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Journal Articles

Non-destructive analysis of samples with a complex geometry by NRTA

Ma, F.; Kopecky, S.*; Alaerts, G.*; Harada, Hideo; Heyse, J.*; Kitatani, Fumito; Noguere, G.*; Paradela, C.*; $v{S}$alamon, L.*; Schillebeeckx, P.*; et al.

Journal of Analytical Atomic Spectrometry, 35(3), p.478 - 488, 2020/03

 Times Cited Count:0 Percentile:100(Chemistry, Analytical)

Journal Articles

Inner structure and inclusions in radiocesium-bearing microparticles emitted in the Fukushima Daiichi Nuclear Power Plant accident

Okumura, Taiga*; Yamaguchi, Noriko*; Dohi, Terumi; Iijima, Kazuki; Kogure, Toshihiro*

Microscopy, 68(3), p.234 - 242, 2019/06

 Times Cited Count:4 Percentile:20.85(Microscopy)

Radiocesium-bearing microparticles (CsMPs), consisting substantially of silicate glass, were released to the environment during the Fukushima nuclear accident in March 2011. We investigated a total of nine CsMPs using transmission electron microscopy (TEM) and inferred the atmosphere in the reactors during the accident. From elemental mapping using energy-dispersive X-ray spectrometry, Fe and Zn showing radial inhomogeneities were found in the CsMPs, in addition to the Cs that had been previously reported. Four of the CsMPs included submicron crystals, which were identified as chromite, franklinite, acanthite, molybdenite, and hessite. The chromium-containing spinels, chromite and franklinite, indicated the presence of ferrous iron (Fe$$^{2+}$$), suggesting that the inside of the reactors was reductive to some extent. Electron energy-loss spectroscopy also confirmed that the CsMPs did not contain boron, and therefore the atmosphere in which they were formed might be boron-free.

Journal Articles

Development of remote sensing technique using radiation resistant optical fibers under high-radiation environment

Ito, Chikara; Naito, Hiroyuki; Ishikawa, Takashi; Ito, Keisuke; Wakaida, Ikuo

JPS Conference Proceedings (Internet), 24, p.011038_1 - 011038_6, 2019/01

A high-radiation resistant optical fiber has been developed in order to investigate the interiors of the reactor pressure vessels and the primary containment vessels at the Fukushima Daiichi Nuclear Power Station. The tentative dose rate in the reactor pressure vessels is assumed to be up to 1 kGy/h. We developed a radiation resistant optical fiber consisting of a 1000 ppm hydroxyl doped pure silica core and 4 % fluorine doped pure silica cladding. We attempted to apply the optical fiber to remote imaging technique by means of fiberscope. The number of core image fibers was increased from 2000 to 22000 for practical use. The transmissive rate of infrared images was not affected after irradiation of 1 MGy. No change in the spatial resolution of the view scope by means of image fiber was noted between pre- and post-irradiation. We confirmed the applicability of the probing system, which consists of a view scope using radiation-resistant optical fibers.

Journal Articles

Quasielastic neutron scattering of brucite to analyse hydrogen transport on the atomic scale

Okuchi, Takuo*; Tomioka, Naotaka*; Purevjav, N.*; Shibata, Kaoru

Journal of Applied Crystallography, 51, p.1564 - 1570, 2018/12

 Times Cited Count:0 Percentile:100(Chemistry, Multidisciplinary)

It is demonstrated that quasielastic neutron scattering (QENS) is a novel and effective method to analyse atomic scale hydrogen transport processes occurring within a mineral crystal lattice. The method was previously characterized as sensitive for analysing the transport frequency and distance of highly diffusive hydrogen atoms or water molecules in condensed matter. Here are shown the results of its application to analyse the transport of much slower hydrogen atoms which are bonded into a crystal lattice as hydroxyls. Two types of hydrogen transport process were observed in brucite, Mg(OH)$$_{2}$$ : a jump within a single two-dimensional layer of the hydrogen lattice and a jump into the next nearest layer of it. These transport processes observed within the prototypical structure of brucite have direct implications for hydrogen transport phenomena occurring within various types of oxides and minerals having layered structures.

