Okita, Shoichiro; Tasaki, Seiji*; Abe, Yutaka*
Nippon Genshiryoku Gakkai Wabun Rombunshi, 19(3), p.178 - 184, 2020/09
The Kyoto University Accelerator-based Neutron Source (KUANS) is a compact neutron source that is mainly used for spectrometer and detector development. In addition, it is also suited for experiments to study the neutronic design of moderators owing to the relatively low neutron generation yield by Be(p,n). We present a neutronic design of the neutron moderator on a reentrant-hole configuration for KUANS to enhance the neutron emission, and some experiments are conducted at KUANS for verification. A polyethylene moderator on a reentrant-hole configuration is designed by PHITS calculation and is introduced to KUANS to obtain intense oblong neutron beams. The intensity of the pulsed neutron beam is experimentally measured. The results reveal that the intensity becomes approximately 1.9 times stronger than that of the conventional rectangular design. In addition, the ratio of its intensity to the conventional intensity increases to approximately threefold as the neutron wavelength increases. It is interesting to note that the longer the neutron wavelength, the more efficiently they are extracted from the inside of the moderator owing to the existence of the reentrant-hole configuration.
Nakamura, Shoji; Endo, Shunsuke; Kimura, Atsushi; Shibahara, Yuji*
KURNS Progress Report 2019, P. 132, 2020/08
Research and development were made for accuracy improvement of neutron capture cross section data on Am among minor actinides. First, the emission probabilities of decay rays were obtained with high accuracy, and the amount of the ground state of Am produced by reactor neutron irradiation of Am was examinded by -ray measurement. Next, the total amount of isomer and ground states was examoned by -ray measurement.
Shibahara, Yuji*; Nakamura, Shoji; Uehara, Akihiro*; Fujii, Toshiyuki*; Fukutani, Satoshi*; Kimura, Atsushi; Iwamoto, Osamu
Journal of Radioanalytical and Nuclear Chemistry, 325(1), p.155 - 165, 2020/07
The measurements of isotopic ratios of Cs samples by thermal ionization mass spectrometry were performed for the analysis of their samples used to evaluate nuclear data obtained for Cs. To obtain a high intensity and stable ion beam, the effects of additive agents on the ionization of Cs were examined. The effect of silicotungstic acid on the ionization of Cs was the largest among the additive agents studied in the present study, while the silicotungstic acid also showed the largest isobaric interference of polyatomic ions. It was demonstrated that as small as 210 g of a Cs sample was sufficient to achieve the analytical precision required to measure the Cs/Cs ratio in the case where an additive agent of TaO/glucose was employed. After examining of the analytical conditions, such as the interference effect due to Ba, the measurements of the isotopic ratios of two Cs samples used in our study using TIMS were conducted, and it was discussed how much the ratios contributed to evaluation of the neutron capture cross-section of Cs.
Nakamura, Shoji; Shibahara, Yuji*; Kimura, Atsushi; Iwamoto, Osamu; Uehara, Akihiro*; Fujii, Toshiyuki*
Journal of Nuclear Science and Technology, 57(4), p.388 - 400, 2020/04
The thermal-neutron capture cross-section () and resonance integral(I) were measured for the Cs(n,)Cs reaction by an activation method and mass spectrometry. We used Cs contained as an impurity in a normally available Cs standard solution. An isotope ratio of Cs and Cs in a standard Cs solution was measured by mass spectrometry to quantify Cs. The analyzed Cs samples were irradiated at the hydraulic conveyer of the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Wires of Co/Al and Au/Al alloys were used as neutron monitors to measure thermal-neutron fluxes and epi-thermal Westcott's indices at an irradiation position. A gadolinium filter was used to measure the , and a value of 0.133 eV was taken as the cut-off energy. Gamma-ray spectroscopy was used to measure induced activities of Cs, Cs and monitor wires. On the basis of Westcott's convention, the and I values were derived as 8.570.25 barn, and 45.33.2 barn, respectively. The obtained in the present study agreed within the limits of uncertainties with the past reported value of 8.30.3 barn.
JAEA-Review 2019-046, 36 Pages, 2020/03
Toward the revision of JENDL-4.0, we conducted a literature survey on how to compute the cross section of thermal neutrons scattered by a liquid. This report summarizes the computational methods for evaluating thermal neutron cross sections with molecular dynamics simulations. The cross section can be expressed with a function called as scattering law. For light and heavy water, the scattering law data instead of the cross sections have been provided in nuclear databases. In this report we review the formulations of the scattering laws. The scattering laws can be derived from both the intermediate scattering function and the space-time correlation function. Features of the derived scattering laws are briefly explained. It is shown that the scattering law data can be evaluated using a molecular dynamics simulation of the liquid that is the target of thermal neutrons.
