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Periez, R.*; Brovchenko, I.*; Jung, K. T.*; Kim, K. O.*; Liptak, L.*; Little, A.*; Kobayashi, Takuya; Maderich, V.*; Min, B. I.*; Suh, K. S.*
Journal of Environmental Radioactivity, 261, p.107138_1 - 107138_8, 2023/05
Times Cited Count:0 Percentile:0(Environmental Sciences)Lagrangian models present several advantages over Eulerian models to simulate the transport of radionuclides in the aquatic environment in emergency situations. A radionuclide release is simulated as a number of particles whose trajectories are calculated along time and thus these models do not require a spatial discretization. In this paper we investigate the dependence of a Lagrangian model output with the grid spacing which is used to calculate concentrations from the final distribution of particles, with the number of particles in the simulation and with the interpolation schemes which are required because of the discrete nature of the water circulation data used to feed the model.
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2022-050, 116 Pages, 2023/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Safe, efficient cementation of challenging radioactive wastes using alkali activated materials with high-flowability and high-anion retention capacity" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. The present study aims to explore alkali activated materials with high anionic nuclide retention and flowability and their recipes for safe storage and disposal of iron flocculant from the water treatment facility at 1F, and to propose a design of a solidification device that is feasible as an actual plant. In order to achieve these objectives, the following five items were carried out in this study.
Togawa, Orihiko; Okura, Takehisa; Kimura, Masanori
JAEA-Review 2022-049, 76 Pages, 2023/01
Before construction and after operation of nuclear facilities, environmental consequence assessments are conducted for normal operation and an emergency. These assessments mainly aim at confirming safety for the public around the facilities and producing relief for them. Environmental consequence assessments are carried out using observations/ measurements by environmental monitoring and/or model predictions by calculation models, sometimes using either of which and at other times using both them, according to the situations and necessities. First, this report investigates methods, roles, merits/demerits and relationship between observations/measurements and model predictions which are used for environmental consequence assessments of nuclear facilities, especially holding up a spent nuclear fuel reprocessing plant at Rokkasho, Aomori as an example. Next, it explains representative examples of utilization of data on observations/measurements and results on model predictions, and considers points of attention at using them. Finally, the report describes future direction, for example, improvements of observations/measurements and model predictions, and fusion of both them.
Collaborative Laboratories for Advanced Decommissioning Science; National Institute for Materials Science*
JAEA-Review 2022-045, 82 Pages, 2023/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms" conducted in FY2021. The present study aims to develop innovative diagnostic techniques such as accelerated test specimens and on-site genetic testing for microbially induced and accelerated corrosion of metallic materials (microbially influenced corrosion, MIC), and to identify the conditions that promote MIC at 1F for proposing methods to prevent MIC through water quality and environmental control. We also aim to develop a research base based on materials, microorganisms, and electrochemistry, to develop technologies that can be used by engineers in the field, and to cultivate
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2022-036, 115 Pages, 2023/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Investigation of environment induced property change and cracking behavior in fuel debris" conducted in FY2021. The present study aims to investigate the environment induced property change and cracking behavior in fuel debris from the viewpoints of materials science. The research objective is cracking behavior in fuel debris which is presumed to be influenced by environment during long-term fuel debris processing period. The degradation models will be established to simulate the oxidation and hydrogenation processes possibly occurred at fuel debris. The evolution of phase constitution and the corresponding property change in the simulated fuel debris under various environmental conditions will be systematically
Maamoun, I.; Eljamal, R.*; Eljamal, O.*
Chemosphere, 312, Part 1, p.137176_1 - 137176_11, 2023/01
Times Cited Count:3 Percentile:98.47(Environmental Sciences)Islam, M. S.*; Maamoun, I.; Falyouna, O.*; Eljamal, O.*; Saha, B. B.*
Journal of Molecular Liquids, 370, p.121005_1 - 121005_11, 2023/01
Times Cited Count:1 Percentile:0.01(Chemistry, Physical)Terada, Hiroaki; Nagai, Haruyasu; Kadowaki, Masanao; Tsuzuki, Katsunori
Journal of Nuclear Science and Technology, 22 Pages, 2023/00
Times Cited Count:1 Percentile:0.04(Nuclear Science & Technology)It is essential to establish a method for reconstructing the source term and spatiotemporal distribution of radionuclides released into the atmosphere due to a nuclear accident for emergency countermeasures. We examined the dependency of a source term estimation method based on Bayesian inference using atmospheric dispersion simulation and environmental monitoring data on the availability of various monitoring data. Additionally, we examined the applicability of this method to a real-time estimation conducted immediately after an accident. A sensitivity analysis of the estimated source term during the Fukushima Daiichi Nuclear Power Station (FDNPS) accident for combinations of various monitoring data indicated that using monitoring data with a high temporal and spatial resolution and the concurrent use of air concentration and surface deposition data is effective for accurate estimation. A real-time source term estimation experiment assuming the situation of monitoring data acquisition during the FDNPS accident revealed that this method could provide the necessary source term for grasping the overview of surface contamination in the early phase and evaluating the approximate accident scale. If the immediate online acquisition of monitoring data and regular operation of an atmospheric dispersion simulation are established, this method can provide the source term in near-real time.
