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Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2021-044, 58 Pages, 2022/01
JAEA-Review-2021-044.pdf:3.53MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of high-resolution imaging camera for alpha dust" conducted in FY2020. The present study aims to develop a novel alpha-ray camera consisting of imaging and an energy spectrometer to find the alpha dust to reduce the risk of health damage in Decommissioning. We have developed the camera in FY2020, and the measurement test for the energy spectra. Moreover, the imaging test has been operated. In addition, we have also developed a high-dose-rate monitor system using novel scintillators with red/infra-red emission.
scintillator under intense 
-ray fields for nuclear decommissioningKaburagi, Masaaki; Shimazoe, Kenji*; Kato, Masahiro*; Kurosawa, Tadahiro*; Kamada, Kei*; Kim, K. J.*; Yoshino, Masao*; Shoji, Yasuhiro*; Yoshikawa, Akira*; Takahashi, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research A, 988, p.164900_1 - 164900_8, 2021/02
Times Cited Count：1 Percentile：81.22(Instruments & Instrumentation)An increasing number of nuclear facilities have been decommissioned worldwide following the 2011 accident of the TEPCO' Fukushima Daiichi Nuclear Power Station. During the decommissioning, radioactive materials have to be retrieved under proper management. In this study, a small cubic CeBr spectrometer with dimensions of 5 mm 
5 mm 5 mm was manufactured to perform -ray spectroscopy under intense -ray fields. Furthermore, thanks to a fast digital process unit and a customized photomultiplier, the device could perform -ray spectroscopy at dose rates of over 1 Sv/h. The energy resolution (FWHM) at 662 keV ranged from 4.4% at 22 mSv/h to 5.2% at 1407 mSv/h for a 
Cs radiation field. Correspondingly, at 1333 keV, it ranged from 3.1% at 26 mSv/h to 4.2% at 2221 mSv/h for a 
Co radiation field, which suggested to realize -ray assessment of 
Cs, Cs, Co, and 
Eu at dose rates of over 1 Sv/h.
Collaborative Laboratories for Advanced Decommissioning Science; Shizuoka University*
JAEA-Review 2020-059, 42 Pages, 2021/01
JAEA-Review-2020-059.pdf:3.07MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Radiation tolerant rapid criticality monitoring with radiation-hardened FPGAs". This research is developing a radiation-hardened optoelectronic FPGA with a 1 Grad total-ionizing-dose tolerance on which optical technologies are introduced onto a semiconductor technology and a radiation hardened FPGA with a 200 Mrad total-ionizing-dose tolerance not using any optical component. Moreover, Japanese research group will support hardware acceleration on FPGAs used for neutron-detection system developed by UK team. Finally, we will provide our radiation-hardened FPGA for the UK neutron-detection system.
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2020-039, 59 Pages, 2021/01
JAEA-Review-2020-039.pdf:4.18MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of high-resolution imaging camera for alpha dust" conducted in FY2019. We have developed an imaging camera with a position resolution of less than approximately 10 
m to monitor alpha dust in the nuclear plant during the decommissioning process, because the operators avoid to drawing in such dusts. Moreover, we have developed real-time monitor system with optical fiber and scintillator under high dose-rate condition.
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2019-038, 57 Pages, 2020/03
JAEA-Review-2019-038.pdf:4.6MB
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Imaging System with Ultra-high Spatial Resolution Aiming to Detect Alpha-dust". In the present study, we have developed a prototype of a system aiming to elucidate the behavior of alpha-dust generated at the time of debris retrieval. In this system, alpha-ray is first converted to visible light by novel scintillator. Then, imaging with ultra-high resolution will be possible using a lens and an Si-semiconductor camera (CMOS camera). Also, it will be possible to identify the species of alpha-ray emitting nuclides by unfolding of the spectra. The demonstration tests of the system will be conducted for dust samplers at the Plutonium Fuel Development Center, JAEA. In the development of the present system, it is important to use scintillator whose emission wavelength is sensitive to the CMOS camera as well as high emission scintillator. Considering these conditions, the key technology will be the improvement of the purity of crystals and optimization of the shapes of the materials including powers.
