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Journal Articles

Estimation of $$Delta$$${it R}$/${it R}$ values by benchmark study of the M$"o$ssbauer Isomer shifts for Ru, Os complexes using relativistic DFT calculations

Kaneko, Masashi; Yasuhara, Hiroki*; Miyashita, Sunao*; Nakashima, Satoru*

Hyperfine Interactions, 238(1), p.36_1 - 36_9, 2017/11

AA2016-0447.pdf:0.46MB

 Times Cited Count:2 Percentile:77.36(Physics, Atomic, Molecular & Chemical)

We aim to evaluate the validity of density functional calculations to the bonding property for Ru and Os complexes. We performed the benchmarking of theoretical computational method with $$^{99}$$Ru, $$^{189}$$Os M$"o$ssbauer isomer shifts. As the result, the computational values of the electron densities at nucleus position correlated with the experimental M$"o$ssbauer isomer shifts.

Journal Articles

Development of a short-term emergency assessment system of the marine environmental radioactivity around Japan

Kobayashi, Takuya; Kawamura, Hideyuki; Fujii, Katsuji*; Kamidaira, Yuki

Journal of Nuclear Science and Technology, 54(5), p.609 - 616, 2017/05

 Times Cited Count:10 Percentile:69.28(Nuclear Science & Technology)

The Japan Atomic Energy Agency has, for many years, been developing a radionuclide dispersion model for the ocean, and has validated the model through application in many sea areas using oceanic flow fields calculated by the ocean model. The Fukushima Dai-ichi Nuclear Power Station accident caused marine pollution by artificial radioactive materials to the North Pacific, especially to coastal waters northeast of mainland Japan. In order to investigate the migration of radionuclides in the ocean caused by this severe accident, studies using marine dispersion simulations have been carried out by JAEA. Based on these as well as the previous studies, JAEA has developed the Short-Term Emergency Assessment system of Marine Environmental Radioactivity (STEAMER) to immediately predict the radionuclide concentration around Japan in case of a nuclear accident.

Journal Articles

Oxidation and reduction behaviors of a prototypic MgO-PuO$$_{2-x}$$ inert matrix fuel

Miwa, Shuhei; Osaka, Masahiko

Journal of Nuclear Materials, 487, p.1 - 4, 2017/04

 Times Cited Count:4 Percentile:37.06(Materials Science, Multidisciplinary)

Oxidation and reduction behaviors of prototypic MgO-based inert matrix fuels (IMFs) containing PuO$$_{2-x}$$ were experimentally investigated by means of thermogravimetry. The oxidation and reduction kinetics of the MgO-PuO$$_{2-x}$$ specimen were determined. The oxidation and reduction rates of the MgO-PuO$$_{2-x}$$ were found to be low compared with those of PuO$$_{2-x}$$. It is note that the changes in O/Pu ratios of MgO-PuO$$_{2-x}$$ from stoichiometry were smaller than those of PuO$$_{2-x}$$ at high oxygen partial pressure. From these results, it can be said that MgO matrix lower the oxygen supply and release of PuO$$_{2-x}$$, which is preferable as the minor actinides incineration devices, since the high oxygen potentials of minor actinide oxides can cause certain problems in terms of thermochemical aspects such as enlarged cladding inner-surface corrosion.

Journal Articles

Magnetic structure and quadrupolar order parameter driven by geometrical frustration effect in NdB$$_4$$

Yamauchi, Hiroki; Metoki, Naoto; Watanuki, Ryuta*; Suzuki, Kazuya*; Fukazawa, Hiroshi; Chi, S.*; Fernandez-Baca, J. A.*

Journal of the Physical Society of Japan, 86(4), p.044705_1 - 044705_9, 2017/04

 Times Cited Count:13 Percentile:64.28(Physics, Multidisciplinary)

Neutron diffraction experiments have been carried out to characterize the magnetic structures and order parameters in an intermediate phase of NdB$$_4$$ showing the successive phase transitions at $$T_{rm 0} = 17.2$$ K, $$T_{rm N1} = 7.0$$ K, and $$T_{rm N2} = 4.8$$ K. The observed patterns in phase II ($$T_{rm N1} < T < T_{rm 0}$$) are successfully explained by postulating a planar structure with static magnetic moments in the tetragonal $$ab$$-plane. We have found that the magnetic structure in phase II can be uniquely determined to be a linear combination of noncolinear "all-in/all-out"-type and "vortex"-type antiferromagnetic structures. We propose that the quadrupolar interaction holds the key to stabilizing the noncollinear magnetic structure and quadrupolar order. Here, the frustration in the Shastry - Sutherland lattice would play an essential role in suppressing the dominance of the magnetic interaction.

Journal Articles

Absence of a polar phase in perovskite chromite $$R$$CrO$$_{3}$$ ($$R$$=La and Pr)

Yoshii, Kenji; Ikeda, Naoshi*; Shimojo, Yutaka; Ishii, Yoshinobu*

Materials Chemistry and Physics, 190, p.96 - 101, 2017/04

 Times Cited Count:15 Percentile:48.52(Materials Science, Multidisciplinary)

Magnetic and dielectric properties have been studied for LaCrO$$_{3}$$, PrCrO$$_{3}$$, and their solid solution La$$_{0.5}$$Pr$$_{0.5}$$CrO$$_{3}$$, belonging to a family of ferroelectricorthochromite series $${it R}$$CrO$$_{3}$$ ($${it R}$$: rare earths). The magnetic measurements confirm that the material shows canted antiferromagnetic ordering at 240-288 K. Neutron diffraction patterns could be fitted with the centrosymmetric $${it Pnma}$$, which is different from the non-centrosymmetric structure proposed for the ferroelectric phase of NdCrO$$_{3}$$. The large dielectric constants are likely due to the hopping of charge carriers as proposed previously for other chromites.

Journal Articles

Influence of mesh non-orthogonality on numerical simulation of buoyant jet flows

Ishigaki, Masahiro; Abe, Satoshi; Shibamoto, Yasuteru; Yonomoto, Taisuke

Nuclear Engineering and Design, 314, p.326 - 337, 2017/04

AA2016-0575.pdf:1.57MB

 Times Cited Count:8 Percentile:56.89(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Intruder configurations in the ground state of $$^{30}$$Ne

Liu, H. N.*; Lee, J.*; Doornenbal, P.*; Scheit, H.*; Takeuchi, Satoshi*; Aoi, Nori*; Li, K. A.*; Matsushita, Masafumi*; Steppenbeck, D.*; Wang, H.*; et al.

Physics Letters B, 767, p.58 - 62, 2017/04

AA2016-0554.pdf:0.67MB

 Times Cited Count:20 Percentile:83.48(Astronomy & Astrophysics)

no abstracts in English

Journal Articles

Selective extraction of Pt(IV) over Fe(III) from HCl with an amide-containing tertiary amine compound

Maeda, Motoki*; Narita, Hirokazu*; Tokoro, Chiharu*; Tanaka, Mikiya*; Motokawa, Ryuhei; Shiwaku, Hideaki; Yaita, Tsuyoshi

Separation and Purification Technology, 177, p.176 - 181, 2017/04

 Times Cited Count:21 Percentile:58.79(Engineering, Chemical)

Journal Articles

Analysis of plutonium isotope ratios including $$^{238}$$Pu/$$^{239}$$Pu in individual U-Pu mixed oxide particles by means of a combination of alpha spectrometry and ICP-MS

Esaka, Fumitaka; Yasuda, Kenichiro; Suzuki, Daisuke; Miyamoto, Yutaka; Magara, Masaaki

Talanta, 165, p.122 - 127, 2017/04

 Times Cited Count:15 Percentile:52.34(Chemistry, Analytical)

The isotope ratios of $$^{238}$$Pu/$$^{239}$$Pu, $$^{240}$$Pu/$$^{239}$$Pu, $$^{241}$$Pu/$$^{239}$$Pu, and $$^{242}$$Pu/$$^{239}$$Pu were measured for individual Pu and U-Pu mixed oxide particles by a combination of alpha spectrometry and inductively coupled plasma mass spectrometry (ICP-MS). As a consequence, we were able to determine the $$^{240}$$Pu/$$^{239}$$Pu, $$^{241}$$Pu/$$^{239}$$Pu, and $$^{242}$$Pu/$$^{239}$$Pu isotope ratios with ICP-MS after particle dissolution and chemical separation of uranium, plutonium and americium with UTEVA resins. Furthermore, $$^{238}$$Pu/$$^{239}$$Pu isotope ratios were able to be calculated by using both the $$^{238}$$Pu/($$^{239}$$Pu+$$^{240}$$Pu) activity ratios that had been measured through alpha spectrometry and the $$^{240}$$Pu/$$^{239}$$Pu isotope ratios determined through ICP-MS. Therefore, the combined use of alpha spectrometry and ICP-MS is useful in determining plutonium isotope ratios, including $$^{238}$$Pu/$$^{239}$$Pu, in individual U-Pu mixed oxide particles.

Journal Articles

Development of fuel temperature calculation code for HTGRs

Inaba, Yoshitomo; Nishihara, Tetsuo

Annals of Nuclear Energy, 101, p.383 - 389, 2017/03

 Times Cited Count:7 Percentile:56.89(Nuclear Science & Technology)

In order to ensure the thermal integrity of fuel in High Temperature Gas-cooled Reactors (HTGRs), it is necessary that the maximum fuel temperature in normal operation is to be lower than a thermal design target. In the core thermal-hydraulic design of block-type HTGRs, the maximum fuel temperature should be evaluated considering data such as thermal power, core geometry, power density and neutron fluence distributions, and core coolant flow distribution. The fuel temperature calculation code used in the design stage of the High Temperature engineering Test Reactor (HTTR) presupposes to run on UNIX systems, and its operation and execution procedure are complicated and are not user-friendly. Therefore, a new fuel temperature calculation code named FTCC which has a user-friendly system such as a simple and easy operation and execution procedure, was developed. This paper describes calculation objects and models, basic equations, improvement points from the HTTR design code in FTCC, and the result of a validation calculation with FTCC. The calculation result obtained by FTCC provides good agreement with that of the HTTR design code, and then FTCC will be used as one of the design codes for HTGRs. In addition, the effect of cooling forms on the maximum fuel temperature is investigated by using FTCC. As a result, it was found that the effect of center hole cooling for hollow fuel compacts and gapless cooling with monolithic type fuel rods on reducing the temperature is very high.

