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Teshigawara, Makoto; Lee, Y.*; Tatsumoto, Hideki*; Hartl, M.*; Aso, Tomokazu; Iverson, E. B.*; Ariyoshi, Gen; Ikeda, Yujiro*; Hasegawa, Takumi*
Nuclear Instruments and Methods in Physics Research B, 557, p.165534_1 - 165534_10, 2024/12
Times Cited Count:1 Percentile:22.55(Instruments & Instrumentation)At Japanese Spallation Neutron Source in J-PARC, the para-hydrogen fraction was measured by using Raman spectroscopy in-situ for an integrated beam power of 9.4 MW
h at 1 MW operation, to evaluate the functionality of the ferric oxyhydroxide catalyst. This result showed that full functionality of the catalyst was retained up to the 1 MW operation. We attempted to study the effect of neutron scattering driven para to ortho-hydrogen back-conversion rate in the absence of the catalyst effect with a bypass line without catalyst. The measured increase of ortho-hydrogen fraction was 0.44% for an integrated beam power of 2.4 MW
h at 500 kW operation, however, which was considered to be due to not only to neutron collisions in cold moderators but also to the high ortho-hydrogen fraction of initially static liquid hydrogen in the bypass line and passive exudation of quasi-static hydrogen in the catalyst vessel to the main loop.
Kai, Tetsuya; Kamiyama, Takashi*; Hiraga, Fujio*; Oi, Motoki; Hirota, Katsuya*; Kiyanagi, Yoshiaki*
Journal of Nuclear Science and Technology, 55(3), p.283 - 289, 2018/03
Times Cited Count:1 Percentile:8.84(Nuclear Science & Technology)Hirade, Tetsuya
Acta Physica Polonica A, 132(5), p.1470 - 1472, 2017/11
Times Cited Count:3 Percentile:25.18(Physics, Multidisciplinary)The positron annihilation lifetime measurements in RTILs showed very strange results. Finally, positron annihilation age-momentum correlation (AMOC) measurements indicated that it was caused by slow bubble formation in RTILs. Then I discovered the oscillation of o-Ps annihilation rates in room temperature ionic liquids (RTILs) which indicated, probably, the oscillation of the Ps bubble. Stepanov et al. calculated change of the bubble size in many liquids and the oscillation of the bubble was not expected except for a liquid He. It means that the structure of RTILs in nanometer scale is very different from usual liquids. Moreover, o-Ps pick-off annihilation rates seems to be too small for the macroscopic surface tension of RTILs. I am going to discuss what you can study by the positron annihilation methods for the structure of RTILs in nanometer scale.
Harada, Masahide; Watanabe, Noboru; Teshigawara, Makoto; Kai, Tetsuya; Ikeda, Yujiro
Nuclear Instruments and Methods in Physics Research A, 539(1-2), p.345 - 362, 2005/02
Times Cited Count:28 Percentile:84.22(Instruments & Instrumentation)Neutronic studies of decoupled hydrogen moderators were performed by calculations taking into account para hydrogen content, decoupling energy, moderator dimensions/shapes and reflector material. Low-energy parts of calculated spectral intensities with different para hydrogen contents were analyzed by a modified Maxwell function to characterize neutron spectra. The result shows that a 100% para hydrogen moderator gives the highest pulse peak intensity together with the narrowest pulse width and the shortest decay times. Pulse broadening with a reflector was explained by time distributions of source neutrons entering into the moderator through a decoupler. Material dependence of time distribution was studied. A decoupling energy higher than 1 eV does not bring about a large improvement in pulse widths and decay times, even at a large penalty in the peak intensity. The optimal moderator thickness was also discussed for a rectangular parallelepiped shape and a canteen shape moderators.
