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JAEA Reports

"J-PARC Hello Science" outreach activity of J-PARC Center

Sakamoto, Shinichi

JAEA-Review 2020-014, 63 Pages, 2020/09


J-PARC Center has been promoting several public relations activities to appeal the cutting-edge research programs and their outputs to the citizen, especially in Ibaraki prefecture and Tokai village. The Public Relations Section put weight to outreach events as the best tool for this purpose, such as site tour, open house, and summer school. Here the outreach activities are summarized mainly from FY2012 to FY2019.

Journal Articles

Measurement of nuclide production cross section for lead and bismuth with proton in energy range from 0.4 GeV to 3.0 GeV

Matsuda, Hiroki; Meigo, Shinichiro; Iwamoto, Hiroki; Maekawa, Fujio

EPJ Web of Conferences, 239, p.06004_1 - 06004_4, 2020/09

For the Accelerator-Driven nuclear transmutation System (ADS), nuclide production yield estimation in the lead-bismuth target is important to manage the target. However, experimental data of nuclide production yield by spallation and high-energy fission reactions are scarce. In order to obtain the experimental data, we experimented in J-PARC using $$^{mathrm{nat}}$$Pb and $$^{mathrm{209}}$$Bi samples. The samples were irradiated with protons at various kinematic energy points between 0.4 and 3.0 GeV. After the irradiation, the nuclide production cross section over $$^{mathrm{7}}$$Be to $$^{mathrm{183}}$$Re was obtained by spectroscopic measurement of decay gamma-rays from the samples with HPGe detectors. The present experimental results were compared with the evaluated data (JENDL-HE/2007) and the calculation with the PHITS code and the INCL++ code. The present experiment data showed consistency with other experimental data with better accuracy than other ones. In reactions to produce light nuclides, JENDL and calculation with the PHITS and INCL++ for $$^{mathrm{7}}$$Be production agreed with the data.$$^{mathrm{22}}$$Na production, however, underestimated about 1/10 times. For middle to heavy nuclide productions cases, both calculations agreed with the experiment by a factor of two. JENDL showed lower energy having a maximum value of excitation function maximal value than the experimental data.

Journal Articles

Strong lattice anharmonicity exhibited by the high-energy optical phonons in thermoelectric material

Wu, P.*; Fan, F.-R.*; Hagihara, Masato*; Kofu, Maiko; Peng, K.*; Ishikawa, Yoshihisa*; Lee, S.*; Honda, Takashi*; Yonemura, Masao*; Ikeda, Kazutaka*; et al.

New Journal of Physics (Internet), 22(8), p.083083_1 - 083083_9, 2020/08

 Times Cited Count:0 Percentile:100(Physics, Multidisciplinary)

Thermoelectric material SnSe has aroused world-wide interests in the past years, and its inherent strong lattice anharmonicity is regarded as a crucial factor for its outstanding thermoelectric performance. However, the understanding of lattice anharmonicity in SnSe system remains inadequate, especially regarding how phonon dynamics are affected by this behavior. In this work, we present a comprehensive study of lattice dynamics on Na$$_{0.003}$$Sn$$_{0.997}$$Se$$_{0.9}$$S$$_{0.1}$$ by means of neutron total scattering, inelastic neutron scattering, Raman spectroscopy as well as frozen-phonon calculations. Lattice anharmonicity is evidenced by pair distribution function, inelastic neutron scattering and Raman measurements. By separating the effects of thermal expansion and multi-phonon scattering, we found that the latter is very significant in high-energy optical phonon modes. The strong temperature-dependence of these phonon modes indicate the anharmonicity in this system. Moreover, our data reveals that the linewidths of high-energy optical phonons become broadened with mild doping of sulfur. Our studies suggest that the thermoelectric performance of SnSe could be further enhanced by reducing the contributions of high-energy optical phonon modes to the lattice thermal conductivity via phonon engineering.

Journal Articles

$$q$$=0 long-range magnetic order in centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O; A Spin-$$frac{1}{2}$$ perfect kagome antiferromagnet with $$J_{1}$$-$$J_{2}$$-$$J_{d}$$

Iida, Kazuki*; Yoshida, Hiroyuki*; Nakao, Akiko*; Jeschke, H. O.*; Iqbal, Y.*; Nakajima, Kenji; Kawamura, Seiko; Munakata, Koji*; Inamura, Yasuhiro; Murai, Naoki; et al.

