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Journal Articles

A Plan of materials irradiation facility at J-PARC for development of ADS and high-power accelerator facilities

Maekawa, Fujio

JPS Conference Proceedings (Internet), 33, p.011042_1 - 011042_6, 2021/03

Development of beam window (BW) materials is one of crucial issues in development of accelerator driven nuclear transmutation systems (ADS). The BW is exposed to high energy protons and spallation neutrons, and also to corrosive lead-bismuth eutectic (LBE) alloy at high temperature of about 500$$^{circ}$$C. Recently, not only high-power accelerators but also high-power targets are the rate-limiting factor for increasing the power of accelerator facilities in terms of radiation damage and heat removal. To study radiation damage on BW and target materials for high-power accelerator facilities including ADS, we are planning a materials irradiation facility by utilizing the proton beam of 400 MeV and 250 kW provided by the J-PARC's Linac. The target is flowing LBE alloy which is a candidate target and coolant material of ADS. When a steel sample is irradiated in the target for one year, the sample receives radiation damage of about 10 dpa at maximum which is equivalent to the yearly radiation damage of ADS's BW. In the current facility concept, the facility is equipped with a hot-laboratory for efficient post-irradiation examination. The facility will be outlined in this presentation.

JAEA Reports

Estimation of oxygen consumption amount in LBE-cooled accelerator-driven system

Sugawara, Takanori; Komatsu, Atsushi

JAEA-Research 2020-016, 44 Pages, 2021/01

JAEA-Research-2020-016.pdf:2.94MB

It is required to control the oxygen concentration in lead-bismuth eutectic (LBE) to prevent the corrosion of structures in LBE-cooled nuclear system. This study estimated the oxygen consumption amount in the LBE-cooled accelerator-driven system (ADS). We used the evaluation formula for the oxide layer thickness, which were derived by various experiments, to estimate the oxygen consumption amount. It was found that the maximum oxide layer thicknesses for the fuel assembly and the beam window were about 35 [$$mu$$m] and 20 [$$mu$$m], respectively. Based on these results, the oxygen consumption amount for the ADS plant was estimated as 30 [kg] during one cycle (one year). Through this study, it was indicated that an oxygen supply device which could supply 3-4 [g/h] oxygen in the normal operation, 150 [g/h] in the peak and about 30 [kg] during one cycle was necessary.

Journal Articles

The Analytical study of inventories and physicochemical configuration of spallation products produced in Lead-Bismuth Eutectic of Accelerator Driven System

Miyahara, Shinya*; Ohdaira, Naoya*; Arita, Yuji*; Maekawa, Fujio; Matsuda, Hiroki; Sasa, Toshinobu; Meigo, Shinichiro

Nuclear Engineering and Design, 352, p.110192_1 - 110192_8, 2019/10

 Times Cited Count:1 Percentile:23.13(Nuclear Science & Technology)

Lead-Bismuth Eutectic (LBE) is used as a spallation neutron target and coolant materials of Accelerator Driven System (ADS), and many kinds of elements are produced as spallation products. It is important to evaluate the release and transport behavior of the spallation products in the LBE. The inventories and the physicochemical composition of the spallation products produced in LBE have been investigated for an LBE loop in the ADS Target Test Facility (TEF-T) in J-PARC. The inventories of the spallation products in the LBE were estimated using the PHITS code. The physicochemical composition of the spallation products in the LBE was calculated using the Thermo-Calc code under the conditions of the operation temperatures of LBE from 350$$^{circ}$$C to 500$$^{circ}$$C and the oxygen concentrations in LBE from 10 ppb to 1 ppm. The calculation showed that the 5 elements of Rb, Tl, Tc, Os, Ir, Pt, Au and Hg were soluble in LBE under the all given conditions and any kinds of compound were not formed in LBE. It was suggested that the oxides of Ce, Sr, Zr and Y were stable as CeO$$_{2}$$, SrO, ZrO$$_{2}$$ and Y$$_{2}$$O$$_{3}$$ in the LBE.