Journal Articles

Effect of flavin compounds on uranium(VI) reduction- kinetic study using electrochemical methods with UV-vis spectroscopy

Yamasaki, Shinya*; Tanaka, Kazuya; Kozai, Naofumi; Onuki, Toshihiko

Applied Geochemistry, 78, p.279 - 286, 2017/03

 Times Cited Count:4 Percentile:18.68(Geochemistry & Geophysics)

This study examined the rate constant for the U(VI) reduction process by three flavin analogues, which are redox-active biomolecules secreted from anaerobic bacteria, to elucidate their substituent group effect on the U(VI) reduction rate by electrochemical methods. The formation of the U(IV) was monitored by UV-vis spectrometry in the presence of the flavins. The rate constant for the U(VI) reduction by the flavins was determined. The apparent reduction potential of U(VI) increased about 0.2 V in the presence of the mediators, which strongly suggests that the biological electron mediator makes the U(VI) reduction possible even under more oxidative conditions.

Journal Articles

Reaction path and product analysis of sodium-water chemical reactions using laser diagnostics

Deguchi, Yoshihiro*; Muranaka, Ryota*; Kamimoto, Takahiro*; Takagi, Taku*; Kikuchi, Shin; Kurihara, Akikazu

Applied Thermal Engineering, 114, p.1319 - 1324, 2017/03

 Times Cited Count:2 Percentile:12.87(Thermodynamics)

The purpose of this study aims to clarify the gas phase sodium-water reaction path and reaction products quantitatively. The counter-flow diffusion experiment device was employed to analyze the reaction path and reaction products using laser diagnostics. The main product of sodium-water reaction was determined to be NaOH and the sodium oxide was not notably measured compared with NaOH.

Journal Articles

Development of the Eulerian atmospheric transport model GEARN-FDM; Validation against the European tracer experiment

Kadowaki, Masanao; Katata, Genki; Terada, Hiroaki; Nagai, Haruyasu

Atmospheric Pollution Research, 8(2), p.394 - 402, 2017/03

 Times Cited Count:2 Percentile:6.87(Environmental Sciences)

We developed a dispersion model based on the finite difference method, GEARN-FDM, for long-range dispersion, which solves the advection-diffusion equation using numerical schemes with low artificial diffusion. The advection and diffusion terms are modeled using a fully mass conservative scheme and the Crank-Nicolson method, respectively. GEARN-FDM was validated using the dataset from the European Tracer Experiment. In the entire domain throughout the simulation period of the observed dataset, GEARN-FDM showed high performance with factors of 2 and 5 of 39% and 78%, respectively. While testing the sensitivity of the horizontal diffusivity with this model, the simulated horizontal diffusivity was distributed heterogeneously in the model domain. High diffusivity was primarily seen over the coastal and mountainous regions. Therefore, for the long-range simulations of radionuclides, we need to consider to the transport caused by horizontal diffusion.

Journal Articles

Preparation of Sr adsorptive fiber by impregnating with crown ether derivative for $$^{90}$$Sr measurement

Horita, Takuma; Asai, Shiho; Konda, Miki; Hanzawa, Yukiko; Saito, Kyoichi*; Fujiwara, Kunio*; Sugo, Takanobu*; Kitatsuji, Yoshihiro

Bunseki Kagaku, 66(3), p.189 - 193, 2017/03

 Times Cited Count:1 Percentile:3.41(Chemistry, Analytical)

A Sr-selective adsorption fiber was prepared for rapid analysis of $$^{90}$$Sr content by using radiation-induced emulsion graft polymerization and subsequent chemical modification. A polyethylene fiber with a diameter of 13 $$mu$$m was first immersed in a methanol solution of an epoxy-group-containing vinyl monomer, glycidyl methacrylate (GMA), and polyoxyethylene sorbitol ester (Tween20) as a surfactant for graft-polymerization of GMA. Octadecylamine was then bound to a polymer chain extending from the fiber surface providing hydrophobicity to the polymer chain. Dicyclohexano-18-crown-6 (DCH18C6) was finally impregnated onto the polymer chain via a hydrophobic interaction between the octadecyl moiety of the polymer chain and the cyclohexyl moiety of DCH18C6. The fiber surface structure, characterized by DCH18C6 molecules loosely entangled with polymer chains, afforded realizes the rapid and selective adsorption of Sr ions with an adsorption rate approximately 100 times higher than that of a commercially available Sr-selective resin (Sr Resin).

Journal Articles

Ionization of protoplanetary disks by galactic cosmic rays, solar protons, and supernova remnants

Kataoka, Ryuho*; Sato, Tatsuhiko

Geoscience Frontiers, 8(2), p.247 - 252, 2017/03

 Times Cited Count:5 Percentile:14.09(Geosciences, Multidisciplinary)

Estimation of the depth-dose profile of ionization in protoplanetary disks by galactic cosmic rays (GCRs), solar protons, and by supernova remnants is of great importance in the analysis of planet formation. We therefore calculated the profile using Particle and Heavy Ion Transport code System PHITS. The attenuation length of GCR ionization is updated as 118 g cm$$^{-2}$$, which is approximately 20% larger than the popular value. Hard and soft possible spectra of solar protons give 5% larger and 20% smaller attenuation lengths compared with those from standard GCR spectra, respectively. Further, all of the attenuation lengths become 10% larger in the compound gas of cosmic abundance, e.g. 128 g cm$$^{-2}$$ for GCRs, which can significantly affect the minimum estimate of the size of dead zones in protoplanetary disks.

Journal Articles

Molecular dynamics simulations of cesium adsorption on illite nanoparticles

Lammers, L.*; Bourg, I. C.*; Okumura, Masahiko; Kolluri, K.*; Sposito, G.*; Machida, Masahiko

Journal of Colloid and Interface Science, 490, p.608 - 620, 2017/03

 Times Cited Count:107 Percentile:93.33(Chemistry, Physical)

no abstracts in English

Journal Articles

Monte Carlo criticality analysis under material distribution uncertainty

Ueki, Taro

Journal of Nuclear Science and Technology, 54(3), p.267 - 279, 2017/03

 Times Cited Count:8 Percentile:61.27(Nuclear Science & Technology)

Analysis framework under material distribution uncertainty is investigated for the Monte Carlo (MC) criticality calculation of continuously mixed media formed via molten core concrete interaction. Deterministic trigonometric functions and randomized Weierstrass functions are utilized to represent the spatially continuous variation. Numerical results indicate that the effective multiplication factor (k$$_{rm eff}$$) under random spatial variation can depart significantly from the k$$_{rm eff}$$ of a reference uniform medium. It is also shown that the deterministic modeling provides an upper-bound measure for extreme results from random realizations.

Journal Articles

Swelling pressure and leaching behaviors of synthetic bituminized waste products with various salt contents under a constant-volume condition

Irisawa, Keita; Meguro, Yoshihiro

Journal of Nuclear Science and Technology, 54(3), p.365 - 372, 2017/03

 Times Cited Count:2 Percentile:19.65(Nuclear Science & Technology)

Journal Articles

Determination of dissolved natural thorium and uranium in Horonobe and Mizunami Underground Research Laboratory groundwater and its thermodynamic analysis

Sasaki, Takayuki*; Kokami, Takayuki*; Kobayashi, Taishi*; Kirishima, Akira*; Murakami, Hiroaki; Amano, Yuki; Mizuno, Takashi; Iwatsuki, Teruki; Sasamoto, Hiroshi; Miyakawa, Kazuya

Journal of Nuclear Science and Technology, 54(3), p.373 - 381, 2017/03

Trace amounts of natural thorium and uranium in deep groundwater were investigated at two underground research laboratories situated at Horonobe and Mizunami, Japan. The groundwater was sampled from underground boreholes, and the colloid contribution was checked by in situ two size-fractionated ultrafiltration systems. A decrease in the concentration after in situ filtration suggested the presence of natural colloids and suspended matter that were carriers of a portion of the elements. The result of the Th and U concentrations in groundwater after 10 kDa filtration was analyzed thermodynamically using existing hydrogeological and geochemical data such as the mineral components in the groundwater at a given pH, ionic strength, concentration of co-existing ions, redox potential, and solid phase assumed. A crystalline solid phase made the solubility very low compared with that of the amorphous phase, and the solubility agreed well with the concentrations measured.

Journal Articles

Development of methods for recovering uranium from sludge-like uranium generated in decontamination of metal wastes

Ohashi, Yusuke; Tanaka, Yoshio; Tsunashima, Yasumichi; Ikeda, Yasuhisa*

Journal of Nuclear Science and Technology, 54(3), p.382 - 390, 2017/03

 Times Cited Count:9 Percentile:61.27(Nuclear Science & Technology)

Sludge-like uranium wastes (SUWs) have been generated with neutralization of acidic aqueous solutions used for decontamination of metal wastes containing a large amount of iron. We have examined the method for recovering uranium from such SUWs using ${{it N-cyclohexyl}}$-2-pyrrolidone (NCP) as a precipitate. As a result, it was found that precipitation ratios (PRs) of uranium in the solutions prepared by dissolving SUWs in HNO$$_{3}$$ is 97.7% at [NCP]/[U(VI)] = 20, and that the PRs of iron, aluminum, fluorine, and sulfate species are less than 1%. This indicates that uranium species are precipitated selectively. The content ratios of U, Fe, Ca, F, and S in the materials after calcining precipitates obtained at [NCP]/[U(VI)] = 20 were in accordance with the conditions of uranium ore concentrate. From these results, it is expected that highly purified uranium can be efficiently recovered from SUWs by using NCP as the precipitant.

Journal Articles

Separation of Zr in the rubble waste generated at the Fukushima Daiichi Nuclear Power Station

Shimada, Asako; Kameo, Yutaka

Journal of Radioanalytical and Nuclear Chemistry, 311(3), p.1613 - 1618, 2017/03

AA2016-0191.pdf:0.23MB

 Times Cited Count:2 Percentile:19.65(Chemistry, Analytical)

Separation method of Zr using trans uranium resin (TRU resin) was developed. Approximately 100% of Zr, Nb, Bi, Th, and U and a part of Mo and Hg were extracted on the TRU resin from 3 M HNO $$_{3}$$ solution and separated from Li, Be, Mg, Al, Ca, V, Cr, Mn, Fe, Co, Ni, Cu, Zn, Ga, As, Se, Rb, Sr,Ag, Cd, In, Cs, Ba. Approximately 100% of Zr, Nb, and U were striped from the TRU resin with 0.01 M HF and 10% of Mo, 7.1% of Hg, 77% of Bi, and 20% of Th were also included in the stripping solution. In order to measure $$^{93}$$Zr with inductively coupled plasma mass spectrometry (ICP-MS), Zr has to be separated from Nb and Mo to avoid isobaric interference. Therefore, further purification of Zr using tetra valent actinide resin (TEVA resin) was applied. The developed method was evaluated with the simulated rubble sample solution. Although a part of Zr was eluted during sample loading, most of Zr was extracted on the TRU resin and separated major elements of the rubble sample. Finally, Zr was separated from Nb and Mo with the TEVA resin.

