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Sun, Haomin; Kunugi, Tomoaki*; Yokomine, Takehiko*; Shen, X.*; Hibiki, Takashi*
Experimental Thermal and Fluid Science, 154, p.111171_1 - 111171_24, 2024/05
Times Cited Count:2 Percentile:56.96(Thermodynamics)Suzuki, Satoshi*; Yuguchi, Takashi*; Ishiguro, Keito*; Endo, Kyoka*; Kato, Asuka*; Yokoyama, Kosuke*; Ogita, Yasuhiro; Yokoyama, Tatsunori; Sakata, Shuhei*; Ono, Takeshi*; et al.
Journal of Mineralogical and Petrological Sciences (Internet), 119(1), p.230807_1 - 230807_18, 2024/02
Times Cited Count:1 Percentile:63.07(Mineralogy)Understanding the crustal evolutionary dynamics of island arc-trench systems requires a thorough evaluation of magma chamber processes, and especially of shallow crustal granitic magma intrusion and emplacement processes. To address this, we studied the petrography and geochronology of the Kuki granite, Kitakami Mountains, northeast Japan, as an example of a non-adakitic granite at the magmatic flare-up stage. Granitic borehole samples reflect vertical variation within a magma chamber. Whole-rock chemical composition and mode data reveal a vertical transition from felsic to mafic composition with increasing depth, potentially due to gravitational fractionation of crystals in the magma chamber. The pressure and temperature history of the Kuki granite indicates no change in the magma depth with cooling from 800 to 730C, and geobarometric calculations indicate the emplacement of magma at a depth of approximately10 km. Simultaneous determination of the zircon U Pb age, Ti concentration, and Th/U yields 1) the time temperature history of granitic magma before its solidification, and 2) the correlation between temperature and Th/U in the magma. The magma chamber cooled from ca. 900 to 700
C at approximately 125 Ma. The change in Th/U with temperature indicates greater fractional crystallization in the magma chamber at temperatures above 800
C than below 800
C. Samples from different depth exhibit common tendencies in terms of the relationship between Th/U and temperature, indicating the same system of fractional crystallization throughout the cooling magma chamber.
Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro
JAEA-Data/Code 2023-011, 32 Pages, 2023/11
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides (H,
C,
Cl,
Ca,
Co,
Ni,
Sr,
Nb,
Ag,
Cs,
Ba,
Eu,
Eu,
Ho,
U,
U,
U,
Pu,
Pu,
Pu,
Am,
Am,
Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.
Sun, Haomin; Kunugi, Tomoaki*; Yokomine, Takehiko*; Shen, X.*; Hibiki, Takashi*
International Journal of Heat and Mass Transfer, 211, p.124214_1 - 124214_17, 2023/09
Times Cited Count:3 Percentile:44.93(Thermodynamics)Ota, Masakazu; Takahara, Shogo; Yoshimura, Kazuya; Nagakubo, Azusa; Hirouchi, Jun; Hayashi, Naho; Abe, Tomohisa; Funaki, Hironori; Nagai, Haruyasu
Journal of Environmental Radioactivity, 264, p.107198_1 - 107198_15, 2023/08
Times Cited Count:0 Percentile:0.00(Environmental Sciences)One of the current major radiation exposure pathways from the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident-fallout is inhalation of the re-suspended Cs occurring in air. While wind-induced soil particle resuspension has been recognized as a primary mechanism of
Cs resuspension, studies following the FDNPP accident suggested that fungal spores can be a significant source of the atmospheric
Cs particularly in the rural areas such as difficult-to-return zone (DRZ). To elucidate the relative importance of the two resuspension phenomena, we propose a model simulating resuspension of
Cs as soil particles and fungal spores, and applied it to DRZ. Our model's calculation showed that soil particle resuspension was responsible for the surface-air
Cs observed during winter-spring, but could not account for the higher
Cs concentrations observed in summer-autumn. The higher concentrations in the summer-autumn were in general reproduced by implementing fungal spore
Cs emission, that replenished low soil particle
Cs resuspension in that period. According to our model's concept,
Cs accumulation in fungal spores and high spore emission rate characterized by the rural environment were likely responsible for the abundance of spore
Cs in the air. It was inferred that the influence of the fungal spores on the atmospheric
Cs would last longer since un-decontaminated forests still exist in DRZ.
Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; Konda, Miki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2023-002, 81 Pages, 2023/05
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2, JRR-3 and Hot laboratory facilities. In this report, we summarized the radioactivity concentrations of 20 radionuclides (H,
C,
Cl,
Co,
Ni,
Sr,
Nb,
Tc,
Ag,
I,
Cs,
Eu,
Eu,
U,
U,
Pu,
Pu,
Pu,
Am,
Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2020.
Abe, Satoshi; Okagaki, Yuria
Nuclear Engineering and Design, 404, p.112165_1 - 112165_14, 2023/04
Times Cited Count:2 Percentile:51.90(Nuclear Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2022-038, 102 Pages, 2023/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Study on rational treatment/disposal of contaminated concrete waste considering leaching alteration" conducted in FY2021. The present study aims to understand migration behaviors of radionuclides in relation to the properties of concrete altered by leaching, to develop a model to predict concentration profiles, and to analyze waste management scenarios, with a focus on underground concrete structures in contact with contaminated water. Migration behaviors depend on radionuclides and their chemical species. Sorption of I is less significant on C-S-H and C-A-S-H than on hardened cement paste with two orders of magnitude smaller distribution coefficient
, while
of U was the same …
Tobita, Minoru*; Konda, Miki; Omori, Takeshi*; Nabatame, Tsutomu*; Onizawa, Takashi*; Kurosawa, Katsuaki*; Haraga, Tomoko; Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; et al.
JAEA-Data/Code 2022-007, 40 Pages, 2022/11
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete, ash, ceramic and brick samples generated from JRR-3, JRR4 and JRTF facilities. In this report, we summarized the radioactivity concentrations of 24 radionuclides (H,
C,
Cl,
Ca,
Co,
Ni,
Sr,
Nb,
Tc,
Ag,
I,
Cs,
Ba,
Eu,
Eu,
Ho,
U,
U,
Pu,
Pu,
Pu,
Am,
Am,
Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2020-2021.
Tsuchida, Daiki; Mitsukai, Akina; Aono, Ryuji; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2022-004, 87 Pages, 2022/07
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until by the beginning of disposal. In order to contribute to this work, we collected and analyzed samples generated from JPDR, JRR-3 and JRR-4. In this report, radioactivity concentrations of 20 radionuclides (H,
C,
Cl,
Co,
Ni,
Sr,
Nb,
Tc,
Ag,
I,
Cs,
Eu,
Eu,
U,
U,
Pu,
Pu,
Am,
Cm) were determined based on radiochemical analysis and summarized as basic data for the study of evaluation method of radioactive concentration.
Komatsu, Atsushi
JAEA-Research 2021-019, 24 Pages, 2022/05
In order to reduce the corrosion rate of materials in molten lead bismuth eutectic (LBE), it is important to adjust the oxygen concentration, and past reports show that the oxygen concentration is often adjusted to about 10 to 10
wt%. However, it is not clearly stated what concentration is optimal, and there are some reports of severe corrosion even within this concentration range. In this study, a corrosion model considering diffusion in oxide and LBE was developed for 9Cr-1Mo steel, and the corrosion control method estimated from the corrosion model were investigated. We also tried to calculate the optimum oxygen concentration to prevent the flow blockage at the low temperature of loop environment while reducing the corrosion of 9Cr-1Mo steel in molten LBE. As a result, it was expected that the corrosion mode of 9Cr-1Mo steel in LBE could be classified into three types, dense film formation, precipitation film formation, and film dissolution, depending on the ratio of oxide film thickness to diffusion layer thickness, iron concentration in LBE, and temperature. In order to inhibit corrosion, it is important to adjust the oxygen concentration so that the conditions for dense film formation can be maintained. For this purpose, it was expected that a pre-oxidized film of more than 10
m should be applied before immersion in LBE. The oxygen concentration of about 10
to 10
wt% is the appropriate oxygen concentration when the oxide film has grown to some extent, and a higher oxygen concentration was expected to be required when the film is thin.
