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JAEA Reports

Review and evaluation on the surface area of vitrified products of high-level waste; Surface area increase factors due to fracturing and their bases for the performance assessment of geological disposal

Igarashi, Hiroshi

JAEA-Review 2020-006, 261 Pages, 2020/09

JAEA-Review-2020-006.pdf:4.42MB

A literature review was conducted on the increase in surface area of vitrified products of HLW due to the fracturing caused by cooling during glass pouring process and by mechanical impact, from the perspective of a parameter of the radionuclide release model in the performance assessment of geological disposal system studied overseas. The review was focused on the value of surface area increase factor set as a parameter in the model, the experimental work to evaluate an increase in surface area, and how the parameters on surface area were determined based on the experimental results. The surface area obtained from the experiments executed in Japan was also discussed in comparison with the overseas studies. On the basis of the investigation, the effects of various conditions on the surface area were studied, such as a diameter of vitrified product, cooling condition during and after the glass pouring, impact on vitrified products during their handling, environment after the closure of disposal facility, and others. The causes of fracturing are associated with the phenomena or events in the waste management process such as production, transport, storage, and disposal. The surface area increase factors set in the nuclide release model of the glass and their bases were reviewed. In addition, the measured values and the experimental methods for surface increase factors published so far were compared. Accordingly, the methods for measuring surface area as the bases were identified for these factors set in the models. The causes of fracturing and features of these factors were studied with respect to the relation with the waste management process. The results from the review and assessment can contribute to the expanding the knowledge for the conservative and realistic application of these factors to performance assessment, and to the developing and upgrading of safety case as a consequence.

Journal Articles

Observation of aerosol particle capturing behavior near gas-liquid interface

Uesawa, Shinichiro; Yoshida, Hiroyuki

Mechanical Engineering Journal (Internet), 7(3), p.19-00539_1 - 19-00539_9, 2020/06

JAEA Reports

Survey of computational methods of cross sections for thermal neutron scattering by liquids

Ichihara, Akira

JAEA-Review 2019-046, 36 Pages, 2020/03

JAEA-Review-2019-046.pdf:1.55MB

Toward the revision of JENDL-4.0, we conducted a literature survey on how to compute the cross section of thermal neutrons scattered by a liquid. This report summarizes the computational methods for evaluating thermal neutron cross sections with molecular dynamics simulations. The cross section can be expressed with a function called as scattering law. For light and heavy water, the scattering law data instead of the cross sections have been provided in nuclear databases. In this report we review the formulations of the scattering laws. The scattering laws can be derived from both the intermediate scattering function and the space-time correlation function. Features of the derived scattering laws are briefly explained. It is shown that the scattering law data can be evaluated using a molecular dynamics simulation of the liquid that is the target of thermal neutrons.

JAEA Reports

Upgrading of recovery method for radioactive microparticles by heavy liquid separation aiming to volume reduction of contaminated soil (Contract research); FY2018 Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development

Collaborative Laboratories for Advanced Decommissioning Science; University of Tsukuba*

JAEA-Review 2019-023, 33 Pages, 2020/01

JAEA-Review-2019-023.pdf:1.97MB

CLADS, JAEA, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the 'Upgrading of Recovery Method for Radioactive Microparticles by Heavy Liquid Separation Aiming to Volume Reduction of Contaminated Soil'. After the accident of the Fukushima Daiichi Nuclear Power Station, radioactive cesium has been heterogeneously distributed in surface soil due to the existence of radioactive microparticles and clay minerals. Therefore, the selective removal of these microparticles will lead to the volume reduction of contaminated soil. The present study examines methods for selectively removing radioactive microparticles from soil. Also, in order to reduce the volume of contaminated soil, we search a possibility to practically apply the separation method that uses the difference in specific gravity of particles (heavy liquid separation method).

