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JAEA Reports

Development of mock-up test loop (IMMORTAL) for LBE spallation target

Obayashi, Hironari; Yamaki, Kenichi*; Yoshimoto, Hidemitsu*; Kita, Satoshi*; Wan, T.*; Sasa, Toshinobu

JAEA-Technology 2021-035, 66 Pages, 2022/03

JAEA-Technology-2021-035.pdf:4.26MB

Construction of Transmutation Experimental Facility (TEF) is under planning in Japan Proton Accelerator Research Complex (J-PARC) program to promote R&Ds on realization of transmutation technology by an accelerator driven system (ADS). As a facility of TEF, ADS Target Test Facility (TEF-T) will provide a spallation target to study target technology and perform post irradiation examination (PIE) of candidate materials of ADS. In ADS, lead-bismuth eutectic (LBE) alloy is used as a spallation target material and a core coolant. As is well known, LBE has corrosive to structural materials hence each component of the target system should provide compatibility with LBE. In addition, instrumentations for LBE are restricted by the target operation condition such as high temperature and irradiation environment. The devices for LBE have been developed individually to achieve the LBE target system. "Integrated Multi-functional MOckup for TEF-T Real-scale TArget Loop, IMMORTAL" was fabricated as a mock-up test loop of the target for the purpose of the integration testing of individually developed devices. This report describes an overview of IMMORTAL and the design of the installed devices.

JAEA Reports

Neutronic analysis of beam window and LBE of an Accelerator-Driven System

Nakano, Keita; Iwamoto, Hiroki; Nishihara, Kenji; Meigo, Shinichiro; Sugawara, Takanori; Iwamoto, Yosuke; Takeshita, Hayato*; Maekawa, Fujio

JAEA-Research 2021-018, 41 Pages, 2022/03

JAEA-Research-2021-018.pdf:2.93MB

Neutronic analysis of beam window of the Accelerator-Driven System (ADS) proposed by Japan Atomic Energy Agency (JAEA) has been conducted using PHITS and DCHAIN-PHITS codes. We investigate gas production of hydrogen and helium isotopes in the beam window, displacement per atom of beam window material, and heat generation in the beam window. In addition, distributions of produced nuclides, heat density, and activity are derived. It was found that at the maximum 12500 appm H production, 1800 appm He production, and damage of 62.1 DPA occurred in the beam window by the ADS operation. On the other hand, the maximum heat generation in the beam window was 374 W/cm$$^3$$. In the analysis of LBE, $$^{206}$$Bi and $$^{210}$$Po were found to be the dominant nuclides in decay heat and radioactivity. Furthermore, the heat generation in the LBE by the proton beam was maximum around 5 cm downstream of the beam window, which was 945 W/cm$$^3$$.

Journal Articles

Development of a miniature electromagnet probe for the measurement of local velocity in heavy liquid metals

Ariyoshi, Gen; Obayashi, Hironari; Sasa, Toshinobu

Journal of Nuclear Science and Technology, 18 Pages, 2022/03

 Times Cited Count:0 Percentile:0.03(Nuclear Science & Technology)

Electromagnetic induction method is one of the effective techniques for local velocity measurement in heavy liquid metals. Ricou and Vives' probe and Von Weissenfluh's probe are famous instrumentations using a permanent magnet. However, sensitivity and measurement volume of the probes show unexpected variation since demagnetization of the magnet is occurred by temperature increase up to the Curie temperature. In this study, electromagnetic probe incorporating a miniature electromagnet was newly developed to overcome such unexpected variation. The diameter and the length of the sensor was 6 mm and 155 mm, respectively. The sensitivity and the measurement volume of the probe were assessed by measurement of local velocity of flowing mercury in a square channel. To clarify the validity for the measured velocity profiles, numerical velocity profiles were calculated and compared with experiment. And the validity for the measured velocity profiles were confirmed by calculated result.

