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JAEA Reports

Analytical study on stress behavior of core graphite components using simplified viscoelastic evaluation model

Saijo, Tomoaki; Shimazaki, Yosuke; Ishihara, Masahiro

JAEA-Technology 2025-010, 126 Pages, 2025/12

JAEA-Technology-2025-010.pdf:12.52MB

During the operation of the High Temperature Engineering Test Reactor (HTTR), thermal stress is generated in the graphite components. In addition, graphite exhibits dimensional shrinkage and creep deformation under neutron irradiation. As a result, residual stress remains in the graphite components during reactor shutdown. Therefore, in the design of the HTTR core graphite structures, stress analyses of the graphite components have previously been performed using the finite element analysis code VIENUS. In the HTTR, the graphite components are exposed to a wide range of temperature, from approximately 400$$^{circ}$$C to 1200$$^{circ}$$C, depending on their location. Consequently, irradiation-induced behaviors such as material property changes and irradiation shrinkage vary among the graphite components. On the other hand, since VIENUS code evaluates stress based on thermal fluid and heat conduction analysis results, it is not suitable for parametric studies. In this study, the influence of irradiation behavior on the stress behavior of graphite components in the wide temperature range (400$$^{circ}$$C to 1200$$^{circ}$$C) was analyzed using simplified viscoelastic evaluation model, consisting of two beam elements, to conduct efficient parametric studies. Operational stress exhibits two distinct patterns depending on whether the irradiation temperature is below or above 800$$^{circ}$$C, due to irradiation shrinkage. Residual stress approaches the thermal stress, preventing excessive increase even when irradiation shrinkage is large. Moreover good agreement in stress behavior trends was observed between the stress analysis results by the simplified viscoelastic evaluation model and VIENUS code. These results indicate that the simplified viscoelastic evaluation model is beneficial in simulating stress behavior.

Journal Articles

Corrosion behavior of extra-high-purity Type 316 austenitic stainless steel in a liquid lead-bismuth eutectic with oxygen saturation or low oxygen concentrations

Irisawa, Eriko; Kato, Chiaki

Corrosion Science, 256, p.113173_1 - 113173_16, 2025/11

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

Journal Articles

Revisiting $$^{9}$$Be nuclear magnetic resonance in UBe$$_{13}$$; Itinerant-localized duality and possible Fermi surface reconstruction at high magnetic field

Matsuki, Rintaro*; Minami, Shoko*; Kotegawa, Hisashi*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; To, Hideki*

Journal of the Physical Society of Japan, 94(12), p.124702_1 - 124702_8, 2025/11

Journal Articles

Improving the analysis method of the Compton camera system mounted on the unmanned helicopter by correcting scintillator coordinates data at each event timing

Shikaze, Yoshiaki

Radioisotopes, 74(3), p.273 - 287, 2025/11

The previous method used the data during the stable period for the position and attitude angles of the unmanned helicopter as a countermeasure to improve the measurement data analysis of the Compton camera system mounted on the unmanned helicopter. However, this reduced the number of events used for analysis, allowing statistical accuracy to be improved in future. Therefore, all event data were corrected and used this time. The scintillator coordinates of two layers fixed in the previous analysis were replaced with those corrected for the ever-changing positions and tilts for each event. I reconstructed gamma-ray images using the corrected events to improve their statistical accuracy and spatial resolution. I compared the ground measurement results to evaluate the improvement in the accuracy of the reconstructed images of gamma-ray intensity. As for the effect of the improved statistics, a decrease in the residual sum of squares (RSS) was noted after improvement, indicating the effectiveness of this method through good correlations with the ground-measured values. Moreover, from the RSS value comparison, compared to changing from the previous method to the improved method, expanding the range of averaging the measured values was confirmed to be more effective, showing better correlations with the ground-measured values.

