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Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2025-048, 56 Pages, 2026/02
JAEA-Review-2025-048.pdf:2.89MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor" conducted in FY2023. The present study aims to develop a high-resolution imaging camera for alpha dust and a high-dose rate monitor. To realize the high-resolution imaging camera for alpha dust, we have developed novel scintillation materials with emission bands of 500-800 nm. Moreover, we have prepared several materials for the camera and software. We have also developed novel scintillation materials with emission bands of 650-1,000 nm, and simulation studies have been conducted for the high-dose-rate monitor system consisting of optical fiber. In addition, we demonstrated this monitoring system, and the dose-rate dynamic range was found to be 20 mSv/h to 1 kSv/h.
Collaborative Laboratories for Advanced Decommissioning Science; University of Fukui*
JAEA-Review 2025-036, 88 Pages, 2025/11
JAEA-Review-2025-036.pdf:6.36MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Development of inspection technology for pipes in high background radiation environments" conducted in FY2023. The following two studies are being conducted with the aim of comprehensively developing technologies to address the three needs indicated in the hearing with TEPCO regarding observation of the inside of piping: (1) Hydrogen content, (2) Presence of precipitates, (3) Presence or absence of 
/
radiation emitting nuclides. First, by downsizing existing nondestructive inspection equipment and developing a dedicated radiation detector capable of nondestructively imaging the inside of piping, we aim to obtain information on the inside of piping by nondestructive inspection using lasers, etc., and to clarify the presence or absence of -nuclides in piping and the internal conditions of piping, etc. In addition, we will develop equipment to visualize -nuclides and discriminate -nuclides in high dose rate environments, as well as technology to investigate the contents of the piping. Deployment of the developed technology is expected to be put into practical use by TEPCO and private companies.
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2024-016, 61 Pages, 2024/12
JAEA-Review-2024-016.pdf:2.88MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor" conducted in FY2022. The present study aims to develop a high-resolution imaging camera for alpha dust and a high-dose rate monitor. To realize the high-resolution imaging camera for alpha dust, we have developed novel scintillation materials with emission bands of 500-800 nm. Moreover, we have prepared several materials for the camera and software. We have also developed novel scintillation materials with emission bands of 650-1,000 nm, and simulation studies have been conducted for the high-dose-rate monitor system consisting of optical fiber.
-rays from slow neutron-induced fission of 
U with STEFFWright, T.*; Harada, Hideo; Kimura, Atsushi; 121 of others*
European Physical Journal A, 60(3), p.70_1 - 70_11, 2024/03
Times Cited Count：0 Percentile：0.00(Physics, Nuclear), , and X-rays (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*
JAEA-Review 2023-022, 93 Pages, 2023/12
JAEA-Review-2023-022.pdf:4.7MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays" conducted from FY2020 to FY2022. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple -ray detection methods, and the Spectral Determination Method (hereinafter referred to as "SDM") was developed. In the research in 2022, we developed a code that handles measurement data of LSC, singles Ge, and 2D spectra (multiple ). In addition, to develop an integrated database, spectral data of 40 nuclides were obtained by actual measurements and simulation calculations.
, , and X-rays (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*
JAEA-Review 2022-037, 118 Pages, 2023/01
JAEA-Review-2022-037.pdf:6.92MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays" conducted in FY2021. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple -ray detection methods, and the Spectral Determination Method (hereafter referred to "SDM") was developed. In the study, the -ray measuring device was installed, and the measurement system consisting of the Ge detector, CeBr
detector, and NaI detector was completed in FY2021. In the SDM development, standard spectra of -ray singles, multiple -ray measurements, …
, , and X-rays (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*
JAEA-Review 2021-060, 105 Pages, 2022/03
JAEA-Review-2021-060.pdf:4.59MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays" conducted in FY2020. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, and develops the measurement system such as multiple -ray detection method. We develop a spectral determination method (SDM method) for integrated analysis by constructing a spectral database for nuclides including -rays and X-rays by measurement using this system and radiation simulation calculation. This method enables simultaneous quantification of multiple nuclides and reduces the chemical separation process.
spectrometry of terrestrial gamma rays using portable germanium detectors in area of 80 km radius around the Fukushima Daiichi Nuclear Power PlantMikami, Satoshi; Tanaka, Hiroyuki*; Okuda, Naotoshi*; Sakamoto, Ryuichi*; Ochi, Kotaro; Uno, Kiichiro*; Matsuda, Norihiro; Saito, Kimiaki
Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(4), p.159 - 178, 2021/12
In order to know the background radiation level where the area affected by the Fukushima Daiichi Nuclear Power Plant accident in 2011, terrestrial gamma rays had been measured by using portable germanium detectors repeatedly from 2013 through 2019, at 370 locations within 80 km radius area centered on the Fukushima Daiichi Nuclear Power Plant. Radioactive concentrations of Uranium 238, Thorium 232, Potassium 40 and kerma rates in air due to terrestrial gamma rays were obtained at those locations based on the method of ICRU report 53. Averaged concentrations of 
U, 
Th and 
K were 18.8, 22.7, 428 Bq/kg, respectively, and kerma rate in air over the area was found to be 0.0402 
Gy/h. The obtained kerma rates in air were compared to those reported in literatures. It was confirmed that the data were correlated with each other, and were agreed within the range of their uncertainty. This is because the kerma rate in air due to terrestrial gamma rays is depend on geology. The similar trend to previous findings was observed that the kerma rate in air at locations geologically classified as Mesozoic era, Granite and Rhyolite were statistically significantly higher than the others.