Journal Articles

Experimental study on local interfacial parameters in upward air-water bubbly flow in a vertical 6$$times$$6 rod bundle

Han, X.*; Shen, X.*; Yamamoto, Toshihiro*; Nakajima, Ken*; Sun, Haomin; Hibiki, Takashi*

International Journal of Heat and Mass Transfer, 144, p.118696_1 - 118696_19, 2019/12

 Times Cited Count:0 Percentile:100(Thermodynamics)

Journal Articles

Experimental evaluation of wall shear stress in a double contraction nozzle using a water mock-up of a liquid Li target for an intense fusion neutron source

Kondo, Hiroo*; Kanemura, Takuji*; Park, C. H.*; Oyaizu, Makoto*; Hirakawa, Yasushi; Furukawa, Tomohiro

Fusion Engineering and Design, 146(Part A), p.285 - 288, 2019/09

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Herein, the wall shear stress in a double contraction nozzle has been evaluated experimentally to produce a liquid lithium (Li) target as a beam target for intense fusion neutron sources such as the International Fusion Materials Irradiation Facility (IFMIF), the Advanced Fusion Neutron Source (A-FNS), and the DEMO Oriented Neutron Source (DONES). The boundary layer thickness and wall shear stress are essential physical parameters to understand erosion-corrosion by the high-speed liquid Li flow in the nozzle, which is the key component in producing a stable Li target. Therefore, these parameters were experimentally evaluated using an acrylic mock-up of the target assembly. The velocity distribution in the nozzle was measured by a laser-doppler velocimeter and the momentum thickness along the nozzle wall was calculated using an empirical prediction method. The resulting momentum thickness was used to estimate the variation of the wall shear stress along the nozzle wall. Consequently, the wall shear stress was at the maximum in the second convergent section in front of the nozzle exit.

Journal Articles

A Noniterative mean-field QM/MM-type approach with a linear response approximation toward an efficient free-energy evaluation

Kido, Kentaro

Journal of Computational Chemistry, 40(24), p.2072 - 2085, 2019/09

 Times Cited Count:0 Percentile:100(Chemistry, Multidisciplinary)

JAEA Reports

SCHERN: Analysis program for chemical behavior of nitrogen oxide in accident of evaporation to dryness by boiling of reprocessed high level liquid waste in Fuel Reprocessing Facilities

Hiyama, Mina*; Tamaki, Hitoshi; Yoshida, Kazuo

JAEA-Data/Code 2019-006, 17 Pages, 2019/07

JAEA-Data-Code-2019-006.pdf:1.84MB

An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. In addition to this, nitrogen oxides (NOx) are also released formed by the thermal decomposition of metal nitrates of fission products (FP) in HLLW. It has been observed experimentally that NOx affects strongly to the transport behavior of Ru at the anticipated atmosphere condition in cells and/or compartments of the facility building. Chemical reactions of NOx with water and nitric acid are also recognized as the complex phenomena to undergo simultaneously in the vapor and liquid phases. An analysis program has been developed to simulate chemical reaction coupled with the thermo-hydraulic condition in the flow paths in the facility building.

Journal Articles

Analysis of chemical behavior of nitrogen oxide formed by thermal decomposition of FP nitrates in accident of evaporation to dryness by boiling of reprocessed high-level liquid waste

Yoshida, Kazuo; Tamaki, Hitoshi; Yoshida, Naoki; Yoshida, Ryoichiro; Amano, Yuki; Abe, Hitoshi

Nippon Genshiryoku Gakkai Wabun Rombunshi, 18(2), p.69 - 80, 2019/06

An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. In addition to this, nitrogen oxides are also released formed by the thermal decomposition of metal nitrates of fission products (FP) in HLLW. It has been observed experimentally that nitrogen oxide affects strongly to the transport behavior of Ru. Chemical reactions of nitrogen oxide with water and nitric acid are also recognized as the complex phenomena to undergo simultaneously in the vapor and liquid phases. An analysis method has been developed with coupling two types of computer codes to simulate not only thermo-hydraulic behavior but also chemical reactions in the flow paths of carrier gases. A simulation study has been also carried out with a typical facility building.

