to minimize the maximum kernel migration rate for nuclear design of pin-in-block type HTGR

Okita, Shoichiro; Fukaya, Yuji; Goto, Minoru

Journal of Nuclear Science and Technology, 58(1), p.9 - 16, 2021/01

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Suppressing the kernel migration rates, which depend on both the fuel temperature and the fuel temperature gradient, under normal operation condition is quite important from the viewpoint of the fuel integrity for High Temperature Gas-cooled Reactors. The presence of the ideal axial power distribution to minimize the maximum kernel migration rate allows us to improve efficiency of design work. Therefore, we propose a new method based on Lagrange multiplier method in consideration of thermohydraulic design in order to obtain the ideal axial power distribution to minimize the maximum kernel migration rate. For one of the existing conceptual designs performed by JAEA, the maximum kernel migration rate for the power distribution to minimize the maximum kernel migration rate proposed in this study is lower by approximately 10% than that for the power distribution as a conventional design target to minimize the maximum fuel temperature.

JAEA Reports

Annual report of Engineering Services Department on JFY2018

Engineering Services Department, Nuclear Science Research Institute

JAEA-Review 2019-044, 96 Pages, 2020/03

JAEA-Review-2019-044.pdf:6.11MB

The Engineering Services Department is in charge of operation and maintenance of utility facilities (water distribution systems, electricity supply systems, steam generation systems and drain water systems etc.) in whole of the institute. And also is in charge of operation and maintenance of specific systems (power receiving and transforming facilities, an emergency electric power supply system, an air/liquid waste treatment system, a compressed air supply system) in nuclear reactor facilities, nuclear fuel treatment facilities and usual facilities or buildings. In addition, the department is in charge of maintenance of buildings, design and repair of electrical/mechanical equipments. This annual report describes summary of activities, operation and maintenance data and technical developments of the department carried out in JFY 2018. We hope that this report may help to future work.

Journal Articles

A Study on self-terminating behavior of sodium-concrete reaction, 2

Kawaguchi, Munemichi; Miyahara, Shinya; Uno, Masayoshi*

Journal of Nuclear Science and Technology, 55(8), p.874 - 884, 2018/08

 Times Cited Count:4 Percentile:30.18(Nuclear Science & Technology)

As parts of severe accident studies in sodium-cooled fast reactor, experiments were performed to investigate the termination mechanism of sodium-concrete reaction (SCR). In the experiment, the reaction time was controlled to investigate the distribution change of sodium (Na) and the reaction products in the pool and around the reaction front. In the results, the Na around the reaction front decreased from the enough amount with the reaction time. The concentrations were 18-24 wt.% for Na, and 22-18 wt.% for Si after the termination. From the thermodynamics calculations, the stable materials around the reaction front comprised more than 90 wt.% solid products such as Na$$_{2}$$SiO$$_{3}$$, and no Na. Further, the distribution of Na and reaction products could be explained by a steady-state sedimentation-diffusion model. At the early stage of SCR, the reaction products were suspended as particles in the Na pool because of the high H$$_{2}$$-generation rate. As the concrete ablation proceeds, they start settling down due to the decreased H$$_{2}$$-generation rate, thereby allowing SCR termination. It was concluded that SCR termination was caused by the sediment of the reaction products and the lack of Na around the reaction front.

Journal Articles

Identification of penetration path and deposition distribution of radionuclides in houses by experiments and numerical model

Hirouchi, Jun; Takahara, Shogo; Iijima, Masashi; Watanabe, Masatoshi; Munakata, Masahiro

Radiation Physics and Chemistry, 140, p.127 - 131, 2017/11

BB2016-0282.pdf:0.39MB

 Times Cited Count:3 Percentile:23.33(Chemistry, Physical)

Journal Articles

On-line subcriticality measurement using a pulsed spallation neutron source

Iwamoto, Hiroki; Nishihara, Kenji; Yagi, Takahiro*; Pyeon, C.-H.*

Journal of Nuclear Science and Technology, 54(4), p.432 - 443, 2017/04

 Times Cited Count:20 Percentile:83.30(Nuclear Science & Technology)

Journal Articles

Application of turbidity measurement for evaluation of two-phase separation in ${it N}$,${it N}$-dialkylamides-nitric acid systems

Tsutsui, Nao; Ban, Yasutoshi; Hakamatsuka, Yasuyuki; Urabe, Shunichi; Matsumura, Tatsuro

Proceedings of 21st International Conference & Exhibition; Nuclear Fuel Cycle for a Low-Carbon Future (GLOBAL 2015) (USB Flash Drive), p.1153 - 1157, 2015/09

${it N}$,${it N}$-Dialkylamides are promising alternative extractants to tri-${it n}$-butyl phosphate in the reprocessing of spent nuclear fuels, but the two-phase separation between their organic and aqueous phases has not been evaluated quantitatively. ${it N}$,${it N}$-Di(2-ethylhexyl)-2,2-dimethylpropanamide (DEHDMPA) in ${it n}$-dodecane were agitated with uranyl nitrate-containing nitric acid, and their turbidities and their uranium distribution ratios were measured with respect to the time for the quantitative evaluation. Increasing DEHDMPA, uranium, and nitric acid concentrations enhanced turbidities. Although turbidities decreased with respect to the time, uranium distribution ratios slightly changed, indicating the observed turbidities did not affect these uranium distribution ratios significantly. Therefore, DEHDMPA may act as suitable extractant for uranium in nitric acid from two-phase separation viewpoint, and turbidity may be an indicator for extractant performance evaluation.

