Shedding light on the origin of Pb, the heaviest -process; Only isotope in the solar system

Casanovas-Hoste, A.*; Harada, Hideo; Kimura, Atsushi; 130 of others*

Physical Review Letters, 133(5), p.052702_1 - 052702_8, 2024/07

https://doi.org/10.1103/PhysRevLett.133.052702

Outlining zircon growth in a granitic pluton using 3D cathodoluminescence patterns, U-Pb age, titanium concentration, and Th/U; Implications for the magma chamber process of Okueyama granite, Kyushu, Japan

Yuguchi, Takashi*; Ito, Daichi*; Yokoyama, Tatsunori; Sakata, Shuhei*; Suzuki, Satoshi*; Ogita, Yasuhiro; Yagi, Koshi*; Imura, Takumi*; Motai, Satoko*; Ono, Takeshi*

Lithos, 440-441, p.107026_1 - 107026_14, 2023/03

https://doi.org/10.1016/j.lithos.2023.107026

We propose a new method for elucidating zircon growth in granitic plutons, based on variations in three-dimensional 3D cathodoluminescence (CL) patterns, U-Pb ages, titanium concentration, and Th/U ratios. We focused on the zircon growth processes in the Okueyama granite (OKG) in central Kyushu, Japan, to obtain interpretations of magma chamber processes that result in the formation of granitic plutons. The OKG consists of three lithofacies: biotite granite (BG), hornblende granite (HG), and hornblende granodiorite (HGD). To determine the 3D internal structure and growth pattern of a zircon crystal, we performed CL observations for multi-sections of the samples. Simultaneously, we also determined the zircon U-Pb age and titanium concentration of the center sections of the samples. The 3D distribution of the oscillatory zoning can be used to determine the crystal nucleus. The simultaneous determination of zircon U-Pb ages and Ti concentrations of the granite samples indicates the time-temperature (t-T) history of granitic magma before its solidification. The t-T histories of the BG, HG, and HGD represented similar cooling behaviors within the magma chamber: rapid cooling from the zircon crystallization temperature to the closure temperature of the biotite K-Ar system between 16 Ma and 10 Ma. The variations in the Th/U ratios against temperature also demonstrate a different trend at the boundary of approximately 670 C. Fractional crystallization in the magma chamber progressed significantly at temperatures above 670 C; below 670 C, crystallization progressed slowly, indicating only minimal changes in the magma composition. The variations in the Th/U ratio against temperature in the BG, HG, and HGD portrayed common tendencies, indicating the same behavior in the progression of fractional crystallization among the three lithofacies, which in turn, represented the same behavior within the entire magma chamber.

Experimental study of nuclear data for Accelerator-Driven Transmutation System (ADS) using Kyoto University FFAG accelerator

Iwamoto, Hiroki; Meigo, Shinichiro; Nakano, Keita*; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.404 - 409, 2023/01

https://www.pasj.jp/web_publish/pasj2022/proceedings/PDF/TUP0/TUP040.pdf

no abstracts in English

Low-lying dipole strength distribution in Pb

Shizuma, Toshiyuki*; Endo, Shunsuke; Kimura, Atsushi; Massarczyk, R.*; Schwengner, R.*; Beyer, R.*; Hensel, T.*; Hoffmann, H.*; Junghans, A.*; Rmer, K.*; et al.

Physical Review C, 106(4), p.044326_1 - 044326_11, 2022/10

https://doi.org/10.1103/PhysRevC.106.044326

no abstracts in English

U-Pb ages of zircons from metamorphic rocks in the upper sequence of the Hidaka metamorphic belt, Hokkaido, Japan; Identification of two metamorphic events and implications for regional tectonics

Takahashi, Hiroshi*; Mikoshiba, Masumi*; Shimura, Toshiaki*; Nagata, Mitsuhiro; Iwano, Hideki*; Danhara, Toru*; Hirata, Takafumi*