Journal Articles

Observation of aerosol particle behavior near gas-liquid interface

Uesawa, Shinichiro; Miyahara, Naoya; Horiguchi, Naoki; Yoshida, Hiroyuki; Osaka, Masahiko

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 5 Pages, 2019/05

Journal Articles

Parametric analysis of bubble and dissolved gas behavior in primary coolant system of sodium-cooled fast reactors

Matsushita, Kentaro; Ito, Kei*; Ezure, Toshiki; Tanaka, Masaaki

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 9 Pages, 2019/05

A numerical simulation code named SYRENA has been developed in JAEA to analyze the behavior of entrained bubbles and dissolved gas in the primary coolant of sodium-cooled fast reactor (SFR). In the present study, a flow network model of SYRENA to a hypothetical pool type reactor was developed and the non-condensable gas behavior was investigated through the comparison with that in the loop type reactor. The effect of the dipped-plate (D/P) tentatively introduced into the pool-type reactor on the gas behavior was investigated through the parametric analyses about the sodium exchange flow rate through the D/P and the gas entrainment rate at the free surface. It was suggested that the increase in the exchange flow rate through the D/P doesn't always work to decrease the bubble volume in the primary coolant system.

Journal Articles

Spectrochemistry of technetium by liquid electrode plasma optical emission spectrometry and its applicability of quantification for highly active liquid waste

Yamamoto, Masahiko; Do, V. K.; Taguchi, Shigeo; Kuno, Takehiko; Takamura, Yuzuru*

Spectrochimica Acta, Part B, 155, p.134 - 140, 2019/05

 Times Cited Count:1 Percentile:100(Spectroscopy)

The emission spectra of technetium (Tc) by liquid electrode plasma optical emission spectrometry have been investigated in this study. From the spectra, 52 emission peaks of Tc were observed in the 250-500 nm wavelength range. All peaks were assigned to the neutral state or singly ionized state. The relative intensities of these peaks were similar to those excited by an electric spark. The strongest intensity peaks were found at 254.3 nm, 261.0 nm, and 264.7 nm. Spectral interferences of coexisting elements in highly active liquid waste of reprocessing stream on those three strongest peaks were investigated using simulated sample. No spectral interferences were observed around the 264.7 nm Tc peak. Therefore, analytical performance using 264.7 nm peak was evaluated. The detection limit, estimated on standard and blank samples in 0.4 M nitric acid, was 1.9 mg/L. The relative standard deviation of Tc standard sample (12.0 mg/L) was 3.8% (N = 5, 1$$sigma$$).

Journal Articles

Waste management in a Hot Laboratory of Japan Atomic Energy Agency, 2; Condensation and solidification experiments on liquid waste

Watanabe, So; Ogi, Hiromichi*; Shibata, Atsuhiro; Nomura, Kazunori

International Journal of Nuclear and Quantum Engineering (Internet), 13(4), p.169 - 174, 2019/04

As a part of STRAD project conducted by JAEA, condensation of radioactive liquid waste containing various chemical compounds using reverse osmosis (RO) membrane filter was examined for efficient and safety treatment of the liquid wastes accumulated inside hot laboratories. NH$$_{4}$$$$^{+}$$ ion in the feed solution was successfully concentrated, and NH$$_{4}$$$$^{+}$$ ion involved in the effluents became lower than target value; 100 ppm. Solidification of simulated aqueous and organic liquid wastes was also tested. Those liquids were successfully solidified by adding cement or coagulants. Nevertheless, optimization in materials for confinement of chemicals is required for long time storage of the final solidified wastes.

