A Study on the methodology for rational treatment/disposal of contaminated concrete waste considering volume reduction of waste (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*

JAEA-Review 2025-037, 103 Pages, 2025/12

JAEA-Review-2025-037.pdf:7.28MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "A study on the methodology for rational treatment/disposal of contaminated concrete waste considering volume reduction of waste" conducted in FY2023. The present study aims to evaluate rational waste management strategies incorporating reuse and recycling focusing on radioactive concrete waste, which will be massively generated from dismantling. Feasibility and challenges of aggregate recycling are considered assuming a typical recycled aggregate production technique, based on the characteristics of the concrete. In 2023, the migration behaviors of radionuclides and ions in cementitious materials having interfacial transition zones (ITZ) were investigated through diffusion and leaching experiments using radioactive and non-radioactive tracers and modeled by random walk particle tracking method with a sampling technique using a probabilistic distribution model for two media with an interface. Properties of surrogate contaminated concrete samples prepared by immersing in Cs solution were examined. Migration of ions was studied for surrogate contaminated aggregates and recycled concrete using the surrogate. In addition, surrogate waste package was prepared using by-product powder to study mechanical and chemical properties as well as leaching behavior of radionuclides. Information on properties of the contaminated concrete and tools to estimate the amount of concrete were organized in order to evaluate different waste management scenarios incorporating reuse/recycling.

Perpendicular magnetic anisotropy of thin films

Takanashi, Koki; Seki, Takeshi*

Magune, 19(3), p.100 - 106, 2024/06

Perpendicular magnetic anisotropy of thin films currently plays an important role in spintronics as well as magnetic recording. Regarding perpendicular magnetic anisotropy, in this article, the fundamentals, the research history, and the recent research trends are reviewed, showing specific examples with perpendicular magnetization such as magnetic multilayers, ordered alloy films, rare earth-transition metal amorphous alloy films, and inhomogeneous or granular films. The physical origins for perpendicular magnetic anisotropy, including interface anisotropy due to structural symmetry breaking, magnetoelastic anisotropy due to strain, bulk-type magnetocrystalline anisotropy, and directional pair ordering of atoms, are discussed in each example.

Understanding muon diffusion in perovskite oxides below room temperature based on harmonic transition state theory

Ito, Takashi; Higemoto, Wataru; Shimomura, Koichiro*

Physical Review B, 108(22), p.224301_1 - 224301_11, 2023/12

https://doi.org/10.1103/PhysRevB.108.224301

Two-step Mott transition in Ni(S,Se); SR studies and charge-spin percolation model

Sheng, Q.*; Kaneko, Tatsuya*; Yamakawa, Kohtaro*; Guguchia, Z.*; Gong, Z.*; Zhao, G.*; Dai, G.*; Jin, C.*; Guo, S.*; Fu, L.*; et al.

Physical Review Research (Internet), 4(3), p.033172_1 - 033172_14, 2022/09

https://doi.org/10.1103/PhysRevResearch.4.033172

Toward mechanistic evaluation of critical heat flux in nuclear reactors, 2; Recent studies and future challenges toward mechanistic and reliable CHF evaluation

Okawa, Tomio*; Mori, Shoji*; Liu, W.*; Ose, Yasuo*; Yoshida, Hiroyuki; Ono, Ayako

Nihon Genshiryoku Gakkai-Shi ATOMO, 63(12), p.820 - 824, 2021/12

https://doi.org/10.3327/jaesjb.63.12_820

The evaluation method of the critical heat flux based on the mechanism is needed for the efficient design and development of fuel in reactors and the appropriate safety evaluation. In this paper, the current researches relating to the mechanism of the critical heat flux are reviewed, and the issue to be considered in the future are discussed.

Observation of longitudinal magnetic fluctuations at a first-order ferromagnetic quantum phase transition in UGe

Noma, Yuichiro*; Kotegawa, Hisashi*; Kubo, Tetsuro*; To, Hideki*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; Ito, Kohei*; Nakamura, Ai*; et al.

