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JAEA Reports

Development of technology for rapid analysis of strontium-90 with low isotopic abundance using laser resonance ionization (Contract research); FY2019 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2020-024, 75 Pages, 2021/01

JAEA-Review-2020-024.pdf:5.43MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Technology for Rapid Analysis of Strontium-90 with Low Isotopic Abundance using Laser Resonance Ionization" conducted in FY2019. In this study, we will develop a rapid analysis technique for strontium-90 using diode laser-based resonance ionization with elemental and isotopic selectivity. Strontium-90 is one of the major difficult-to-measure nuclides released into the environment due to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station. Our method is particularly intended for real samples which contain high concentrations of strontium stable isotopes such as marine samples.

JAEA Reports

Development of technology for rapid analysis of strontium-90 with low isotopic abundance using laser resonance ionization (Contract research); FY2018 Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2019-027, 70 Pages, 2020/01

JAEA-Review-2019-027.pdf:5.18MB

JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Technology for Rapid Analysis of Strontium-90 with Low Isotopic Abundance Using Laser Resonance Ionization". In this study, we will develop a rapid analysis technique for strontium-90 using diode laser-based resonance ionization with elemental and isotopic selectivity. Strontium-90 is one of the major difficult-to-measure nuclides released into the environment due to the accident at Tokyo Electric Power Company (TEPCO)'s Fukushima Daiichi Nuclear Power Station. Our method is particularly intended for real samples which contain high concentrations of strontium stable isotopes such as marine samples.

Journal Articles

Preparation of an H$$_{2}$$-permselective silica membrane for the separation of H$$_{2}$$ from the hydrogen iodide decomposition reaction in the iodine-sulfur process

Myagmarjav, O.; Ikeda, Ayumi*; Tanaka, Nobuyuki; Kubo, Shinji; Nomura, Mikihiro*

International Journal of Hydrogen Energy, 42(9), p.6012 - 6023, 2017/03

 Times Cited Count:17 Percentile:59.75(Chemistry, Physical)

Journal Articles

Investigation of ligand immobilized nano-composite adsorbent for efficient cerium(III) detection and recovery

Awual, M. R.; Hasan, M. M.*; Shahat, A.*; Naushad, M.*; Shiwaku, Hideaki; Yaita, Tsuyoshi

Chemical Engineering Journal, 265, p.210 - 218, 2015/04

 Times Cited Count:179 Percentile:99.3(Engineering, Environmental)

Journal Articles

Organic-inorganic based nano-conjugate adsorbent for selective palladium(II) detection, separation and recovery

Awual, M. R.; Hasan, M. M.*; Znad, H.*

Chemical Engineering Journal, 259, p.611 - 619, 2015/01

 Times Cited Count:158 Percentile:99.03(Engineering, Environmental)

Journal Articles

Selective separation of Am(III) from lanthanides(III) by solvent extraction with hydrophobic field of "superweak" anion

Naganawa, Hirochika; Suzuki, Hideya*; Noro, Junji*; Kimura, Takaumi

Chemical Communications, (23), p.2963 - 2965, 2005/06

A "superweak" anion, TFPB-, gives rise to a field effect on the selectivity for Am$$^{3+}$$ over Ln$$^{3+}$$ in their extraction from aqueous HNO$$_{3}$$ solution into benzene containing a "hard donor" extractant that shows no selectivity for these metal ions in traditional solvent extraction.

Journal Articles

Thermo- and pH-sensitive gel membranes based on poly-(acryloyl-$$L$$-proline methyl ester)-${it graft}$-poly(acrylic acid) for selective permeation of metal ions

Hasegawa, Shin; Ohashi, Hitoshi; Maekawa, Yasunari; Katakai, Ryoichi*; Yoshida, Masaru

Radiation Physics and Chemistry, 72(5), p.595 - 600, 2005/04

 Times Cited Count:16 Percentile:74.09(Chemistry, Physical)

Thermo- and pH-responsive gel membranes were synthesized by $$gamma$$-ray grafting of pH-responsive poly (acrylic acid) (AAc) onto thermo-responsive polymer gel of acryloyl-$$L$$-proline methyl ester (A-ProOMe). The gel membranes of poly (A-ProOMe) with 15 mol% graft chains of AAc exhibited both thermo- and pH-responses. Under the condition (pH 6.0, 30$$^{circ}$$C) in which the thermo-sensitive unit shrinks and the pH-sensitive unit swells, the selective permeation of Li ion over Co and Ni ions can be achieved.