Journal Articles

Conceptual design and verification of long-distance laser-probe system for Li target diagnostics of intense fusion neutron source

Kondo, Hiroo*; Kanemura, Takuji*; Hirakawa, Yasushi; Furukawa, Tomohiro

Fusion Engineering and Design, 136(Part A), p.24 - 28, 2018/11

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

In the IFMIF-EVEDA project, we designed and constructed the IFMIF-EVEDA Li Test Loop (ELTL), and we performed experiments to validate the stability of the Li target. This project required a diagnostic tool to be developed in order to examine the Li target; as such, we developed a unique laser-based method that we call the laser-probe method; this method combines a high-precision laser distance meter with a statistical data analysis method. Following the successful development of the laser-probe method, we proposes a long-distance-measurement of the laser probe method (long-distance LP method) as a diagnostics tool in off-beam conditions for IFMIF or the relevant neutron sources. In this study, the measurement uncertainty resulting from coherency of the laser in a long-distance-measurement has been verified by using stationary objects and a water jet simulating the liquid Li target.

Journal Articles

Cesium liquid-liquid extraction by calix-crown ethers; Solvent effect

Simonnet, M.; Miyazaki, Yuji; Suzuki, Shinichi; Yaita, Tsuyoshi

Progress in Nuclear Science and Technology (Internet), 5, p.66 - 69, 2018/11

Journal Articles

Development on high-power spallation neutron sources with liquid metals

Futakawa, Masatoshi

Proceedings of 13th International Symposium on Advanced Science and Technology in Experimental Mechanics (13th ISEM'18) (USB Flash Drive), 6 Pages, 2018/10

Issues on the engineering technologies relating to high-power spallation neutron sources with liquid metals are introduced. The present status on research activities and results was reviewed.

Journal Articles

Dynamic properties of nano-confined water in an ionic liquid

Abe, Hiroshi*; Yamada, Takeshi*; Shibata, Kaoru

Journal of Molecular Liquids, 264, p.54 - 57, 2018/08

 Times Cited Count:6 Percentile:34.28(Chemistry, Physical)

Journal Articles

Local gas-liquid two-phase flow characteristics in rod bundle geometry

Xiao, Y.*; Shen, X.*; Miwa, Shuichiro*; Sun, Haomin; Hibiki, Takashi*

Konsoryu Shimpojiumu 2018 Koen Rombunshu (Internet), 2 Pages, 2018/08

In order to develop constitutive equations of two-fluid model in rod bundle flow channels, experiments of adiabatic air-water upward two-phase flow in 6$$times$$6 rod bundle flow channel were performed. Local flow parameters such as void fraction, interfacial area concentration (IAC) and so on were measured by a double-sensor optical probe. The area-averaged void fraction and IAC data were compared with the predictions from a drift-flux model and an IAC correlation.

Journal Articles

Visualization study on droplet-entrainment in a high-speed gas jet into a liquid pool

Sugimoto, Taro*; Saito, Shimpei*; Kaneko, Akiko*; Abe, Yutaka*; Uchibori, Akihiro; Ohshima, Hiroyuki

Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 7 Pages, 2018/07

A computational fluid dynamics code for a sodium-water reaction phenomenon in a steam generator of sodium-cooled fast reactors has been developed. In order to provide the data for validation of this code, the visualization experiment on liquid droplet entrainment in the high-pressure air jet submerged in the water pool was carried out. The experiment successfully elucidated the behavior, such as atomization of the relatively large diameter liquid droplet generated from the gas-liquid interface.

Journal Articles

Quantitative determination of total cesium in highly active liquid waste by using liquid electrode plasma optical emission spectrometry

Do, V. K.; Yamamoto, Masahiko; Taguchi, Shigeo; Takamura, Yuzuru*; Surugaya, Naoki; Kuno, Takehiko

Talanta, 183, p.283 - 289, 2018/06

 Times Cited Count:2 Percentile:77.08(Chemistry, Analytical)

We develop a novel analytical method employing liquid electrode plasma optical emission spectrometry for measurement of total cesium in highly active liquid wastes. Limit of detection and limit of quantification are 0.005 mg/L and 0.02 mg/L, respectively. The method is validated and applied to the real samples.

306 (Records 1-20 displayed on this page)