Hosoda, Masahiro*; Nugraha, E. D.*; Akata, Naofumi*; Yamada, Ryohei; Tamakuma, Yuki*; Sasaki, Michiya*; Kelleher, K.*; Yoshinaga, Shinji*; Suzuki, Takahito*; Rattanapongs, C. P.*; et al.
Science of the Total Environment, 750, p.142346_1 - 142346_11, 2021/01
The biological effects of low dose-rate radiation exposures on humans remains unknown. In fact, the Japanese nation still struggles with this issue after the Fukushima Dai-ichi Nuclear Power Plant accident. Recently, we have found a unique area in Indonesia where naturally high radiation levels are present, resulting in chronic low dose-rate radiation exposures. We aimed to estimate the comprehensive dose due to internal and external exposures at the particularly high natural radiation area, and to discuss the enhancement mechanism of radon. A car-borne survey was conducted to estimate the external doses from terrestrial radiation. Indoor radon measurements were made in 47 dwellings over three to five months, covering the two typical seasons, to estimate the internal doses. Atmospheric radon gases were simultaneously collected at several heights to evaluate the vertical distribution. The absorbed dose rates in air in the study area vary widely between 50 nGy h and 1109 nGy h. Indoor radon concentrations ranged from 124 Bq m to 1015 Bq m. That is, the indoor radon concentrations measured exceed the reference levels of 100 Bq m recommended by the World Health Organization. Furthermore, the outdoor radon concentrations measured were comparable to the high indoor radon concentrations. The annual effective dose due to external and internal exposures in the study area was estimated to be 27 mSv using the median values. It was found that many residents are receiving radiation exposure from natural radionuclides over the dose limit for occupational exposure to radiation workers. This enhanced outdoor radon concentration might be as a result of the stable atmospheric conditions generated at an exceptionally low altitude. Our findings suggest that this area provides a unique opportunity to conduct an epidemiological study related to health effects due to chronic low dose-rate radiation exposure.
Goto, Akira; Sasaki, Akimichi*; Komatsu, Tetsuya; Miwa, Atsushi*; Terusawa, Shuji*; Kagohara, Kyoko*; Shimada, Koji
JAEA-Research 2020-013, 88 Pages, 2020/11
Improvement of the investigation techniques to identify active faults is important for the implementation of geological disposal projects from the viewpoint of avoiding locations where permeability increases due to fault displacement. Generally, the existence of active faults is confirmed by aerial photography interpretation of fault displacement topography, which is a topographical trace of fault movement, and on-site geological surveys. However, the investigation method for cases where the topographical traces are unclear is not sufficiently developed. Therefore, to improve existing topographical methods, this study deciphered lineaments up to the rank of poorly defined features, which are almost neglected in general active fault research. The investigation area is one of the geodetic strain concentration zone, called the southern Kyushu shear zone, where the seismogenic faults of the 1997 Kagoshima northwest earthquakes are concealed. We conducted aerial photography interpretation of 62 sheets of 1/25,000 topographic maps, and obtained 1,327 lineaments. Distribution density, direction and length of lineaments were also investigated with topographic and geologic information. As a result, it was clarified that the east-west lineaments in the south Kyushu shear zone predominate in the western part, and the lineaments are densely distributed in the aftershock distribution area of the Kagoshima northwest earthquake. Along with these results, we have compiled a catalog of typical 13 lineaments based on combinations of clarity, direction, length and geomorphic characters of lineaments.
Kokusen, Junya; Akasaka, Shingo*; Shimizu, Osamu; Kanazawa, Hiroyuki; Honda, Junichi; Harada, Katsuya; Okamoto, Hisato
JAEA-Technology 2020-011, 70 Pages, 2020/10
The Uranium Enrichment Laboratory in the Japan Atomic Energy Agency (JAEA) was constructed in 1972 for the purpose of uranium enrichment research. The smoke emitting accident on 1989 and the fire accident on 1997 had been happened in this facility. The research on uranium enrichment was completed in JFY1998. The decommissioning work was started including the transfer of the nuclear fuel material to the other facility in JFY2012. The decommissioning work was completed in JFY2019 which are consisting of removing the hood, dismantlement of wall and ceiling with contamination caused by fire accident. The releasing the controlled area was performed after the confirmation of any contamination is not remained in the target area. The radioactive waste was generated while decommissioning, burnable and non-flammable are 1.7t and 69.5t respectively. The Laboratory will be used as a general facility for cold experiments.
