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Tomioka, Dai; Kochiyama, Mami; Ozone, Kenji; Nakata, Hisakazu; Sakai, Akihiro
JAEA-Technology 2024-023, 38 Pages, 2025/03
JAEA-Technology-2024-023.pdf:1.54MB
Japan Atomic Energy Agency is an implementing organization of near-surface disposal for low-level radioactive wastes generated from research, industrial and medical facilities in Japan. Information on the radioactivity concentration of these radioactive wastes is dispensable for the design and conformity assessment of the waste disposal facilities for the licensing application of the disposal project and its safety review. Radioactive Wastes Disposal Center has been improving the radioactivity evaluation procedure for the dismantling waste generated from the research reactors based on the activation calculation. In order to investigate the applicability of the ORIGEN code (included in SCALE6.2.4), which enables more accurate activation calculations using multigroup neutron spectra, we performed activation calculations with the ORIGEN-code and the ORIGEN-S code (included in SCALE6.0), which has been widely used in the past, for the dismantled wastes from the Rikkyo University Research Reactor, where radioactivity analysis data for the structural materials around the reactor core were compiled. As a result, the calculation time difference between ORIGEN and ORIGEN-S was small and the evaluated radioactivity concentrations of the former were in the range of 0.8-1.0 times those of the latter, which was in good agreement with those of radiochemical analysis in the range of 0.5-3.0 times. The applicability of ORIGEN was confirmed. In addition, activation calculations assuming trace elements in structural materials of nuclear reactor were performed with ORIGEN and ORIGEN-S and the results were compared. The causes of the large differences among 170 nuclides that are important for dose assessment in near-surface disposal were assessed each nuclide.
Aono, Ryuji; Haraga, Tomoko; Kameo, Yutaka
JAEA-Technology 2024-006, 48 Pages, 2024/06
JAEA-Technology-2024-006.pdf:1.77MB
In the future, radioactive waste which generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried for the near surface disposal. It is necessary to establish the method to evaluate the radioactivity concentrations of the radioactive wastes. In this work, we studied the evaluation methodology of the radioactivity concentrations in concrete waste generated from JPDR. In order to construct the evaluation methodology of the radioactivity concentration, the validity of the evaluation methods was confirmed by mainly theoretical calculation and using the result of radiochemical analysis. Correcting the theoretical calculations using results of nuclide analysis, it is possible to evaluate the radioactivity concentrations of nuclides preliminary selected.
Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro
JAEA-Data/Code 2023-011, 32 Pages, 2023/11
JAEA-Data-Code-2023-011.pdf:0.93MB
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides (
H, 
C, 
Cl, 
Ca, 
Co, 
Ni, 
Sr, 
Nb, 
Ag, 
Cs, 
Ba, 
Eu, 
Eu, 
Ho, 
U, 
U, 
U, Pu, 
Pu, 
Pu, 
Am, 
Am, 
Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.
Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; Konda, Miki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2023-002, 81 Pages, 2023/05
JAEA-Data-Code-2023-002.pdf:3.0MB
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2, JRR-3 and Hot laboratory facilities. In this report, we summarized the radioactivity concentrations of 20 radionuclides (H, C, Cl, Co, Ni, Sr, Nb, 
Tc, Ag, 
I, Cs, Eu, Eu, U, U, Pu, Pu, Pu, Am, Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2020.
Tobita, Minoru*; Konda, Miki; Omori, Takeshi*; Nabatame, Tsutomu*; Onizawa, Takashi*; Kurosawa, Katsuaki*; Haraga, Tomoko; Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; et al.
JAEA-Data/Code 2022-007, 40 Pages, 2022/11
JAEA-Data-Code-2022-007.pdf:1.99MB
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete, ash, ceramic and brick samples generated from JRR-3, JRR4 and JRTF facilities. In this report, we summarized the radioactivity concentrations of 24 radionuclides (H, C, Cl, Ca, Co, Ni, Sr, Nb, Tc, Ag, I, Cs, Ba, Eu, Eu, Ho, U, U, Pu, Pu, Pu, Am, Am, Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2020-2021.
Tsuchida, Daiki; Mitsukai, Akina; Aono, Ryuji; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2022-004, 87 Pages, 2022/07
JAEA-Data-Code-2022-004.pdf:6.73MB
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until by the beginning of disposal. In order to contribute to this work, we collected and analyzed samples generated from JPDR, JRR-3 and JRR-4. In this report, radioactivity concentrations of 20 radionuclides (H, C, Cl, Co, Ni, Sr, Nb, Tc, Ag, I, Cs, Eu, Eu, U, U, Pu, 
Pu, Am, Cm) were determined based on radiochemical analysis and summarized as basic data for the study of evaluation method of radioactive concentration.
