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Journal Articles

In-situ measurement of radiation driven back-conversion from para to ortho liquid hydrogen state in cold moderators at J-PARC

Teshigawara, Makoto; Lee, Y.*; Tatsumoto, Hideki*; Hartl, M.*; Aso, Tomokazu; Iverson, E. B.*; Ariyoshi, Gen; Ikeda, Yujiro*; Hasegawa, Takumi*

Nuclear Instruments and Methods in Physics Research B, 557, p.165534_1 - 165534_10, 2024/12

 Times Cited Count:1 Percentile:22.55(Instruments & Instrumentation)

At Japanese Spallation Neutron Source in J-PARC, the para-hydrogen fraction was measured by using Raman spectroscopy in-situ for an integrated beam power of 9.4 MW$$cdot$$h at 1 MW operation, to evaluate the functionality of the ferric oxyhydroxide catalyst. This result showed that full functionality of the catalyst was retained up to the 1 MW operation. We attempted to study the effect of neutron scattering driven para to ortho-hydrogen back-conversion rate in the absence of the catalyst effect with a bypass line without catalyst. The measured increase of ortho-hydrogen fraction was 0.44% for an integrated beam power of 2.4 MW$$cdot$$h at 500 kW operation, however, which was considered to be due to not only to neutron collisions in cold moderators but also to the high ortho-hydrogen fraction of initially static liquid hydrogen in the bypass line and passive exudation of quasi-static hydrogen in the catalyst vessel to the main loop.

Journal Articles

Measurements of neutronic characteristics of rectangular and cylindrical coupled hydrogen moderators

Kai, Tetsuya; Kamiyama, Takashi*; Hiraga, Fujio*; Oi, Motoki; Hirota, Katsuya*; Kiyanagi, Yoshiaki*

Journal of Nuclear Science and Technology, 55(3), p.283 - 289, 2018/03

 Times Cited Count:1 Percentile:8.84(Nuclear Science & Technology)

Journal Articles

Ortho-positronium annihilation in room temperature ionic liquids

Hirade, Tetsuya

Acta Physica Polonica A, 132(5), p.1470 - 1472, 2017/11

 Times Cited Count:3 Percentile:25.18(Physics, Multidisciplinary)

The positron annihilation lifetime measurements in RTILs showed very strange results. Finally, positron annihilation age-momentum correlation (AMOC) measurements indicated that it was caused by slow bubble formation in RTILs. Then I discovered the oscillation of o-Ps annihilation rates in room temperature ionic liquids (RTILs) which indicated, probably, the oscillation of the Ps bubble. Stepanov et al. calculated change of the bubble size in many liquids and the oscillation of the bubble was not expected except for a liquid He. It means that the structure of RTILs in nanometer scale is very different from usual liquids. Moreover, o-Ps pick-off annihilation rates seems to be too small for the macroscopic surface tension of RTILs. I am going to discuss what you can study by the positron annihilation methods for the structure of RTILs in nanometer scale.

Journal Articles

Neutronic studies on decoupled hydrogen moderator for a short-pulse spallation source

Harada, Masahide; Watanabe, Noboru; Teshigawara, Makoto; Kai, Tetsuya; Ikeda, Yujiro

Nuclear Instruments and Methods in Physics Research A, 539(1-2), p.345 - 362, 2005/02

 Times Cited Count:28 Percentile:84.22(Instruments & Instrumentation)

Neutronic studies of decoupled hydrogen moderators were performed by calculations taking into account para hydrogen content, decoupling energy, moderator dimensions/shapes and reflector material. Low-energy parts of calculated spectral intensities with different para hydrogen contents were analyzed by a modified Maxwell function to characterize neutron spectra. The result shows that a 100% para hydrogen moderator gives the highest pulse peak intensity together with the narrowest pulse width and the shortest decay times. Pulse broadening with a reflector was explained by time distributions of source neutrons entering into the moderator through a decoupler. Material dependence of time distribution was studied. A decoupling energy higher than 1 eV does not bring about a large improvement in pulse widths and decay times, even at a large penalty in the peak intensity. The optimal moderator thickness was also discussed for a rectangular parallelepiped shape and a canteen shape moderators.

Journal Articles

CARS study of deuterium clusters stabilized in solid helium

Gordon, E. B.*; Kumada, Takayuki; Ishiguro, Masazumi; Aratono, Yasuyuki

Journal of Experimental and Theoretical Physics, 99(4), p.776 - 783, 2004/10

The solid Deuterium clusters for the first time isolated in a matrix of solid Helium have been investigated at T = 1.3K and P = 3 MPa by CARS (Coherent anti-Stokes Raman spectroscopy) technique. The Q1(J=0) and Q1(J=1) lines intensity, shape and positions have been studied as the functions of ortho- para content in the solid, as well as of clusters size. The strong effect of Raman scattering cross section sensitivity to the molecular environment nuclear spin state has been found in CARS; the ratio of probabilities for the scattering by para (J=1) and ortho (J=0) deuterium being equal to 1 in a gas is as high as 10,000 in nearly pure o-D2, whereas it is about 50 in spontaneous Raman scattering. This effect has been shown to give rise starting from cluster size corresponding to the phonon band onset.