Department of Decommissioning and Waste Management
JAEA-Review 2020-012, 103 Pages, 2020/08
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2018 to March 31, 2019. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM.
Udagawa, Yutaka; Fuketa, Toyoshi*
Comprehensive Nuclear Materials, 2nd Edition, Vol.2, p.322 - 338, 2020/08
Rodriguez, D.; Koizumi, Mitsuo; Rossi, F.; Seya, Michio; Takahashi, Toon; Bogucarska, T.*; Crochemore, J.-M.*; Pedersen, B.*; Takamine, Jun
Journal of Nuclear Science and Technology, 57(8), p.975 - 988, 2020/08
Igarashi, Kai*; Onuki, Ryoji*; Sakai, Takaaki*; Kato, Shinya; Matsuba, Kenichi; Kamiyama, Kenji
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08
Ioka, Ikuo; Kuriki, Yoshiro*; Iwatsuki, Jin; Kawai, Daisuke*; Yokota, Hiroki*; Inagaki, Yoshiyuki; Kubo, Shinji
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 5 Pages, 2020/08
A thermochemical water-splitting iodine-sulfur processes (IS process) is one of candidates for the large-scale production of hydrogen using heat from solar power. Severe corrosive environment which is thermal decomposition of sulfuric acid exists in the IS process. A hybrid material with the corrosion-resistance and the ductility was made by a plasma spraying and laser treatment. The specimen had excellent corrosion resistance in the condition of 95 mass% boiling sulfuric acid. This was attributed to the formation of SiO on the surface. The container using the hybrid material was experimentally made. The pre-oxidized container using hybrid technique was prepared for the corrosion test in boiling sulfuric acid to evaluate the corrosion characteristics of the container. There was no detaching of the surface with the weld part and the R processing. We proposed the calculation method of corrosion rate from the ions dissolved in the sulfuric acid solution after the corrosion test.
JAEA-Data/Code 2020-005, 48 Pages, 2020/07
In order to discuss the technological development and human resource development necessary for the future nuclear fuel cycle, various quantitative analyzes were conducted assuming a wide range of future nuclear power generation scenarios. In the evaluation of quantities, the future power generation of LWR and fast reactor, the amount of spent fuel reprocessing, etc. were assumed, and the amount of uranium demand, the accumulation of spent fuel, plutonium, vitrified waste etc. were estimated.
Aoyagi, Kazuhei; Sakurai, Akitaka; Miyara, Nobukatsu; Sugita, Yutaka
JAEA-Research 2020-004, 68 Pages, 2020/06
In construction and operational phase of a high-level radioactive waste disposal project, it is necessary to monitor on mechanical stability of underground facility for long term. In this research, we measured the displacement of the rock around the gallery and the stress acting on support materials. Furthermore, we investigated the durability of measurement sensor installed in the rock mass and the support material such as concreate lining and steel support. As a result, optical fiber sensor is appropriate for measurement of the displacement of rock mass around the gallery, while it is enough to apply the conventional electric sensor for the measurement of stress acting on the support material in the geological environment (soft rock and low inflow). The result of the measurement in the fault zone in 350 m gallery, show that the stresses acting on both shotcrete and steel arch lib exceeded the value which will cause the instability of the gallery. However, as, we found no crack on the surface of the shotcrete. By observation on the surface of shotcrete, thus, it was concluded that careful observation of shotcrete around that section in addition to the monitoring the measured stress was necessary to continue. In other measurement sections, there was no risk for the instability of the gallery as a result of the investigation of the measurement result.
