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Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Kimijima, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; et al.
Canadian Journal of Physics, 103(12), p.1225 - 1231, 2025/12
Times Cited Count：0 Percentile：0.00(Physics, Multidisciplinary)Science using neutrons in the nanometer (nm) wavelength region as probes is expanding into a wide range of fields, from basic research in materials and life science to industrial applications. Dramatic increase in the intensity of the beam source is required to drive such research. We have focused on coherent scattering caused by nano-sized particle aggregations to increase the intensity of neutron beams. Nanodiamond is being vigorously researched and developed with the aim of practical application. On the other hand, we have focused on graphene, which has higher van der Waals forces by an order of magnitude and stronger bonding, sp2, between carbons than nanodiamond. This is expected to lead to its processability into a lumped for and to adapt to higher radiation fields. By promoting chemical vapor deposition (CVD), we have established a technique to form nano-sized graphene (called graphene flower) with a shape similar to a sunflower flower. In this talk, we report on the neutron scattering properties that contribute to the coherent scattering of the newly developed graphene flower.
Hirota, Noriaki; Takeda, Ryoma; Ide, Hiroshi; Tsuchiya, Kunihiko; Kobayashi, Yoshinao*
Nuclear Materials and Energy (Internet), 45, p.102009_1 - 402009_10, 2025/12
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Using SUS304L stainless steel, which is employed in reactor structural components, the effects of grain refinement on stress corrosion cracking occurring under nuclear reactor operating conditions were investigated. As a result, after conducting slow strain rate testing (SSRT) in air and nuclear reactor operating environments, a comparison of the tensile properties of SUS304L with the same grain size revealed that elongation significantly decreased with increasing grain size under nuclear reactor operating conditions. In SSRT conducted in air, the 
-value obtained from the Hall-Petch relationship was lower than the conventional values. Observations showed the absence of cracks on SUS304L with 0.59 and 1.52 
m grains; however, SUS304L with larger grains exhibited rougher fracture surfaces and side cracks. Thin oxide films were formed on SUS304L with 0.59 m and 1.52 m grains, while SUS304L with coarse grains of 28.4 m or larger enabled the formation of oxide films with over 2 m thickness. Cr
O
films were formed on SUS304L with 0.59 m, 1.52 m, and 28.4 m, while CrO and Fe based oxides were formed on SUS304L with 39.5 m and 68.6 m. Crystal orientation analysis revealed linear surface layers without cracks in the 
-phase for SUS304L with 0.59 m and 1.52 m. In materials with Larger grain sizes, surface irregularities and cracks were observed in the -phase. In fine-grained SUS304L, lattice diffusion caused uniform O diffusion in the -phase, resulting in the formation of a thin CrO layer that suppressed cracks. In coarse-grained SUS304L, grain boundary diffusion caused Fe oxide formation at the grain boundaries, weakening them, and supersaturated O led to the formation of thick films comprising CrO and Fe-based oxides, resulting in peeling and cracking.
Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Journal of Neutron Research, 26(2-3), p.69 - 74, 2024/09
Slow neutrons, such as cold neutrons, are important non-destructive probes not only for basic physics but also for the structural genomics advancements in the life sciences and the battery technology advancements needed for the transition to a hydrogen society. Neutron-based science is also known as high-neutron-intensity-dependent science. A new unique method focusing on nanosized particle aggregation has been proposed to increase neutron intensity in that energy region. The method is based on intensity enhancement by multiple coherent scatterings with nanosized particle aggregation. The aggregation of nanosized particles matches the wavelength of below cold neutrons, causing a similar effect to coherent scattering, so-called Bragg scattering, leading to neutron intensity enhancement by several orders of magnitude. Nanodiamonds and magnesium hydride have recently been studied numerically and experimentally. The major challenge with nanodiamonds in practical applications is the molding method. Another carbon structure, graphene is focused on to find a solution to this problem. It is hypothesized that nanosized graphene could aid coherent neutron scattering under particle size conditions similar to nanodiamonds. We report the potential of nanosized graphene as a reflector material below cold neutrons, together with experimental results.