Kochiyama, Mami; Sakai, Akihiro
JAEA-Technology 2022-009, 56 Pages, 2022/06
JAEA-Technology-2022-009.pdf:4.15MB
It is necessary to evaluate radioactivity inventory in wastes before disposal of low-level radioactive wastes generated from dismantling research reactors. It is efficient for owners of each research reactor to use a common radioactive evaluation method in order to comply with the license application for disposal facility. In this report, neutron transport and activation calculations were carried out for the Rikkyo University research reactor in order to examine a common radioactivity evaluation method for burial disposal of radioactive wastes generated by dismantling. We adopted the neutron transport codes DORT and MCNP and the activation code ORIGEN-S with cross-section libraries based on JENDL-4.0 and JENDL/AD-2017. The radioactivity concentrations obtained by the radiochemical analysis and both calculation codes were in agreement by 0.4 to 3 times. Therefore, by appropriately considering this difference, the radioactivity evaluation method by DORT, MCNP and ORIGEN-S can be applied to the radioactivity evaluation for buried disposal. In order to classify wastes from dismantling by clearance or buried disposal method according to their radioactivity levels, we also created radioactivity concentration distributions in the concrete area and graphite thermal column area.
Tobita, Minoru*; Haraga, Tomoko; Endo, Tsubasa*; Omori, Hiroyuki*; Mitsukai, Akina; Aono, Ryuji; Ueno, Takashi; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2021-013, 30 Pages, 2021/12
JAEA-Data-Code-2021-013.pdf:1.47MB
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JPDR facility. In this report, we summarized the radioactivity concentrations of 21 radionuclides (H, C, Cl, Ca, Co, Ni, Sr, Nb, Ag, Cs, Eu, Eu, Ho, U, U, Pu, Pu, Pu, Am, Am, Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2018-2019.
Kochiyama, Mami; Okada, Shota; Sakai, Akihiro
JAEA-Technology 2021-010, 61 Pages, 2021/07
JAEA-Technology-2021-010.pdf:3.56MBJAEA-Technology-2021-010(errata).pdf:0.75MB
It is necessary to evaluate the radioactivity inventory in wastes in order to dispose of radioactive wastes generated from dismantling nuclear reactor in the shallow ground. In this report, we examined radioactivity evaluation method for near surface disposal about biological shield concrete near the core generated from the dismantling of JPDR. We calculated radioactive concentration of the target biological concrete using the DORT code and the ORIGEN-S code, and we estimated radioactivity concentration Di (Bq/t). For DORT calculation, the cross-section library created from the MATXSLIB-J40 file from JENDL-4.0 was used, and for ORIGEN-S, the attached library of SCALE6.0 was used. As a result of comparing the calculation results of the radioactivity concentration with the past measured values in the radial direction and the vertical direction, we found that the trends were generally the same. We calculated radioactive concentration of the target biological concrete Di (Bq/t), and we compared with the estimated Ci (Bq/t) equivalent to the dose criteria of trench disposal calculated for 140 nuclides. As a result we inferred that the except for about 2% of target waste could be disposed of in the trench disposal facility. We also preselected important nuclides for trench disposal based on the ratios (Di/Ci) for each nuclide, H-3, C-14, Cl-36, Ca-41, Co-60, Sr-90, Eu-152 and Cs-137 were selected as important nuclides.
Nagao, Rina; Namekawa, Maki*; Totsuka, Masayoshi*; Nakata, Hisakazu; Sakai, Akihiro
JAEA-Technology 2021-009, 139 Pages, 2021/06
JAEA-Technology-2021-009.pdf:13.96MB
Japan Atomic Energy Agency is the implementing body of the near surface disposal of low-level radioactive waste (LLW) generated from research facilities and other facilities. Concrete-pit disposal are considered as a method of disposing of the LLW. Since the concrete-pits are placed at deeper position than the groundwater level, we need to consider that radionuclides might migrate with the flow of groundwater. Accordingly, in order to explain the safety of the concrete-pit disposal facility, it is necessary to investigate the flow of groundwater and the volumetric flow rate of leaching water from the facility. Therefore, in this report, sensitivity analysis of the volumetric flow rate of leaching water from concrete-pit was carried out by varying the permeability of cover-soil filled with in outside of the lateral sides of the bentonite mixed soil (BMS) and the conditions of the BMS on the upper part of the concrete-pits. As a result of the analysis, when the BMS is normal condition, the volumetric flow rate of leaching water from the concrete-pits is reduced by lowering permeability of the lateral cover-soil. However, in the case of occurring the deterioration of the function of BMS on the upper part of the concrete-pit, significant reduction of the volumetric flow rate of leaching water is not seen even if the permeability of the lateral cover-soil is lowered. Therefore, taking into consideration the possibility of the deterioration of the function of BMS on the upper part of the concrete-pit, it is necessary to consider that cover-soil with low permeability is equipped on the upper part of the BMS.