Journal Articles

Ten-year temporal changes in the supply source of $$^{137}$$Cs released by the Fukushima Daiichi Nuclear Power Plant to the coastal area

Sato, Shun; Wakiyama, Yoshifumi*; Takahashi, Fumiaki; Takata, Hyoe*

Science of the Total Environment, 1000, p.180380_1 - 180380_14, 2025/10

We compared the ongoing direct release of $$^{137}$$Cs from the Fukushima Daiichi Nuclear Power Plant (FDNPP) and riverine inputs of $$^{137}$$Cs that have contributed to the persistent elevated $$^{137}$$Cs in coastal waters around the plant since 2012. The direct release of $$^{137}$$Cs clearly decreased from 17.5 TBq during 2012$$sim$$2014 to 0.6 TBq during 2019$$sim$$2021 because of measures implemented by the FDNPP. The riverine input decreased slightly from 2.2 TBq during 2012$$sim$$2014 to 2.0 TBq during 2019$$sim$$2021. The ratio of direct release to the total $$^{137}$$Cs flux into the coastal water around the FDNPP decreased from 89% during 2012$$sim$$2014 to 23% during 2019$$sim$$2021. This change resulted in part from a lowering of the limit of detection of $$^{137}$$Cs activities to avoid overestimation of Cs fluxes from the facility, but also from installation of an impermeable seaside wall. The trend of decreasing riverine $$^{137}$$Cs input might have been due entirely to environmental remediation. Our results indicate that the contribution of riverine input to the coastal waters will continue for a long time. Precise prediction of the long-term distribution of $$^{137}$$Cs in the marine environment will require consideration of a variety of environmental factors and anthropogenic effects.

Journal Articles

Pressure-driven solid-state radical polymerization toward carbon nanothread

Che, G.*; Tang, X.*; Liu, J.*; Lang, P.*; Fei, Y.*; Yang, X.*; Wang, Y.*; Gao, D.*; Wang, X.*; Ju, J.*; et al.

Nano Letters, 25(39), p.14467 - 14472, 2025/09

Mechanochemical radical polymerization has unique advantages in the synthesis of polymer due to its reduced solvent consumption and adaptability of insoluble monomers. However, it suffers from the uncontrollable degradation of the formed polymers during reaction and new synthetic strategy with precise controllability needs to be developed. Here, by employing high static pressure up to 30 GPa, we found 1,3,5-trifluorobenzene undergoes radical polymerization by breaking the conjugated $$pi$$-bonds, and forms a carbon nanothread with high selectivity (Polymer-I polymorph). Based on the crystal structure at the threshold pressure and the calculated energy barriers for the bonding pathway, we concluded that the benzene-rings react via a 1-2 radical polymerization pathway. Our work highlights high pressure is a robust method to initiate the solid-state radical polymerization, even for very stable aromatics, and offers fresh insights for the synthesis of polymeric carbon-based materials with high selectivity.

Journal Articles

Tensile properties of irradiated modified 316 stainless steel (PNC316) at slow strain rates

Yano, Yasuhide; Miyazawa, Takeshi; Tanno, Takashi; Akasaka, Naoaki; Yoshitake, Tsunemitsu; Kaito, Takeji; Otsuka, Satoshi

Journal of Nuclear Science and Technology, 62(8), p.748 - 755, 2025/08

 Times Cited Count:0 Percentile:76.46(Nuclear Science & Technology)

The effects of strain rate on tensile properties of irradiated modified 316 stainless steel (PNC316) claddings were investigated. PNC316 claddings were irradiated at the experimental fast reactor Joyo using CRT402 control rod assembly at 400$$^{circ}$$C up to 25 dpa. Post-irradiation ring tensile tests were carried out at strain rates of 3.3$$times$$10$$^{-6}$$, 3.3$$times$$10$$^{-7}$$ and 3.3$$times$$10$$^{-8}$$ s$$^{-1}$$ at a test temperature of 350$$^{circ}$$C. The results showed no obvious dependence of all strain rates on tensile properties, although a slight decrease in total elongation was observed at the slowest strain rate of 3.3$$times$$10$$^{-8}$$ s$$^{-1}$$. In addition, only a part of fracture surface at the slowest strain rate showed intergranular type region in the inner surface area, although the grain boundary separation occurred on inner surfaces near the fracture region at all strain rates. It is suggested that presence of a high content of helium near the inner surfaces would be related to the fracture behavior.

