In-vessel source term analysis code TRACER Version 2.4.1 (User's manual)

Ono, Masahiro*; Uchibori, Akihiro; Okano, Yasushi; Takata, Takashi*

JAEA-Testing 2022-004, 193 Pages, 2023/03

JAEA-Testing-2022-004.pdf:3.31MB

A computer code TRACER (Transport phenomena of Radionuclides for Accident Consequence Evaluation of Reactor) version 2.4.1 has been developed to evaluate species and quantities of fission products (FPs) released into cover gas due to a fuel pin failure in an LMFBR. The TRACER version 2.4.1 includes the models related to NUREG-0772 and also new or modified computational program codes in order to possess a new function shown below, and partial modify of coefficient of FP transition model between coolant and cover gas. This manual includes manual conventions for TRACER Version 2.3, addition of reference such as formula, improvement of explanation of input file creation method, addition of improvement of NUREG-0772 model added to TRACER code, modification of figure of sample analysis performed in appendix. It includes modifications and additions of sample analysis.

Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms (Contract Research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; National Institute for Materials Science*

JAEA-Review 2022-045, 82 Pages, 2023/01

JAEA-Review-2022-045.pdf:4.6MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms" conducted in FY2021. The present study aims to develop innovative diagnostic techniques such as accelerated test specimens and on-site genetic testing for microbially induced and accelerated corrosion of metallic materials (microbially influenced corrosion, MIC), and to identify the conditions that promote MIC at 1F for proposing methods to prevent MIC through water quality and environmental control. We also aim to develop a research base based on materials, microorganisms, and electrochemistry, to develop technologies that can be used by engineers in the field, and to cultivate

Measurement of fragments of a wall-impinging liquid jet in a shallow pool

Horiguchi, Naoki; Yoshida, Hiroyuki; Kaneko, Akiko*; Abe, Yutaka*

Proceedings of 12th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS12) (Internet), 6 Pages, 2022/10

For safety evaluation of nuclear reactors in severe accidents, it is important to estimate physical quantities of fragments generated from the molten fuel jet, which falls in a pool and breaks up. The evaluation method has been developed for the behavior as liquid jet with hydrodynamic interaction including fuel coolant interaction (FCI). In case of a shallow pool assumed in ex-vessel, the molten fuel jet is assumed to behave as wall-impinging liquid jet and to form liquid film flow spreading on the floor with/without fragmentation. In our research, focusing on hydrodynamic interaction and the transient 3-dimensional spreading on the floor, we have developed the evaluation method by numerical simulation using the two-phase flow simulation code with interface tracking method (TPFIT) developed by JAEA and, the experimental method using the 3D-LIF method in liquid-liquid system for the validation data. In our previous studies, we investigated the wall-impinging liquid jet behavior with fragmentation and observed that the liquid film flow had some characteristic parts transiently. Since it indicates that the quantities change depending on the parts and affect the safety evaluation, it is important to measure the quantities of the fragments generated from each part. This paper explains the measurement of the physical quantities of the fragments generated from each part of the wall-impinging liquid jet in a shallow pool for the validation of the numerical simulation. We conducted an experiment with the 3D-LIF method and segmented the experimental data based on the fragmentation point over the liquid film flow using the dispersed phase tracking method, developed by JAEA. Then, we measured the diameter and amount of the fragments from the segmented experimental data and investigated their changing trend.

Development of the simplified boiling model applied for the large scale simulation by the detailed two-phase flow analysis based on the surface tracking

Ono, Ayako; Yamashita, Susumu; Sakashita, Hiroto*; Suzuki, Takayuki*; Yoshida, Hiroyuki

Dai-26-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 4 Pages, 2022/07

https://doi.org/10.1299/jsmepes.2022.26.B211

JAEA is implementing a simulation of a two-phase flow in the reactor core by TPFIT and JUPITER which are developed by JAEA based on the surface tracking method. However, it is impossible to simulate a boiling on the heating surface in the large-scale domain by this type of simulation method since the simulation of boiling based on the surface tracking method needs the fine mesh which sufficiently resolves the initiation of boiling. Therefore, JAEA started to develop the simplified boiling model applied for the two-phase flow in the fuel assemblies. In this study, the simulation results of the convection boiling on a vertical heating surface and the comparison between the simulation results and experimental results are shown.