Journal Articles

CFD analysis of natural circulation in LBE-cooled accelerator-driven system

Sugawara, Takanori; Watanabe, Nao; Ono, Ayako; Nishihara, Kenji; Ichihara, Kyoko*; Hanzawa, Kohei*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 10 Pages, 2022/03

Japan Atomic Energy Agency (JAEA) has investigated an accelerator-driven system (ADS) to transmute minor actinides (MAs) included in high level wastes discharged from nuclear power plants. The ADS is a lead-bismuth cooled tank-type reactor with 800 MW thermal power. It is supposed that the ADS is safer than conventional critical reactors because it is operated in a subcritical state. The previous study performed the transient analyses for the typical ADS accidents such as unprotected loss of flow or beam overpower. It was shown that all calculation cases except loss of heat sink (LOHS) satisfied the no-damage criteria. To avoid the damage by LOHS, the ADS equips Direct Reactor Auxiliary Cooling System (DRACS) to remove the decay heat. The most important points of a DRACS operation are its reliability and to ensure the flowrate in a natural circulation state. This study aims to perform the CFD analysis of the natural circulation to clarify the flowrate in the ADS reactor vessel.

Journal Articles

A Plan of materials irradiation facility at J-PARC for development of ADS and high-power accelerator facilities

Maekawa, Fujio

JPS Conference Proceedings (Internet), 33, p.011042_1 - 011042_6, 2021/03

Development of beam window (BW) materials is one of crucial issues in development of accelerator driven nuclear transmutation systems (ADS). The BW is exposed to high energy protons and spallation neutrons, and also to corrosive lead-bismuth eutectic (LBE) alloy at high temperature of about 500$$^{circ}$$C. Recently, not only high-power accelerators but also high-power targets are the rate-limiting factor for increasing the power of accelerator facilities in terms of radiation damage and heat removal. To study radiation damage on BW and target materials for high-power accelerator facilities including ADS, we are planning a materials irradiation facility by utilizing the proton beam of 400 MeV and 250 kW provided by the J-PARC's Linac. The target is flowing LBE alloy which is a candidate target and coolant material of ADS. When a steel sample is irradiated in the target for one year, the sample receives radiation damage of about 10 dpa at maximum which is equivalent to the yearly radiation damage of ADS's BW. In the current facility concept, the facility is equipped with a hot-laboratory for efficient post-irradiation examination. The facility will be outlined in this presentation.

JAEA Reports

Estimation of oxygen consumption amount in LBE-cooled accelerator-driven system

Sugawara, Takanori; Komatsu, Atsushi

JAEA-Research 2020-016, 44 Pages, 2021/01

JAEA-Research-2020-016.pdf:2.94MB

It is required to control the oxygen concentration in lead-bismuth eutectic (LBE) to prevent the corrosion of structures in LBE-cooled nuclear system. This study estimated the oxygen consumption amount in the LBE-cooled accelerator-driven system (ADS). We used the evaluation formula for the oxide layer thickness, which were derived by various experiments, to estimate the oxygen consumption amount. It was found that the maximum oxide layer thicknesses for the fuel assembly and the beam window were about 35 [$$mu$$m] and 20 [$$mu$$m], respectively. Based on these results, the oxygen consumption amount for the ADS plant was estimated as 30 [kg] during one cycle (one year). Through this study, it was indicated that an oxygen supply device which could supply 3-4 [g/h] oxygen in the normal operation, 150 [g/h] in the peak and about 30 [kg] during one cycle was necessary.

Journal Articles

The Analytical study of inventories and physicochemical configuration of spallation products produced in Lead-Bismuth Eutectic of Accelerator Driven System

Miyahara, Shinya*; Ohdaira, Naoya*; Arita, Yuji*; Maekawa, Fujio; Matsuda, Hiroki; Sasa, Toshinobu; Meigo, Shinichiro

Nuclear Engineering and Design, 352, p.110192_1 - 110192_8, 2019/10

 Times Cited Count:1 Percentile:17.7(Nuclear Science & Technology)