Journal Articles

Neutronic study on coupled hydrogen moderator for J-PARC spallation neutron source

Kai, Tetsuya; Harada, Masahide; Teshigawara, Makoto; Watanabe, Noboru; Ikeda, Yujiro

Proceedings of ICANS-XVI, Volume 3, p.657 - 666, 2003/07

Neutronic design studies were carried out on the J-PARC coupled H$$_{2}$$ moderator. The highest time- and energy- integrated intensity below 15 meV, pulse peak intensity at 2 meV and 10 meV, were given by 100% para-H$$_{2}$$ moderators, but the optimal moderator thickness was different for each: more than 220 mm, about 120 mm and 80 mm, respectively. Finally, we concluded 140 mm was the optimal thickness for the 100% para-H$$_{2}$$ coupled moderator. Cold neutron distributions on the moderator viewed surface were found to exhibit an intensity-enhanced region at a picture frame part near premoderator. This rather peculiar distribution suggested that the moderator and the viewed surface must be designed so as to take the brighter region near premoderator in use. The intensity decreases along with beam-extraction angle to the normal direction down to about 70% at 25.4$$^{rm o}$$. Then, we propose a cylindrical shape coupled moderator which brings about a slight intensity decrease for 0$$^{rm o}$$ but a increase in the averaged intensity over the angles of interest.

Journal Articles

Magnetic study of the mixed orthotitanate La$$_{1-x}$$Sm$$_{x}$$TiO$$_{3}$$(0≦x≦1)

Yoshii, Kenji; Nakamura, Akio; Abe, Hideki*

Journal of Alloys and Compounds, 290(1-2), p.236 - 243, 1999/00

 Times Cited Count:11 Percentile:60.43(Chemistry, Physical)

no abstracts in English

Journal Articles

Magnetic studies of orthotitanate Ln$$_{1-x}$$Nd$$_{x}$$TiO$$_{3}$$(Ln=Ce and Pr; 0≦x≦1)

Yoshii, Kenji; Nakamura, Akio

Journal of Solid State Chemistry, 137(1), p.181 - 183, 1998/00

 Times Cited Count:10 Percentile:63.79(Chemistry, Inorganic & Nuclear)

no abstracts in English

Journal Articles

Gas permeation through CVD modified anodic alumina membrane

Onuki, Kaoru; ; Nakajima, Hayato; Shimizu, Saburo

J. Chem. Eng. Jpn., 30(2), p.359 - 362, 1997/00

 Times Cited Count:3 Percentile:34.81(Engineering, Chemical)

no abstracts in English

Journal Articles

Vacancy spectroscopy of radiation cross-linked and degraded polytetrafluoroethylenes

Ito, Yasuo*; F.M.H.Mohamed*; Seguchi, Tadao;

Radiation Physics and Chemistry, 48(6), p.775 - 779, 1996/00

 Times Cited Count:24 Percentile:85.64(Chemistry, Physical)

no abstracts in English

JAEA Reports

Treatment of Liguid Waste from the Production of Molybdenum-99 by $$^{2}$$$$^{3}$$$$^{5}$$U(n,f)$$^{9}$$$$^{9}$$ Moreaction,III(Treatment of the Very Hot Liguid Waste)

Motoki, Ryozo; ; ; Motoishi, Shoji; ; ; ;

JAERI-M 84-015, 34 Pages, 1984/02

JAERI-M-84-015.pdf:1.12MB

no abstracts in English

JAEA Reports

ROTAX; A Nonlinear Optimization Program By Axes Rotation Method

JAERI-M 7255, 30 Pages, 1977/09

JAERI-M-7255.pdf:0.87MB

no abstracts in English

Journal Articles

Theory of omega-d modes

Asahi, Yoshiro

Journal of Nuclear Science and Technology, 12(2), p.92 - 106, 1975/02

 Times Cited Count:6

no abstracts in English

Journal Articles

Steric effects of ortho-groups on hydrogen bond formation in phenyl derivatives as studies by nuclear magnetic resonance

Yamaguchi, Ichiro

Bulletin of the Chemical Society of Japan, 34(3), p.451 - 452, 1961/00

 Times Cited Count:15

no abstracts in English

Journal Articles

Inorganic extraction studies on the system between bis (2-ethyl hexyl)-ortho-phosphoric acid and hydrochloric acid, 2

Bulletin of the Chemical Society of Japan, 34(1), p.63 - 68, 1961/00

 Times Cited Count:73

no abstracts in English

Journal Articles

Inorganic extraction studies on the system between bis (2-ethyl hexyl)-ortho-phosphoric acid and hydrochloric acid, 1

Bulletin of the Chemical Society of Japan, 33(8), P. 1038, 1960/00

no abstracts in English

Journal Articles

Inorganic extraction studies on the system between bis(2-ethyl hexyl) orthophosphoric acid and hydrochloric acid, 1

Bulletin of the Chemical Society of Japan, 33(8), p.1038 - 1046, 1960/00

 Times Cited Count:110

no abstracts in English

17 (Records 1-17 displayed on this page)
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