Yuguchi, Takashi*; Yamazaki, Hayato*; Ishibashi, Kozue*; Sakata, Shuhei*; Yokoyama, Tatsunori; Suzuki, Satoshi*; Ogita, Yasuhiro; Sando, Kazusa*; Imura, Takumi*; Ono, Takeshi*
Journal of Asian Earth Sciences, 226, p.105075_1 - 105075_9, 2022/04
Times Cited Count:8 Percentile:61.96(Geosciences, Multidisciplinary)Simultaneous determination of the U-Pb age of zircon and concentration of titanium in a single analysis spot, using inductively coupled plasma mass spectrometry with laser ablation sample introduction, produces paired age and temperature data of zircon crystallisation, potentially revealing time-temperature () histories for evolved magma. The Kurobegawa granite, central Japan, contains abundant mafic magmatic enclaves (MMEs). We applied this method to evaluate MMEs and their host (enclosing) granites. Cooling behaviour common to both MMEs and host rocks was found between 1.5 and 0.5 Ma. Rapid cooling from the zircon crystallisation temperature to the closure temperature of biotite K-Ar system was within
1 million year. Combining the obtained
paths of MMEs and host rocks with petrological information can provide insights into magma chamber processes. This suggests that MME flotation, migration, and spread through the magma chamber ceased at 1.5-0.5 Ma, indicating the emplacement age of the Kurobegawa granitic pluton, as no large-scale reheating episodes have occurred since then.
Tobita, Minoru*; Haraga, Tomoko; Endo, Tsubasa*; Omori, Hiroyuki*; Mitsukai, Akina; Aono, Ryuji; Ueno, Takashi; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2021-013, 30 Pages, 2021/12
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JPDR facility. In this report, we summarized the radioactivity concentrations of 21 radionuclides (H,
C,
Cl,
Ca,
Co,
Ni,
Sr,
Nb,
Ag,
Cs,
Eu,
Eu,
Ho,
U,
U,
Pu,
Pu,
Pu,
Am,
Am,
Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2018-2019.
Kakiuchi, Kazuo; Udagawa, Yutaka; Amaya, Masaki
Annals of Nuclear Energy, 155, p.108171_1 - 108171_11, 2021/06
Times Cited Count:2 Percentile:22.08(Nuclear Science & Technology)Dohi, Terumi; Omura, Yoshihito*; Yoshimura, Kazuya; Sasaki, Takayuki*; Fujiwara, Kenso; Kanaizuka, Seiichi*; Nakama, Shigeo; Iijima, Kazuki
PLOS ONE (Internet), 16(5), p.e0251828_1 - e0251828_16, 2021/05
Times Cited Count:8 Percentile:38.10(Multidisciplinary Sciences)Tsuchida, Daiki; Haraga, Tomoko; Tobita, Minoru*; Omori, Hiroyuki*; Omori, Takeshi*; Murakami, Hideaki*; Mitsukai, Akina; Aono, Ryuji; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2020-022, 34 Pages, 2021/03
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JRR-3 and JPDR. In this report, we summarized the radioactivity concentrations of 22 radionuclides(H,
C,
Cl,
Ca,
Co,
Ni,
Sr,
Nb,
Ag,
Ba,
Cs,
Eu,
Eu,
Ho,
U,
U,
Pu,
Pu,
Am,
Am,
Cm) which were obtained from radiochemical analysis of the samples.