Lead-Bismuth Eutectic (LBE) is used as a spallation neutron target and coolant materials of Accelerator Driven System (ADS), and many kinds of elements are produced as spallation products. It is important to evaluate the release and transport behavior of the spallation products in the LBE. The inventories and the physicochemical composition of the spallation products produced in LBE have been investigated for an LBE loop in the ADS Target Test Facility (TEF-T) in J-PARC. The inventories of the spallation products in the LBE were estimated using the PHITS code. The physicochemical composition of the spallation products in the LBE was calculated using the Thermo-Calc code under the conditions of the operation temperatures of LBE from 350$$^{circ}$$C to 500$$^{circ}$$C and the oxygen concentrations in LBE from 10 ppb to 1 ppm. The calculation showed that the 5 elements of Rb, Tl, Tc, Os, Ir, Pt, Au and Hg were soluble in LBE under the all given conditions and any kinds of compound were not formed in LBE. It was suggested that the oxides of Ce, Sr, Zr and Y were stable as CeO$$_{2}$$, SrO, ZrO$$_{2}$$ and Y$$_{2}$$O$$_{3}$$ in the LBE.

Journal Articles

Thermal-hydraulic analysis of the LBE spallation target head in JAEA

Wan, T.; Obayashi, Hironari; Sasa, Toshinobu

Nuclear Technology, 205(1-2), p.188 - 199, 2019/01

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

JAEA Reports

Measurement experiment of oxygen concentration in liquid lead-bismuth eutectic; Basic Tests and estimation of gamma-ray irradiation effect

Sugawara, Takanori; Kita, Satoshi*; Yoshimoto, Hidemitsu*; Okubo, Nariaki

JAEA-Technology 2018-008, 26 Pages, 2018/09

JAEA-Technology-2018-008.pdf:10.35MB

The oxygen sensors to measure the oxygen concentration in liquid LBE (lead-bismuth eutectic) were fabricated and tested for future use in LBE-cooled ADS (accelerator-driven system) or LBE test loops. The following tests were performed; estimation of catalyst application range, freeze seal structure and estimation of gamma-ray irradiation effect. For the estimation of the catalyst application range, it was confirmed that the measurement accuracy became worse in low LBE temperature as the application range became small. For the freeze seal structure, we realized the structure to prevent the LBE leakage with 0.5 MPa pressure condition. For the estimation of gamma-ray irradiation effect, the ex-situ test was carried out and it was observed that there was little effect by 4 MGy gamma-ray irradiation.

JAEA Reports

Assessment of lead-bismuth-eutectic leak at ADS Target Test Facility in Transmutation Experimental Facility of J-PARC

Iwamoto, Hiroki; Maekawa, Fujio; Matsuda, Hiroki; Meigo, Shinichiro

JAEA-Technology 2017-029, 39 Pages, 2018/01

JAEA-Technology-2017-029.pdf:2.68MB

Under an assumption that an incident of lead-bismuth eutectic (LBE) leak from an LBE circulation system occurred during a 250-kW beam operation, an estimation of radiation dose at the site boundary for the ADS Target Test Facility (TEF-T) in Transmutation Experimental Facility (TEF) of J-PARC was conducted using various conservative assumptions. As a result, the radiation dose at the site boundary was estimated to be about 660 $$mu$$Sv, which were dominated by mercury, noble gas, and iodine produced as spallation products from the LBE. Even though the incident scenario was made conservatively, it was shown that the estimated total dose was lower than the annual radiation dose due to natural sources, and the TEF-T has sufficient safety margin for the leak of radioactivity.

Journal Articles

Electrochemical impedance analysis on solid electrolyte oxygen sensor with gas and liquid reference electrodes for liquid LBE

Adhi, P. M.*; Okubo, Nariaki; Komatsu, Atsushi; Kondo, Masatoshi*; Takahashi, Minoru*

Energy Procedia, 131, p.420 - 427, 2017/12

 Times Cited Count:0 Percentile:0.03

The ionic conductivity of solid electrolyte may insufficient, and the sensor output signal will deviate from the theoretical one in low temperature. The performance of oxygen sensor with Ag/air reference electrode (RE) and liquid Bi/Bi$$_{2}$$O$$_{3}$$ RE was tested in low-temperature LBE at 300$$sim$$450$$^{circ}$$C and the charge transfer reactions impedance at the electrode-electrolyte interface was analyzed by electrochemical impedance analysis (EIS). After steady state condition, both of the sensors performed well and can be used at 300$$sim$$450$$^{circ}$$C. Bi/Bi/Bi$$_{2}$$O$$_{3}$$ RE has lower impedance than Ag/air RE. Therefore, the response time of the oxygen sensor with Bi/Bi/Bi$$_{2}$$O$$_{3}$$ RE is faster than the oxygen sensor with Ag/air RE in the low-temperature region.