Idham, M. F.*; Falyouna, O.*; Eljamal, R.*; Maamoun, I.; Eljamal, O.*
Journal of Water Process Engineering (Internet), 50, p.103289_1 - 103289_16, 2022/12
Times Cited Count:6 Percentile:86.8(Engineering, Environmental)Urushidate, Tadayuki*; Yoda, Tomoyuki; Otani, Shuichi*; Yamaguchi, Toshio*; Kunii, Nobuaki*; Kuriki, Kazuki*; Fujiwara, Kenso; Niizato, Tadafumi; Kitamura, Akihiro; Iijima, Kazuki
JAEA-Review 2022-023, 8 Pages, 2022/09
After the accident of the Fukushima Daiichi Nuclear Power Station, the Japan Atomic Energy Agency has newly set up a laboratory in Fukushima and started measuring radioactivity concentrations of environmental samples. In October 2015, Fukushima Radiation Measurement Group has been accredited the ISO/IEC 17025 standard by the Japan Accreditation Board (JAB) as a testing laboratory for radioactivity analysis (Cs,
Cs) based on Gamma-ray spectrometry with germanium semiconductor detectors. The laboratory has measured approximately 60,000 of various environmental samples at the end of March 2022. The laboratory quality control and measurement techniques have been accredited by regular surveillance of JAB. In September 2019, the laboratory renewed accreditation as a testing laboratory for radioactivity analysis.
Nakashio, Nobuyuki*; Osugi, Takeshi; Kurosawa, Shigenobu; Ishikawa, Joji; Hemmi, Ko; Iketani, Shotaro; Yokobori, Tomohiko
JAEA-Technology 2022-016, 47 Pages, 2022/08
The Nuclear Science Research Institute (NSRI) of the Japan Atomic Energy Agency (JAEA) started operation of the Advanced Volume Reduction Facilities (AVWF) for production of waste packages for disposal of low-level radioactive solid wastes (LLW). To clarify the operating conditions for homogenization of non-metallic LLW, preliminary tests were carried out using the plasma melting furnace of the non-metal melting unit. The fluidity of molten waste influences homogenization conditions of solidified products. It was clarified that the viscosity, which is determined by the chemical composition and the melting temperature, influence the fluidity of molten waste greatly through previous literature review and the small-scale melting tests. In the preliminary tests, the simulated waste with a cold tracer loaded in 200 L drums were melted. Using the waste chemical components (basicity, iron oxide concentration) as an experimental parameter, the homogeneity of the chemical components of the solidified product was investigated and the homogenization conditions of melting tests were examined. The retention ratio of the tracer in the molten bath was also confirmed. The viscosity of the molten wastes was measured and the correlation with homogeneity was examined. In addition, the technical requirements that should be concerned in advance for future actual operation were discussed.
Safety and Environmental Management Section, Safety and Nuclear Security Administration Department
JAEA-Review 2022-013, 210 Pages, 2022/07
In September, 2021 Japan Atomic Energy Agency (JAEA) published the Environmental Report 2021 concerning the activities of FY 2020 under "Law Concerning the Promotion of Business Activities with Environmental Consideration by Specified Corporations, etc., by Facilitating Access to Environmental Information, and Other Measures". This report has been edited to show detailed environmental performance data in FY 2020 as the base of the Environmental Report 2021. This report would not only ensure traceability of the data in order to enhance the reliability of the environmental report, but also make useful measures for promoting activities of environmental considerations in JAEA.
Honda, Maki; Martschini, M.*; Marchhart, O.*; Priller, A.*; Steier, P.*; Golser, R.*; Sato, Tetsuya; Tsukada, Kazuaki; Sakaguchi, Aya*
Analytical Methods, 14(28), p.2732 - 2738, 2022/07
Times Cited Count:2 Percentile:76.85(Chemistry, Analytical)The sensitive Sr analysis with accelerator mass spectrometry (AMS) was developed for the advances of environmental radiology. One advantage of AMS is the ability to analyze various environmental samples with
Sr/
Sr atomic ratios of 10
in a simple chemical separation. Three different IAEA samples with known
Sr concentrations (moss-soil, animal bone, Syrian soil: 1 g each) were analyzed to assess the validity of the chemical separation and the AMS measurement. The
Sr measurements were conducted on the AMS system combined with the Ion Laser InterAction MasSpectrometry (ILIAMS) setup at the University of Vienna, which has excellent isobaric separation performance. The isobaric interference of
Zr in the
Sr AMS was first removed by chemical separation. The separation factor of Zr in two-step column chromatography with Sr resin and anion exchange resin was 10
. The
Zr remaining in the sample was removed by ILIAMS effectively. This simple chemical separation achieved a limit of detection
0.1 mBq in the
Sr AMS, which is lower than typical
-ray detection. The agreement between AMS measurements and nominal values for the
Sr concentrations of IAEA samples indicated that the new highly-sensitive
Sr analysis in the environmental samples with AMS is reliable even for high matrix samples of soil and bone.