Rodriguez, D. C.; Abbas, K.*; Koizumi, Mitsuo; Lee, H.-J.; Nonneman, S.*; Pedersen, B.*; Rossi, F.; Takahashi, Tone
Proceedings of 2021 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC) (Internet), 3 Pages, 2021/10
Rodriguez, D. C.; Koizumi, Mitsuo; Rossi, F.; Seya, Michio; Takahashi, Tone; Bogucarska, T.*; Crochemore, J.-M.*; Pedersen, B.*; Takamine, Jun
Journal of Nuclear Science and Technology, 57(8), p.975 - 988, 2020/08
Times Cited Count：4 Percentile：31.93(Nuclear Science & Technology)Rodriguez, D. C.; Rossi, F.; Seya, Michio; Koizumi, Mitsuo
Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11
-ray pipe monitoring for comprehensive safeguards process monitoring of reprocessing facilitiesRodriguez, D. C.; Tanigawa, Masafumi; Mukai, Yasunobu; Isomae, Hidemi; Nakamura, Hironobu; Rossi, F.; Koizumi, Mitsuo; Seya, Michio
Proceedings of INMM 58th Annual Meeting (Internet), 9 Pages, 2017/07
Safegaurding nuclear material at reprocessing facilities utilizes sampling to verify the quantity and process monitoring to maintain continuity-of-knowledge to reduce re-verification. Solution Monitoring and Measurement Systems that determine the solution density and volume are installed at solution tanks, though this only provides indirect verification. To offset this safeguards limitation we propose measuring rays from solutions passing through the pipes and at the tanks to provide improved continuous monitoring and direct verification. This can provide both real-time flow measurements and Pu isotopic composition quantification through passive nondestructive assay. This concept was tested by recent experimental studies performed at the Japan Atomic Energy Agency's Plutonium Conversion Development Facility of flowing Pu-nitrate rays. This presentation will describe the concept details and analysis of using ray pipe monitoring as a capability for real-time safeguards verification.
-ray polarization in NRF-based nondestructive assay of nuclear materialsOmer, M.; Hajima, Ryoichi*; Shizuma, Toshiyuki*; Koizumi, Mitsuo
Proceedings of INMM 58th Annual Meeting (Internet), 7 Pages, 2017/07
Nuclear resonance fluorescence (NRF) is a process in which the electric and/or the magnetic dipole excitations of the nucleus take place. Since these excitations are unique signatures of each nucleus, the NRF provides a practical tool for a non-destructive detection and assay of nuclear materials. Using a polarized -ray beam, distinguishing the nature of the excitation is straightforward. At a scattering angle of 90
, the electric dipole excitations are radiated normal to the polarization plane whereas the magnetic dipole excitations are radiated in the same plane as the incident beam polarization. By contrast, other -ray interactions with the atom may exhibit different responses regarding the polarization of the incident beam. For example, the elastic scattering is expected to give approximately 60% lower yield in the direction of the incident beam polarization than the other direction. This fact significantly affects the sensitivity of the NRF technique because it is not possible to separate the NRF and the elastic scattering on the basis of the photon energy. We report the results of a photon scattering experiment on U using a 100% linearly polarized -ray beam with an energy of 2.04 MeV. We demonstrate how the elastic scattering responds to the polarization of the incident beam. Accordingly, we are able to resolve the effects of the polarization of incident photon in an NRF measurement.
Yagmur, A.*; Uchida, Kenichi*; Ihara, Kazuki*; Ioka, Ikuo; Kikkawa, Takashi*; Ono, Madoka*; Endo, Junichi*; Kashiwagi, Kimiaki*; Nakashima, Tetsuya*; Kirihara, Akihiro*; et al.
Applied Physics Letters, 109(24), p.243902_1 - 243902_4, 2016/12
Times Cited Count：3 Percentile：12.87(Physics, Applied)Thermoelectric devices based on the spin Seebeck effect (SSE) were irradiated with gamma () rays with the total dose of around 3
10
Gy in order to investigate the -radiation resistance of the devices. To demonstrate this, Pt/Ni
Zn
Fe
O
/Glass and Pt/Bi
Y
Fe
O
/GdGaO SSE devices were used. We confirmed that the thermoelectric, magnetic, and structural properties of the SSE devices are not affected by the -ray irradiation. This result demonstrates that SSE devices are applicable to thermoelectric generation even in high radiation environments.