Collaborative Laboratories for Advanced Decommissioning Science; Kyushu University*
JAEA-Review 2019-039, 104 Pages, 2020/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Research and Development of Transparent Materials for Radiation Shield using Nanoparticles". The present study aims to reduce radiation exposure of workers in debris retrieval/analysis and reduce deterioration of optical and electronic systems in remote cameras. For these purposes, we develop transparent radiation shield by making the shield materials into nanoparticles, and dispersing/solidifying them in epoxy resin. By making BC and W into nanoparticles, we will also develop a radiation shield that shields both neutrons and gamma-rays, and also suppresses secondary gamma-rays produced from neutrons.
Nakamura, Shoji; Kimura, Atsushi; Iwamoto, Osamu; Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*
KURNS Progress Report 2018, P. 106, 2019/08
Under the ImPACT project, the neutron capture cross-section measurements of Cesium-135 (Cs) among the long-lived fission products have been performed at Kyoto University. This paper reports measurements of the thermal-neutron capture cross-section of Cs at the Kyoto University Research Reactor (KUR).
Nakamura, Shoji; Kitatani, Fumito; Kimura, Atsushi; Uehara, Akihiro*; Fujii, Toshiyuki*
Journal of Nuclear Science and Technology, 56(6), p.493 - 502, 2019/06
The thermal-neutron capture cross-section()and resonance integral(I) were measured for the Np(n,)Np reaction by an activation method. A method with a Gadolinium filter, which is similar to the Cadmium difference method, was used to measure the with paying attention to the first resonance at 0.489 eV of Np, and a value of 0.133 eV was taken as a cut-off energy. Neptunium-237 samples were irradiated at the pneumatic tube of the Kyoto University Research Reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Wires of Co/Al and Au/Al alloys were used as monitors to determine thermal-neutron fluxes and epi-thermal Westcott's indices at an irradiation position. A -ray spectroscopy was used to measure activities of Np, Np and neutron monitors. On the basis of Westcott's convention, the and I values were derived as 186.96.2 barn, and 100990 barn, respectively.
Hamon, 28(4), p.204 - 207, 2018/11
A Neutron guide is one of the devices to transport neutron beam for long distance without sacrificing much neutrons; therefore, it can supply neutrons to many experimental instruments distributed in a large experimental hall. Also, by using a curved guide, only the neutrons in a required energy range can be transported, and rays and fast neutrons can be effectively eliminated, therefore the signal to background ratio is improved. In addition, a neutron beam can be branched by applying curved guides. Neutron guides are also used to control the divergence angle and intensity of the neutron beam supplied to the neutron instrument.
Proceedings of 13th International Symposium on Advanced Science and Technology in Experimental Mechanics (13th ISEM'18) (USB Flash Drive), 6 Pages, 2018/10
Issues on the engineering technologies relating to high-power spallation neutron sources with liquid metals are introduced. The present status on research activities and results was reviewed.
Suwa, Tomone*; Hemmi, Tsutomu*; Saito, Toru*; Takahashi, Yoshikazu*; Koizumi, Norikiyo*; Luzin, V.*; Suzuki, Hiroshi; Harjo, S.
IEEE Transactions on Applied Superconductivity, 28(3), p.6001104_1 - 6001104_4, 2018/04
Inoue, Rintaro*; Kanaya, Toshiji*; Yamada, Takeshi*; Shibata, Kaoru; Fukao, Koji*
Physical Review E, 97(1), p.012501_1 - 012501_6, 2018/01
In this study, we investigate the process of a polystyrene thin film using inelastic neutron scattering (INS), dielectric relaxation spectroscopy (DRS), and thermal expansion spectroscopy (TES). The DRS and TES measurements exhibited a decrease in glass transition temperature () with film thickness. On the other hand, an increase in was observed in INS studies. In order to interpret this contradiction, we investigated the temperature dependence of the peak frequency () of the process probed by DRS and TES. The experiments revealed an increase in the peak frequency () with decreasing film thickness in the frequency region. This observation is consistent with the observed decrease in with thickness. The discrepancy between INS and DRS or TES descriptions of the process is likely to be attributed to a decrease in the apparent activation energy with film thickness and reduced mobility, due to the impenetrable wall effect.