Physical Review B, 101(22), p.220408_1 - 220408_6, 2020/06

Crystal and magnetic structures of the mineral centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O are investigated by means of synchrotron X-ray diffraction and neutron diffraction measurements complemented by density functional theory (DFT) and pseudofermion functional renormalization group (PFFRG) calculations. In CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O, Cu$$^{2+}$$ ions form a geometrically perfect kagome network with antiferromagnetic $$J_{1}$$. No intersite disorder between Cu$$^{2+}$$ and Ca$$^{2+}$$ ions is detected. CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O enters a magnetic long-range ordered state below $$T_{rm N}$$ = 7.2 K, and the $$q$$=0 magnetic structure with negative vector spin chirality is obtained. The ordered moment at 0.3 K is suppressed to 0.58(2)$$mu$$B. Our DFT calculations indicate the presence of antiferromagnetic $$J_{2}$$ and ferromagnetic $$J_{d}$$ superexchange couplings of a strength which places the system at the crossroads of three magnetic orders (at the classical level) and a spin-$$frac{1}{2}$$ PFFRG analysis shows a dominance of $$q$$=0 type magnetic correlations, consistent with and indicating proximity to the observed $$q$$=0 spin structure. The results suggest that this material is located close to a quantum critical point and is a good realization of a $$J_{1}$$-$$J_{2}$$-$$J_{d}$$ kagome antiferromagnet.

Journal Articles

Ultralow thermal conductivity from transverse acoustic phonon suppression in distorted crystalline $$alpha$$-MgAgSb

Li, X.*; Liu, P.-F.*; Zhao, E.*; Zhang, Z.*; Guide, T.*; Le, M. D.*; Avdeev, M.*; Ikeda, Kazutaka*; Otomo, Toshiya*; Kofu, Maiko; et al.

Nature Communications (Internet), 11(1), p.942_1 - 942_9, 2020/02

 Times Cited Count:2 Percentile:28.87(Multidisciplinary Sciences)

In high-performance thermoelectric materials, there are two main low thermal conductivity mechanisms: the phonon anharmonic and phonon scattering resulting from the dynamic disorder, which have been successfully revealed by inelastic neutron scattering. Using neutron scattering and ab initio calculations, we report here a mechanism of static local structure distortion combined with phonon-anharmonic-induced ultralow lattice thermal conductivity in $$alpha$$-MgAgSb. Since the transverse acoustic phonons are almost fully scattered by the intrinsic distorted rocksalt sublattice in this compound, the heat is mainly transported by the longitudinal acoustic phonons. The ultralow thermal conductivity in $$alpha$$-MgAgSb is attributed to its atomic dynamics being altered by the structure distortion, which presents a possible microscopic route to enhance the performance of similar thermoelectric materials.

Journal Articles

J-PARC RCS; High-order field components inherent in the injection bump magnets and their effects on the circulating beam during multi-turn injection

Hotchi, Hideaki; Harada, Hiroyuki; Takayanagi, Tomohiro

Journal of Physics; Conference Series, 1350, p.012102_1 - 012102_5, 2019/11

 Times Cited Count:1 Percentile:17.12

Journal Articles

The Analytical study of inventories and physicochemical configuration of spallation products produced in Lead-Bismuth Eutectic of Accelerator Driven System

Miyahara, Shinya*; Ohdaira, Naoya*; Arita, Yuji*; Maekawa, Fujio; Matsuda, Hiroki; Sasa, Toshinobu; Meigo, Shinichiro

Nuclear Engineering and Design, 352, p.110192_1 - 110192_8, 2019/10

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Lead-Bismuth Eutectic (LBE) is used as a spallation neutron target and coolant materials of Accelerator Driven System (ADS), and many kinds of elements are produced as spallation products. It is important to evaluate the release and transport behavior of the spallation products in the LBE. The inventories and the physicochemical composition of the spallation products produced in LBE have been investigated for an LBE loop in the ADS Target Test Facility (TEF-T) in J-PARC. The inventories of the spallation products in the LBE were estimated using the PHITS code. The physicochemical composition of the spallation products in the LBE was calculated using the Thermo-Calc code under the conditions of the operation temperatures of LBE from 350$$^{circ}$$C to 500$$^{circ}$$C and the oxygen concentrations in LBE from 10 ppb to 1 ppm. The calculation showed that the 5 elements of Rb, Tl, Tc, Os, Ir, Pt, Au and Hg were soluble in LBE under the all given conditions and any kinds of compound were not formed in LBE. It was suggested that the oxides of Ce, Sr, Zr and Y were stable as CeO$$_{2}$$, SrO, ZrO$$_{2}$$ and Y$$_{2}$$O$$_{3}$$ in the LBE.