Journal Articles

Numerical study on the potential of cavitation damage in a lead-bismuth eutectic spallation target

Wan, T.; Naoe, Takashi; Kogawa, Hiroyuki; Futakawa, Masatoshi; Obayashi, Hironari; Sasa, Toshinobu

Materials, 12(4), p.681_1 - 681_15, 2019/02

 Times Cited Count:0 Percentile:0(Chemistry, Physical)

Journal Articles

Thermal-hydraulic analysis of the LBE spallation target head in JAEA

Wan, T.; Obayashi, Hironari; Sasa, Toshinobu

Nuclear Technology, 205(1-2), p.188 - 199, 2019/01

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

JAEA Reports

Measurement experiment of oxygen concentration in liquid lead-bismuth eutectic; Basic Tests and estimation of gamma-ray irradiation effect

Sugawara, Takanori; Kita, Satoshi*; Yoshimoto, Hidemitsu*; Okubo, Nariaki

JAEA-Technology 2018-008, 26 Pages, 2018/09

JAEA-Technology-2018-008.pdf:10.35MB

The oxygen sensors to measure the oxygen concentration in liquid LBE (lead-bismuth eutectic) were fabricated and tested for future use in LBE-cooled ADS (accelerator-driven system) or LBE test loops. The following tests were performed; estimation of catalyst application range, freeze seal structure and estimation of gamma-ray irradiation effect. For the estimation of the catalyst application range, it was confirmed that the measurement accuracy became worse in low LBE temperature as the application range became small. For the freeze seal structure, we realized the structure to prevent the LBE leakage with 0.5 MPa pressure condition. For the estimation of gamma-ray irradiation effect, the ex-situ test was carried out and it was observed that there was little effect by 4 MGy gamma-ray irradiation.

JAEA Reports

Assessment of lead-bismuth-eutectic leak at ADS Target Test Facility in Transmutation Experimental Facility of J-PARC

Iwamoto, Hiroki; Maekawa, Fujio; Matsuda, Hiroki; Meigo, Shinichiro

JAEA-Technology 2017-029, 39 Pages, 2018/01

JAEA-Technology-2017-029.pdf:2.68MB

Under an assumption that an incident of lead-bismuth eutectic (LBE) leak from an LBE circulation system occurred during a 250-kW beam operation, an estimation of radiation dose at the site boundary for the ADS Target Test Facility (TEF-T) in Transmutation Experimental Facility (TEF) of J-PARC was conducted using various conservative assumptions. As a result, the radiation dose at the site boundary was estimated to be about 660 $$mu$$Sv, which were dominated by mercury, noble gas, and iodine produced as spallation products from the LBE. Even though the incident scenario was made conservatively, it was shown that the estimated total dose was lower than the annual radiation dose due to natural sources, and the TEF-T has sufficient safety margin for the leak of radioactivity.

Journal Articles

Electrochemical impedance analysis on solid electrolyte oxygen sensor with gas and liquid reference electrodes for liquid LBE

Adhi, P. M.*; Okubo, Nariaki; Komatsu, Atsushi; Kondo, Masatoshi*; Takahashi, Minoru*

Energy Procedia, 131, p.420 - 427, 2017/12

 Times Cited Count:0 Percentile:0.03

The ionic conductivity of solid electrolyte may insufficient, and the sensor output signal will deviate from the theoretical one in low temperature. The performance of oxygen sensor with Ag/air reference electrode (RE) and liquid Bi/Bi$$_{2}$$O$$_{3}$$ RE was tested in low-temperature LBE at 300$$sim$$450$$^{circ}$$C and the charge transfer reactions impedance at the electrode-electrolyte interface was analyzed by electrochemical impedance analysis (EIS). After steady state condition, both of the sensors performed well and can be used at 300$$sim$$450$$^{circ}$$C. Bi/Bi/Bi$$_{2}$$O$$_{3}$$ RE has lower impedance than Ag/air RE. Therefore, the response time of the oxygen sensor with Bi/Bi/Bi$$_{2}$$O$$_{3}$$ RE is faster than the oxygen sensor with Ag/air RE in the low-temperature region.