Collaborative Laboratories for Advanced Decommissioning Science; Kyoto University*
JAEA-Review 2019-036, 65 Pages, 2020/03
JAEA-Review-2019-036.pdf:4.46MB
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Quantitative Analysis Method for Radiation Distribution in High Radiation Environment by Gamma-ray Image Spectroscopy". Electron-tracking Compton camera (ETCC) has been developed originally for nuclear gamma-ray astronomy, and also applied to medical use as a technology that greatly improves the resolution of conventional Compton camera by measuring three-dimensional tracking of electrons using a gaseous 3-dimensional position detector (so called Time Projection Chamber) in the first stage. In the present study, based on the ETCC that has been developed for medical use, we produce a prototype of light weight ETCC with the emphasis on the operability at the site, and evaluate its practicability by field tests.
Arikawa, Yasunobu*; Ikeda, Yujiro; Shimizu, Hirohiko*; Hanayama, Ryohei*; Kondo, Yasuharu*; Kurosawa, Shunsuke*
Reza Kenkyu, 46(11), p.634 - 640, 2018/11
Compact neutron sources have been used as various diagnostics such as a neutron diffraction, neutron resonant analysis, and neutron radiography. The developments of the neutron detectors are essential for all of these applications, while the techniques are strongly dependent on the neutron energy and the aim of the measurement. This paper reviews neutron detection techniques pertinent to promote compact neutron source uses. Along with general neutron detection systems with conventional counters for slow neutrons, we have highlighted detectors for high energy neutrons with high time resolution and high sensitivity which could be applied in a laser-driven compact neutron source.
Seya, Michio; Kobayashi, Naoki; Naoi, Yosuke; Hajima, Ryoichi; Soyama, Kazuhiko; Kureta, Masatoshi; Nakamura, Hironobu; Harada, Hideo
Book of Abstracts, Presentations and Papers of Symposium on International Safeguards; Linking Strategy, Implementation and People (Internet), 8 Pages, 2015/03
JAEA-ISCN has been implementing basic development programs of the advanced NDA technologies for nuclear material (NM) since 2011JFY (Japanese Fiscal Year), which are (1) NRF (Nuclear resonance fluorescence) NDA technology using laser Compton scattered (LCS) -rays (intense mono-energetic -rays), (2) Alternative to 
He neutron detection technology using ZnS/B
O
ceramic scintillator, and (3) NRD (Neutron resonance densitometry) using NRTA (Neutron resonance transmission analysis) and NRCA (Neutron resonance capture analysis). These programs are going to be finished in 2014JFY and have demonstration tests in February - March 2015.
Arita, Ren*; Nakazato, Tomoharu*; Shimizu, Toshihiko*; Yamanoi, Kohei*; Empizo, M.*; Hori, Tatsuhiro*; Fukuda, Kazuhito*; Minami, Yuki*; Sarukura, Nobuhiko*; Maruyama, Momoko; et al.
Optical Materials, 36(12), p.2012 - 2015, 2014/10
Times Cited Count：7 Percentile：38.97(Materials Science, Multidisciplinary)A single shot image of a ZnO crystal excited by the EUV laser of Kansai Photon Science Institute was captured. The evaluated EUV beam waist radii from the ZnO emission pattern along the horizontal and vertical axes are 5.0 and 4.7m, respectively. The expected focal spot size of EUV laser and the spatial resolution of the magnifier (including the Schwarzschild objectives and lenses) are however 1 and 4m, respectively. The discrepancy on the spatial resolutions is attributed to exciton diffusion. We estimated the ZnO exciton diffusion length from the effective decay time which is shortened by exciton-exciton collision quenching and which is dependence on excitation energy density. Our results indicate that the short lifetime of ZnO is required to improve the spatial resolution.