Tsuchida, Daiki; Haraga, Tomoko; Tobita, Minoru*; Omori, Hiroyuki*; Omori, Takeshi*; Murakami, Hideaki*; Mitsukai, Akina; Aono, Ryuji; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2020-022, 34 Pages, 2021/03
JAEA-Data-Code-2020-022.pdf:1.74MB
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JRR-3 and JPDR. In this report, we summarized the radioactivity concentrations of 22 radionuclides(H, C, Cl, Ca, Co, Ni, Sr, Nb, Ag, Ba, Cs, Eu, Eu, Ho, U, U, Pu, Pu, Am, Am, Cm) which were obtained from radiochemical analysis of the samples.
Aono, Ryuji; Mitsukai, Akina; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2020-006, 70 Pages, 2020/08
JAEA-Data-Code-2020-006.pdf:2.59MB
Radioactive wastes which generated from research and testing reactors in Japan Atomic Energy Agency are planning to be buried at the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes by the time it starts disposal. In order to contribute to this work, we collected and analyzed the samples generated from JPDR and JRR-4. In this report, we summarized the radioactivity concentrations of 19 radionuclides (H, C, Cl, Co, Ni, Sr, Nb, Tc, Ag, I, Cs, Eu, Eu, U, U, Pu, Pu, Am, Cm) which were obtained from radiochemical analysis of those samples.
Fukui, Toshiki*; Maki, Takashi*; Miura, Nobuyuki; Tsukada, Takeshi*
Genshiryoku Bakkuendo Kenkyu (CD-ROM), 23(2), p.169 - 173, 2016/12
The basic research programs for the next generation vitrification technology, which are commissioned project from Ministry of Economy, Trade and Industry of Japan, have been implemented from 2014 until 2018 for developing the advanced vitrification technology of low level wastes and high level liquid wastes.
Sakai, Akihiro; Hasegawa, Makoto; Sakamoto, Yoshiaki; Nakatani, Takayoshi
Proceedings of International Conference on the Safety of Radioactive Waste Management (Internet), p.98_1 - 98_4, 2016/11
The radioactivity of uranium-bearing waste contaminated by refined uranium increases with the production of its progeny on a long-term timescale. Therefore, the long-term safety concept of the near surface disposal of uranium-bearing waste is very important. The Japan Atomic Energy Agency (JAEA) examines disposal safety by controlling the average uranium radioactivity concentration in each section of disposal facility and performing safety assessment for very conservative assumptions.
Sakai, Akihiro; Kurosawa, Ryohei*; Nakata, Hisakazu; Okada, Shota; Izumo, Sari; Sato, Makoto*; Kitamura, Yoichi*; Honda, Yasutake*; Takaoka, Katsuki*; Amazawa, Hiroya
JAEA-Technology 2016-019, 134 Pages, 2016/10
JAEA-Technology-2016-019.pdf:8.25MB
Japan Atomic Energy Agency has been developing to design trench disposal facility with impermeable layers in order to dispose of miscellaneous waste. Geomembrane liners have a function that prevent seepage of leachant and collect the leachant. However, the geomembrane liners do not necessarily provide the expected performance due to damage generated when heavy equipment contacts with the liner. Therefore, we studied the impermeable layers having high performance of preventing seepage of leachant including radioactivity taking into account characteristics of low permeable materials and effect of multiple layer structure. As results, we have evaluated that the composite layers composed by a drainage layer, geomembrane liners and a low permeable layer are most effective structure to prevent seepage of leachant. Taking into account disposal of waste including cesium, we also considered zeolite containing sheets for adsorption of cesium were installed in the impermeable layers.
Higuchi, Hidekazu; Momma, Toshiyuki; Nakashio, Nobuyuki; Kozawa, Kazushige; Tohei, Toshio; Sudo, Tomoyuki; Mitsuda, Motoyuki; Kurosawa, Shigenobu; Hemmi, Ko; Ishikawa, Joji; et al.