Omer, M.; Hajima, Ryoichi*; Angell, C.*; Shizuma, Toshiyuki*; Hayakawa, Takehito*; Seya, Michio; Koizumi, Mitsuo
Proceedings of INMM 57th Annual Meeting (Internet), 9 Pages, 2016/07
Isotope-specific -rays emitted in the nuclear resonance fluorescence (NRF) process provide a good technique for a non-destructive detection and assay of nuclear materials. We are developing technologies relevant to -ray nondestructive detection and assay utilizing NRF. A Monte Carlo code to simulate NRF process is necessary for design and evaluation of NDA systems. We are developing NRFGeant4, a Geant4-based simulation code, for this purpose. In NRF experiments, highly-enriched targets are generally used such that the NRF signals are dominant and easily measured. In contrast, a real situation may involve very small contents of isotopes of interest. This results in a difficulty in measuring NRF signals because of the interference with other interactions, e.g. elastic scattering. For example, a typical nuclear fuel pellet contains about 90% of U as a host material and less than 1% of 
Pu as an isotope of interest. When measuring NRF of Pu, there would be a huge background coming from the elastic scattering of U. Therefore, an estimation of the elastic scattering with the host material is essential for precise determination of isotope of interest. Satisfying estimation of elastic scattering is currently not available except for some calculations. In the present study, we upgrade our simulation code to include the calculation of elastic scattering events.
Se(, n) cross section and uncertainty evaluation of the 
Se(n, ) cross sectionKitatani, Fumito; Harada, Hideo; Goko, Shinji*; Iwamoto, Nobuyuki; Utsunomiya, Hiroaki*; Akimune, Hidetoshi*; Toyokawa, Hiroyuki*; Yamada, Kawakatsu*; Igashira, Masayuki*
Journal of Nuclear Science and Technology, 53(4), p.475 - 485, 2016/04
Times Cited Count：5 Percentile：37.96(Nuclear Science & Technology)Yokoseki, Takashi; Abe, Hiroshi; Makino, Takahiro; Onoda, Shinobu; Tanaka, Yuki*; Kandori, Mikio*; Yoshie, Toru*; Hijikata, Yasuto*; Oshima, Takeshi
Materials Science Forum, 821-823, p.705 - 708, 2015/07
Nakamoto, Tatsushi*; Idesaki, Akira; Morishita, Norio; Ito, Hisayoshi; Kamiya, Tomihiro; Kimura, Nobuhiro*; Makida, Yasuhiro*; Ogitsu, Toru*; Ohata, Hirokatsu*; Yamamoto, Akira*
AIP Conference Proceedings 824, p.225 - 232, 2006/03
Radiation resistance with respect to mechanical properties of organic materials used in the superconducting magnets for the 50 GeV - 750 kW proton beam line for the J-PARC neutrino experiment was studied. Specimens cooled at liquid nitrogen temperature of 77 K were irradiated by gamma rays beyond 10 MGy. The flexural strength of glass-fiber reinforced plastics (GFRPs), the tear strength of polyimide films and the tensile lap-shear strength of adhesive films were evaluated. It was verified that the organic materials used in the superconducting magnet have a sufficient radiation resistance, and the degradation of their mechanical properties after 10 years operation was estimated to be negligible.
(Ce) scintillation detector applications for environmental -ray measurements of low to high dose ratesTsutsumi, Masahiro; Tanimura, Yoshihiko
Nuclear Instruments and Methods in Physics Research A, 557(2), p.554 - 560, 2006/02
Times Cited Count：16 Percentile：72.62(Instruments & Instrumentation)A new cerium-doped LaCl(Ce) scintillator is evaluated with respect to the application in environmental -ray dosimetry and spectrometry. The scintillator is very attractive for -ray spectrometry in the case of high count rate, because it has excellent energy resolution and fast decay time. The performance characteristics of a scintillator with a 25.4 mm 25.4 mm LaCl(Ce) crystal are studied and compared to those of a NaI(Tl) scintillator with the same size crystal. Acquired pulse-height spectra are converted to dose rates by using the G(E) function method. Though the LaCl(Ce) crystal itself produces a rather high background in the crystal itself, the scintillator provides good energy information and dose-rate readings from low to high-level (several mGy/h) by subtracting the self-background. The properties of LaCl(Ce) scintillator suggest that the scintillator could be a promising candidate for monitoring at high-dose levels as in emergencies, as well as at ordinary levels of background radiation.
Taguchi, Mitsumasa; Kojima, Takuji
JAEA-Review 2005-001, TIARA Annual Report 2004, p.181 - 182, 2006/01
The yields of OH radicals in water containing phenol have been investigated for several ten MeV/n C ion and Ne ion having the same LET value, as a function of the residual ion energy at the specific depth in water. In this study, beside such energy dependence, the dependence of reaction time of OH radical yield was examined by changing the concentration of phenol as solute. The defferential G'-values of OH radicals, those G-values per kinetic energy of ions increase with specific energy of Ne ions. The G'-value just after irradiation(1.5ns) is relatively high but become lower with reaction time to be the value (2.7) obtained for 
Co -rays. It suggests the diffusion behavior of OH radicals locally induced in water.