Journal Articles

Anthropogenic radionuclides in seawater of the Japan Sea; The Results of recent observations and the temporal change of concentrations

Ito, Toshimichi; Aramaki, Takafumi*; Otosaka, Shigeyoshi; Suzuki, Takashi; Togawa, Orihiko; Kobayashi, Takuya; Kawamura, Hideyuki; Amano, Hikaru; Senju, Tomoharu*; Chaykovskaya, E. L.*; et al.

Journal of Nuclear Science and Technology, 42(1), p.90 - 100, 2005/01

 Times Cited Count:14 Percentile:65.85(Nuclear Science & Technology)

During 1996-2002, a wide-area research project on anthropogenic radionuclides was done in the Japanese and Russian EEZ of the Japan Sea to investigate their migration. As the results of expeditions in 2001 and 2002, (1) the concentrations and distributions of radionuclides are similar to the results of previous, (2) inventories of these radionuclides indicate accumulation in the Japan Sea seawater compared to the amounts supplied by global fallout, (3) $$^{90}$$Sr and $$^{137}$$Cs concentrations in intermediate layer show temporal variations, and 4) the variations may reflect the water mass movement in upper part of the Japan Sea.

Journal Articles

Neutron spectra and angular distributions of concrete-moderated neutron calibration fields at JAERI

Yoshizawa, Michio; Tanimura, Yoshihiko; Saegusa, Jun; Nemoto, Hisashi*; Yoshida, Makoto

Radiation Protection Dosimetry, 110(1-4), p.81 - 84, 2004/09

 Times Cited Count:3 Percentile:22.47(Environmental Sciences)

The facility of Radiation Standards (FRS) of JAERI has equipped with the concrete-moderated neutron calibration fields as simulated workplace neutron fields. The fields use an Am-Be (37GBq) neutron source placed in the narrow space surrounded by concrete wall and bricks to produce scattered neutrons. The neutron spectra of the fields were measured with Bonner multi-sphere spectrometer system (BMS), spherical recoil-proton proportional counters (RPCs), and a liquid scintillation counter (NE-213). The results were compared with each other, and the neutron spectra and the ambient dose equivalent rate, ${it H}$$$^{*}$$(10), were agreed well within the uncertainty. The angular distributions of neutron fluence were calculated by the MCNP-4B2 Monte Carlo code to obtain the reference personal dose equivalent rate, ${it H}$$$_{p}$$(10). The calculated results show that the scattered neutrons have a wide variety of incident angles. The reference ${it H}$$$_{p}$$(10) values considered the angular distribution were found to be 10-18% smaller than those without consideration.

Journal Articles

Coupled hydrogen moderator optimization with ortho/para hydrogen ratio

Kai, Tetsuya; Harada, Masahide; Teshigawara, Makoto; Watanabe, Noboru; Ikeda, Yujiro

Nuclear Instruments and Methods in Physics Research A, 523(3), p.398 - 414, 2004/05

 Times Cited Count:40 Percentile:89.82(Instruments & Instrumentation)

Neutronic performance of a coupled hydrogen moderator was studied as a function of para hydrogen concentration, moderator thickness, height and premoderator thickness. It was found that a thick (120$$sim$$140mm) moderator with 100% para hydrogen was optimal to provide the highest time- and energy- integrated neutron intensity below 15 meV together with the highetst possible pulse-peak intensity. Low-energy neutron distribution on the moderator viewed surface was found to exhibit an intensity-enhanced region at a picture frame part near premoderator. The rather peculiar distribution suggested that the moderator and the viewed surface must be designed so as to take the brighter region near premoderator in use.

Journal Articles

Subchannel analysis of CHF experiments for tight-lattice core

Nakatsuka, Toru; Tamai, Hidesada; Kureta, Masatoshi; Okubo, Tsutomu; Akimoto, Hajime; Iwamura, Takamichi

Proceedings of International Conference on Global Environment and Advanced Nuclear Power Plants (GENES4/ANP 2003) (CD-ROM), 6 Pages, 2003/09

It is important to evaluate thermal margin of the tight lattice core in the Reduced-Moderation Water reactor (RMWR). In the present study, to assess the applicability of subchannel analysis for tight lattice cores, tight lattice CHF experiments were analyzed with COBRA-TF code. For the axial uniform heated rod bundle, the code gives good prediction of critical power for mass velocity of around 500kg/(m$$^{2}$$s), while the code underestimates it for lower mass velocity and overestimates for higher mass velocity. The predicted BT position was outer channels and differed from the measured position. For the axially double-humped heated bundle, the code gives good prediction for mass velocity of around 200kg/(m$$^{2}$$s), and overestimates for higher mass velocity. It turned out that the two-phase multiplier of friction loss have a large influences on the flow distribution among the subchannels. To improve the calculation accuracy, it is required to predict precisely the flow distribution including the prediction of pressure distribution in a tight lattice bundle.

64 (Records 1-20 displayed on this page)