Journal Articles

Neutron powder diffraction study on the magnetic structure of NdPd$$_5$$Al$$_2$$

Metoki, Naoto; Yamauchi, Hiroki; Kitazawa, Hideaki*; Suzuki, Hiroyuki*; Hagihara, Masato*; Frontzek, M. D.*; Matsuda, Masaaki*; Fernandez-Baca, J. A.*

Journal of the Physical Society of Japan, 86(3), p.034710_1 - 034710_5, 2017/03

 Times Cited Count:9 Percentile:56.98(Physics, Multidisciplinary)

Magnetic structure of NdPd$$_5$$Al$$_2$$ has been studied by means of neutron powder diffraction. We observed remarkable magnetic reflections with the modulation vector $$q$$= (1/2 0 0) below the ordering temperature $$T_{rm N}$$ = 1.2 K. We found a collinear magnetic structure of Nd moment of 2.9(1) $${mu}_{rm B}$$ at 0.3 K parallel to the $$c$$-axis, where the ferromagnetically ordered $$a$$ planes stack with four Nd layer period of ++-- sequence along the $$a$$ direction with the distance between adjuscent Nd layers to be $$a/2$$. This is very similar to CePd$$_5$$Al$$_2$$ with $$q$$ = (0.23 0.23 0) and the Ce moment parallel to the $$c$$-axis. These structures with in-plane modulation $$q_{|}$$ is a consequence of the two dimensional nature of fermi surface topology in this family, coming from unique crystal structure with very long tetragonal unit cell and large distance $$>$$ 7${AA}$ between the rare earth layers separated by Al and two Pd layers.

Journal Articles

Development of multi-colored neutron talbot-lau interferometer with absorption grating fabricated by imprinting method of metallic glass

Seki, Yoshichika; Shinohara, Takenao; Parker, J. D.*; Yashiro, Wataru*; Momose, Atsushi*; Kato, Kosuke*; Kato, Hidemi*; Sadeghilaridjani, M.*; Otake, Yoshie*; Kiyanagi, Yoshiaki*

Journal of the Physical Society of Japan, 86(4), p.044001_1 - 044001_5, 2017/03

 Times Cited Count:13 Percentile:66.28(Physics, Multidisciplinary)

For the effective phase imaging at pulsed neutron sources, we have designed and developed the multi-colored Talbot-Lau interferometer which works at several wavelengths. At the Energy Resolved Neutron Imaging System RADEN in J-PARC, we demonstrated its operation by observing the visibilities of moire fringes derived from different wavelengths (0.25, 0.50, and 0.75 nm). We also investigated the variation of moire fringes dependent on the wavelength resolution from 18% to 50% and showed the advantage of pulsed beams. At the central wavelength of 0.5 nm, we have succeeded in interferometric imaging for the samples of metal rods made of aluminum, lead, and copper. An absorption grating as an analyzer was fabricated by imprinting of metallic glass for the first time, and showed a clear moire fringe with the high visibility of 68% and a well-controlled shape in comparison with previous ones fabricated by oblique evaporation of gadolinium.

Journal Articles

Evaluation of influence of splay fault growth on groundwater flow around geological disposal system

Takai, Shizuka; Takeda, Seiji; Sakai, Ryutaro*; Shimada, Taro; Munakata, Masahiro; Tanaka, Tadao

Nihon Genshiryoku Gakkai Wabun Rombunshi, 16(1), p.34 - 48, 2017/03

In geological disposal, direct effect on geological repositories by active faults is avoided at a stage of site characterization; however, uncertainty remains for avoidance of faults derived from the active faults, which are concealed deep under the ground and difficult to detect in advance. In this research, the influence of growth of undetected splay faults on natural barrier in a geological disposal system, which will caused by attack of the faults in the future, was evaluated. We investigated examples of splay faults in Japan and set conditions for growth of splay faults. Furthermore, we assumed a disposal site composed of sedimentary rocks and made a hydrogeological model of growth of splay faults. We carried out groundwater flow analyses, changing parameters such as location and depth of repository and growth velocity of splay faults. The results indicate that main flow path from the repository is changed into upward flow along the splay fault due to its growth and the average velocity to the ground surface becomes one or two orders of magnitude higher than that before its growth. The results also suggest that the splay fault growth leads into the possibility of downward flow of oxidizing groundwater from ground surface area.

Journal Articles

Development of a method of safety assessment for geological disposal considering long-term evolution of geological and topographical environment by uplift and erosion

Wakasugi, Keiichiro; Yamaguchi, Masaaki; Koo, Shigeru*; Nagao, Fumiya; Kato, Tomoko; Suzuki, Yuji*; Ebashi, Takeshi; Umeki, Hiroyuki*; Niibori, Yuichi*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 16(1), p.15 - 33, 2017/03

This study provides a method of safety assessment for the geological disposal of HLW to evaluate the effects of uplift and erosion which are widespread phenomena identified on regional and global scales, and are more or less difficult to avoid in Japan. This method enables to deal with different uplift rate and erosion rate, and to evaluate repository depth, the time required for a repository to reach the weathered zone and surface of the ground, and the number of waste packages eroded as a function of time by using a landform evolution model. Based on trial analysis, the result shows that the maximum dose in the Base Case (uplift rate: 0.3 mm/y) is less than the targeted criterion suggested by the international organization even if the repository reaches the ground surface. Furthermore, the diversifying effect on timing the waste packages to reach to weathered zone due to heterogeneity on altitude of bottom of weathered zone reduces one order magnitude of result of the existed dose assessment. The new method is applicable to evaluate safety of geological disposal based on realistic phenomena of uplift and erosion and to quantify a safety margin and robustness of the disposal system.

Journal Articles

Prospects for researches on environmental and health effects of the Fukushima Dai-ichi NPP accident

Hirouchi, Jun; Okura, Takehisa; Satoh, Daiki

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 59(3), p.152 - 155, 2017/03

no abstracts in English

Journal Articles

Research and development of probabilistic risk assessment methodology for combination event of low temperature and snow

Nishino, Hiroyuki; Yamano, Hidemasa; Kurisaka, Kenichi

Nihon Kikai Gakkai Rombunshu (Internet), 83(847), p.16-00392_1 - 16-00392_13, 2017/03

Journal Articles

Applicability of the two-angle differential method to response measurement of neutron-sensitive devices at the RCNP high-energy neutron facility

Masuda, Akihiko*; Matsumoto, Tetsuro*; Iwamoto, Yosuke; Hagiwara, Masayuki*; Satoh, Daiki; Sato, Tatsuhiko; Iwase, Hiroshi*; Yashima, Hiroshi*; Nakane, Yoshihiro; Nishiyama, Jun*; et al.

Nuclear Instruments and Methods in Physics Research A, 849, p.94 - 101, 2017/03

 Times Cited Count:1 Percentile:10.62(Instruments & Instrumentation)

Quasi-monoenergetic high-energy neutron fields induced by $$^{7}$$Li(p,n) reactions are used for the response evaluation of neutron-sensitive devices. The quasi-monoenergetic high-energy field consists of high-energy monoenergetic peak neutrons and unwanted continuum neutrons down to the low-energy region. A two-angle differential method has been developed to compensate for the effect of the continuum neutrons in the response measurements. In this study, the two-angle differential method was demonstrated for Bonner sphere detectors, which are typical examples of moderator-based neutron-sensitive detectors, to investigate the method's applicability and its dependence on detector characteristics. Through this study, the adequacy of the two-angle differential method was experimentally verified, and practical suggestions were made pertaining to this method.

Journal Articles

Gas retention behavior of carbonate slurry under $$gamma$$-ray irradiation

Motooka, Takafumi; Nagaishi, Ryuji; Yamagishi, Isao

QST-M-2; QST Takasaki Annual Report 2015, P. 95, 2017/03

We conducted $$gamma$$ ray irradiation test using simulated carbonate slurry to investigate the cause of stagnant water over the high integrity container (HIC). This test was performed at Co-60 irradiation facility in Takasaki Advanced Radiation Research Institute. We observed a rise in water level, air bubbles in the slurry, a supernatant when the carbonate slurry with 95 g/L density was irradiated by $$gamma$$ ray at a dose rate of 8.5 kGy/h. The cause of the rise in water level was regarded as the volume expansion by the gas retention of the carbonate slurry. It was suggested that the cause of stagnant water over the high integrity container might be the volume expansion by the gas retention.

Journal Articles

Degradation behavior of surface-mounted LED by $$gamma$$ irradiation

Takeuchi, Tomoaki; Otsuka, Noriaki; Uehara, Toshiaki; Kumahara, Hajime*; Tsuchiya, Kunihiko

QST-M-2; QST Takasaki Annual Report 2015, P. 80, 2017/03

no abstracts in English

Journal Articles

Effect of twin boundary on crack propagation behavior in magnesium binary alloys; Experimental and calculation studies

Somekawa, Hidetoshi*; Tsuru, Tomohito

Scripta Materialia, 130, p.114 - 118, 2017/03

 Times Cited Count:25 Percentile:74.12(Nanoscience & Nanotechnology)

The impact of alloying elements on crack propagation and atomistic phenomenon at {10$$bar{1}$$2}-type twin boundaries in magnesium was investigated via both experiments and calculations. The alloying elements clearly affected crack propagation behavior. Cracks were difficult to propagate along matrix-deformation twinning interfaces in alloys that had high fracture toughness. In such magnesium alloys, the solute atoms, e.g., silver, manganese and zinc atoms, create adhesive interactions between magnesium atoms. Closed-shell and covalent-like bonding of these kinds of solute atoms would influence strong adhesion, which impedes the nucleation of a new surface at the twin boundary.

Journal Articles

Dynamic behavior of secondary electrons produced by a high-energy electron in liquid water

Kai, Takeshi; Yokoya, Akinari*; Fujii, Kentaro*; Watanabe, Ritsuko*

Yodenshi Kagaku, (8), p.11 - 17, 2017/03

It is thought to that the biological effects such as cell death or mutation are induced by complex DNA damage which are formed by several damage sites within a few nm. We calculated dynamic behavior of secondary electrons produced by primary electron and positon of high energy in water whose composition ratio is similar to biological context. The secondary electrons induce the ionization or electronic excitation near the parent cations. The decelerated electrons about 10% are distributed to their parent cations by the attractive Coulombic force. From the results, we predicted the following formation mechanism for the complex DNA damage. The electrons ejected from DNA could induce the ionization or the electronic excitation within the DNA. The electrons attracted by the Coulombic force are pre-hydrated in water layer of the DNA. The pre-hydrated electrons could induce to the DNA damage by dissociative electron transfer. As the results, the complex DNA damage with 1 nm could be formed by the interaction of not only the primary electron or positon but also the secondary electrons.