Journal Articles

Study on neutron beam pulse width dependence in the nuclear fuel measurement by the neutron resonance transmission analysis

Kitatani, Fumito; Tsuchiya, Harufumi; Toh, Yosuke; Hori, Junichi*; Sano, Tadafumi*; Takahashi, Yoshiyuki*; Nakajima, Ken*

KURRI Progress Report 2017, P. 99, 2018/08

Journal Articles

Effect of nitrogen concentration on nano-structure and high-temperature strength of 9Cr-ODS steel

Oka, Hiroshi; Tanno, Takashi; Otsuka, Satoshi; Yano, Yasuhide; Kaito, Takeji

Nuclear Materials and Energy (Internet), 16, p.230 - 237, 2018/08

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Journal Articles

Neutron resonance transmission analysis for measurement of nuclear materials in nuclear fuel

Tsuchiya, Harufumi; Kitatani, Fumito; Toh, Yosuke; Paradela, C.*; Heyse, J.*; Kopecky, S.*; Schillebeeckx, P.*

Proceedings of INMM 59th Annual Meeting (Internet), 6 Pages, 2018/07

Journal Articles

Implementation of a low-activation Au-In-Cd decoupler into the J-PARC 1 MW short pulsed spallation neutron source

Teshigawara, Makoto; Ikeda, Yujiro; Oi, Motoki; Harada, Masahide; Takada, Hiroshi; Kakishiro, Masanori*; Noguchi, Gaku*; Shimada, Tsubasa*; Seita, Kyoichi*; Murashima, Daisuke*; et al.

Nuclear Materials and Energy (Internet), 14, p.14 - 21, 2018/01

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

We developed an Au-In-Cd (AuIC) decoupler material to reduce induced radioactivity instead of Ag-In-Cd one, which has a cut off energy of 1eV. In order to implement it into an actual moderator-reflector assembly, a number of critical engineering issues need to be resolved with regard to large-sized bonding between AuIC and A5083 alloys by the hot isostatic pressing process. We investigated this process in terms of the surface conditions, sizes, and heat capacities of large AuIC alloys. We also show a successful implementation of an AuIC decoupler into a reflector assembly, resulting in a remarkable reduction of radioactivity by AuIC compared to AIC without sacrificing neutronic performance.

Journal Articles

Influence of the neutron transport tube on neutron resonance densitometry

Kitatani, Fumito; Tsuchiya, Harufumi; Koizumi, Mitsuo; Takamine, Jun; Hori, Junichi*; Sano, Tadafumi*

EPJ Web of Conferences, 146, p.09032_1 - 09032_3, 2017/09

 Times Cited Count:0 Percentile:100

Journal Articles

Effect of thermo-mechanical treatments on nano-structure of 9Cr-ODS steel

Oka, Hiroshi; Tanno, Takashi; Otsuka, Satoshi; Yano, Yasuhide; Uwaba, Tomoyuki; Kaito, Takeji; Onuma, Masato*

Nuclear Materials and Energy (Internet), 9, p.346 - 352, 2016/12

 Times Cited Count:10 Percentile:18.31(Nuclear Science & Technology)

Journal Articles

Novel neutron scattering techniques using neutron transmission spectra

Oba, Yojiro*; Morooka, Satoshi; Sato, Hirotaka*; Sato, Nobuhiro*; Inoue, Rintaro*; Sugiyama, Masaaki*

Hamon, 26(4), p.170 - 173, 2016/11

Journal Articles

Magnetic scattering in the simultaneous measurement of small-angle neutron scattering and Bragg edge transmission from steel

Oba, Yojiro*; Morooka, Satoshi; Oishi, Kazuki*; Sato, Nobuhiro*; Inoue, Rintaro*; Adachi, Nozomu*; Suzuki, Junichi*; Tsuchiyama, Toshihiro*; Gilbert, E. P.*; Sugiyama, Masaaki*

Journal of Applied Crystallography, 49(5), p.1659 - 1664, 2016/10

 Times Cited Count:7 Percentile:38.97(Chemistry, Multidisciplinary)

Journal Articles

Journal Articles

Generalized analysis method for neutron resonance transmission analysis

Harada, Hideo; Kimura, Atsushi; Kitatani, Fumito; Koizumi, Mitsuo; Tsuchiya, Harufumi; Becker, B.*; Kopecky, S.*; Schillebeeckx, P.*

Journal of Nuclear Science and Technology, 52(6), p.837 - 843, 2015/06

 Times Cited Count:4 Percentile:54.36(Nuclear Science & Technology)

Journal Articles

JAEA-ISCN development programs of advanced NDA technologies of nuclear material

Seya, Michio; Kobayashi, Naoki; Naoi, Yosuke; Hajima, Ryoichi; Soyama, Kazuhiko; Kureta, Masatoshi; Nakamura, Hironobu; Harada, Hideo

Book of Abstracts, Presentations and Papers of Symposium on International Safeguards; Linking Strategy, Implementation and People (Internet), 8 Pages, 2015/03

JAEA-ISCN has been implementing basic development programs of the advanced NDA technologies for nuclear material (NM) since 2011JFY (Japanese Fiscal Year), which are (1) NRF (Nuclear resonance fluorescence) NDA technology using laser Compton scattered (LCS) $$gamma$$-rays (intense mono-energetic $$gamma$$-rays), (2) Alternative to $$^{3}$$He neutron detection technology using ZnS/B$$_{2}$$O$$_{3}$$ ceramic scintillator, and (3) NRD (Neutron resonance densitometry) using NRTA (Neutron resonance transmission analysis) and NRCA (Neutron resonance capture analysis). These programs are going to be finished in 2014JFY and have demonstration tests in February - March 2015.