Journal Articles

Development of a theoretical scaling factor method for the inventory estimation of difficult-to-measure nuclide Cs-135 in fuel debris and radioactive wastes

Sakamoto, Masahiro; Okumura, Keisuke; Kanno, Ikuo; Matsumura, Taichi; Terashima, Kenichi; Riyana, E. S.; Kaneko, Junichi*; Mizokami, Masato*; Mizokami, Shinya*

Journal of Nuclear Science and Technology, 62(8), p.756 - 765, 2025/08

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Distribution of cesium-bearing microparticles in the paddy field and their effect on transfer factor of radioactive cesium for brown rice

Tatsuno, Takahiro*; Nihei, Naoto*; Yoshimura, Kazuya

Journal of Radioanalytical and Nuclear Chemistry, 334(8), p.5719 - 5727, 2025/08

Journal Articles

A New analytical technique utilizing the PdI$$_{2}$$ target for measurement of $$^{129}$$I in environmental samples by accelerator mass spectrometry

Honda, Maki; Takaku, Yuichi*; Sakaguchi, Aya*; Matsuzaki, Hiroyuki*; Sueki, Keisuke*

Journal of Radioanalytical and Nuclear Chemistry, 12 Pages, 2025/08

 Times Cited Count:0 Percentile:0.00

A series of in-house PdI$$_{2}$$ standards appropriate for AMS was prepared by quantitatively mixing the $$^{129}$$I/$$^{127}$$I isotope standard solution and $$^{127}$$I solution. The dominant interferences from $$^{104, 105}$$Pd $$^{4+}$$ were successfully suppressed by adjusting the electrostatic cylindrical analyser, etc., to select the ion beams finely. As a result, the $$^{129}$$I/$$^{127}$$I atom ratios of PdI$$_{2}$$ prepared from the seawater and dolomite samples agreed with those prepared as AgI, respectively. The pretreatment time for the new method was shortened by 33% compared to the conventional method. This study demonstrated a new approach to $$^{129}$$I analysis in AMS that departs from conventional methods.

Journal Articles

Experimental and modeling studies on the oxygen ingression behavior at the crevices of stainless steels in high-temperature water

Soma, Yasutaka; Komatsu, Atsushi; Kaji, Yoshiyuki; Yamamoto, Masahiro*; Igarashi, Takahiro

Corrosion Science, 251, p.112897_1 - 112897_15, 2025/07

 Times Cited Count:1 Percentile:61.86(Materials Science, Multidisciplinary)

Experimental and modeling studies of the oxygen ingression at the crevices of stainless steels were conducted in high-temperature water (288$$^{circ}$$C). The limiting distance of oxygen ingression, $$d_{rm lim}$$, was defined as the point beyond which the primary surface oxide changed (hematite $$rightarrow$$ magnetite), regardless of crevice gap, oxygen concentration, and time. In situ measurements revealed increased electrical conductivity around the $$d_{rm lim}$$ position indicating ion enrichment due to a differential oxygen concentration cell. $$d_{rm lim}$$ increased with increasing crevice gap, oxygen concentration, and immersion time. Modeling study suggested that oxide layer growth reduced anodic dissolution and slowed oxygen consumption, allowing oxygen ingression with time.

Journal Articles

Which radionuclides contribute most to seafood ingestion dose?