Journal Articles

Mechanism of Cs removal from Fukushima weathered biotite by heat treatment with a NaCl-CaCl$$_{2}$$ mixed salt

Honda, Mitsunori; Okamoto, Yoshihiro; Shimoyama, Iwao; Shiwaku, Hideaki; Suzuki, Shinichi; Yaita, Tsuyoshi

ACS Omega (Internet), 2(2), p.721 - 727, 2017/02

 Times Cited Count:19 Percentile:55.31(Chemistry, Multidisciplinary)

Journal Articles

Gyroscopic $$g$$ factor of rare earth metals

Ogata, Yudai; Chudo, Hiroyuki; Ono, Masao; Harii, Kazuya; Matsuo, Mamoru; Maekawa, Sadamichi; Saito, Eiji

Applied Physics Letters, 110(7), p.072409_1 - 072409_4, 2017/02

 Times Cited Count:19 Percentile:65.79(Physics, Applied)

Journal Articles

Development of rapid analytical method for radioactive samples by capillary electrophoresis with absorbance and fluorescence detection

Haraga, Tomoko

Bunseki Kagaku, 66(2), p.123 - 124, 2017/02

no abstracts in English

Journal Articles

Interaction of rare earth elements and components of the Horonobe deep groundwater

Kirishima, Akira*; Kuno, Atsushi*; Amamiya, Hiroki; Kubota, Takumi*; Kimuro, Shingo*; Amano, Yuki; Miyakawa, Kazuya; Iwatsuki, Teruki; Mizuno, Takashi; Sasaki, Takayuki*; et al.

Chemosphere, 168, p.798 - 806, 2017/02

 Times Cited Count:3 Percentile:10.21(Environmental Sciences)

For better understanding of the migration behavior of minor actinides (MA) in deep groundwater, the interaction of doped rare earth elements (REEs) and components in Horonobe deep groundwater was studied. Appx. 10 ppb of rare earth elements, i.e., Y, La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Er, Tm and Yb were doped to the sample groundwater collected from a packed sections in borehole drilled from 140 m depth experiment drift of Horonobe underground research laboratory (URL), Hokkaido, Japan. Then, that groundwater was sequentially filtrated by 0.2 micron pore filter, 10 kDa, 3 kDa and 1 kDa of nominal molecular weight limit (NMWL) ultrafilters by keeping inert condition. After that, the filtrate solutions were analyzed by ICP-MS to determine the concentrations of retained REEs at each filtration steps, while the used filters were analyzed by the neutron activation analysis (NAA) and TOF-SIMS element mapping to know the amount and chemical speciation of trapped fraction of the REEs on each filter. A remarkable relation between the retention ratios of REEs in the filtrate solutions and the ionic radius was observed, i.e., smaller rare earth element solves more in liquid phase under the Horonobe groundwater condition. NAA and TOF-SIMS analyses revealed that certain portions of REEs were trapped by 0.2 micron pore filters as rare earth phosphates which corresponded with the predicted predominant species by a chemical equilibrium calculation for the Horonobe groundwater condition, while small portions of colloidal REEs were trapped by 10 kDa and 3 kDa NMWL ultrafilters. The result suggested that phosphate anion plays an important role in the chemical behavior of REEs in saline (seawater based) groundwater, which could be referred for the prediction of migration behavior of trivalent actinide released from the repository of radioactive waste in far future.

Journal Articles

The Peak structure in the in-flight $$^{3}$$He$$(K^{-}, Lambda p) n$$ reaction around the $$bar{K} N N$$ Threshold

Sekihara, Takayasu; Oset, E.*; Ramos, A.*

JPS Conference Proceedings (Internet), 13, p.020002_1 - 020002_5, 2017/02

Journal Articles

Experimental investigation of the influence of Mo contained in stainless steel on Cs chemisorption behavior

Di Lemma, F. G.; Nakajima, Kunihisa; Yamashita, Shinichiro; Osaka, Masahiko

Journal of Nuclear Materials, 484, p.174 - 182, 2017/02

 Times Cited Count:22 Percentile:90.44(Materials Science, Multidisciplinary)

Chemisorption phenomena can affect fission products retention in the nuclear reactor vessel during a Severe Accident (SA). This paper will describe the influence of molybdenum contained in type 316 stainless steel (SS) on Cs chemisorption. Our experiments showed the formation of Cs-Mo compounds in addition to CsFeSiO$$_{4}$$, observed previously on SS304. The results of high temperature stability tests on the deposits are also presented. These tests aimed at simulating the revaporization of FP from structural materials during a SA. From our results, it can be inferred that Cs-Mo deposits may revaporize, contributing as a delayed source to the radioactive release.

Journal Articles

Evaluation of neutron nuclear data on platinum isotopes

Shibata, Keiichi

Journal of Nuclear Science and Technology, 54(2), p.147 - 157, 2017/02

 Times Cited Count:4 Percentile:37.06(Nuclear Science & Technology)

Neutron nuclear data on platinum isotopes have been evaluated for the next version of Japanese Evaluated Nuclear Data Library general-purpose file in the energy region from $$10^{-5}$$ eV to 20 MeV. Resolved resonance parameters of naturally-occurring isotopes were taken from the compilation work of Mughabghab. Unresolved resonance parameters were obtained by fitting to the total and capture cross sections calculated from nuclear models. A statistical model code CCONE was applied to evaluate cross sections above the resolved resonance region. Compound, pre-equilibrium and direct-reaction processes were considered for cross-section calculation. Coupled-channel optical model parameters were employed for the interaction between neutrons and nuclei. The present results reproduce experimental data very well, and are much better than the existing evaluations. The evaluated data are compiled into ENDF-formatted data files.

Journal Articles

Improvement of neutron startup source handling work by developing new transportation container for High-Temperature engineering Test Reactor (HTTR)

Shimazaki, Yosuke; Sawahata, Hiroaki; Shinohara, Masanori; Yanagida, Yoshinori; Kawamoto, Taiki; Takada, Shoji

Journal of Nuclear Science and Technology, 54(2), p.260 - 266, 2017/02

 Times Cited Count:2 Percentile:19.65(Nuclear Science & Technology)

The High-Temperature engineering Test Reactor (HTTR) has three neutron startup sources (NSs) in the reactor core, each of which consists of $$^{252}$$Cf with 3.7 GBq and is contained in a small capsule, installed in NS holder and subsequently in a control guide block (CR block). The NSs are exchanged at the interval of approximately 7 years. The NS holders are transported from the dealer's hot cell to the reactor facility of HTTR using a transportation container. The loading work of NS holders to the CR blocks is subsequently carried out in the fuel handling machine maintenance pit of HTTR. Technical issues, which are the reduction and prevention of radiation exposure of workers and the exclusion of falling of NS holder, were extracted from the experiences in past two exchange works of NSs to develop a safety handling procedure. Then, a new transportation container special to the NSs of HTTR was developed to solve the technical issues while keeping the cost as low as that for overhaul of conventional container. As the results, the NS handling work using the new transportation container was safely accomplished by developing the new transportation container which can reduce the risks of radiation exposure dose of workers and exclude the falling of NS holder.

Journal Articles

Cs-Te corrosion depth dependence on distribution of chromium carbide precipitation in high chromium steel

Sasaki, Koei; Fujimura, Ryota*; Tanigaki, Takanori; Matsubara, Masanori*; Fukumoto, Kenichi*; Uno, Masayoshi*

Journal of Nuclear Science and Technology, 54(2), p.139 - 146, 2017/02

AA2016-0211.pdf:2.83MB

 Times Cited Count:6 Percentile:51.46(Nuclear Science & Technology)

In an attempt to investigate Cs-Te corrosion depth dependence on distribution of chromium carbide precipitation in high chromium steel, Cs-Te corrosion out-pile tests of two 9Cr steels with different distributions of chromium carbide were carried out at 975K for 100h and their corrosion depths were compared. The corrosion is obviously more advanced in a specimen which has grain boundary carbide than in the one that does not. A considerable reason of the result is that the carbide distributed at grain boundaries promoted the corrosion reaction and the corrosion extended along the grain boundary. This is the first case in which the Cs-Te corrosion depth dependence on distribution of chromium carbide precipitation in Fe-Cr steel is clarified experimentally.

Journal Articles

Positron annihilation in the near surface of room temperature ionic liquids

Hirade, Tetsuya; O'Rourke, B. E.*; Kobayashi, Yoshinori*

Journal of Physics; Conference Series, 791(1), p.012029_1 - 012029_4, 2017/02

 Times Cited Count:2 Percentile:62.67(Physics, Multidisciplinary)

We tried to observe the positron annihilation rates near surface of (room temperature ionic liquids) IL's, such as N,N,N-trimethyl-N-propylammonium bis(trifluoromethanesulfonyl)imide (TMPA-TFSI) by use of the perpendicular slow positron beamline installed at AIST. The vaper pressure of TMPA-TFSI is very small and hence it is possible to measure the positron annihilation rate in vacuum chamber directly. This represents the first energy variable experimental results of the positron annihilation rate at the near surface of an IL. The triplet positronium annihilation rate seems to be larger at nearer region to the surface of the IL's.

Journal Articles

Structure of nitride layer formed on titanium alloy surface by N$$_{2}$$-gas exposure at high temperatures

Takeda, Yusuke; Iida, Kiyoshi*; Sato, Shinji*; Matsuo, Tadatoshi*; Nagashima, Yasuyuki*; Okubo, Nariaki; Kondo, Keietsu; Hirade, Tetsuya

Journal of Physics; Conference Series, 791(1), p.012022_1 - 012022_4, 2017/02

 Times Cited Count:1 Percentile:42.05(Physics, Multidisciplinary)

Titanium alloy is widely used for applications such as golf club heads and structural materials for aircrafts. The surface can be exceedingly hardened by nitriding treatment that initiates defects, but there are some difficulties on use of titanium nitride because the layer can be exfoliated by stress. Therefore, we prepared samples in two different treatment conditions, (1) 810$$^{circ}$$C 600 min and (2) 850$$^{circ}$$C 720 min and performed depth profile analysis of Doppler broadening of positron annihilation $$gamma$$-rays (DB) for these samples. According to a calculation of nitrogen diffusion depth, the nitride layer should be only about 0.05-0.1$$mu$$m. However, the depth profile analysis of the DB measurement indicated that the defects introduced by nitriding treatment extended to a depth of 0.5$$mu$$m.