Journal Articles

Development of a dc 1MV power supply technology for NB injectors

Watanabe, Kazuhiro; Kashiwagi, Mieko; Kawashima, Shuichi*; Ono, Yoichi*; Yamashita, Yasuo*; Yamazaki, Choji*; Hanada, Masaya; Inoue, Takashi; Taniguchi, Masaki; Okumura, Yoshikazu; et al.

Nuclear Fusion, 46(6), p.S332 - S339, 2006/06

 Times Cited Count:22 Percentile:36.5(Physics, Fluids & Plasmas)

no abstracts in English

Journal Articles

Temperature dependence of the transmission loss in KU-1 and KS-4V quartz glasses for the ITER diagnostic window

Nishitani, Takeo; Sugie, Tatsuo; Morishita, Norio; Yokoo, Noriko*

Fusion Engineering and Design, 74(1-4), p.871 - 874, 2005/11

 Times Cited Count:13 Percentile:30.82(Nuclear Science & Technology)

no abstracts in English

JAEA Reports

Standard of radiation monitor based on LAN and PLC technology for J-PARC

Miyamoto, Yukihiro; Sakamaki, Tsuyoshi*; Maekawa, Osamu*; Nakashima, Hiroshi

JAERI-Tech 2004-054, 72 Pages, 2004/08

JAERI-Tech-2004-054.pdf:7.3MB

A standard is provided for the radiation monitor based on LAN (Local Area Network) and PLC (Programmable Logic Controller) technology at the introduction to the Japan Proton Accelerator Research Complex (J-PARC). The monitor consists of radiation measurement equipments and the central monitoring panel. The formers are installed in the radiation field, and the latter is installed in the control room and composed of PLC, which are connected with LAN. Extension of the existing standard and the conformity to the international standard were thought as important in providing the standard. The standard is expected to improve the compatibility, maintenancability and productivity of the components.

JAEA Reports

Experimental study on accelerator driven subcritical reactor, JAERI's nuclear research promotion program, H12-031 (Contract research)

Shiroya, Seiji*; Misawa, Tsuyoshi*; Unesaki, Hironobu*; Ichihara, Chihiro*; Kobayashi, Keiji*; Nakamura, Hiroshi*; Shin, Kazuo*; Imanishi, Nobutsugu*; Kanazawa, Satoshi*; Mori, Takamasa

JAERI-Tech 2004-025, 93 Pages, 2004/03

JAERI-Tech-2004-025.pdf:6.69MB

In view of the future plan of Research Reactor Institute, Kyoto University, the present study consisted of (1) the transmission experiments of high energy neutrons through materials, (2) experimental simulation of ADSR using the Kyoto University Critical Assembly(KUCA), and (3) conceptual neutronics design study on KUR type ADSR using the MCNP-X code. Through the present study, valuable knowledge on the basic nuclear characteristics of ADSR, which is indispensable to promote the study on ADSR, was obtained both theoretically and experimentally. For the realization of ADSR, it is considered to be necessary to accumulate results of research steadily. For this purpose, it is inevitable (1) to compile the more precise nuclear data for the wide energy range, (2) to establish experimental techniques for reactor physics study on ADSR including subcriticality measurement and absolute neutron flux measurement, and (3) to develop neutronics calculation tools which take into account the neutron generation process by the spallation reaction and the delayed neutron behavior.

Journal Articles

Neutron transmission experiment of boron-doped resin for the JT-60SC neutron shield using 2.45 MeV neutron source

Morioka, Atsuhiko; Sato, Satoshi; Ochiai, Kentaro; Sakasai, Akira; Hori, Junichi; Yamauchi, Michinori*; Nishitani, Takeo; Kaminaga, Atsushi; Masaki, Kei; Sakurai, Shinji; et al.

Journal of Nuclear Science and Technology, 41(Suppl.4), p.109 - 112, 2004/03

Neutron shielding material of the port section of JT-60 superconducting modification (JT-60SC) serves as a design which used resin (KRAFTON-HB4) excellent in the temperature characteristic from polyethylene. In order to make port weight mitigate and reduce the nuclear heating of the superconducting coil, we were developed the resin which added natural BORON to resin. The 2.45MeV neutron generated in the D-D reaction was irradiated, the penetration of the neutron was measured in some kinds of samples which changed the amount of BORON, and the shielding performance of the resin containing BORON was compared with them. The penetration rates of fast neutron flux do not depend on the doped density of boron in both measurements. Whereas the penetration rates of thermal neutron flux in the resin with 2 wt% B are about 25% lower than those with 1 wt% at the back surface of the test specimens.

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