Gordon, E. B.*; Kumada, Takayuki; Ishiguro, Masazumi; Aratono, Yasuyuki
Journal of Experimental and Theoretical Physics, 99(4), p.776 - 783, 2004/10
The solid Deuterium clusters for the first time isolated in a matrix of solid Helium have been investigated at T = 1.3K and P = 3 MPa by CARS (Coherent anti-Stokes Raman spectroscopy) technique. The Q1(J=0) and Q1(J=1) lines intensity, shape and positions have been studied as the functions of ortho- para content in the solid, as well as of clusters size. The strong effect of Raman scattering cross section sensitivity to the molecular environment nuclear spin state has been found in CARS; the ratio of probabilities for the scattering by para (J=1) and ortho (J=0) deuterium being equal to 1 in a gas is as high as 10,000 in nearly pure o-D2, whereas it is about 50 in spontaneous Raman scattering. This effect has been shown to give rise starting from cluster size corresponding to the phonon band onset.
Kai, Tetsuya; Harada, Masahide; Teshigawara, Makoto; Watanabe, Noboru; Ikeda, Yujiro
Proceedings of ICANS-XVI, Volume 3, p.657 - 666, 2003/07
Neutronic design studies were carried out on the J-PARC coupled H
moderator. The highest time- and energy- integrated intensity below 15 meV, pulse peak intensity at 2 meV and 10 meV, were given by 100% para-H
moderators, but the optimal moderator thickness was different for each: more than 220 mm, about 120 mm and 80 mm, respectively. Finally, we concluded 140 mm was the optimal thickness for the 100% para-H
coupled moderator. Cold neutron distributions on the moderator viewed surface were found to exhibit an intensity-enhanced region at a picture frame part near premoderator. This rather peculiar distribution suggested that the moderator and the viewed surface must be designed so as to take the brighter region near premoderator in use. The intensity decreases along with beam-extraction angle to the normal direction down to about 70% at 25.4
. Then, we propose a cylindrical shape coupled moderator which brings about a slight intensity decrease for 0
but a increase in the averaged intensity over the angles of interest.
Sm
TiO
(0≦x≦1)Yoshii, Kenji; Nakamura, Akio; Abe, Hideki*
Journal of Alloys and Compounds, 290(1-2), p.236 - 243, 1999/00
Times Cited Count:11 Percentile:60.43(Chemistry, Physical)no abstracts in English
Nd
TiO
(Ln=Ce and Pr; 0≦x≦1)Yoshii, Kenji; Nakamura, Akio
Journal of Solid State Chemistry, 137(1), p.181 - 183, 1998/00
Times Cited Count:10 Percentile:63.79(Chemistry, Inorganic & Nuclear)no abstracts in English
Onuki, Kaoru; ; Nakajima, Hayato; Shimizu, Saburo
J. Chem. Eng. Jpn., 30(2), p.359 - 362, 1997/00
Times Cited Count:3 Percentile:34.81(Engineering, Chemical)no abstracts in English
Ito, Yasuo*; F.M.H.Mohamed*; Seguchi, Tadao;
Radiation Physics and Chemistry, 48(6), p.775 - 779, 1996/00
Times Cited Count:24 Percentile:85.64(Chemistry, Physical)no abstracts in English


U(n,f)
Moreaction,III(Treatment of the Very Hot Liguid Waste)Motoki, Ryozo; ; ; Motoishi, Shoji; ; ; ;
JAERI-M 84-015, 34 Pages, 1984/02
no abstracts in English
JAERI-M 7255, 30 Pages, 1977/09
no abstracts in English
Asahi, Yoshiro
Journal of Nuclear Science and Technology, 12(2), p.92 - 106, 1975/02
Times Cited Count:6no abstracts in English
Yamaguchi, Ichiro
Bulletin of the Chemical Society of Japan, 34(3), p.451 - 452, 1961/00
Times Cited Count:15no abstracts in English
Bulletin of the Chemical Society of Japan, 34(1), p.63 - 68, 1961/00
Times Cited Count:73no abstracts in English
Bulletin of the Chemical Society of Japan, 33(8), P. 1038, 1960/00
no abstracts in English
Bulletin of the Chemical Society of Japan, 33(8), p.1038 - 1046, 1960/00
Times Cited Count:110no abstracts in English