Journal Articles

Research progress at the Slow Positron Facility in the Institute of Materials Structure Science, KEK

Hyodo, Toshio*; Wada, Ken*; Mochizuki, Izumi*; Kimura, Masao*; Toge, Nobukazu*; Shidara, Tetsuo*; Fukaya, Yuki; Maekawa, Masaki*; Kawasuso, Atsuo*; Iida, Shimpei*; et al.

Journal of Physics; Conference Series, 791(1), p.012003_1 - 012003_8, 2017/02

 Times Cited Count:3 Percentile:74.29(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Dissolved radiocaesium in seawater off the coast of Fukushima during 2013-2015

Fukuda, Miho*; Aono, Tatsuo*; Yamazaki, Shinnosuke*; Nishikawa, Jun*; Otosaka, Shigeyoshi; Ishimaru, Takashi*; Kanda, Jota*

Journal of Radioanalytical and Nuclear Chemistry, 311(2), p.1479 - 1484, 2017/02

 Times Cited Count:6 Percentile:51.46(Chemistry, Analytical)

In order to investigate processes affecting distribution of radiocaesium in seawater in the adjacent region of Fukushima Daiichi Nuclear Power Plant (FDNPP), relationships between $$^{137}$$Cs activity in seawater and physical properties of seawater (salinity, temperature, and potential density) were observed in seven stations within 10 km radius from the FDNPP. As a whole, $$^{137}$$Cs concentrations in seawater were higher in the vicinity of the FDNPP, and were negatively correlated with potential density. From these results, it can be considered that river water discharge or export of seawater from the FDNPP's harbor has affected the higher activity levels of $$^{137}$$Cs in seawater. It was also observed that the $$^{137}$$Cs-elevated seawater can be advected to the 20$$sim$$50 m depths.

Journal Articles

Algebraic design of multi-dimensional transfer function using transfer function synthesizer

Kawamura, Takuma; Idomura, Yasuhiro; Miyamura, Hiroko; Takemiya, Hiroshi

Journal of Visualization, 20(1), p.151 - 162, 2017/02

 Times Cited Count:3 Percentile:18.26(Computer Science, Interdisciplinary Applications)

In this paper, we propose a novel transfer function design interface for multivariate volume rendering. In the conventional multivariate volume rendering, GUI based transfer function design interfaces were limited to two-dimensional variables space. In order to design higher dimensional transfer functions in an interactive and intuitive manner, a Transfer Function Synthesizer (TFS) is developed. On the TFS, multi-dimensional transfer functions are generated by algebraic synthesis of one-dimensional transfer functions, which are designed based on the conventional GUIs or algebraic expressions. The TFS enables not only multivariate volume rendering but also general visualization techniques such as surface visualization and image composition within the framework of volume rendering. The TFS is implemented on the remote visualization system PBVR, and applied to various multivariate scalar volume data generated from nuclear applications.

Journal Articles

Application of $$^{67}$$Cu produced by $$^{68}$$Zn($$n,n'p+d$$)$$^{67}$$Cu to biodistribution study in tumor-bearing mice

Sugo, Yumi*; Hashimoto, Kazuyuki*; Kawabata, Masako*; Saeki, Hideya*; Sato, Shunichi*; Tsukada, Kazuaki; Nagai, Yasuki*

Journal of the Physical Society of Japan, 86(2), p.023201_1 - 023201_3, 2017/02

 Times Cited Count:14 Percentile:68.14(Physics, Multidisciplinary)

$$^{67}$$Cu produced by the $$^{68}$$Zn($$n,n'p+d$$)$$^{67}$$Cu reaction was used for the first time to determine the biodistribution of $$^{67}$$CuCl$$_{2}$$ in colorectal tumor-bearing mice. High uptake of $$^{67}$$Cu was observed in the tumor as well as in the liver and kidney which are the major organs for copper metabolism. The result showing $$^{67}$$Cu accumulation in the tumor suggests that $$^{67}$$CuCl$$_{2}$$ can be a potential radionuclide agent for cancer radiotherapy. It would also encourage further studies on the therapeutic effect in small animals using an increased dose of $$^{67}$$Cu produced by the $$^{68}$$Zn($$n,n'p+d$$)$$^{67}$$Cu reaction using intense neutrons available at present.

Journal Articles

Influence of inlet velocity condition on unsteady flow characteristics in piping with a short elbow under a high-Reynolds-number condition

Ono, Ayako; Tanaka, Masaaki; Kobayashi, Jun; Kamide, Hideki

Mechanical Engineering Journal (Internet), 4(1), p.16-00217_1 - 16-00217_15, 2017/02

In the design of the Advanced Sodium-cooled Fast Reactor in Japan, the Reynolds number in the primary hot leg (H/L) piping reaches 4.2$$times$$10$$^{7}$$. Furthermore, a short elbow is used in the H/L piping to achieve a compact plant layout. In the H/L piping, flow-induced vibration is a concern due to the excitation force caused by pressure fluctuation in the short elbow. In this report, the influence of inlet velocity condition on the unsteady velocity characteristics in the short elbow was studied by controlling the flow patterns at the elbow inlet. Measured velocity distributions indicated that the inlet velocity profiles affected a circumferential secondary flow, which then affected an area of flow separation at the elbow. It was also found that the velocity fluctuation at low frequency components observed upstream of the elbow could remain in downstream of the elbow though its intensity was attenuated.

Journal Articles

Thermodynamic evidence for nematic superconductivity in Cu$$_{x}$$Bi$$_{2}$$Se$$_{3}$$

Yonezawa, Shingo*; Tajiri, Kengo*; Nakata, Suguru*; Nagai, Yuki; Wang, Z.*; Segawa, Koji*; Ando, Yoichi*; Maeno, Yoshiteru*

Nature Physics, 13(2), p.123 - 126, 2017/02

 Times Cited Count:198 Percentile:99.01(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Progress of thermal hydraulic evaluation methods and experimental studies on a sodium-cooled fast reactor and its safety in Japan

Kamide, Hideki; Ohshima, Hiroyuki; Sakai, Takaaki; Tanaka, Masaaki

Nuclear Engineering and Design, 312, p.30 - 41, 2017/02

 Times Cited Count:6 Percentile:51.46(Nuclear Science & Technology)

In the framework of the Generation-IV International Forum, the safety design criteria (SDC) incorporating safety-related Research and Development results on innovative technologies and lessons learned from Fukushima Dai-ichi Nuclear Power Plants accident has been established to provide the set of general criteria for the safety designs of structures, systems and components of Generation-IV Sodium-cooled Fast Reactors (Gen-IV SFRs). A number of thermal-hydraulic evaluations are necessary to meet the concept of the criteria in the design studies of Gen-IV SFRs. This paper focuses on four kinds of thermal-hydraulic issues associated with the SDC, i.e., fuel subassembly thermal-hydraulics, natural circulation decay heat removal, core disruptive accidents, and thermal striping. Progress of evaluation methods on these issues is shown with activities on verification and validation (V and V) and experimental studies towards commercialization of SFR in Japan. These evaluation methods are planned to be eventually integrated into a comprehensive numerical simulation system that can be applied to all possible phenomena in SFR systems and that can be expected to become an effective tool for the development of human resource and the handing our knowledge and technologies down.

Journal Articles

Influence of lattice structure on multipole interactions in $$Gamma_3$$ non-Kramers doublet systems

Kubo, Katsunori; Hotta, Takashi*

Physical Review B, 95(5), p.054425_1 - 054425_6, 2017/02

 Times Cited Count:27 Percentile:76.04(Materials Science, Multidisciplinary)

Journal Articles

Dislocations near elastic instability in high-pressure body-centered-cubic magnesium

Winter, I. S.*; Poschmann, M.*; Tsuru, Tomohito; Chrzan, D. C.*

Physical Review B, 95(6), p.064107_1 - 064107_9, 2017/02

 Times Cited Count:4 Percentile:22.14(Materials Science, Multidisciplinary)

At high pressure, Mg is expected to transform to the body centered cubic (BCC) phase. We use density functional theory to explore the structure of $$langle 111 rangle$$ type dislocation cores in BCC Mg as a function of pressure. As the pressure is reduced from the region of absolute stability for the BCC phase, the dislocation cores spread. When dislocation cores overlap the displacements of columns of atoms resemble the nanodisturbances observed in TiNb alloys known as Gum Metal. The ideal tensile strength of BCC Mg is also computed as a function of pressure. Despite its low shear modulus, BCC Mg is predicted to be intrinsically brittle at absolute zero.

Journal Articles

$$beta$$ decay of $$^{38,40}$$Si ($$T_z$$ = +5, +6) to low-lying core excited states in odd-odd $$^{38,40}$$P isotopes

Tripathi, V.*; Lubna, R. S.*; Abromeit, B.*; Crawford, H. L.*; Liddick, S. N.*; Utsuno, Yutaka; Bender, P. C.*; Crider, B. P.*; Dungan, R.*; Fallon, P.*; et al.

Physical Review C, 95(2), p.024308_1 - 024308_7, 2017/02

AA2016-0485.pdf:0.5MB

 Times Cited Count:7 Percentile:51.81(Physics, Nuclear)

no abstracts in English

Journal Articles

Two-body wave functions and compositeness from scattering amplitudes; General properties with schematic models

Sekihara, Takayasu

Physical Review C, 95(2), p.025206_1 - 025206_16, 2017/02

AA2016-0539.pdf:1.06MB

 Times Cited Count:21 Percentile:83.48(Physics, Nuclear)

Journal Articles

The Recent improvements on circulation of research results at the Japan Atomic Energy Agency (JAEA)

Inagaki, Satomi; Hayakawa, Misa; Ebisawa, Naomi; Gonda, Mayuki; Nozawa, Takashi; Itabashi, Keizo

Proceedings of 18th International Conference on Grey Literature (GL-18), p.24 - 31, 2017/02

Sharing information of scientific research results on the Internet have developed in the global advancement of the open science today, such as archiving and disseminating scientific papers on institutional repositories, facilitating access to and use of research data etc. Accessibility to those contents in large volumes of information on the Internet is very important issue. Those contents might be grey literature without solving this accessibility issue. This presentation introduces the case study of the Japan Atomic Energy Agency (JAEA) Library as an example of efforts to improve circulation of research results in terms of grey literature. JAEA has disseminate information of our research results through the JAEA Originated Papers Searching System (JOPSS) on the Internet over decade, but we have three main issues to solve aiming at improving the accessibility of grey literature in the open science era; (1) to ensure accessibility of our Internet contents, (2) to consider how our target users find our contents, (3) to improve user interface of contents. We will continue to improve the system aiming to distribute various information of JAEA R&D results.