Proceedings of International Conference on Nuclear Energy System for Future Generation and Global Sustainability (GLOBAL 2005) (CD-ROM), 6 Pages, 2005/10
The JAERI constructed the Advanced Volume Reduction Facilities(AVRF). The AVRF consists of the Waste Size Reduction and Storage Facilities(WSRSF) and the Waste Volume Reduction Facilities(WVRF). By operating the AVRF, it will be able to produce waste packages for final disposal and to reduce the amount of the low level solid wastes. Cutting installations for large wastes such as tanks in the WSRSF have been operating since June 1999. The wastes treated so far amount to 600 m and the volume reduction ratio is around 1/3. The waste volume reduction is carried out by a high-compaction process or melting processes in the WVRF. The metal wastes from research reactors are treated by the high-compaction process. The other wastes are treated by the melting processes that enable to estimate radioactivity levels easily by homogenization and get chemical and physical stability. The WVRF have been operating with non-radioactive wastes since February 2003 for the training and the homogeneity investigation in the melting processes. The operation with radioactive wastes will start in FY2005.
Akutsu, Atsushi; Kishimoto, Katsumi; Sukegawa, Takenori; Shimada, Taro
JAERI-Tech 2003-090, 75 Pages, 2004/01
JAERI-Tech-2003-090.pdf:6.83MB
The Japan Research Reactor No.1 (JRR-1) that was constructed first in Japan was permanently shut down after operation from 1957 to 1968. At present, the reactor part is in safe store conditions. The JRR-1 facility is being used as an exhibition room for the time being, and will be dismantled in the future. In consideration of future dismantling of the facility, the radioactive inventory in reactor part was calculated using computer codes that are Two-Dimensional Discrete Ordinates Transport Code (DORT) and Oak Ridge Isotope Generation and Depletion Code (ORIGEN-MD). The average concentration of radioactivity is estimated to be 6.40
Bq/g in the core tank as of April, 2002. It is also expected that the low level waste (LLW) weights approximately 400kg and very low level waste (VLLW) weights approximately 14,000kg, and the waste which doesn't need to deal as a radioactive material weights approximately 250,000kg.
Sumita, Junya; Sawa, Kazuhiro; Tsuchie, Yasuo*; Urakami, Masao*; Kunitomi, Kazuhiko
JAERI-Tech 2002-104, 23 Pages, 2003/02
JAERI-Tech-2002-104.pdf:1.15MB
This report describes the result of study on disposal method of graphite blocks in future block-type reactor. Present study was carried out within a framework of joint research, "Research of Modular High Temperature Gas-cooled Reactors (No. 3)", between Japan Atomic Energy Research Institute (JAERI) and the Japan Atomic Power Company (JAPCO), in 2000. In this study, activities in fuel and reflector graphite blocks were evaluated and were compared with the disposal limits defined as low-level of radioactive waste. As a result, it was found that the activity for only C-14 was higher than disposal limits for the low-level of radioactive waste and that the amount of air in the graphite is important to evaluate precisely of C-14 activity. In addition, spent fuels can be stored in air-cooled condition at least after two years cooling in the storage pool.
Okuno, Hiroshi; Akiyama, Hideo*; Mochizuki, Hiroki*
Journal of Nuclear Science and Technology, 40(1), p.57 - 60, 2003/01
Times Cited Count：1 Percentile：10.60(Nuclear Science & Technology)Low-level waste (LLW) drums are required to transport as fissile material if the current IAEA's Regulations for the Safe Transport of Radioactive Material are rigorously applied. This problem is a consequence that water contents of concrete in LLW drums contained deuterium (D) in quantities more than 0.1% of fissile material mass, therefore they are not excepted from packages containing fissile material. Consideration of differences in the absorption cross sections of light hydrogen and D shows that the relative increase in the neutron multiplication factor by a presence of D in natural water for hydrogen (H)-moderated systems is not larger than 0.015%. A numerical calculation confirms that the infinite multiplication factor of a mixture of U-metal and water in a U/H mass ratio of 5% increases proportionally to the D/H atomic ratio, and that its relative increase is less than 0.03% for the D/H atomic ratio of 0.015%. The limiting fissile-to-H mass ratio of 5% in the exception rule is concluded to be applicable to H-moderated systems including D in natural water.
ray detection systemsOishi, Tetsuya; Tsutsumi, Masahiro; Sugita, Takeshi*; Yoshida, Makoto
Proceedings of 1st Asian and Oceanic Congress for Radiation Protection (AOCRP-1) (CD-ROM), 9 Pages, 2002/10
An EGS4 user code has been developed to design gamma ray detection systems for complex shapes of radioactive sources. The code is fundamentally based on the PRESTA-CG, which is improved on the electron transport in the EGS4 and specialized for using a combinatorial geometry (CG) method. The newly added functions are classified mainly into two parts of the transport of particles and the definition of sources. This user code was applied to some detectors used for low-level radioactive wastes monitoring in order to demonstrate the availability of this code. As the result, it was found that the response of anti-Compton spectrometer and the radiation background in a concrete building could be suitably estimated.