Wakui, Takashi; Takagishi, Yoichi*; Futakawa, Masatoshi
Zairyo, 73(6), p.520 - 526, 2024/06
Cavitation damage is one of crucial issues to predict the structural endurability of the mercury targets for highly intensive pulsed neutron sources. Based on the comparison with numerical simulation on the pit shape and results of the basic test, the cavitation bubble collapsing was assumed to be resulted in the micro jet with the impact velocity of 160-200 m/s, imposing then impact pressure of 3-4 GPa at the input power simulating the operation condition in the mercury targets. It was statistically understandable that cavitation damage evolution was proportional to 4th power of the input power approximately, as taking the aggressivity of cavitation bubbles, the distribution of the maximum diameter of grown bubbles and the space of distribution of bubbles in the mercury into account.
Collaborative Laboratories for Advanced Decommissioning Science; Ibaraki University*
JAEA-Review 2023-021, 112 Pages, 2024/02
JAEA-Review-2023-021.pdf:7.1MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Contribution to Risk Reduction in Decommissioning Works by the Elucidation of Basic Property of Radioactive Microparticles" conducted from FY2018 to FY2021 (this contract was extended to FY2021). The present study aims to understand the basic properties (size, chemical composition, isotopic composition - including concentration of 
-emitters, electrostatic properties, and optical properties, etc.) of fine particles composed of silicate with insoluble properties which contain regions of highly concentrated radioactive cesium (Cs) released to the environment by the accident at the Fukushima Daiichi Nuclear Power Station of TEPCO in 2011 March.
Terada, Atsuhiko; Nagaishi, Ryuji
Nuclear Science and Engineering, 197(4), p.647 - 659, 2023/04
Times Cited Count：5 Percentile：49.89(Nuclear Science & Technology)In order to understand dispersion of hydrogen leaked in a partially open space practically, which can be considered as a basic model for all processes of transfer, treatment, storage and disposal of radioactive materials containing fuel debris in the decommissioning of nuclear facilities after a severe accident, by using a CFD code, the effects of vent size and outer wind on the H dispersion were analytically studied by adopting the experimental Hallway model, which has H release hole on the ceiling, one vent on the Roof vent and Door vent. Air flowed in the model from the Door vent, while H was discharged outside from the Roof vent. The discharged amount of H increased in conjunction with the air inflow when the size of Roof and or Door vents was increased. The effect of wind depended on the direction to the Door vent: wind from the same direction as the Door vent promoted the H discharge, while wind from the opposite direction suppressed. The dispersion characteristics of indoor leaked H was clarified for comparing model tests with the same Froude number and different scales. It was found from the analysis results of comparing model tests with the same Froude number and different scales that when the H leaked into the room and diffused to the air, the flow generated by the buoyancy of mixed gas created the stack effect which caused the natural ventilation by drawing in the air from the outside through vent. In addition, it was speculated that the H concentration decreased after its leak by quickly mixing with the air which flowed in from the vents and reached to the floor due to the Coanda effect, which is the effect of the free jet being drawn to a nearby wall.
Yuan, X.*; Hu, Q.*; Lin, X.*; Zhao, C.*; Wang, Q.*; Tachi, Yukio; Fukatsu, Yuta; Hamamoto, Shoichiro*; Siitari-Kauppi, M.*; Li, X.*
Journal of Hydrology, 618, p.129172_1 - 129172_15, 2023/03
Times Cited Count：11 Percentile：70.69(Engineering, Civil)Teshigawara, Makoto; Ikeda, Yujiro*; Yan, M.*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Nanomaterials (Internet), 13(1), p.76_1 - 76_9, 2023/01
Times Cited Count：8 Percentile：57.39(Chemistry, Multidisciplinary)To enhance neutron intensity below cold neutrons, it is proposed that nanosized graphene aggregation could facilitate neutron coherent scattering under particle size conditions similar to nanodiamond. It might also be possible to use it in high neutron radiation conditions due to graphene's strong sp2 bonds. Using the RIKEN accelerator-driven compact neutron source and iMATERIA at J-PARC, we performed neutron measurement experiments, total neutron cross-section, and small-angle neutron scattering on nanosized graphene aggregation. The measured data revealed, for the first time, that nanosized graphene aggregation increased the total cross-sections and small-angle scattering in the cold neutron energy region, most likely due to coherent scattering, resulting in higher neutron intensities, similar to nanodiamond.