Journal Articles

Unitization for portability of emergency response surveillance robot system; Experiences and lessons learned from the deployment of the JAEA-3 emergency response robot at the Fukushima Daiichi Nuclear Power Plants

Kawatsuma, Shinji; Mimura, Ryuji; Asama, Hajime*

ROBOMECH Journal (Internet), 4, p.6_1 - 6_7, 2017/02

It was cleared that portability of emergency response reconnaissance robot had been very important. So, RESQ-A robots, which had been developed by Japan Atomic Energy Research Institute (present Japan Atomic Energy Agency), had been considered from the view point of portability. After Fukushima Daiichi NPPs' accidents occurred, JAEA had modified a RESQ-A robot to JAEA-3 robot in order to meet the anticipated situation of the accidents. However, actual situation was beyond the anticipated situation, and additional modification was required. The actual confused situation was many rubble were scattered and temporary cables and hoses were constructed in the reactor buildings, so that reconnaissance robots should be conveyed by operators through limited route, should be reassembled in short time and should be able to remove cable and tiers for reduce the operators' exposure dose during maintenance. JAEA modified again JAEA-3 robot system, with cooperation of operators from Fukushima Daiichi NPPs. It was lesson learned that emergency response reconnaissance robot needed to be unitized for portability, and "Unitization Policy for emergency response reconnaissance robot" was developed.

Journal Articles

A Study on dynamics of non-crystalline materials and superionic conductors by chopper spectrometers in J-PARC

Nakamura, Mitsutaka

Radioisotopes, 66(2), p.93 - 99, 2017/02

Studying the dynamical properties of structurally isotropic materials such as glass, liquid, and polycrystalline powder samples, the inelastic neutron scattering measurement by chopper spectrometer in pulsed neutron source shows the whelming strength compared with that by triple axis spectrometer in research reactor. When a new material exhibiting the unusual physical properties is discovered, it might be difficult to grow the single crystal and only possible to obtain the powder form in the early stage of research. The strong neutron beam of J-PARC can provide opportunity promptly for the dynamical study of newly-discovered materials. The chopper spectrometers in J-PARC have the potential to create innovative research outcomes.

Journal Articles

Effect of specimen size and oxygen partial pressure on creep characteristics for mod. 9Cr-1Mo steel

Kanayama, Hideyuki; Hiyoshi, Noritake*; Ito, Takamoto*; Ogawa, Fumio*; Wakai, Takashi

Zairyo, 66(2), p.86 - 92, 2017/02

This study presents creep characteristics of Mod. 9Cr-1Mo steel with various sized specimens and environment. Creep tests were performed using three different sizes of specimen and three different type of testing environment. Specimens are a bulk specimen which has 6mm diameter and 30mm gage length, a miniature specimen which has 2mm diameter and 10mm gage length and a thin plate specimen which has 0.76mm thickness, 1.5mm width and 7.62mm gage length. Three different type of testing environment are air, 99.99% Ar gas and vacuum. In the same environmental condition, there was no effect of specimen size on time to rupture. Time to rupture of Mod. 9Cr-1Mo steel in Ar gas was shorter than that in air and vacuum. Oxide thickness is not dominant factor in time to rupture. Fracture mode at specimen surface in Ar gas might be dominant factor in shorter time to rupture. Effect of specimen size and environment on creep strength of Mod. 9Cr-1Mo steel was evaluated on the basis of thinning.

Journal Articles

Influence of cyclic softening on high temperature material properties in Mod.9Cr-1Mo steel

Onizawa, Takashi; Nagae, Yuji; Kato, Shoichi; Wakai, Takashi

Zairyo, 66(2), p.122 - 129, 2017/02

The applicability of Modified 9Cr-1Mo steel (ASME Grade 91 steel) as the main structural material in advanced loop-type sodium cooled fast reactor has been explored to enhance the safety, the credibility and the economic competitiveness of fast reactor plants. It is well-known that the steel exhibits cyclic softening behavior. Decrease of tensile and creep strength in softened materials has been already reported by other researchers. This paper discusses the relationship between cyclic softening conditions and high temperature material properties. Grade 91 steel was softened by repeat of plastic strain. The softening behavior could be evaluated by the index of the softening rate. Decrease of tensile and creep strength in softened materials can be evaluated by the softening rate and it depends on the cyclic softening conditions.

Journal Articles

A Spin-crossover phenomenon depending on the environment around an iron atom for the assembled coordination polymers

Nakashima, Satoru*; Kaneko, Masashi

Advances in Chemistry Research, Vol.36, p.171 - 195, 2017/01

Spin-crossover (SCO) phenomena of the assembled coordination polymers are introduced. When the bridging ligand is flexible like 1,2-bis(4-pyridyl)ethane, 1,3-bis(4-pyridyl)propane, a variety of assembled structure can be obtained, depending on the conformer of the ligand and the guest molecules. Guest-dependent SCO phenomena of the assembled iron complexes are shown. Density functional theory is applied to know the cause of guest-dependent SCO phenomena. The validity of an iron mono-nucleus model is evaluated for the coordination polymers. It is shown that SCO occurs or not depends on the local structure around iron ion.

Journal Articles

Sustainable and safe energy supply with seawater uranium fueled HTGR and its economy

Fukaya, Yuji; Goto, Minoru

Annals of Nuclear Energy, 99, p.19 - 27, 2017/01

AA2015-0534.pdf:0.56MB

 Times Cited Count:9 Percentile:65.76(Nuclear Science & Technology)

Sustainable and safe energy supply with seawater fueled HTGR have been investigated to sustain the nuclear energy safely by electricity generation with HTGR, the uranium resources must be inexhaustible. The seawater uranium is expected to be alternative resources to conventional resources. It is said that 4.5 billion tons of uranium is dissolved in the seawater, which corresponds to a consumption of approximately 72 thousand years. The uranium dissolved in seawater is in an equilibrium state with the uranium on surface of sea floor, which is approximately a thousand times of the amount, that is 72 million years. It can be recoverable. In other words, the uranium from seawater is almost inexhaustible natural resource. The cost of extracting uranium from seawater with current technology is still expensive compared with that of conventional uranium. However, the economy of nuclear power generation fueled by seawater uranium should be assessed for entire electricity generation cost. In the present study, the economy of electricity generation using uranium from seawater is assessed using a commercial HTGR. Compared with ordinary LWR using conventional uranium, HTGR can realize lower cost of electricity owing to small volume of simple direct gas turbine system compared with water and steam systems of LWR, rationalization by modularizing, and high thermal efficiency, even if fueled by seawater uranium. It is concluded that the HTGR fueled by seawater uranium with the current technology enables the energy sustainability to be maintained for a long term approximately 70 million years with superior inherent safety features and low cost of 7.28 yen/kWh, which is lower than the 8.80 yen/kWh cost of LWR using conventional uranium.

Journal Articles

The Role of low-temperature organic matter diagenesis in carbonate precipitation within a marine deposit

Miyakawa, Kazuya; Ishii, Eiichi; Hirota, Akinari*; Komatsu, Daisuke*; Ikeya, Kosuke*; Tsunogai, Urumu*

Applied Geochemistry, 76, p.218 - 231, 2017/01

 Times Cited Count:18 Percentile:62.15(Geochemistry & Geophysics)

no abstracts in English

Journal Articles

Inelastic and quasi-elastic neutron scattering spectrometers in J-PARC

Seto, Hideki; Ito, Shinichi; Yokoo, Tetsuya*; Endo, Hitoshi*; Nakajima, Kenji; Shibata, Kaoru; Kajimoto, Ryoichi; Kawamura, Seiko; Nakamura, Mitsutaka; Kawakita, Yukinobu; et al.

Biochimica et Biophysica Acta; General Subjects, 1861(1), p.3651 - 3660, 2017/01

 Times Cited Count:32 Percentile:80.67(Biochemistry & Molecular Biology)

J-PARC, Japan Proton Accelerator Research Complex provides short pulse proton beam at a repetition rate 25 Hz and the maximum power is expected to be 1 MW. Materials and Life Science Experimental Facility (MLF) has 23 neutron beam ports and 21 instruments have already been operated or under construction / commissioning. There are 6 inelastic / quasi-elastic neutron scattering spectrometers and the complementary use of these spectrometers will open new insight for life science.

Journal Articles

Analysis of $$^{134}$$Cs, $$^{137}$$Cs and $$^{40}$$K in the certified reference material of Brown Rice by $$gamma$$-ray spectrometry using a Ge detector, 2; Uncertainty evaluation

Yonezawa, Chushiro*; Shirono, Katsuhiro*; Haraga, Tomoko

Bunseki Kagaku, 66(1), p.27 - 37, 2017/01

 Times Cited Count:0 Percentile:0(Chemistry, Analytical)

no abstracts in English

Journal Articles

Elastically-homogeneous lattice models of damage in geomaterials

Asahina, Daisuke*; Aoyagi, Kazuhei; Kim, K.*; Birkholzer, J.*; Birkholzer, J. T.*; Bolander, J. E.*

Computers and Geotechnics, 81, p.195 - 206, 2017/01

 Times Cited Count:33 Percentile:82.55(Computer Science, Interdisciplinary Applications)

Journal Articles

Assessment of the functions of the impervious plug based on several monitoring results for groundwater recovery experiment

Matsui, Hiroya; Mikake, Shinichiro; Ikeda, Koki; Sasaki, Sadao

Dai-14-Kai Iwa No Rikigaku Kokunai Shimpojiumu Koen Rombunshu (Internet), 6 Pages, 2017/01

Japan Atomic Energy Agency (JAEA) has been conducting the groundwater recovery experiment to develop the methodology to estimate the recovery of geological environment after drift closure at GL-500m in Mizunami Underground Research Laboratory, Gifu prefecture, Japan. For the experiment, the impervious concrete plug was constructed to keep a recovered water pressure. The authors assessed the functions of the pluge based on monitoring and interpretation of the several kinds of measurements inside and outside of the plug during groundwater recovery process in a drift. As the results, the design concept and the expected function of the impervious plug assessed almost satisfied and it is supposed no problem will occur on the groundwater recovery experiment for several months.

Journal Articles

Hydrogeomechanical properties of excavation damaged zones along galleries in different depths of the Horonobe underground research laboratory

Aoyagi, Kazuhei; Ishii, Eiichi

Dai-14-Kai Iwa No Rikigaku Kokunai Shimpojiumu Koen Rombunshu (Internet), 6 Pages, 2017/01

The objective of this research is to investigate the hydro-mechanical properties of excavation damaged zones (EDZs) along the galleries excavated in 250 m and 350 m depths. We conducted hydraulic tests, BTV observations and core analyses. As a result, in the 250 m gallery, the extent of the EDZ was 1.0 m into the gallery wall. The hydraulic conductivity was increased by 2 to 3 orders of magnitudes compared with that of intact rock. On the other hand, in the 350 m gallery, the extent of the EDZ was 0.4 m into the gallery wall; the hydraulic conductivity was increased by 5 orders of magnitudes compared with that of intact rock. We investaged the difference of the characteristics of the EDZs on the basis of competence factor and ductility index. As a result, it was estimated that an extent of an EDZ decreases with decrease of competence factor; a hydraulic conductivity in an EDZ increases with decrease of ductility index.