Journal Articles

Design of 250kW LBE spallation target for the Japan Proton Accelerator Research Complex (J-PARC)

Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Sugawara, Takanori; Wan, T.; Yamaguchi, Kazushi*; Yoshimoto, Hidemitsu

NEA/CSNI/R(2017)2 (Internet), p.111 - 116, 2017/06

Japan Atomic Energy Agency (JAEA) proposes to reduce the environmental impact caused from high-level radioactive waste by using Accelerator-driven system (ADS). To realize ADS, JAEA plans to build the Transmutation Experimental Facility (TEF) within the framework of J-PARC project. For the JAEA-proposed ADS, lead-bismuth eutectic alloy (LBE) is adopted as a coolant for subcritical core and spallation target. By using TEF in J-PARC, we are planning to solve technical difficulties for LBE utilization by completion of the data for the design of ADS. The 250kW LBE spallation target will be located in TEF facility to prepare material irradiation database. Various R&Ds for important technologies required to build the facilities are investigated such as oxygen content control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for 250kW target mock up and material corrosion studies are also manufactured and ready for various experiments. The latest status of 250kW LBE spallation target optimization will be described in the presentation.

JAEA Reports

Technical design report on J-PARC Transmutation Experimental Facility; ADS Target Test Facility (TEF-T)

Nuclear Transmutation Division, J-PARC Center

JAEA-Technology 2017-003, 539 Pages, 2017/03

JAEA-Technology-2017-003.pdf:59.1MB

JAEA is pursuing R&D on volume reduction and mitigation of degree of harmfulness of high-level radioactive waste based on the "Strategic Energy Plan" issued in April 2014. Construction of Transmutation Experimental Facility is under planning as one of the second phase facilities in the J-PARC program to promote R&D on the transmutation technology with using accelerator driven systems (ADS). The TEF consists of two facilities: ADS Target Test Facility (TEF-T) and Transmutation Physics Experimental Facility (TEF-P). Development of spallation target technology and study on target materials are to be conducted in TEF-T with impinging a high intensity proton beam on a lead-bismuth eutectic target. Whereas in TEF-P, by introducing a proton beam to minor actinide loaded subcritical cores, physical properties of the cores are to be studied, and operation experiences are to be acquired. This report summarizes results of technical design for construction of one of two TEF facilities, TEF-T.

Journal Articles

Design study around beam window of ADS

Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Kikuchi, Kenji; Kurata, Yuji; Sasa, Toshinobu; Umeno, Makoto*; Nishihara, Kenji; Saito, Shigeru; Mizumoto, Motoharu; Takano, Hideki*; et al.

Proceedings of 4th International Workshop on the Utilisation and Reliability of High Power Proton Accelerators, p.325 - 334, 2005/11

The Japan Atomic Energy Research Institute (JAERI) is conducting the research and development (R&D) on the Accelerator-Driven Subcritical System (ADS) for the effective transmutation of minor actinides (MAs). The ADS proposed by JAERI is the 800 MWth, Pb-Bi cooled, tank-type subcritical reactor loaded with (MA+Pu) nitride fuel. The Pb-Bi is also used as the spallation target. In this study, the feasibility of the ADS was discussed with putting the focus on the design around the beam window. The partition wall was placed between the target region and the ductless-type fuel assemblies to keep the good cooling performance for the hot-spot fuel pin. The flow control nozzle was installed to cool the beam window effectively. The thermal-hydraulic analysis showed that the maximum temperature at the outer surface of the beam window could be repressed below 500 $$^{circ}$$C even in the case of the maximum beam power of 30 MW. The stress caused by the external pressure and the temperature distribution of the beam window was also below the allowable limit.

