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Journal Articles

Quantum critical behavior of the hyperkagome magnet Mn$$_3$$CoSi

Yamauchi, Hiroki; Sari, D. P.*; Yasui, Yukio*; Sakakura, Terutoshi*; Kimura, Hiroyuki*; Nakao, Akiko*; Ohara, Takashi; Honda, Takashi*; Kodama, Katsuaki; Igawa, Naoki; et al.

Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02

https://doi.org/10.1103/PhysRevResearch.6.013144

Journal Articles

Magnetic susceptibility of multiorbital systems

Kubo, Katsunori; Hotta, Takashi

Journal of the Physical Society of Japan, 75(1), p.013702_1 - 013702_4, 2006/01

https://doi.org/10.1143/JPSJ.75.013702
 Times Cited Count：12 Percentile：57.69(Physics, Multidisciplinary)

Effects of orbital degeneracy on magnetic susceptibility in paramagnetic phases are investigated within a mean-field theory. Under certain crystalline electric fields, the magnetic moment consists of two independent moments, e.g., spin and orbital moments. In such a case, the magnetic susceptibility is given by the sum of two different Curie-Weiss relations, leading to the deviation from the Curie-Weiss law. Such behavior may be observed in $$d$$- and $$f$$-electron systems with $$t_{2g}$$ and $$Gamma_8$$ ground states, respectively. As a potential application of our theory, we attempt to explain the difference in the temperature dependence of magnetic susceptibilities of UO$$_2$$ and NpO$$_2$$. Then, we find that the difference in the temperature dependence can be naturally explained by considering the effects of the octupole moments in NpO$$_2$$.

Journal Articles

High-temperature magnetic investigations on uranium compounds

Galatanu, A.; Haga, Yoshinori; Matsuda, Tatsuma; Ikeda, Shugo; Yamamoto, Etsuji; Aoki, Dai*; Takeuchi, Tetsuya*; Onuki, Yoshichika

Journal of the Physical Society of Japan, 74(5), p.1582 - 1597, 2005/05

https://doi.org/10.1143/JPSJ.74.1582
 Times Cited Count：39 Percentile：79.87(Physics, Multidisciplinary)

We investigated the magnetic property of typical uranium compounds by measuring the magnetic susceptibility in an extended temperature range up to about 800 K. The magnetic susceptibility follows the Curie-Weiss law for a localized 5$$f^2$$-electron compound UPd$$_3$$ and a ferromagnetic insulator UFe$$_4$$P$$_{12}$$. In most of the investigated compounds we observed a crossover effect of the 5$$f$$ electrons from a low-temperature itinerant nature to a high-temperature localized one. This is found to be characteristic for ferromagnetic superconductors such as UGe$$_{2}$$ and UIr, and also for antiferromagnets like USb$$_{2}$$ or UNiSb$$_{2}$$. To assess an extension of this characteristic property in the uranium compounds we also investigated typical 5$$f$$-itinerant compounds like UGa$$_{3}$$ and UPtGa$$_5$$. The crossover effect is essentially important in heavy fermion compounds such as UPt$$_3$$, UPd$$_2$$Al$$_3$$ and URu$$_2$$Si$$_2$$. Even in the paramagnetic compound of UB$$_4$$, the magnetic susceptibility is not temperature-independent, but approaches a 5$$f$$-localized tendency at high temperatures. Since the samples were single crystals, we were also able to trace the evolution of the magnetic anisotropy. The high-temperature anisotropic susceptibility data were analyzed on the basis of the crystalline electric field scheme.

Journal Articles

Antiferromagnetic and ferromagnetic phases of UCu$$_2$$Si$$_2$$

Matsuda, Tatsuma; Haga, Yoshinori; Ikeda, Shugo; Galatanu, A.; Onuki, Yoshichika

Physica B; Condensed Matter, 359-361, p.1069 - 1071, 2005/04

https://doi.org/10.1016/j.physb.2005.01.289
 Times Cited Count：3 Percentile：16.35(Physics, Condensed Matter)

We have succeeded in growing a high-quality single crystal of UCu$$_2$$Si$$_2$$ with the tetragonal structure by the Sn-flux method and measured the magnetic susceptibility and magnetization. UCu$$_2$$Si$$_2$$ is confirmed to order antiferromagnetically below $$T_{rm N}$$ = 106 K, and follows a successive ferromagnetic ordering at $$T_{rm C}$$ = 100 K. The magnetic properties are highly anisotropic, reflecting the crystal structure. An easy-axis of magnetization is found to be the [001] direction ($$c$$-axis), while the [100] direction ($$a$$-axis) corresponds to the hard-axis in magnetization. The saturation moment is determined as 1.8$$mu_{rm B}$$/U.

Journal Articles

Magnetic properties of tetragonal Ce$$_{1-x}$$Lu$$_x$$B$$_2$$C$$_2$$(0$$<$$x$$<$$0.31) compounds

Tobo, Aya*; Ishimoto, Kenichi*; Konno, Junya*; Oyama, Kenji*; Kaneko, Koji; Yamaguchi, Yasuo*; Onodera, Hideya*

Journal of the Physical Society of Japan, 72(12), p.3231 - 3236, 2003/12

https://doi.org/10.1143/JPSJ.72.3231
 Times Cited Count：1 Percentile：12.69(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Magnetic study of the mixed orthotitanate La$$_{1-x}$$Sm$$_{x}$$TiO$$_{3}$$(0≦x≦1)

Yoshii, Kenji; Nakamura, Akio; Abe, Hideki*

Journal of Alloys and Compounds, 290(1-2), p.236 - 243, 1999/00

https://doi.org/10.1016/S0925-8388(99)00107-3
 Times Cited Count：11 Percentile：60.92(Chemistry, Physical)

no abstracts in English

Journal Articles

Magnetic studies of orthotitanate Ln$$_{1-x}$$Nd$$_{x}$$TiO$$_{3}$$(Ln=Ce and Pr; 0≦x≦1)

Yoshii, Kenji; Nakamura, Akio

Journal of Solid State Chemistry, 137(1), p.181 - 183, 1998/00

https://doi.org/10.1006/jssc.1998.7824
 Times Cited Count：10 Percentile：65.52(Chemistry, Inorganic & Nuclear)

no abstracts in English

JAEA Reports

Magnetic and Electrical Properties of Uranium Carbonitride and Oxycarbide

JAERI-M 4519, 75 Pages, 1971/07

JAERI-M-4519.pdf:2.76MB

no abstracts in English

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