Journal Articles

Estimation of rock mass stress state based on the convergence measurement result during tunnel excavation

Kamemura, Katsumi*; Aoyagi, Kazuhei; Nago, Makito*; Sugawara, Kentaro*; Matsubara, Makoto*

Dai-14-Kai Iwa No Rikigaku Kokunai Shimpojiumu Koen Rombunshu (Internet), 6 Pages, 2017/01

In the design of deep underground structures such as high-level radioactive waste disposal repositories, the estimation of rock mass stress state is important as well as the estimation of mechanical characteristics of rock mass. This study establishes a practical and effective method for estimating in situ stress based on the convergence measurement results obtained during gallery construction of URL. The convergence was measured in various directions of the URL loop gallery at 350 m depth, and this will allow determination of the stress state over a large area using a back analysis method. In order to improve the accuracy of initial stress estimation, the relationship between convergence measurement results and geological situation of existing fractures were studied. The analysis results show good agreement with the in situ stress state results reported in previous studies and confirm the applicability of the proposed method.

Journal Articles

Long-term evaluation of excavation damaged zone by optical measurement in Horonobe Underground Research Laboratory

Hata, Koji*; Niunoya, Sumio*; Aoyagi, Kazuhei

Dai-14-Kai Iwa No Rikigaku Kokunai Shimpojiumu Koen Rombunshu (Internet), 6 Pages, 2017/01

The objective of this research is to investigate the long-term hydro-mechanical behavior of rock mass around the shaft in the Horonobe Underground Research Laboratory (URL). The long-term monitoring has been carried out by optical AE sensors, optical water pressure sensors, and optical temperature sensors below 350m depth of the shaft in the Horonobe URL. From the measurement results, the extent of an excavation damaged zone was 1.5m within the shaft wall. After the excavation, it was observed that the unsaturated zone of the groundwater was spread more than 1.5m within the shaft wall.

Journal Articles

Numerical analysis of the grout injection conducted in the ventilation shaft of the Horonobe Underground Research Laboratory

Nakashima, Hiroyoshi*; Koyama, Tomofumi*; Tatsuta, Keisuke*; Katayama, Tatsuo*; Aoyagi, Kazuhei

Dai-14-Kai Iwa No Rikigaku Kokunai Shimpojiumu Koen Rombunshu (Internet), 6 Pages, 2017/01

In this study, we created the three dimensional model based on equivalent continuum approach to study the penetration length and enhancement of the hydraulic conductivity of the rock mass. The developed numerical model was applied to the in situ grout injection conducted in the ventilation shaft of the Horonobe Underground Research Laboratory. We evaluated the hydraulic conductivity of the rock mass after the grout operation. As a result, hydraulic conductivity of the highly permeable fault was decreased in 4 orders of magnitude, which is almost consistent with the in situ hydraulic conductivity obtained from in situ Luegeon test after the grout injection. Thus the simulation method described in this paper can be applied to the evaluation of the efficiency of in situ grout injection.

Journal Articles

Higher harmonic imaging of small defects in ODS steel cladding tubes and characterization of the defects with SEM

Kawashima, Koichiro*; Yano, Yasuhide; Tanno, Takashi; Kaito, Takeji

Dai-24-Kai Choompa Ni Yoru Hihakai Hyoka Shimpojiumu Koen Rombunshu (USB Flash Drive), p.99 - 104, 2017/01

no abstracts in English

Journal Articles

Inferring partial orders of nodes for hierarchical network layout

Wu, H.-Y.*; Takahashi, Shigeo*; Miyamura, Hiroko; Ozahata, Satoshi*; Nakao, Akihiro*

Electronic Imaging, 2017(1), p.118 - 130, 2017/01

Extracting hierarchical structures from networks provides us with an effective means of visualizing them, especially when they contain complicated node connectivities such as those in traffic and distributed networks. This paper presents an algorithm for inferring such partial orders by optimizing the network hierarchies along flow paths that are given as input. We study several network examples to demonstrate the feasibility of the proposed approach including course dependency charts, railway networks, and P2P networks.

Journal Articles

Proposal of maintenance management of nuclear power plants at R&D stage by taking account of their features

Takaya, Shigeru; Chikazawa, Yoshitaka; Hayashida, Kiichi; Tagawa, Akihiro; Kubo, Shigenobu; Yamashita, Atsushi

Hozengaku, 15(4), p.71 - 78, 2017/01

A maintenance management suitable to nuclear power plants (NPP) at R&D stage was discussed. Objectives of maintenance management of NPP at R&D stage was first clarified. Next, applicability of codes for maintenance management of commercial NPP to NPP at R&D stage was discussed. Then, requirements and consideration for maintenance management of NPP at R&D stage was proposed. Finally, an example that the proposal was applied to setting maintenance program of sodium-cooled fast reactor was presented.

Journal Articles

Comprehensive study on initial thermal oxidation of GaN(0001) surface and subsequent oxide growth in dry oxygen ambient

Yamada, Takahiro*; Ito, Joyo*; Asahara, Ryohei*; Watanabe, Kenta*; Nozaki, Mikito*; Nakazawa, Satoshi*; Anda, Yoshiharu*; Ishida, Masahiro*; Ueda, Tetsuzo*; Yoshigoe, Akitaka; et al.

Journal of Applied Physics, 121(3), p.035303_1 - 035303_9, 2017/01

 Times Cited Count:66 Percentile:91.84(Physics, Applied)

Initial oxidation of GaN(0001) epilayers and subsequent growth of thermal oxides in dry oxygen ambient were investigated by means of X-ray photoelectron spectroscopy, spectroscopic ellipsometry, atomic force microscopy and X-ray diffraction measurements. It was found that, whereas initial oxide formation tends to saturate at temperatures below 800$$^{circ}$$C, selective growth of small oxide grains proceeds at dislocations in the epilayers, followed by noticeable grain growth leading to rough surface morphology at higher oxidation temperatures. This indicates that oxide growth and its morphology are crucially dependent on the defect density in the GaN epilayers. Structural characterizations also revealed that polycrystalline $$alpha$$- and $$beta$$-phase Ga$$_{2}$$O$$_{3}$$ grains in an epitaxial relation with the GaN substrate are formed from the initial stage of the oxide growth. On the basis of these experimental findings, we also developed a comprehensive model for GaN oxidation mediated by nitrogen removal and mass transport.

Journal Articles

Assessment of residual doses to population after decontamination in Fukushima Prefecture

Mori, Airi; Takahara, Shogo; Ishizaki, Azusa; Iijima, Masashi; Sanada, Yukihisa; Munakata, Masahiro

Journal of Environmental Radioactivity, 166(Part 1), p.74 - 82, 2017/01

 Times Cited Count:8 Percentile:26.82(Environmental Sciences)

Large quantities of radioactive materials were released into the environment as a result of the Fukushima Daiichi Nuclear Power Station accident. Many inhabitants residing in the affected areas are now exposed to radiation in their daily lives. In an attempt to manage this radiation dose, an additional radiation dose of 1 mSv/y was adopted as a long-term dosimetric target. An activity level reading of 0.23 $$mu$$Sv/h was then determined as a guidance value to achieve the target by implementing decontamination measures. The objectives of this study are to assess the effects of decontamination based on this guidance value and to predict any possible future problems with the decontamination strategy. Using a probabilistic approach, we assessed the annual effective dose of indoor workers, outdoor workers, and pensioners in the Fukushima Prefecture. Our probabilistic model considers the variabilities in behavioral patterns and Cs-137 surface-activity levels. Five years after the initial contamination, the 95th percentiles of indoor workers and pensioners in 53 of the 59 municipalities were found to receive annual effective doses of below 1 mSv/y (0.026-0.73 mSv/y). However, for outdoor workers in 25 municipalities, the annual doses were over 1 mSv/y (1.0-35 mSv/y). Therefore, the guidance value is effective for indoor workers and pensioners; to determine whether additional countermeasures for outdoor workers should be implemented, a detailed assessment that uses more realistic assumptions is required.

Journal Articles

Spectrum-dose conversion operator of NaI(Tl) and CsI(Tl) scintillation detectors for air dose rate measurement in contaminated environments

Tsuda, Shuichi; Saito, Kimiaki

Journal of Environmental Radioactivity, 166(Part 3), p.419 - 426, 2017/01

 Times Cited Count:27 Percentile:65.77(Environmental Sciences)

Air dose rate monitoring in the environment has been performed since the Fukushima Dai-ichi Nuclear Power Plant accident happened. In the measurement, NaI(Tl) and CsI(Tl) scintillation detectors are used, which are usually used in nuclear power plants and calibrated in a uniform irradiation condition in a radiation calibration field. In general, however, the detector responses are dependent on incident direction and in reality, the incident direction of the photons is not uniform in the environment. In this study, to evaluate the dependence of dose on the photon incident direction, the spectrum - dose conversion operator (G(E) function) for air kerma in a semi-infinite radiation field were obtained using the PHITS code for commonly used NaI(Tl) and CsI(Tl) scintillation detectors. The results indicate that the commonly used scintillation detectors overestimate the doses by a maximum of 40% for mono-energetic photons but under the real environment, one could obtain the dose in the semi-infinite radiation field within 20%.

Journal Articles

Measurements of air dose rates in and around houses in the Fukushima Prefecture in Japan after the Fukushima accident

Matsuda, Norihiro; Mikami, Satoshi; Sato, Tetsuro*; Saito, Kimiaki

Journal of Environmental Radioactivity, 166(Part 3), p.427 - 435, 2017/01

 Times Cited Count:16 Percentile:48.19(Environmental Sciences)

Journal Articles

Implementation of muon interaction models in PHITS

Abe, Shinichiro; Sato, Tatsuhiko

Journal of Nuclear Science and Technology, 54(1), p.101 - 110, 2017/01

 Times Cited Count:9 Percentile:61.27(Nuclear Science & Technology)

There are several researches for application of muons, e.g. the visualization of inner-structure of nuclear reactors by using high-energy cosmic-ray muons, nuclear transmutation of long-lived fission products (LLFPs) and nondestructive elemental analysis by using low-energy negative muon. In this study, we construct models for muon interactions (i.e., bremsstrahlung, electron-positron pair production, muon photonuclear interaction, and negative muon capture reaction) and implement them into PHITS in order to make PHITS available for investigations of muon application. The improved PHITS agrees well with experimental data not only for the vertical intensities of cosmic-ray muons in water and standard rock, but also for neutron production by muon photonuclear interaction and negative muon capture reaction. The improved PHITS can also reproduce the cross-section of radionuclide production by muons passing through a concrete wall very well. These results indicate the applicability of the improved PHITS to the shielding design of muon facilities in which estimations of attenuation length and induced radioactivity are important.