JAEA Reports

Improvement of accumulator in cryogenic hydrogen system used for 1-MW pulsed spallation neutron source

Aso, Tomokazu; Tatsumoto, Hideki*; Otsu, Kiichi*; Kawakami, Yoshihiko*; Komori, Shinji*; Muto, Hideki*; Takada, Hiroshi

JAEA-Technology 2019-013, 77 Pages, 2019/09


At Materials and Life Science experimental Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), a 1-MW pulsed spallation neutron source is equipped with a cryogenic hydrogen system which circulates liquid hydrogen (20 K and 1.5 MPa) to convert high energy neutrons generated at a mercury target to cold neutrons at three moderators with removing nuclear heat of 3.8 kW deposited there. The cryogenic system includes an accumulator with a bellows structure in order to absorb pressure fluctuations generated by the nuclear heat deposition in the system. Welded inner bellows of the first accumulator was failured during operation, forcing us to improve the accumulator to have sufficient pressure resistance and longer life-time. We have developed elemental technologies for manufacturing welded bellows of the accumulator by a thick plate with high pressure resistance, succeeding to find optimum welding conditions. We fabricated a prototype bellows block and carried out an endurance test by adding a pressure change of 2 MPa repeatedly. As a result, the prototype bellows was successfully in use exceeding the design life of 10,000 times. Since distortions given during welding and assembling affect functionality and lifetime of the bellows, we set the levelness of each element of the bellows as within 0.1$$^{circ}$$. The improved accumulator has already been in operation for about 25,000 hours as of January 2019, resulting that the number of strokes reached to 16,000. In July 2018, we demonstrated that the accumulator could suppress the pressure fluctuation generated by the 932 kW beam injection as designed. As current operational beam power is 500 kW, the current cryogenic hydrogen system could be applicable for stable operation at higher power in the future.

JAEA Reports

Development of prototype for TEF-T integral control system of J-PARC

Sakai, Kenji; Obayashi, Hironari; Saito, Shigeru; Sasa, Toshinobu; Sugawara, Takanori; Watanabe, Akihiko*

JAEA-Technology 2019-009, 18 Pages, 2019/07


Construction of Transmutation Experimental Facility (TEF) is under planning in the Japan Proton Accelerator Research Complex (J-PARC) program to promote R&D on the transmutation technology with using accelerator driven systems (ADS). ADS Target Test Facility (TEF-T) in TEF will develop spallation target technology and study on target materials with irradiating high intensity proton beams on a lead-bismuth eutectic (LBE) target. For safe and efficient beam operation, a general control system (GCS) will be constructed in TEF-T. GCS comprises several subsystems, such as a network system (LAN), an integral control system (ICS), an interlock system (ILS), and a timing distribution system (TDS) according to their roles. Especially, the ICS plays the important role that executes integral operations in the entire facility, acquires, stores and distributes operation data. We planned to develop a prototype of the ICS, to evaluate its concrete performances such as data transmission speeds, data storage capability, control functions, long-term stability of the system, and to utilize them for design of the actual ICS. This report mentions to product the prototype of ICS and to apply it to remote operations of instruments for developing LBE target technology.

Journal Articles

Beam dynamics study for beam loss mitigation in the J-PARC RCS

Hotchi, Hideaki; Harada, Hiroyuki; Okabe, Kota; Saha, P. K.; Shobuda, Yoshihiro; Tamura, Fumihiko; Yoshimoto, Masahiro

Kasokuki, 16(2), p.109 - 118, 2019/07

no abstracts in English

Journal Articles

Background issues encountered by cold-neutron chopper spectrometer AMATERAS

Kikuchi, Tatsuya*; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro; Nakamura, Mitsutaka; Wakai, Daisuke*; Aoyama, Kazuhiro*; Iwahashi, Takaaki*; Kambara, Wataru*

Physica B; Condensed Matter, 564, p.45 - 53, 2019/07

 Times Cited Count:0 Percentile:100(Physics, Condensed Matter)

Details of the background, that is, unwanted signals accumulated by the data acquisition system of neutron instruments, observed by the cold-neutron chopper spectrometer AMATERAS installed at the Materials and Life Science Experimental Facility at J-PARC are reported. In the design phase of AMATERAS, we carefully considered the achievement of high signal-to-noise ratio, and possible countermeasures were implemented. Actually, recent scientific outputs from AMATERAS indicates that the spectrometer is one of excellent neutron instruments with low background. In spite of that, in nine years of AMATERAS operation, we have encountered unwanted signals due to various reasons, including gamma-rays emitted at materials on or near the beam line including the sample itself, scattered neutrons from the beam line devices, air scattering, electronic noise in data acquisition system, cosmic rays, T0 burst, and other unknown sources. In this report, we discuss the background observed by AMATERAS, especially in the conditions of without samples, comprehensively. The possible sources of these signals and the countermeasures considered against the above sources are discussed, which may be helpful to those who are engaged in other existing or planned neutron-scattering instruments.