Island Arc, 30(1), p.e12393_1 - e12393_15, 2021/01

https://doi.org/10.1111/iar.12393

The Hidaka metamorphic belt is an excellent example of island-arc-type crust, and in this belt the metamorphic grade increases westwards from unmetamorphosed sediment up to the granulite facies. The metamorphic age of the belt had previously been considered to be ca. 55 Ma. However, zircons from the granulites in the lower sequence have given U-Pb ages of ca. 21-19 Ma and a preliminary report on zircons from pelitic gneiss in the upper sequence gave a U-Pb age of ca. 40 Ma. In this paper we provide new U-Pb ages for zircons from the pelitic gneisses in the upper sequence in order to assess the metamorphic age and also the maximum depositional age of the sedimentary protolith. The weighted mean Pb/U ages and 2 sigma errors for zircons from biotite gneiss in the central area of the belt are 39.6 0.9 Ma for metamorphic overgrowth rims and 53.1 0.9 Ma for the youngest inherited detrital cores. The ages of zircons from cordierite-biotite gneiss in the southern area are 35.9 0.7 Ma for overgrowth rims and 46.5 2.8 Ma for the youngest detrital cores. These results indicate that the metamorphism of the upper sequence took place at ca. 40-36 Ma, and that the sedimentary protolith was deposited after ca. 53-47 Ma. These metamorphic ages are consistent with the reported ages of ca. 37-36 Ma plutonic rocks in the upper sequence, but contrast with the ca. 21-19 Ma ages of metamorphic and plutonic rocks in the lower sequence. Therefore, we conclude, that the upper and lower metamorphic sequences developed independently but became coupled before ca. 19 Ma as a result of dextral reverse tectonic movements, as indicated by the intrusion of ca. 19-18 Ma magmas, possibly generated in the lower sequence, into the upper sequence.

Interactive in-situ steering and visualization of GPU-accelerated simulations using particle-based volume rendering

Kawamura, Takuma; Hasegawa, Yuta; Idomura, Yasuhiro

Proceedings of Joint International Conference on Supercomputing in Nuclear Applications + Monte Carlo 2020 (SNA + MC 2020), p.187 - 192, 2020/10

In order to realize the atmospheric dispersion prediction of pollutants, a fluid simulation by adaptive mesh refinement (AMR) optimized for GPU supercomputer has been developed, and interactive visualization and parameter steering of the simulation results are needed. In this study, we extend particle-based in-situ visualization method for structured grids into AMR, and enables in-situ steering of the simulation parameters by utilizing an in-situ control mechanism via files. By combining the developed method with plume dispersion simulation in urban areas running on a GPU platform, it was shown that human-in-the-loop pollution source search is possible without enormous parameter scanning.

Special issue on accelerator-driven system benchmarks at Kyoto University Critical Assembly

Pyeon, C. H.*; Talamo, A.*; Fukushima, Masahiro

Journal of Nuclear Science and Technology, 57(2), p.133 - 135, 2020/02

https://doi.org/10.1080/00223131.2019.1680324

Sample worth measurements with systematically changed mixing ratios of lead and bismuth in A-core of KUCA for ADS

Fukushima, Masahiro; Oizumi, Akito; Yamanaka, Masao*; Pyeon, C. H.*

KURNS Progress Report 2018, P. 143, 2019/08

https://www.rri.kyoto-u.ac.jp/PUB/report/PR/ProgRep2018/ProgRep2018.html

For the design study of ADS, integral experimental data of nuclear characteristics of LBE is necessary to validate cross sections of lead (Pb) and bismuth (Bi). In present study, sample worth measurements were carried out with systematically changed mixing ratios of lead and bismuth, which would be complementary to the previous data of Pb and Bi samples individually measured in FY 2013 and FY 2017, respectively.

U-Pb dating of calcite using LA-ICP-MS; Instrumental setup for non-matrix-matched age dating and determination of analytical areas using elemental imaging

Yokoyama, Tatsunori; Kimura, Junichi*; Mitsuguchi, Takehiro; Danhara, Toru*; Hirata, Takafumi*; Sakata, Shuhei*; Iwano, Hideki*; Maruyama, Seiji*; Chang, Q.*; Miyazaki, Takashi*; et al.

Geochemical Journal, 52(6), p.531 - 540, 2018/12

https://doi.org/10.2343/geochemj.2.0541

Lead void reactivity worth in two critical assembly cores with differing uranium enrichments

Fukushima, Masahiro; Goda, J.*; Bounds, J.*; Cutler, T.*; Grove, T.*; Hutchinson, J.*; James, M.*; McKenzie, G.*; Sanchez, R.*; Oizumi, Akito; et al.

Nuclear Science and Engineering, 189, p.93 - 99, 2018/01

https://doi.org/10.1080/00295639.2017.1373520

To validate lead (Pb) nuclear cross sections, a series of integral experiments to measure lead void reactivity worths was conducted in a high-enriched uranium (HEU)/Pb system and a low enriched uranium (LEU)/Pb system using the Comet Critical Assembly at NCERC. The critical experiments were designed to provide complementary data sets having different sensitivities to scattering cross sections of lead. The larger amount of the U present in the LEU/Pb core increases the neutron importance above 1 MeV compared with the HEU/Pb core. Since removal of lead from the core shifts the neutron spectrum to the higher energy region, positive lead void reactivity worths were observed in the LEU/Pb core while negative values were observed in the HEU/Pb core. Experimental analyses for the lead void reactivity worths were performed with the Monte Carlo calculation code MCNP6.1 together with nuclear data libraries, JENDL 4.0 and ENDF/B VII.1. The calculation values were found to overestimate the experimental ones for the HEU/Pb core while being consistent for the LEU/Pb core.