Seya, Michio; Kureta, Masatoshi; Soyama, Kazuhiko; Nakamura, Hironobu; Harada, Hideo; Hajima, Ryoichi
Proceedings of INMM 55th Annual Meeting (Internet), 10 Pages, 2014/07
JAEA has been implementing development programs of basic technologies of the following advanced NDA (non-destructive assay) of nuclear material (NM) for nuclear safeguards and security. (1) Alternative to He neutron detection using ZnS/BO ceramic scintillator, (2) NRD (neutron resonance densitometry) using NRTA (neutron resonance transmission analysis) and NRCA (neutron resonance capture analysis), (3) NRF (nuclear resonance fluorescence)-NDA using laser Compton scattered (LCS) -rays (intense mono-energetic -rays). The development program (1) is for NDA systems that use ZnS/BO ceramic scintillator as alternative neutron detector to He for coming shortage of its supply. The program (2) is for a NDA system of isotopic composition measurement (non-destructive mass spectroscopy) in targets such as particle-like melted fuel debris using NRTA and NRCA. The program (3) is for NDA systems using a specific NRF reaction of certain Pu/U isotope caused by mono-energetic LCS -ray with energy tuned to the specific excited state of the isotope. This paper introduces above three programs.
BO ceramic scintillator detector as an alternative to a He-gas-based detector for a plutonium canister assay systemNakamura, Tatsuya; Ozu, Akira; To, Kentaro; Sakasai, Kaoru; Suzuki, Hiroyuki; Honda, Katsunori; Birumachi, Atsushi; Ebine, Masumi; Yamagishi, Hideshi*; Takase, Misao; et al.
Nuclear Instruments and Methods in Physics Research A, 763, p.340 - 346, 2014/05
Times Cited Count：3 Percentile：30.04(Instruments & Instrumentation)A neutron-sensitive ZnS/BO ceramic scintillator detector was developed as an alternative to a He-gas-based detector for use in a plutonium canister assay system. The detector has a modular structure, with a flat ZnS/BOceramic scintillator strip that is installed diagonally inside a light-reflecting aluminium case with a square cross section. The prototype detectors, which have a neutron-sensitive area of 30 mm 250 mm, exhibited a sensitivity of 21.7-23.4 
0.1 cps
nv for thermal neutrons, a Cs -ray sensitivity of 1.1-1.9 
0.2 10
and a count variation of less than 6% over the detector length. A trial experiment revealed a temperature coefficient of less than -0.24 0.05% / 
C over the temperature range of 20-50C.
(Ce) scintillation detector applications for environmental -ray measurements of low to high dose ratesTsutsumi, Masahiro; Tanimura, Yoshihiko
Nuclear Instruments and Methods in Physics Research A, 557(2), p.554 - 560, 2006/02
Times Cited Count：12 Percentile：65.95(Instruments & Instrumentation)A new cerium-doped LaCl(Ce) scintillator is evaluated with respect to the application in environmental -ray dosimetry and spectrometry. The scintillator is very attractive for -ray spectrometry in the case of high count rate, because it has excellent energy resolution and fast decay time. The performance characteristics of a scintillator with a 25.4 mm 25.4 mm LaCl(Ce) crystal are studied and compared to those of a NaI(Tl) scintillator with the same size crystal. Acquired pulse-height spectra are converted to dose rates by using the G(E) function method. Though the LaCl(Ce) crystal itself produces a rather high background in the crystal itself, the scintillator provides good energy information and dose-rate readings from low to high-level (several mGy/h) by subtracting the self-background. The properties of LaCl(Ce) scintillator suggest that the scintillator could be a promising candidate for monitoring at high-dose levels as in emergencies, as well as at ordinary levels of background radiation.
Sato, Tatsuhiko; Satoh, Daiki; Endo, Akira; Yamaguchi, Yasuhiro
Journal of Nuclear Science and Technology, 42(9), p.768 - 778, 2005/09
Times Cited Count：16 Percentile：74.09(Nuclear Science & Technology)A new inventive radiation monitor, designated to DARWIN (Dose Assessment system applicable to various Radiations with WIde energy raNges), has been developed for monitoring doses at workspaces of high energy accelerator facilities and on ground. Characteristics of DARWIN were studied by both calculation and experiment. The calculated results indicate that DARWIN gives reasonable estimations of doses at most radiation fields. It was found from the experiment that DARWIN has an excellent property of measuring doses from all particles that significantly contribute to the background dose - photon, muon and neutron with wide energy ranges.