Journal Articles

Localized magnetic excitations in the fully frustrated dimerized magnet Ba$$_{2}$$CoSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$

Kurita, Nubuyuki*; Yamamoto, Daisuke*; Kanesaka, Takuya*; Furukawa, Nobuo*; Kawamura, Seiko; Nakajima, Kenji; Tanaka, Hidekazu*

Physical Review Letters, 123(2), p.027206_1 - 027206_6, 2019/07

 Times Cited Count:0 Percentile:100(Physics, Multidisciplinary)

Journal Articles

Recent progress of the J-PARC RCS beam commissioning and operation; Efforts to realize a higher beam power beyond 1 MW

Hotchi, Hideaki; Harada, Hiroyuki; Hayashi, Naoki; Kinsho, Michikazu; Okabe, Kota; Saha, P. K.; Shobuda, Yoshihiro; Tamura, Fumihiko; Yamamoto, Kazami; Yamamoto, Masanobu; et al.

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.574 - 578, 2019/07

no abstracts in English

Journal Articles

Study of heavy ion acceleration in J-PARC

Harada, Hiroyuki; Saha, P. K.; Kinsho, Michikazu

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.179 - 182, 2019/07

Recently, humankind had big discovery about neutron star, which is great big nuclear in the space. They are discovery of neutron star with twice mass of solar in 2010 and observation of gravity wave when two neutron start incorporate in 2017. In order to understand the high dense matter like the neutron star, project of experimental researches by using accelerated heavy ion beams become heated in the world, such RHIC-BES-II program, FAIR project, NICA project, etc. The J-PARC provides MW class high intensity proton beams to many experiments and researches. We have study of the heavy ion beam in J-PARC to fully utilize high intensity ability of J-PARC. We propose the accelerator scheme of the beam in J-PARC and the intensity will reach to the world record. In our talk, we will report the current status of proton beam and the accelerator scheme for the high-intensity heavy ion beam in J-PARC.

Journal Articles

Progress of long-time operation and industrial use of negative ion source for particle accelerator

Oguri, Hidetomo

Purazuma, Kaku Yugo Gakkai-Shi, 95(7), p.340 - 344, 2019/07

no abstracts in English

JAEA Reports

Assessment report on research and development activities in FY 2018; Activity "Research and development on J-PARC" (Interim report)

J-PARC Center

JAEA-Evaluation 2019-003, 52 Pages, 2019/06


Evaluation Committee of Research Activities for J-PARC for interim assessment of Japan Proton Accelerator Research Complex evaluated the management and research activities of J-PARC center on the explanatory documents and oral presentations during the period from April 2015 to December 2018. This report summarizes the results of the assessment by the Committee with the Committee report attached.

Journal Articles

Study on beam dynamics of high intensity proton beam and mitigation of beam loss in J-PARC RCS

Hotchi, Hideaki

FAS Dayori (Internet), (18), p.20 - 26, 2019/06

no abstracts in English

Journal Articles

Measurements of the $$^{243}$$Am neutron capture and total cross sections with ANNRI at J-PARC

Kimura, Atsushi; Nakamura, Shoji; Terada, Kazushi*; Nakao, Taro*; Mizuyama, Kazuhito*; Iwamoto, Nobuyuki; Iwamoto, Osamu; Harada, Hideo; Katabuchi, Tatsuya*; Igashira, Masayuki*; et al.

Journal of Nuclear Science and Technology, 56(6), p.479 - 492, 2019/06

 Times Cited Count:1 Percentile:56.06(Nuclear Science & Technology)

Journal Articles

Evidence for singular-phonon-induced nematic superconductivity in a topological superconductor candidate Sr$$_{0.1}$$Bi$$_{2}$$Se$$_{3}$$

Wang, J.*; Ran, K.*; Li, S.*; Ma, Z.*; Bao, S.*; Cai, Z.*; Zhang, Y.*; Nakajima, Kenji; Kawamura, Seiko; $v{C}$erm$'a$k, P.*; et al.

Nature Communications (Internet), 10, p.2802_1 - 2802_6, 2019/06

 Times Cited Count:7 Percentile:12.06(Multidisciplinary Sciences)

Journal Articles

J-PARC RCS; High-order field components inherent in the injection bump magnets and their effects on the circulating beam during multi-turn injection

Hotchi, Hideaki; Harada, Hiroyuki; Takayanagi, Tomohiro

Proceedings of 10th International Particle Accelerator Conference (IPAC '19) (Internet), p.2009 - 2012, 2019/06

456 (Records 1-20 displayed on this page)