Kawaguchi, Koichi; Segawa, Tomoomi; Ishii, Katsunori
Funtai Kogakkai-Shi, 59(6), p.283 - 290, 2022/06
In the Japan Atomic Energy Agency, in order to effectively use the out-of-standard pellets in the fuel manufacturing process for high-speed furnaces, we are developing techniques for crushing and reusing them with raw material powder. By analyzing in detail the particle size distribution before and after grinding, it was shown that the grinding powder is composed of three different component particles having different characteristics of the particle size distribution. In addition, we examined the method of predicting pulverized powder particle size distribution from the supply powder particle size distribution.
Soba, A.*; Prudil, A.*; Zhang, J.*; Dethioux, A.*; Han, Z.*; Dostal, M.*; Matocha, V.*; Marelle, V.*; Lasnel-Payan, J.*; Kulacsy, K.*; et al.
Proceedings of TopFuel 2021 (Internet), 10 Pages, 2021/10
Miyahara, Shinya*; Kawaguchi, Munemichi; Seino, Hiroshi; Atsumi, Takuto*; Uno, Masayoshi*
Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 6 Pages, 2021/08
In a postulated accident of fuel pin failure of sodium cooled fast reactor, a fission product cesium will be released from the failed pin as an aerosol such as cesium iodide and/or cesium oxide together with a fission product noble gas such as xenon and krypton. As the result, the xenon and krypton released with cesium aerosol into the sodium coolant as bubbles have an influence on the removal of cesium aerosol by the sodium pool in a period of bubble rising to the pool surface. In this study, cesium aerosol removal behavior due to inertial deposition, sedimentation and diffusion from a noble gas bubble rising through liquid sodium pool was analyzed by a computer program which deals with the expansion and the deformation of the bubble together with the aerosol absorption considering the effects of particle size distribution and agglomeration in aerosols. In the analysis, initial bubble diameter, sodium pool depth and temperature, aerosol particle diameter and density, initial aerosol concentration in the bubble were changed as parameter, and the results for the sensitivities of these parameters on decontamination factor (DF) of cesium aerosol were compared with the results of the previous study in which the effects of particle size distribution and agglomeration in aerosols were not considered. From the results, it was concluded that the sensitivities of initial bubble diameter, the aerosol particle diameter and density to the DF became significant due to the inertial deposition of agglomerated aerosols. To validate these analysis results, the simulation experiments have been conducted using a simulant particles of cesium aerosol under the condition of room temperature in water pool and air bubble systems. The experimental results were compared with the analysis results calculated under the same condition.
Zhou, Q.*; Saito, Takumi*; Suzuki, Seiya; Yano, Kimihiko; Suzuki, Shunichi*
Journal of Nuclear Science and Technology, 58(4), p.461 - 472, 2021/04
Times Cited Count：11 Percentile：70.86(Nuclear Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; Ibaraki University*
JAEA-Review 2020-033, 84 Pages, 2021/01
JAEA-Review-2020-033.pdf:4.9MB
JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project in FY2019. Among the adopted proposals in FY2018, this report summarizes the research results of the "Contribution to Risk Reduction in Decommissioning Works by the Elucidation of Basic Property of Radioactive Microparticles" conducted in FY2019.
Kawaguchi, Koichi; Segawa, Tomoomi; Yamamoto, Kazuya; Makino, Takayoshi; Iso, Hidetoshi; Ishii, Katsunori
Funtai Kogakkai-Shi, 57(9), p.478 - 484, 2020/09
A collision plate type jet mill is assumed to be a pulverizer that can control the particle size for nuclear fuel fabrication. The collision plate type jet mill consists of two modules, a classifier and a mill chamber. Coarse component of powder is cycled in the equipment and finally pulverized into objective particle size. In this report, simulated crushed powders were classified and pulverized step by step, and particle size distribution were compared. The collision plate type jet mil can produce objective size particles with low overgrinding.