Johansen, M. P.*; Gwynn, J. P.*; Carpenter, J. G.*; Charmasson, S.*; Mori, Airi; Orr, B.*; Simon-Cornu, M.*; Osvath, I.*; McGinnity, P.*

Journal of Environmental Radioactivity, 287, p.107706_1 - 107706_8, 2025/07

 Times Cited Count:1 Percentile:61.99(Environmental Sciences)

Journal Articles

Measurements of neutron capture cross-sections for nuclides of interest in decommissioning (IV); $$^{165}$$Ho(n,$$gamma$$)$$^{rm 166m,166g}$$Ho reactions

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Rovira Leveroni, G.; Kimura, Atsushi

Journal of Nuclear Science and Technology, 14 Pages, 2025/07

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Measurements of neutron capture cross-section for nuclides of interest in decommissioning (III); $$^{170}$$Er(n,$$gamma$$)$$^{171}$$Er and $$^{180}$$Hf(n,$$gamma$$)$$^{181}$$Hf reactions

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Rovira Leveroni, G.; Kimura, Atsushi

Journal of Nuclear Science and Technology, 62(7), p.617 - 630, 2025/07

 Times Cited Count:1 Percentile:76.46(Nuclear Science & Technology)

Journal Articles

${it Gaoshiqia hydrogeniformans}$ sp. nov., a novel hydrogen-producing bacterium isolated from a deep diatomaceous shale formation

Ueno, Akio*; Sato, Kiyoshi*; Tamamura, Shuji*; Murakami, Takuma*; Inomata, Hidenori*; Tamazawa, Satoshi*; Amano, Yuki; Miyakawa, Kazuya; Naganuma, Takeshi*; Igarashi, Toshifumi*

International Journal of Systematic and Evolutionary Microbiology, 75(6), p.006802_1 - 006802_11, 2025/06

 Times Cited Count:0 Percentile:0.00(Microbiology)

no abstracts in English

Journal Articles

Neutron capture cross-section measurement at TC-Pn in KUR for holmium among nuclides in decommissioning

Nakamura, Shoji; Endo, Shunsuke; Rovira Leveroni, G.; Kimura, Atsushi; Shibahara, Yuji*

KURNS Progress Report 2024, P. 31, 2025/06

no abstracts in English

Journal Articles

Evaluation of stability of precipitates under irradiation in 316FR steel used as fast reactor structural material

Toyota, Kodai; Onizawa, Takashi; Wakai, Eiichi*

Research & Development in Material Science (Internet), 21(5), p.2632 - 2637, 2025/06

Journal Articles

Ingestion doses from radionuclides in seafood before and after the Fukushima Daiichi Nuclear Power Plant accident

Mori, Airi; Johansen, M. P.*; McGinnity, P.*; Takahara, Shogo

Communications Earth & Environment (Internet), 6, p.356_1 - 356_11, 2025/05

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Operational quantities for external radiation exposure proposed in ICRU Report 95

Endo, Akira

ESI-News, 43(2), p.37 - 41, 2025/04

The International Commission on Radiation Units and Measurements (ICRU) published ICRU Report 95 in 2020, revising the operational quantities for external exposure. This article provides an overview of the developments in the discussions within the ICRU, the International Commission on Radiological Protection (ICRP), and experts from Japan, and explores the background and process that led the ICRU to revise the operational quantities, as well as future responses and challenges. The article aims to enhance the understanding of the experts of the new operational quantities and to contribute to their smooth implementation in the future.

Journal Articles

Comparison of analysis results based on flight methods using a CZT detector system on an unmanned aerial vehicle near the Fukushima nuclear power plant

Joung, S.*; Ji, Y.-Y.*; Choi, Y.*; Lee, E.*; Ji, W.*; Sasaki, Miyuki; Ochi, Kotaro; Sanada, Yukihisa

Journal of Instrumentation (Internet), 20(4), p.P04027_1 - P04027_10, 2025/04

 Times Cited Count:0 Percentile:65.93(Instruments & Instrumentation)

3126 (Records 1-20 displayed on this page)