Journal Articles

Design of 250kW LBE spallation target for the Japan Proton Accelerator Research Complex (J-PARC)

Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Sugawara, Takanori; Wan, T.; Yamaguchi, Kazushi*; Yoshimoto, Hidemitsu

NEA/CSNI/R(2017)2 (Internet), p.111 - 116, 2017/06

Japan Atomic Energy Agency (JAEA) proposes to reduce the environmental impact caused from high-level radioactive waste by using Accelerator-driven system (ADS). To realize ADS, JAEA plans to build the Transmutation Experimental Facility (TEF) within the framework of J-PARC project. For the JAEA-proposed ADS, lead-bismuth eutectic alloy (LBE) is adopted as a coolant for subcritical core and spallation target. By using TEF in J-PARC, we are planning to solve technical difficulties for LBE utilization by completion of the data for the design of ADS. The 250kW LBE spallation target will be located in TEF facility to prepare material irradiation database. Various R&Ds for important technologies required to build the facilities are investigated such as oxygen content control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for 250kW target mock up and material corrosion studies are also manufactured and ready for various experiments. The latest status of 250kW LBE spallation target optimization will be described in the presentation.

JAEA Reports

Technical design report on J-PARC Transmutation Experimental Facility; ADS Target Test Facility (TEF-T)

Nuclear Transmutation Division, J-PARC Center

JAEA-Technology 2017-003, 539 Pages, 2017/03

JAEA-Technology-2017-003.pdf:59.1MB

JAEA is pursuing R&D on volume reduction and mitigation of degree of harmfulness of high-level radioactive waste based on the "Strategic Energy Plan" issued in April 2014. Construction of Transmutation Experimental Facility is under planning as one of the second phase facilities in the J-PARC program to promote R&D on the transmutation technology with using accelerator driven systems (ADS). The TEF consists of two facilities: ADS Target Test Facility (TEF-T) and Transmutation Physics Experimental Facility (TEF-P). Development of spallation target technology and study on target materials are to be conducted in TEF-T with impinging a high intensity proton beam on a lead-bismuth eutectic target. Whereas in TEF-P, by introducing a proton beam to minor actinide loaded subcritical cores, physical properties of the cores are to be studied, and operation experiences are to be acquired. This report summarizes results of technical design for construction of one of two TEF facilities, TEF-T.

JAEA Reports

Thermal design study of lead-bismuth cooled accelerator driven system, 1; Study on thermal hydraulic behavior under normal operation condition

Akimoto, Hajime; Sugawara, Takanori

JAEA-Data/Code 2016-008, 87 Pages, 2016/09

JAEA-Data-Code-2016-008.pdf:15.62MB

Thermal hydraulic behavior in a lead-bismuth cooled accelerator driven system (ADS) is analyzed under normal operation condition. Input data for the ADS version of J-TRAC code have been constructed to integrate the conceptual design. The core part of the ADS is modeled in detail to evaluate the core radial power profile effect on the core cooling. As the result of the analyses, the followings are found; (1) Both maximum clad temperature and fuel temperature are below the design limits. (2) The radial power profile has little effect on the coolant flow distribution among fuel assemblies. (3) The radial power profile has little effect on the heat transfer coefficients along fuel rods. (4) The thermal hydraulic behaviors along four steam generators are identical. The thermal hydraulic behaviors along two pumps are also identical. A fast running input data is developed by the simplification of the detailed input data based on the findings mentioned above.

JAEA Reports

Proceedings of the first topical meeting on Asian network for accelerator-driven systems and nuclear transmutation technology

Sasa, Toshinobu

JAEA-Review 2015-042, 213 Pages, 2016/03

JAEA-Review-2015-042.pdf:166.0MB

The first topical meeting on Asian Network for Accelerator-driven System (ADS) and Nuclear Transmutation Technology (NTT) was held on 26-27 October 2015 at the J-PARC Center, Japan Atomic Energy Agency, Japan. The meeting was an optional one in-between the regular meeting, which will be held in every second year. Instead of the regular meeting, which covers all research fields for ADS and NTT, such as accelerator, spallation target, subcritical reactor, fuel, and material, this topical meeting is focused on the specific topic to make technical discussions more deeply. In this meeting, the technology for lead-bismuth eutectic alloy was selected as one of the hot issues in the world and had deep discussions with specialists in Asian countries. Through the discussion, the importance of cooperation in Again region is recognized to solve the issues for application of LBE. This report summarizes all presentation materials discussed in the meeting.