Journal of the Physical Society of Japan, 90(7), p.073707_1 - 073707_5, 2021/07

https://doi.org/10.7566/JPSJ.90.073707

Devil's staircase transition of the electronic structures in CeSb

Kuroda, Kenta*; Arai, Yosuke*; Rezaei, N.*; Kunisada, So*; Sakuragi, Shunsuke*; Alaei, M.*; Kinoshita, Yuto*; Bareille, C.*; Noguchi, Ryo*; Nakayama, Mitsuhiro*; et al.

Nature Communications (Internet), 11, p.2888_1 - 2888_9, 2020/06

https://doi.org/10.1038/s41467-020-16707-6

Flow separation at inlet causing transition and intermittency in circular pipe flow

Ogawa, Masuro*

JAEA-Technology 2019-010, 22 Pages, 2019/07

JAEA-Technology-2019-010.pdf:1.5MB

Transition phenomena from laminar to turbulent flow are roughly classified into three categories. Circular pipe flow of the third category is linearly stable against any small disturbance, despite that flow actually transitions and transitional flow exhibits intermittency. These are among major challenges that are yet to be resolved in fluid dynamics. Thus, author proposes hypothesis as follows; "Flow in a circular pipe transitions from laminar flow because of vortices released from separation bubble forming in vicinity of inlet of pipe, and transitional flow becomes intermittent because vortex-shedding is intermittent." Present hypothesis can easily explain why linear stability theory has not been able to predict transition in circular pipe flow, why circular pipe flow actually transitions, why transitional flow actually exhibits intermittency even due to small disturbance, and why numerical analysis has not been able to predict intermittency of transitional flow in circular pipe.

Heat conduction analyses on rewetting front propagation during transients beyond anticipated operational occurrences for BWRs

Yonomoto, Taisuke; Shibamoto, Yasuteru; Satou, Akira; Okagaki, Yuria

Journal of Nuclear Science and Technology, 53(9), p.1342 - 1352, 2016/09

AA2015-0497.pdf:1.05MB

https://doi.org/10.1080/00223131.2015.1108882

Our previous study investigated the rewetting behavior of dryout fuel surface during transients beyond anticipated operational occurrences (AOOs) for BWRs, which indicated the rewetting velocity was significantly affected by the precursory cooling defined as cooling immediately before rewetting. The present study further investigated the previous experiments by conducting additional experimental and numerical heat conduction analyses to characterize the precursory cooling. For the characterization, the precursory cooling was firstly defined quantitatively based on evaluated heat transfer rates; the rewetting velocity was investigated as a function of the cladding temperature immediately before the onset of the precursory cooling. The results indicated that the propagation velocity appeared to be limited by the maximum heat transfer rate near the rewetting front. This limitation was consistent with results of the heat conduction analysis.

In situ synthesis of volatile carbonyl complexes with short-lived nuclides

Even, J.*; Ackermann, D.*; Asai, Masato; Block, M.*; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; Eichler, R.*; Fan, F.*; Haba, Hiromitsu*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(3), p.2457 - 2466, 2015/03

https://doi.org/10.1007/s10967-014-3793-7

Rapid In situ synthesis of metal carbonyl complexes has been demonstrated using short-lived isotopes produced in nuclear fission and fusion reactions. The short-lived isotopes with high recoil energy directly react with carbon-monoxides and form carbonyl complexes. Only highly volatile complexes were fast transported in a gas stream to counting and chemistry devices. Short-lived Mo, Tc, Ru, Rh, W, Re, Os, and Ir were found to form volatile carbonyl complexes, while no volataile complex of Hf and Ta were detected. This technique has been applied to a chemical investigation of the superheavy element Sg (atomic number 106), and will be applicable to various fields of nuclear science with short-lived transition metal isotopes.