Aoki, Tomoyuki*; Tani, Takuya*; Sakai, Kazuo*; Koga, Yoshihisa*; Aoyagi, Kazuhei; Ishii, Eiichi
JAEA-Research 2020-002, 83 Pages, 2020/06
The Japan Atomic Energy Agency (JAEA) has conducted with the Horonobe Underground Research Project in Horonobe, Teshio-gun, Hokkaido for the purpose of research and development related to geological disposal technology for high-level radioactive wastes in sedimentary soft rocks. The geology around the Horonobe Underground Research Laboratory (HURL) is composed of the Koetoi diatomaceous mudstone layer and the Wakkanai siliceous layer, both of which contain a large amount of diatom fossils. Since these rocks exhibit relatively high porosity but low permeability, it is important to investigate the poro-elastic characteristics of the rock mass. For this objective, it is necessary to measure parameters based on the poro-elastic theory. However, there are few measurement results of the poro-elastic parameters for the geology around HURL, and the characteristics such as dependence on confining pressure are not clearly understood. One of the reasons is that the rocks show low permeability and the pressure control during testing is difficult. Therefore, a poro-elastic parameter measurement test was conducted on the siliceous mudstone of the Wakkanai formation to accumulate measurement results on the poro-elastic parameters and to examine the dependence of the parameters on confining pressure. As a result, some dependency of the poro-elastic parameters on confining pressure was observed. Among the measured or calculated poro-elastic parameters, the drained bulk modulus increased, while the Skempton's pressure coefficient, and the Biot-Wills coefficient in the elastic region decreased with the increase in confining pressure. The measurement results also inferred that the foliation observed in the rock specimens might impact a degree of dependency of those parameters on confining pressure.
Kubo, Shigenobu; Chikazawa, Yoshitaka; Ohshima, Hiroyuki; Uchita, Masato*; Miyagawa, Takayuki*; Eto, Masao*; Suzuno, Tetsuji*; Matoba, Ichiyo*; Endo, Junji*; Watanabe, Osamu*; et al.
Mechanical Engineering Journal (Internet), 7(3), p.19-00489_1 - 19-00489_16, 2020/06
The authors are developing the design concept of pool-type sodium-cooled fast reactor (SFR) that addresses Japan's specific siting conditions such as earthquakes and meets safety design criteria (SDC) and safety design guidelines (SDGs) for Generation IV SFRs. The development of this concept will broaden not only options for reactor types in Japan but also the range and depth of international cooperation. A design concept of 1,500 MWt (650 MWe) class pool-type SFR was thought up by applying design technology obtained from the design of advanced loop-type SFR, named JSFR, equipped with safety measures that reflect results from the feasibility study on commercialized fast reactor cycle systems and fast reactor cycle technology development, improved maintainability and repairability, and lessons learned from the Fukushima Daiichi Nuclear Power Plants accident.
Abe, Yuta; Yamashita, Takuya; Sato, Ikken; Nakagiri, Toshio; Ishimi, Akihiro
Journal of Nuclear Engineering and Radiation Science, 6(2), p.021113_1 - 021113_9, 2020/04
Hotta, Akitoshi*; Akiba, Miyuki*; Morita, Akinobu*; Konovalenko, A.*; Vilanueva, W.*; Bechta, S.*; Komlev, A.*; Thakre, S.*; Hoseyni, S. M.*; Skld, P.*; et al.
Journal of Nuclear Science and Technology, 57(4), p.353 - 369, 2020/04
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2019-038, 57 Pages, 2020/03
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Imaging System with Ultra-high Spatial Resolution Aiming to Detect Alpha-dust". In the present study, we have developed a prototype of a system aiming to elucidate the behavior of alpha-dust generated at the time of debris retrieval. In this system, alpha-ray is first converted to visible light by novel scintillator. Then, imaging with ultra-high resolution will be possible using a lens and an Si-semiconductor camera (CMOS camera). Also, it will be possible to identify the species of alpha-ray emitting nuclides by unfolding of the spectra. The demonstration tests of the system will be conducted for dust samplers at the Plutonium Fuel Development Center, JAEA. In the development of the present system, it is important to use scintillator whose emission wavelength is sensitive to the CMOS camera as well as high emission scintillator. Considering these conditions, the key technology will be the improvement of the purity of crystals and optimization of the shapes of the materials including powers.
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2019-037, 90 Pages, 2020/03
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Technology to Prevent Scattering of Radioactive Materials in Fuel Debris Retrieval". The objective of the present study is to clarify the behavior of microparticles in gas and liquid phases in order to steadily confine radioactive microparticles at the time of debris retrieval in Fukushima Daiichi Nuclear Power Station. In addition, as measures to prevent scattering, we will evaluate and develop methods by experiments and simulation as to; (1) a method to suppress the scattering with minimum amount of water utilizing water spray etc., and (2) a method to suppress the scattering by solidifying fuel debris.