Tachi, Yukio; Sato, Tomofumi*; Akagi, Yosuke*; Kawamura, Makoto*; Nakane, Hideji*; Terashima, Motoki; Fujiwara, Kenso; Iijima, Kazuki
Science of the Total Environment, 724, p.138098_1 - 138098_11, 2020/07
Times Cited Count：21 Percentile：57.07(Environmental Sciences)To understand and predict radiocesium transport behaviors in the environment, highly contaminated sediments from Ukedo and Odaka rivers around the Fukushima Daiichi Nuclear Power Plant were investigated systematically focusing on key factors controlling radiocesium sorption and fixation, including particle size, clay mineralogy and organic matter.
2 mMatsubara, Akihiro; Fujita, Natsuko; Kimura, Kenji
Proceedings of the 8th East Asia Accelerator Mass Spectrometry Symposium and the 22nd Japan Accelerator Mass Spectrometry symposium (EA-AMS 8 & JAMS-22), p.57 - 59, 2020/00
no abstracts in English
Idomura, Yasuhiro
Physics of Plasmas, 26(12), p.120703_1 - 120703_5, 2019/12
Times Cited Count：7 Percentile：34.29(Physics, Fluids & Plasmas)This Letter presents the impacts of the hydrogen isotope mass and the normalized gyroradius 
on L-mode like hydrogen (H) and deuterium (D) plasmas dominated by ion temperature gradient driven (ITG) turbulence using global full-f gyrokinetic simulations. In ion heated numerical experiments with adiabatic electrons, the energy confinement time shows almost no isotope mass dependency, and is determined by Bohm like scaling. Electron heated numerical experiments with kinetic electrons show clear isotope mass dependency caused by the isotope effect on the collisional energy transfer from electrons to ions, and the H and D plasmas show similar ion and electron temperature profiles at an H to D heating power ratio of 
. The normalized collisionless ion gyrokinetic equations for H and D plasmas become identical at the same , and collisions weakly affect ITG turbulence. Therefore, the isotope mass dependency is mainly contributed by the scaling and the heating sources.
Takasaki, Koji; Yasumune, Takashi; Hashimoto, Makoto; Maeda, Koji; Kato, Masato; Yoshizawa, Michio; Momose, Takumaro
JAEA-Review 2019-003, 48 Pages, 2019/03
JAEA-Review-2019-003.pdf:3.81MB
June 6, 2017, at Plutonium Fuel Research Facility in Oarai Research and Development Center of JAEA, when five workers were inspecting storage containers containing plutonium and uranium, resin bags in a storage container ruptured, and radioactive dust spread. Though they were wearing a half face mask respirator, they inhaled radioactive materials. In the evaluation of the internal exposure dose, the aerodynamic radioactive median diameter (AMAD) is an important parameter. We measured 14 smear samples and a dust filter paper with imaging plates, and estimated the AMAD by image analysis. As a result of estimating the AMAD, from the 14 smear samples, the AMADs are 4.3 to 11 m or more in the case of nitrate plutonium, and the AMADs are 5.6 to 14 m or more in the case of the oxidized plutonium. Also, from the dust filter paper, the AMAD is 3.0 m or more in the case of nitrate plutonium, and the AMAD is 3.9 m or more in the case of the oxidized plutonium.
Wan, T.; Naoe, Takashi; Wakui, Takashi; Futakawa, Masatoshi; Obayashi, Hironari; Sasa, Toshinobu
Materials, 10(7), p.753_1 - 753_17, 2017/07
Times Cited Count：34 Percentile：76.70(Chemistry, Physical)Kitamura, Yasunori*; Fukushima, Masahiro
Nuclear Science and Engineering, 186(2), p.168 - 179, 2017/05
Times Cited Count：1 Percentile：8.58(Nuclear Science & Technology)An inconsistency between the reactivity worth of short-size samples measured by the critical-water-level (CWL) method and that conventionally analysed for validating the nuclear data and the nuclear calculation methods has been known. The present study investigated this inconsistency in terms of a simple theoretical framework and proposed a simple and practical technique for correcting the measured sample reactivity worth without making supplementary experiments. A series of Monte Carlo calculations that simulated typical sample reactivity worth measurement by the CWL method showed that this inconsistency is effectively reduced by the present correction technique.