Eljamal, R.*; Maamoun, I.; Bensaida, K.*; Yilmaz, G.*; Sugihara, Yuji*; Eljamal, O.*
Renewable and Sustainable Energy Reviews, 158, p.112192_1 - 112192_13, 2022/04
Times Cited Count:12 Percentile:94.32(Green & Sustainable Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; National Institute for Materials Science*
JAEA-Review 2021-059, 71 Pages, 2022/02
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms" conducted in FY2020. The present study aims to develop innovative diagnostic techniques such as accelerated test specimens and on-site genetic testing for microbially induced and accelerated corrosion of metallic materials (microbially influenced corrosion, MIC), and to identify the conditions that promote MIC at 1F for proposing methods to prevent MIC through water quality and environmental control. We also aim to develop a research base based on materials, microorganisms, and electrochemistry, to develop technologies that can be used by engineers in the field, and to cultivate leade
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2021-058, 75 Pages, 2022/02
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Investigation of environment induced property change and cracking behavior in fuel debris" conducted in FY2020. The present study aims to investigate the environment induced property change and cracking behavior in fuel debris from the viewpoints of materials science. The research objective is cracking behavior in fuel debris which is presumed to be influenced by environment during long-term fuel debris processing period. The degradation models will be established to simulate the oxidation and hydrogenation processes possibly occurred at fuel debris. The evolution of phase constitution and the corresponding property change in the simulated fuel debris under various environmental conditions will be systematically
Collaborative Laboratories for Advanced Decommissioning Science; Keio University*
JAEA-Review 2021-048, 181 Pages, 2022/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Study of corrosion and degradation of the objects in the nuclear reactor by microorganisms" conducted in FY2019 and FY2020. Since the final year of this proposal was FY2020, the results for two fiscal years were summarized. The purpose of the study is to obtain knowledge related to microorganisms that will be useful in the decommissioning process of 1F. Therefore, we clarified the current conditions of the microbial community inhabiting the power plant and its premises. Environmental samples were taken from several sites such as, topsoil from the south of the plant site boundary (south of the treated water tanks), seabed soil and its above water near the plant, surface water 3km offshore, and metagenomic
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2021-036, 95 Pages, 2021/12
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Safe, efficient cementation of challenging radioactive wastes using alkali activated materials with high-flowability and high-anion retention capacity" conducted in FY2020. For safe storage and disposal of iron sludge generated from contaminated water treatment, the present study aims to 1) explore alkali activated materials (AAM) with high-flowability and high-anion retention capacity and its recipe, 2) try mock-up manufacture and evaluation for one-tenth the size of real waste and propose the concept of the manufacturing equipment for a real plant, 3) show potential of AAM as the material for the solidification of waste with various physicochemical properties and radioactive nuclide compositions from the result of
Nakamoto, Yukihiro*; Doyama, Kohei*; Haruma, Toshikatsu*; Lu, X.*; Tanaka, Kazuya; Kozai, Naofumi; Fukuyama, Kenjin; Fukushima, Shigeru; Ohara, Yoshiyuki; Yamaji, Keiko*
Minerals (Internet), 11(12), p.1337_1 - 1337_17, 2021/12
Times Cited Count:1 Percentile:0.02(Geochemistry & Geophysics)Mine drainage is a vital water problem in the mining industry worldwide because of the heavy metal elements and low pH. Rhizofiltration using wetland plants is an appropriate method to remove heavy metals from the water via accumulation in the rhizosphere. is one of the candidate plants for this method because of metal accumulation, forming iron plaque around the roots. At the study site, which was the mill tailings pond in the Ningyo-toge uranium mine,
has been naturally growing since 1998. The results showed that
accumulated Fe, Mn, and
U in the nodal roots without/with iron plaque compared with other plant tissues. Among the 837 bacterial colonies isolated from nodal roots, 88.6% showed siderophore production activities. Considering iron plaque formation around
roots, we hypothesized that microbial siderophores might influence iron plaque formation because bacterial siderophores have catechol-like functional groups. The complex of catechol or other phenolics with Fe was precipitated due to the networks between Fe and phenolic derivatives. The experiment using bacterial products of root endophytes, such as
spp. and
spp., showed precipitation with Fe ions, and we confirmed that several
spp. and
spp. produced unidentified phenolic compounds. In conclusion, root-endophytic bacteria such as
spp. and
spp., isolated from metal-accumulating roots of
, might influence iron plaque formation as the metal accumulation site. Iron plaque formation is related to tolerance in
, and
spp. and
spp. might indirectly contribute to tolerance.
Safety and Environmental Management Section, Safety and Nuclear Security Administration Department
JAEA-Review 2021-005, 209 Pages, 2021/11
In September, 2020 Japan Atomic Energy Agency (JAEA) published the Environmental Report 2020 concerning the activities of FY 2019 under "Law Concerning the Promotion of Business Activities with Environmental Consideration by Specified Corporations, etc., by Facilitating Access to Environmental Information, and Other Measures". This report has been edited to show detailed environmental performance data in FY 2019 as the base of the Environmental Report 2020. This report would not only ensure traceability of the data in order to enhance the reliability of the environmental report, but also make useful measures for promoting activities of environmental considerations in JAEA.