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Journal Articles

Development of nanosized graphene material for neutron intensity enhancement below cold neutron energy

Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*

Journal of Neutron Research, 26(2-3), p.69 - 74, 2024/09

Slow neutrons, such as cold neutrons, are important non-destructive probes not only for basic physics but also for the structural genomics advancements in the life sciences and the battery technology advancements needed for the transition to a hydrogen society. Neutron-based science is also known as high-neutron-intensity-dependent science. A new unique method focusing on nanosized particle aggregation has been proposed to increase neutron intensity in that energy region. The method is based on intensity enhancement by multiple coherent scatterings with nanosized particle aggregation. The aggregation of nanosized particles matches the wavelength of below cold neutrons, causing a similar effect to coherent scattering, so-called Bragg scattering, leading to neutron intensity enhancement by several orders of magnitude. Nanodiamonds and magnesium hydride have recently been studied numerically and experimentally. The major challenge with nanodiamonds in practical applications is the molding method. Another carbon structure, graphene is focused on to find a solution to this problem. It is hypothesized that nanosized graphene could aid coherent neutron scattering under particle size conditions similar to nanodiamonds. We report the potential of nanosized graphene as a reflector material below cold neutrons, together with experimental results.

Journal Articles

New material exploration to enhance neutron intensity below cold neutrons; Nanosized graphene flower aggregation

Teshigawara, Makoto; Ikeda, Yujiro*; Yan, M.*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*

Nanomaterials (Internet), 13(1), p.76_1 - 76_9, 2023/01

 Times Cited Count:4 Percentile:60.72(Chemistry, Multidisciplinary)

To enhance neutron intensity below cold neutrons, it is proposed that nanosized graphene aggregation could facilitate neutron coherent scattering under particle size conditions similar to nanodiamond. It might also be possible to use it in high neutron radiation conditions due to graphene's strong sp2 bonds. Using the RIKEN accelerator-driven compact neutron source and iMATERIA at J-PARC, we performed neutron measurement experiments, total neutron cross-section, and small-angle neutron scattering on nanosized graphene aggregation. The measured data revealed, for the first time, that nanosized graphene aggregation increased the total cross-sections and small-angle scattering in the cold neutron energy region, most likely due to coherent scattering, resulting in higher neutron intensities, similar to nanodiamond.

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