Journal Articles

Adsorption efficiency of a new adsorbent towards uranium and vanadium ions at low concentrations

Kavakli, P. A.*; Seko, Noriaki; Tamada, Masao; G$"u$ven, O.*

Separation Science and Technology, 39(7), p.1631 - 1643, 2005/00

 Times Cited Count:52 Percentile:84.2(Chemistry, Multidisciplinary)

A new type of fibrous adsorbent with excess amidoxime groups was synthesized by radiation-induced graft polymerization. Glycidyl methacrylate (GMA) was first radiation-grafted on polyethylene-coated polypropylene nonwoven fabrics and chemically modified with 3,30-iminodipropionitrile [NH (-CH$$_{2}$$-CH$$_{2}$$-CN)$$_{2}$$] (IDPN), which was further reacted with hydroxylamine to obtain graft chains containing two amidoxime groups per graft repeating units. The adsorption properties of this new adsorbent for uranium (U), vanadium (V), lead (Pb), copper (Cu), and cobalt (Co) ions at low concentrations (3.3-1000 ppb).

Journal Articles

Stability of a silica membrane prepared by CVD using $$gamma$$- and $$alpha$$-alumina tube as the support tube in the Hi-H$$_{2}$$O gaseous mixture

Hwang, G.*; Kim, J.*; Choi, H.*; Onuki, Kaoru

Journal of Membrane Science, 215(1-2), p.293 - 302, 2003/04

 Times Cited Count:15 Percentile:56.82(Engineering, Chemical)

no abstracts in English

Journal Articles

Simulation study on the catalytic decomposition of hydrogen iodide in a membrane reactor with a silica membrane for the thermochemical water-splitting IS process

Hwang, G.; Onuki, Kaoru

Journal of Membrane Science, 194(2), p.207 - 215, 2001/12

 Times Cited Count:59 Percentile:88.71(Engineering, Chemical)

no abstracts in English

Journal Articles

Separation of hydrogen from H$$_{2}$$-H$$_{2}$$O-HI gaseous mixture using a silica membrane

Hwang, G.; Onuki, Kaoru; Shimizu, Saburo

AIChE Journal, 46(1), p.92 - 98, 2000/01

 Times Cited Count:38 Percentile:79.42(Engineering, Chemical)

no abstracts in English

Journal Articles

Hydrogen separation in H$$_{2}$$-H$$_{2}$$O-HI gaseous mixture using the silica membrance prepared by chemical vapor deposition

Hwang, G.*; Onuki, Kaoru; Shimizu, Saburo; *

J. Membr. Sci., 162(1-2), p.83 - 90, 1999/00

 Times Cited Count:62 Percentile:90.42(Engineering, Chemical)

no abstracts in English

JAEA Reports

Statistical thermodynamic properties of uranium hexafluoride

Oda, Tetsuzo

JAERI-M 93-052, 49 Pages, 1993/03

JAERI-M-93-052.pdf:1.11MB

no abstracts in English

Journal Articles

Cation exchange selectivity of some fission products on strongly acidic cation exchanger of sulfonic acid type nitric acid system

Sato, Tadashi

Journal of Radioanalytical and Nuclear Chemistry, 139(1), p.79 - 87, 1990/00

 Times Cited Count:4 Percentile:47.93(Chemistry, Analytical)

no abstracts in English

Journal Articles

Radiation effects on methane in the presence of molecular sieves

; ;

J.Chem.Soc.,Faraday Trans.,I, 79, p.1973 - 1986, 1983/00

no abstracts in English

Journal Articles

The Influence of the laser linewidth on the selectivity in laser isotope separation

; ; ; Naruse, Yuji

J.Phys.,D, 16, p.2415 - 2424, 1983/00

no abstracts in English

16 (Records 1-16 displayed on this page)
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