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2019-030, 66 Pages, 2020/03
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. Among the adopted proposals in FY2018, this report summarizes the research results of the "Identification of Altered Phases of Fuel Debris by Laser Fluorescence Spectroscopy". In the present study, we focus on uranium that is the main component element in debris, and identify the altered phase produced on the debris surface under various conditions by time-resolved laser fluorescence spectroscopy (TRLFS) with high sensitivity to hexavalent uranium (U(VI)) that is stable in oxidation environment. In particular, further high-sensitive and high-resolution measurements are implemented by improving the fluorescence yields and suppressing the broadening of the peaks through the measurements at ultra-low temperature. In addition, with the supports by quantum chemical calculations, multivariate analysis, and machine learning, the method will lead to the identification of multicomponent and heterogeneous altered phase of fuel debris.
Sugiura, Yuki; Suyama, Tadahiro*; Tachi, Yukio
JAEA-Data/Code 2019-022, 40 Pages, 2020/03
Sorption behavior of radionuclides (RNs) in buffer materials, rocks and cementitious materials is one of the key processes in a safe geological disposal. This report focuses on updating of JAEA sorption database (JAEA-SDB) as a basis of integrated approach for the performance assessment (PA)-related distribution coefficient (K) setting and development of mechanistic sorption models. K data and their quality assurance (QA) results were updated by focusing on the following systems as potential needs extracted from our recent activities on the K setting and development of mechanistic models, i.e., clay minerals, sedimentary rocks and cementitious materials. As a result, 6,702 K data from 60 references were added and the total number of K values in JAEA-SDB reached 69,679. The QA/classified K data reached about 72% for all K data in JAEA-SDB.
Sato, Junya; Shiota, Kenji*; Takaoka, Masaki*
Journal of Hazardous Materials, 385, p.121109_1 - 121109_9, 2020/03
Lead is a hazardous heavy metal that can be stabilized by incorporation into the matrix of aluminosilicate bearing phases as they solidify. The actual mechanism by which lead is stabilized, however, continues to be unclear because the individual mechanisms of Pb incorporation into crystalline and amorphous aluminosilicate phases have not yet been studied separately. A detailed investigation of the incorporation of Pb into the amorphous phase of aluminosilicate solids was therefore performed. Amorphous aluminosilicate solids were synthesized with 0.7, 1.5, and 3.7 wt% of Pb from aluminosilicate gel produced from chemical reagents. Based on Raman spectroscopy, the Si-O stretching vibration bond shifted to lower wavenumbers with increasing Pb concentration. This shift suggested that covalent bonding between Pb and O in the matrix of the aluminosilicate solids increased. In addition, sequential extraction revealed that most of the Pb (75-90%) in the aluminosilicate solids was in a poorly soluble form (i.e. reducible, oxidizable, and residual fractions). These findings indicate that most of Pb is bonded covalently to the amorphous phase in aluminosilicate solids.
Nakayama, Masashi; Ono, Hirokazu
JAEA-Research 2019-007, 132 Pages, 2019/12
The Horonobe Underground Research Laboratory (URL) Project has being pursued by Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies through investigations of the deep geological environment within the host sedimentary formation at Horonobe, northern Hokkaido. The URL Project consists of two major research areas, "Geoscientific Research" and "Research and Development on Geological Disposal Technologies". The in-situ experiment for performance confirmation of engineered barrier system (EBS experiment) had been prepared from 2013 to 2014 fiscal year at GL-350m gallery, and heating by electric heater in simulated overpack had started in January, 2015. One of objectives of the EBS experiment is acquiring data concerned with Thermal-Hydrological-Mechanical-Chemical (THMC) coupled behavior. These data will be used in order to confirm the performance of engineered barrier system. This report shows following works had carried out at the GL-350 m gallery. Excavation of a test niche and a test pit, Setting buffer material blocks and a simulated overpack into the test pit, Backfilling the niche by compaction backfilling material and setting backfilling material blocks, Casting concrete type plug and contact grouting, Consolidate measurement system and start measuring.