Akita, Koichi; Shibahara, Masakazu*; Ikushima, Kazuki*; Nishikawa, Satoru*; Furukawa, Takashi*; Suzuki, Hiroshi; Harjo, S.; Kawasaki, Takuro; Vladimir, L.*
Yosetsu Gakkai Rombunshu (Internet), 35(2), p.112s - 116s, 2017/06
Harjo, S.; Kawasaki, Takuro; Hemmi, Tsutomu; Ito, Takayoshi*; Nakamoto, Tatsushi*; Aizawa, Kazuya
JPS Conference Proceedings (Internet), 8, p.031001_1 - 031001_5, 2015/09
Suzuki, Satoshi; Enoeda, Mikio; Hatano, Toshihisa; Hirose, Takanori; Hayashi, Kimio; Tanigawa, Hisashi; Ochiai, Kentaro; Nishitani, Takeo; Tobita, Kenji; Akiba, Masato
Nuclear Fusion, 46(2), p.285 - 290, 2006/02
This paper presents significant progress in R&D of key technologies on the water-cooled solid breeder blanket for the ITER-TBM in JAERI. By the improvement of heat treatment process for blanket module fabrication, a fine-grained microstructure of F82H, can be obtained by homogenizing it at 1150 C followed by normalizing at 930 C after the HIP process. Moreover, a promising bonding process for a tungsten armor and an F82H structural material was developed by using a uniaxial hot compression without any artificial compliant layer. Also, it has been confirmed that a fatigue lifetime correlation, which was developed for ITER divertor, can be applicable for F82H first wall mock-up. As for R&D on a breeder material, LiTiO, the effect of compression loads on thermal conductivity of pebble beds has been clarified. JAERI have extensively developed key technologies for ITER-TBM, and now steps up into an engineering R&D stage, where integrated performance of TBM structures will be demonstrated by scalable mock-ups.
Asano, Yoshihiro; Sugita, Takeshi*; Suzaki,Takenori; Hirose, Hideyuki
Radiation Protection Dosimetry, 116(1-4), p.284 - 289, 2005/12
no abstracts in English
Asano, Yoshihiro; Sugita, Takeshi*; Hirose, Hideyuki; Suzaki,Takenori
Nuclear Science and Engineering, 151(2), p.251 - 259, 2005/10
no abstracts in English
JAERI-Research 2005-016, 127 Pages, 2005/08
no abstracts in English
Tanimura, Yoshihiko; Saegusa, Jun; Yoshizawa, Michio; Yoshida, Makoto
Nuclear Instruments and Methods in Physics Research A, 547(2-3), p.592 - 600, 2005/08
The moderator structure of a neutron spectrometer was optimized with a Monte Carlo code of MCNP-4B. The spectrometer consists of a cylindrical moderator and a position-sensitive thermal neutron detector. It can obtain an energy spectrum from thermal neutron distribution along the cylindrical axis of the moderator. The structure of the moderator was improved by putting a low hydrogen density material in the front of a high hydrogen density one and inserting a neutron absorber which eliminated thermal neutrons diffusing in the moderator. These improvements make energy resolution of the spectrometer better especially for the low energy neutrons from a few tens to 100 keV. The designed spectrometer can be applied to the measurement of energy spectrum over a neutron energy range from a few keV to 20 MeV.
Ishikura, Shuichi*; Shiga, Akio*; Futakawa, Masatoshi; Kogawa, Hiroyuki; Sato, Hiroshi; Haga, Katsuhiro; Ikeda, Yujiro
JAERI-Tech 2005-026, 65 Pages, 2005/03
Failure probability analysis was carried out to estimate the lifetime of the mercury target which will be installed into the JSNS (Japan spallation neutron source) in J-PARC (Japan Proton Accelerator Research Complex). The lifetime was estimated as taking loading condition and materials degradation into account. Considered loads imposed on the target vessel were the static stresses due to thermal expansion and static pre-pressure on He-gas and mercury and the dynamic stresses due to the thermally shocked pressure waves generated repeatedly at 25 Hz. Materials used in target vessel will be degraded by the fatigue, neutron and proton irradiation, mercury immersion and pitting damages, etc. The imposed stresses were evaluated through static and dynamic structural analyses. The material-degradations were deduced based on published experimental data. As results, it was quantitatively confirmed that the failure probability for the lifetime expected in the design is very much lower, 10 in the safety hull, meaning that it will be hardly failed during the design lifetime. On the other hand, the beam window of mercury vessel suffered with high-pressure waves exhibits the failure probability of 12%. It was concluded, therefore, that the leaked mercury from the failed area at the beam window is adequately kept in the space between the safety hull and the mercury vessel to detect mercury-leakage sensors.