A Comparative CFD exercise on bubble hydrodynamics using Euler-Euler and interface tracking approaches

Dehbi, A.*; Cheng, X.*; Liao, Y.*; Okagaki, Yuria; Pellegrini, M.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 15 Pages, 2022/03

Numerical simulation of two-phase flow in fuel assemblies with a spacer grid using a mechanistically based method

Ono, Ayako; Yamashita, Susumu; Suzuki, Takayuki*; Yoshida, Hiroyuki

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

JAEA is developing the methodology to predict the critical heat flux based on a mechanism in order to reduce the cost for full mock-up test. The evaluation method based on a mechanism is expected to be able to predict in the wide range of parameter under the unexpected conditions including the severe accident. In this study, the JUPITER code developed by JAEA is examined to apply for the two-phase flow simulation of LWR fuel assembly with the spacer grid. The benchmark data of single-phase flow in the bundle with the spacers by KAERI were used to validate the simulation result by JUPITER. Moreover, the single-phase flow simulation was conducted by another simulation method, STAR-CCM+, as a supplemental analysis to consider the effect of the different simulation methods. Finally, the two-phase flow simulation for the bundle with the spacer was conducted by JUPITER. The effect of the spacer with a vane on the bubble behavior is discussed.

Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; National Institute for Materials Science*

JAEA-Review 2021-059, 71 Pages, 2022/02

JAEA-Review-2021-059.pdf:4.25MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms" conducted in FY2020. The present study aims to develop innovative diagnostic techniques such as accelerated test specimens and on-site genetic testing for microbially induced and accelerated corrosion of metallic materials (microbially influenced corrosion, MIC), and to identify the conditions that promote MIC at 1F for proposing methods to prevent MIC through water quality and environmental control. We also aim to develop a research base based on materials, microorganisms, and electrochemistry, to develop technologies that can be used by engineers in the field, and to cultivate leade

Separation of light and middle lanthanides using multistage extraction with diglycolamide extractant

Matsutani, Takafumi; Sasaki, Yuji; Katsuta, Shoichi*

Analytical Sciences, 37(11), p.1603 - 1609, 2021/11

https://doi.org/10.2116/analsci.21P120

We investigated the chemical behavior of lanthanides (Ln) using diglycolamide extractant with multistage extraction. We obtained the breakthrough curves for light and middle Ln. Our study reveals that the metal extraction limit depends on their values and metal concentrations used in the experiments. From the multistage extractions of 15 aqueous phases and 15 organic phases, three curves (extraction curves, back-extraction curves, and separation curves) were obtained by changing the nitric acid concentration. As an example, under a condition of the separation curve experiment (aqueous phase: 0.5 M HNO, organic phase: 0.1 M TDDGA (-tetradecyl-diglycolamide) in -dodecane), a recovery of more than 99% of Sm in the organic phase with less than 1% Nd can be obtained.

Study on phenanthroline carboxamide for lanthanide separation; Influence of amide substituents

Simonnet, M.; Kobayashi, Toru; Shimojo, Kojiro; Yokoyama, Keiichi; Yaita, Tsuyoshi

Inorganic Chemistry, 60(17), p.13409 - 13418, 2021/09

https://doi.org/10.1021/acs.inorgchem.1c01729

Fundamental study on multistage extraction using TDdDGA for separation of lanthanides present in Nd magnets

Sasaki, Yuji; Morita, Keisuke; Matsumiya, Masahiko*; Ono, Ryoma*; Shiroishi, Hidenobu*

JOM, 73(4), p.1037 - 1043, 2021/04

https://doi.org/10.1007/s11837-021-04586-1

The separation of Dy from Nd is studied from the viewpoint of recycling Dy from Nd magnets. Both metals are lanthanide elements, which means their mutual separation is difficult because of their similar chemical behaviors. All lanthanide elements can be extracted easily by using tetradodecyl-diglycolamide (TDdDGA) extractants, and it has a relatively high separation factor (SF) between Dy and Nd (SF over 10). In the present study, by performing eight extraction steps with the organic phase (0.1M TDdDGA in dodecane), ten steps with an aqueous phase (0.7 M HNO with metals), and six steps with another aqueous phase (0.7 M HNO without metals), approximately 99% Dy was recovered into the organic phase with 1% co-extraction of Nd.