JAEA Reports

Development of thermal-hydraulic design code for transmutation system with lead-bismuth cooled accelerator driven reactor

Akimoto, Hajime

JAEA-Data/Code 2014-031, 75 Pages, 2015/03

JAEA-Data-Code-2014-031.pdf:37.23MB

A thermal-hydraulic analysis code for transmutation system with lead-bismuth cooled accelerator-driven system (ADS) has been developed using the Japanese-version of Transient Reactor Analysis Code (J-TRAC) as the framework to apply the design studies of ADS. To identify the required capabilities of the thermal-hydraulic analysis code for ADS, previous thermal-hydraulic analyses of light water reactors, sodium-cooled fast reactor and ADS have been surveyed. To make up for insufficient capabilities of the J-TRAC code as a thermal-hydraulic analysis code of ADS, physical properties of lead-bismuth eutectic (LBE), argon gas and nitride nuclear fuel were implemented to the J-TRAC code. It was confirmed that the implemented capabilities worked as expected through verification calculations on (1) single-phase LBE flow, (2) heat transfer in a fuel assembly, and (3) heat transfer in a steam generator.

Journal Articles

Shielding analysis at the upper section of the accelerator-driven system

Sasa, Toshinobu; Yang, J. A.*; Oigawa, Hiroyuki

Radiation Protection Dosimetry, 116(1-4), p.256 - 258, 2005/12

 Times Cited Count:0 Percentile:0.01(Environmental Sciences)

The proton beam duct of the accelerator-driven system (ADS) acts a streaming path for spallation neutrons and photons and causes the activation of the magnets and other devices above the subcritical core. We have performed a streaming analysis at the upper section of the lead-bismuth target/cooled ADS (800MWth). MCNPX was used to calculate the radiation dose from streamed neutrons and photons through the beam duct. For the secondary photon production calculation, cross sections for several actinides were substituted for plutonium because of the lack of gamma production cross section. From the results of this analysis, the neutron dose from the beam duct is about 20 orders higher than that of the bulk shield. The magnets and shield plug were heavily irradiated by streaming neutrons according to the DCHAIN-SP analysis.

Journal Articles

Concept of transmutation experimental facility

Oigawa, Hiroyuki; Sasa, Toshinobu; Kikuchi, Kenji; Nishihara, Kenji; Kurata, Yuji; Umeno, Makoto*; Tsujimoto, Kazufumi; Saito, Shigeru; Futakawa, Masatoshi; Mizumoto, Motoharu; et al.

Proceedings of 4th International Workshop on the Utilisation and Reliability of High Power Proton Accelerators, p.507 - 517, 2005/11

Under the framework of J-PARC, the Japan Atomic Energy Research Institute (JAERI) plans to construct the Transmutation Experimental Facility (TEF). The TEF consists of two facilities: the Transmutation Physics Experimental Facility (TEF-P) and the ADS Target Test Facility (TEF-T). The TEF-P is a critical facility which can accept a 600 MeV - 10 W proton beam. The TEF-T is a material irradiation facility using a 600 MeV - 200 kW proton beam, where a Pb-Bi target is installed, but neutron multiplication by nuclear fuel will not be attempted. This report describes the purposes of the facility, the present status of the conceptual design, and the expected experiments to be performed.

Journal Articles

Design study around beam window of ADS

Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Kikuchi, Kenji; Kurata, Yuji; Sasa, Toshinobu; Umeno, Makoto*; Nishihara, Kenji; Saito, Shigeru; Mizumoto, Motoharu; Takano, Hideki*; et al.

Proceedings of 4th International Workshop on the Utilisation and Reliability of High Power Proton Accelerators, p.325 - 334, 2005/11

The Japan Atomic Energy Research Institute (JAERI) is conducting the research and development (R&D) on the Accelerator-Driven Subcritical System (ADS) for the effective transmutation of minor actinides (MAs). The ADS proposed by JAERI is the 800 MWth, Pb-Bi cooled, tank-type subcritical reactor loaded with (MA+Pu) nitride fuel. The Pb-Bi is also used as the spallation target. In this study, the feasibility of the ADS was discussed with putting the focus on the design around the beam window. The partition wall was placed between the target region and the ductless-type fuel assemblies to keep the good cooling performance for the hot-spot fuel pin. The flow control nozzle was installed to cool the beam window effectively. The thermal-hydraulic analysis showed that the maximum temperature at the outer surface of the beam window could be repressed below 500 $$^{circ}$$C even in the case of the maximum beam power of 30 MW. The stress caused by the external pressure and the temperature distribution of the beam window was also below the allowable limit.