Tsutsumi, Masahiro; Oishi, Tetsuya*; Yamasoto, Kotaro; Yoshida, Makoto
JAERI-Research 2004-021, 43 Pages, 2004/12
JAERI-Research-2004-021.pdf:8.55MB
We have designed and developed a measurement system to certify radioactive wastes below the clearance level. By advancing non-destructive -ray assay technology, it aims at quantitative determination of radionuclides contained in 200 litter drum/container wastes. Unlike the waste from a nuclear power plant, you have to assume that the waste originating from radioisotope usage and nuclear research laboratory have a variety of contents and a complex mixture of radionuclides, and furthermore the uniformity of activity concentration is unknown. To cope with the problems, we have developed the -ray measuring instruments (units) with effective improvement of capability against each problem. They are (1) germanium spectrometry unit for enhanced peak identification, (2) positioning detection unit for positioning of interactions and (3)high-efficiency detection unit for separation of low-energy component. This report summarizes the direction of the clearance level measuring system and the three developed measuring units with their performances.
Li+ZnS(Ag) sheetSato, Tatsuhiko; Endo, Akira; Yamaguchi, Yasuhiro; Takahashi, Fumiaki
Radiation Protection Dosimetry, 110(1-4), p.255 - 261, 2004/09
Times Cited Count：8 Percentile：50.96(Environmental Sciences)For monitoring of neutron doses in high-energy accelerator facilities, we have developed a neutron-monitor detector applicable to energies from the thermal energy to 100 MeV. The detector is composed of a cylindrical (12.7 cm in diameter and 12.7 cm in length) liquid organic scintillator BC501A covered with Li+ZnS(Ag) sheets. Characteristics of this phoswitch-type detector were studied experimentally in moderated neutron fields of 
Am-Be and 
Cf sources, and in quasi-monoenergetic neutron fields of 40 and 70 MeV. It was found from the experiments that the detector is enough sensitive to both thermal and fast neutrons, and has an excellent property of pulse-shape discrimination between them. We concluded, therefore, that the detector can be used for monitoring of neutron doses over a wide energy range from the thermal to 100 MeV.
Matsubayashi, Masahito; Katagiri, Masaki
Nuclear Instruments and Methods in Physics Research A, 529(1-3), p.389 - 393, 2004/08
Times Cited Count：2 Percentile：18.72(Instruments & Instrumentation)no abstracts in English
Endo, Akira; Kim, E.; Yamaguchi, Yasuhiro; Sato, Tatsuhiko; Yoshizawa, Michio; Tanaka, Susumu; Nakamura, Takashi; Rasolonjatovo, A. H. D.*
Journal of Nuclear Science and Technology, 41(Suppl.4), p.510 - 513, 2004/03
no abstracts in English
JAERI's Internal Investigation Group on the Ruptured Glove; Department of Decommissioning and Waste Management
JAERI-Review 2002-017, 121 Pages, 2002/09
JAERI-Review-2002-017.pdf:13.36MB
On November 21st, 2001, the glove rupture arose at an incinerator of Waste Treatment Building No.1 in JAERI Tokai Research Establishment. In order to examine the cause and recurrence prevention measure of the rupture, JAERI's Internal Investigation Group on the Ruptured Glove investigated the conditions of the incinerator including ash removing equipment and the glove, types and properties of waste which was incinerated on that day, and background factor of the trouble in cooperation with Department of Decommissioning and Waste Management.As the result, the causes of the rupture were that the solidification of liquid scintillator waste was insufficient, that the protective cover of the glove does not have pressure resistance and the degraded glove was used. For preventing the recurrence of the trouble, the direct confirmation of the solidification condition, the installation of protective cover for the glove, the improvement of the management of the glove, review of manuals and education and training were carried out.
Li glass scintillator for wide energy rangeKim, E.; Endo, Akira; Yamaguchi, Yasuhiro; Yoshizawa, Michio; Nakamura, Takashi*; Rasolonjatovo, D. R. D.*
Nihon Genshiryoku Gakkai Wabun Rombunshi, 1(3), p.317 - 319, 2002/09
no abstracts in English
To, Kentaro; Katagiri, Masaki; Sakasai, Kaoru; Matsubayashi, Masahito; Birumachi, Atsushi; Takahashi, Hiroyuki*; Nakazawa, Masaharu*
Nuclear Instruments and Methods in Physics Research A, 485(3), p.571 - 575, 2002/09
Times Cited Count：2 Percentile：19.85(Instruments & Instrumentation)no abstracts in English