Journal Articles

Experimental investigation of lead-bismuth evaporation behavior

Ohno, Shuji*; Miyahara, Shinya*; Kurata, Yuji

Journal of Nuclear Science and Technology, 42(7), p.593 - 599, 2005/07

no abstracts in English

Journal Articles

R&D activities on accelerator-driven transmutation system in JAERI

Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Kikuchi, Kenji; Kurata, Yuji; Sasa, Toshinobu; Umeno, Makoto*; Saito, Shigeru; Nishihara, Kenji; Mizumoto, Motoharu; Takano, Hideki*; et al.

EUR-21227 (CD-ROM), p.483 - 493, 2005/00

JAERI is conducting the study on the dedicated transmutation system using the accelerator driven subcritical system (ADS). A subcritical reactor with the thermal power of 800 MW has been proposed. Many research and development activities including the conceptual design study are under way and planned at JAERI to examine the feasibility of the ADS. In the field of the proton accelerator, a superconducting LINAC is being developed. In the field of the spallation target using lead-bismuth eutectic (LBE), material corrosion, thermal-hydraulics, polonium behavior, and irradiation effect on materials are being studied. Moreover, in the framework of the J-PARC project, JAERI plans to construct the Transmutation Experimental Facility (TEF) to study the feasibility of the ADS using a high-energy proton beam and nuclear fuel and to establish the technology for the LBE spallation target and relevant materials.

Journal Articles

Experimental investigation of evaporation behavior for lead-bismuth eutectic and its impurity tellurium

Ohno, Shuji*; Miyahara, Shinya*; Kurata, Yuji

Proceedings of 12th International Conference on Nuclear Engineering (ICONE-12) (CD-ROM), 6 Pages, 2004/00

no abstracts in English

Journal Articles

Research and development on accelerator-driven transmutation system at JAERI

Sasa, Toshinobu; Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Nishihara, Kenji; Kikuchi, Kenji; Kurata, Yuji; Saito, Shigeru; Futakawa, Masatoshi; Umeno, Makoto*; Ouchi, Nobuo; et al.

Proceedings of 11th International Conference on Nuclear Engineering (ICONE-11) (CD-ROM), 9 Pages, 2003/04

JAERI carries out research and development on accelerator-driven system (ADS) to transmute minor actinides and long-lived fission products in high-level radioactive waste. The system is composed of high intensity proton accelerator, lead-bismuth spallation target and lead-bismuth cooled subcritical core with nitride fuel. About 2500 kg of minor actinide is loaded into the subcritical core. Annual transmutation amount using this system is 250 kg with 800MW of thermal output. A superconducting linear accelerator with the beam power of 20 - 30MW is connected to drive the subcritical core. The nitride fuel without uranium, such as (Np, Am, Pu)N, is selected. The fuel irradiated in the ADS is reprocessed by pyrochemical process followed by the re-fabrication of the fuel. Many research and development activities are under way. Especially, to study and evaluate the feasibility of the ADS from physics and engineering aspects, the Transmutation Experimental Facility (TEF) is proposed under a framework of the High-Intensity Proton Accelerator Project.

Journal Articles

Present status and perspective on nuclear transmutation, C; Accelerator driven transmutation system

Oigawa, Hiroyuki

Genshikaku Kenkyu, 47(6), p.39 - 52, 2003/03

Minor actinide (MA) and long-lived fission product (LLFP) keep their radiological toxicity in high level waste of nuclear fuel cycle for long period. In order to transmute such nuclides to short-lived or stable ones, the Accelerator-Driven Transmutation System (ADS) is proposed and developed. This article presents the current status of the research and development on ADS, technical issues to be solved, the experimental program under the framework of the High-Intensity Proton Accelerator Project (J-PARC), and worldwide activities.

JAEA Reports

Research on the behavior of polonium produced in lead-bismuth eutectic irradiated with neutrons, JAERI's nuclear research promotion program, H10-026 (Contract research)

Sekimoto, Hiroshi*; Igashira, Masayuki*; Yano, Toyohiko*; Obara, Toru*; Osaki, Toshiro*

JAERI-Tech 2002-008, 58 Pages, 2002/03

JAERI-Tech-2002-008.pdf:3.6MB

no abstracts in English

25 (Records 1-20 displayed on this page)