Journal Articles

Research and development program on accelerator driven subcritical system in JAERI

Tsujimoto, Kazufumi; Oigawa, Hiroyuki; Ouchi, Nobuo; Kikuchi, Kenji; Kurata, Yuji; Mizumoto, Motoharu; Sasa, Toshinobu; Nishihara, Kenji; Saito, Shigeru; Umeno, Makoto*; et al.

Proceedings of International Conference on Nuclear Energy System for Future Generation and Global Sustainability (GLOBAL 2005) (CD-ROM), 6 Pages, 2005/10

The Japan Atomic Energy Research Institute (JAERI) has been proceeding with the research and development (R&D) on accelerator-driven subcritical system (ADS). The ADS proposed by JAERI is a lead-bismuth (Pb-Bi) eutectic cooled fast subcritical core with 800 MWth. To realize such an ADS, some technical issues should be studied, developed and demonstrated. JAERI has started a comprehensive R&D program since the fiscal year of 2002 to acquire knowledge and elemental technology that are necessary for the validation of engineering feasibility of the ADS. The first stage of the program had been continued for three years. The program is conducted by JAERI, and many institutes, universities and private companies were involved. Items of R&D are concentrated on three technical areas peculiar to the ADS: (1) superconducting linear accelerator (SC-LINAC), (2) Pb-Bi eutectic as spallation target and core coolant, and (3) subcritical core design and technology. In the present work, the outline and the results in the first stage of the program are reported.

Journal Articles

Experimental investigation of lead-bismuth evaporation behavior

Ohno, Shuji*; Miyahara, Shinya*; Kurata, Yuji

Journal of Nuclear Science and Technology, 42(7), p.593 - 599, 2005/07

no abstracts in English

Journal Articles

R&D activities on accelerator-driven transmutation system in JAERI

Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Kikuchi, Kenji; Kurata, Yuji; Sasa, Toshinobu; Umeno, Makoto*; Saito, Shigeru; Nishihara, Kenji; Mizumoto, Motoharu; Takano, Hideki*; et al.

EUR-21227 (CD-ROM), p.483 - 493, 2005/00

JAERI is conducting the study on the dedicated transmutation system using the accelerator driven subcritical system (ADS). A subcritical reactor with the thermal power of 800 MW has been proposed. Many research and development activities including the conceptual design study are under way and planned at JAERI to examine the feasibility of the ADS. In the field of the proton accelerator, a superconducting LINAC is being developed. In the field of the spallation target using lead-bismuth eutectic (LBE), material corrosion, thermal-hydraulics, polonium behavior, and irradiation effect on materials are being studied. Moreover, in the framework of the J-PARC project, JAERI plans to construct the Transmutation Experimental Facility (TEF) to study the feasibility of the ADS using a high-energy proton beam and nuclear fuel and to establish the technology for the LBE spallation target and relevant materials.

Journal Articles

Research activities for accelerator-driven transmutation system at JAERI

Sasa, Toshinobu

Progress in Nuclear Energy, 47(1-4), p.314 - 326, 2005/00

 Times Cited Count:12 Percentile:65.49(Nuclear Science & Technology)

JAERI performs R&D of accelerator-driven systems (ADS) for transmutation of long-lived nuclides under national OMEGA program since 1988. To study the basic characteristics of ADS, Transmutation Experimental Facility is proposed under a framework of JAERI-KEK joint J-PARC project. A comprehensive R&D program for future ADS plant is also performed since 2002. R&D items are categorized into three fields, (1) accelerator (superconducting LINAC design), (2) lead-bismuth target/coolant (material compatibility, thermal-hydraulics around beam window and polonium behavior) and (3) subcritical core (system design, nuclear data, subcriticality measurement, and safety issues of ADS). First phase of the program will be done within three years. Assemble test of the cryomodule, heat transfer experiment using Pb-Bi thermal-hydraulics loop, cold test of polonium vaporization, design study of the 800MW ADS subcritical core are now underway. Part of this job was funded by the MEXT as one of the public offered R&D program for innovative nuclear systems.

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