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Journal Articles

Quantum optimal control of the isotope-selective rovibrational excitation of diatomic molecules

Kurosaki, Yuzuru*; Yokoyama, Keiichi

Chemical Physics, 493, p.183 - 193, 2017/08

AA2017-0230.pdf:8.02MB

 Times Cited Count:3 Percentile:77.34(Chemistry, Physical)

Electric field of laser pulses which gives maximum selectivity in the isotope-selective rovibrational excitation of lithium chloride molecules is calculated. Applying the optimal control theory, we calculate optimal electric field to produce mixture of LiCl-35 ($$nu$$=0, $$J$$=0) and LiCl-37 ($$nu$$=1, $$J$$=1) from molecular ensemble of LiCl-35 ($$nu$$=0, $$J$$=0) and LiCl-37 ($$nu$$=0, $$J$$=0). As a result, it is found that electric field which permit rotational excitations only gives high yield in the selective excitation compared to the electric field which permit both rotational and vibrational excitations.

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Quantum optimal control of isotope-selective rovibrational excitation of diatomic molecules

Kurosaki, Yuzuru*; Yokoyama, Keiichi

no journal, , 

Electric field of laser pulses is designed by the optimal control theory. The target process is isotope-selective rovibrational excitation of two isotopologues of the lithium chloride molecule, Li$$^{35}$$Cl or Li$$^{37}$$Cl. The calculation includes both radial and angular motion of atoms in molecule. As a result, it is found that a laser pulse field which can cause isotope-selective rovibrational excitation with high yield exists.

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