Nakano, Masanao
Hoken Butsuri (Internet), 56(1), p.17 - 25, 2021/03
The Tokai Reprocessing Plant is the first reprocessing plant in Japan which started hot test in 1977, and had reprocessed 1140 tons of spent nuclear fuel by May 2007. The gaseous and liquid radioactive wastes has been discharged to the environment. Since iodine-129 (I) is one of the most important nuclides for environmental impact assessment. Therefore,
I in the exhaust and effluent has been controlled, and a precise analysis method of
I in the environmental samples was developed, and the concentration of 129I in the environment was investigated. This report presents an overview of these activities. Not limited to
I on reprocessing facilities, it is essential for nuclear operators to reduce the amount released to the environment in the spirit of ALARA, and to continuously develop the further upgrading environmental monitoring methods and evaluation methods in order to foster a sense of safety and security among residents living in the vicinity of the facilities.
Yokoyama, Kenji; Lahaye, S.*
Proceedings of Joint International Conference on Supercomputing in Nuclear Applications + Monte Carlo 2020 (SNA + MC 2020), p.109 - 116, 2020/10
CEA/DEN/DM2S/SERMA and JAEA/NSEC are working on benchmarks for burnup, isotopic concentrations and decay heat calculations in the collaboration framework between both organisms. Both actors of this benchmark are independently developing their own simulation code systems for computing quantities of interest in nuclear fuel cycle domain: MENDEL in CEA and MARBLE in JAEA. The purpose of the benchmark is to verify each system by comparing both calculation results on specific applications. MENDEL uses a several solvers for the resolution of Bateman equation. Runge-Kutta method or Chebyshev Rational Approximation method (CRAM) are used for irradiation computations. An analytical solver can also be used for decay calculations. MARBLE can use Krylov subspace method or CRAM method. As the first phase of the benchmark, we compared the calculated results of decay heat and isotropic concentrations following by a Pu-239 fast fission pulse. We applied nuclear data from three libraries: (1) JEFF-3.1.1, (2) JENDL/DDF-2015 + JENDL/FPY-2011, and (3) ENDF/B-VII.1. Nuclear data and burnup chain were generated from these libraries independently on each system. We confirmed that the results for both systems were in very good agreement with each other. Numerical results were also compared to experimental data. As the second phase of the benchmark, we are proceeding with a burnup calculation benchmark of MENDEL and MARBLE using the nuclear data and burnup chain provided by ORLIBJ33, which is a set of cross-section data based on JENDL-3.3 for ORIGEN-2 code system. We will also compare with calculation results by the ORIGEN-2 code with ORLIBJ33. Since the series of ORLIB, that is, ORLIBJ32, ORLIBJ33, and ORLIBJ40, have been widely used especially in Japan for many years, the comparison with ORLIB is effective for confirming the performance of MENDEL and MARBLE.
Aono, Ryuji; Mitsukai, Akina; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2020-006, 70 Pages, 2020/08
Radioactive wastes which generated from research and testing reactors in Japan Atomic Energy Agency are planning to be buried at the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes by the time it starts disposal. In order to contribute to this work, we collected and analyzed the samples generated from JPDR and JRR-4. In this report, we summarized the radioactivity concentrations of 19 radionuclides (H,
C,
Cl,
Co,
Ni,
Sr,
Nb,
Tc,
Ag,
I,
Cs,
Eu,
Eu,
U,
U,
Pu,
Pu,
Am,
Cm) which were obtained from radiochemical analysis of those samples.
Nakano, Masanao; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Okura, Takehisa; Kuramochi, Akihiko; Kawasaki, Masatsugu; Takeuchi, Erina; Fujii, Yutaka*; Jinno, Tsukasa*; et al.
Hoken Butsuri (Internet), 55(2), p.102 - 109, 2020/06
After the Fukushima-Daiichi Nuclear Power Station (1F) Accident in March 2011, the increase was significantly observed in a part of the result of the environmental radiation monitoring in Ibaraki prefecture. "The review meeting of the environmental effect from 1F accident" was established to discuss technically the fluctuation of monitoring data. The review meeting collected the monitoring data from the four nuclear operators, and discussed a fluctuating trend, Cs/
Cs activity ratio, and so on. In this report, the results of the dose rate and
Cs in fallout, surface soil, flatfish and seabed sediment are introduced. Also the problem solving in the review meeting is introduced.