Journal Articles

Investigation of absorption characteristics for thermal-load fluctuation using HTTR

Tochio, Daisuke; Honda, Yuki; Sato, Hiroyuki; Sekita, Kenji; Homma, Fumitaka; Sawahata, Hiroaki; Takada, Shoji; Nakagawa, Shigeaki

Journal of Nuclear Science and Technology, 54(1), p.13 - 21, 2017/01

 Times Cited Count:1 Percentile:10.62(Nuclear Science & Technology)

GTHTR300C is designed and developed in JAEA. The reactor system is required to continue a stable and safety operation as well as a stable power supply in the case that thermal-load is fluctuated by the occurrence of abnormal event in the heat utilization system. Then, it is necessary to demonstrate that the thermal-load fluctuation should be absorbed by the reactor system so as to continue the stable and safety operation could be continued. The thermal-load fluctuation absorption tests without nuclear heating were planned and conducted in JAEA to clarify the absorption characteristic of thermal-load fluctuation mainly by the reactor and by the IHX. As the result it was revealed that the reactor has the larger absorption capacity of thermal-load fluctuation than expected one, and the IHX can be contributed to the absorption of the thermal-load fluctuation generated in the heat utilization system in the reactor system. It was confirmed from there result that the reactor and the IHX has effective absorption capacity of the thermal-load fluctuation generated in the heat utilization system. Moreover it was confirmed that the safety estimation code based on RELAP5/MOD3 can represents the thermal-load fluctuation absorption behavior conservatively.

Journal Articles

Correction of the thermal neutron capture cross section of $$^{241}$$Am obtained by the Westcott convention

Mizuyama, Kazuhito; Iwamoto, Nobuyuki; Iwamoto, Osamu

Journal of Nuclear Science and Technology, 54(1), p.74 - 80, 2017/01

Journal Articles

Vertical distributions of global fallout $$^{137}$$Cs and $$^{14}$$C in a Japanese forest soil profile and their implications for the fate and migration processes of Fukushima-derived $$^{137}$$Cs

Koarashi, Jun; Atarashi-Andoh, Mariko; Amano, Hikaru*; Matsunaga, Takeshi

Journal of Radioanalytical and Nuclear Chemistry, 311(1), p.473 - 481, 2017/01

 Times Cited Count:17 Percentile:85.35(Chemistry, Analytical)

Vertical distributions of global fallout $$^{137}$$Cs and $$^{14}$$C were investigated in a Japanese forest soil in 2001. Even 38 years after the fallout, $$^{137}$$Cs was still observed mostly in the uppermost 5 cm. A preferential accumulation of $$^{137}$$Cs was found in a 1-cm-thick transition layer between organic-rich A and underlying B horizons. This unique observation indicated that $$^{137}$$Cs migrated through the A horizon at a rate of 0.20% y$$^{-1}$$ and the transition layer acted as a barrier for $$^{137}$$Cs migration to deeper layers. The vertical distributions of $$^{137}$$Cs and $$^{14}$$C were significantly correlated, suggesting a coupled downward migration of $$^{137}$$Cs and organic matter on a time scale of decades, along the same physical pathways.

Journal Articles

Applicability of polyvinylpolypyrrolidone adsorbent to treatment process of wastes containing uranium

Ohashi, Yusuke; Harada, Masayuki*; Asanuma, Noriko*; Ando, Shion; Tanaka, Yoshio; Ikeda, Yasuhisa*

Journal of Radioanalytical and Nuclear Chemistry, 311(1), p.491 - 502, 2017/01

 Times Cited Count:1 Percentile:10.62(Chemistry, Analytical)

In order to assess the feasibility of method for recovering U from wastes containing uranium (scrap uranium) using polyvinylpolypyrrolidone (PVPP) adsorbent, we have examined the adsorption and desorption behavior of metal species in HCl aqueous solutions dissolving scrap uranium. It was found that the U(VI) species are selectively adsorbed onto PVPP regardless of the presence of a large amount of Na(I) and Al(III), that the adsorbed U(VI) species are desorbed from PVPP column selectively by water. Pure uranium was efficiently recovered from the eluates. From these results, the PVPP resin is expected to be used as the adsorbent in the treatment process of scrap uranium.

Journal Articles

Generation method of underwater landmarks for ocean observation

Takahashi, Satoru*; Nota, Yoshiki*; Matsuda, Asahi*; Kawabata, Kuniaki; Suzuki, Tsuyoshi*; Takemura, Fumiaki*; Ogasawara, Kei*; Kaneko, Shunichi*

Journal of Signal Processing, 21(1), p.15 - 24, 2017/01

In recent years, many researchers try to observe the state of the global environment from marine information for the understanding of the global environment change. First, we introduce the recording system of underwater environment which is made by the authors. By using this system, we want to observe the change of global environment from the coral bleaching. In this paper, especially, we propose the generation method of underwater landmark which is used to measure the position of robot of oceanographic observation based on the dynamic image processing. In here, underwater landmark means the feature point in underwater image.

Journal Articles

Reduced-shifted conjugate-gradient method for a Green's function; Efficient numerical approach in a nano-structured superconductor

Nagai, Yuki; Shinohara, Yasushi*; Futamura, Yasunori*; Sakurai, Tetsuya*

Journal of the Physical Society of Japan, 86(1), p.014708_1 - 014708_9, 2017/01

 Times Cited Count:8 Percentile:53.85(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Variational wavefunction for the periodic Anderson model with onsite correlation factors

Kubo, Katsunori; Onishi, Hiroaki

Journal of the Physical Society of Japan, 86(1), p.013701_1 - 013701_4, 2017/01

 Times Cited Count:3 Percentile:21.19(Physics, Multidisciplinary)

Journal Articles

Alloy design and mechanical properties; First-principles calculations of dislocation core

Tsuru, Tomohito

Materia, 56(1), p.5 - 13, 2017/01

Elements strategy becomes important to investigate alternative materials of rare metals. We have dedicated to establish a new approach based on computational methods. In the present paper, we propose two approaches based on first-principles and theory of dislocations. These methods are introduced to magnesium alloys.

Journal Articles

Modeling of Phosphorus Transport by Interstitial Dumbbell in $$alpha$$-Iron Using First-Principles-Based Kinetic Monte Carlo

Ebihara, Kenichi; Suzudo, Tomoaki; Yamaguchi, Masatake

Materials Transactions, 58(1), p.26 - 32, 2017/01

 Times Cited Count:8 Percentile:38.56(Materials Science, Multidisciplinary)

In order to evaluate grain boundary (GB) phosphorous (P) segregation in nuclear reactor pressure vessel steels under irradiation, the rate-theory model based on first-principles calculations is developed. In this study, we evaluated the diffusion coefficient of the mixed interstitial dumbbell of a P atom and an iron(Fe) atom using a kinetic Monte Carlo (kMC) simulation based on first-principles calculations. The evaluated diffusion coefficient was almost the same with the diffusion coefficient of P atoms which migrate via octahedral interstitial sites, and was much faster than that for P transport by vacancies. Furthermore, from the simulation of the irradiation induced GB P segregation using the model which was modified to include P atoms of octahedral interstitial sites, it was found that the boundary condition at GB is not valid for P atoms of octahedral interstitial sites

Journal Articles

Investigation of error estimation method of observational data and comparison method between numerical and observational results toward V&V of seismic simulation

Suzuki, Yoshio; Kawakami, Yoshiaki*; Nakajima, Norihiro

Mechanical Engineering Reviews, 4(1), p.15-00525_1 - 15-00525_18, 2017/01

The method to estimate errors included in observational data and the method to compare numerical results with observational results are investigated toward the verification and validation (V&V) of a seismic simulation. For the method to estimate errors, it is found that errors are caused by the resolution, the linearity, the temperature coefficient for sensitivity, the temperature coefficient for zero shift, the transverse sensitivity, the seismometer property, the aliasing, and so on. Thus, it is needed to estimate errors individually for those factors and integrate them. For the method to compare numerical results with observational results, it is found that six methods have been mainly proposed in existing researches. Evaluating those methods using nine items, advantages and disadvantages for those methods are arranged. The method is not well established so that it is necessary to employ those methods by compensating disadvantages and/or to search for a solution to a novel method.

Journal Articles

Composite behavior of lath martensite steels induced by plastic strain, a new paradigm for the elastic-plastic response of martensitic steels

Ung$'a$r, T.*; Harjo, S.; Kawasaki, Takuro; Tomota, Yo*; Rib$'a$rik, G.*; Shi, Z.*

Metallurgical and Materials Transactions A, 48(1), p.159 - 167, 2017/01

AA2016-0372.pdf:2.81MB

 Times Cited Count:46 Percentile:90.37(Materials Science, Multidisciplinary)

Journal Articles

Hydrogenation of iron in the early stage of Earth's evolution

Iizuka, Riko*; Yagi, Takehiko*; Goto, Hirotada*; Okuchi, Takuo*; Hattori, Takanori; Sano, Asami

Nature Communications (Internet), 8, p.14096_1 - 14096_7, 2017/01

AA2016-0524.pdf:0.73MB

 Times Cited Count:44 Percentile:88.82(Multidisciplinary Sciences)

Density of the Earth's core is lower than that of pure iron and the light element(s) in the core is a long-standing problem. Hydrogen is the most abundant element in the solar system and thus one of the important candidates. However, the dissolution process of hydrogen into iron remained unclear. Here we carry out high-pressure and high-temperature in situ neutron diffraction experiments and clarify that when the mixture of iron and hydrous minerals are heated, iron is hydrogenized soon after the hydrous mineral is dehydrated. This implies that early in the Earth's evolution, as the accumulated primordial material became hotter, the dissolution of hydrogen into iron occurred before any other materials melted. This suggests that hydrogen is likely the first light element dissolved into iron during the Earth's evolution and it may affect the behaviour of the other light elements in the later processes.

Journal Articles

One-dimensional spinon spin currents

Hirobe, Daichi*; Sato, Masahiro*; Kawamata, Takayuki*; Shiomi, Yuki*; Uchida, Kenichi*; Iguchi, Ryo*; Koike, Yoji*; Maekawa, Sadamichi; Saito, Eiji

Nature Physics, 13(1), p.30 - 34, 2017/01

 Times Cited Count:99 Percentile:96.76(Physics, Multidisciplinary)

Journal Articles

Cesiated surface H$$^{-}$$ ion source; Optimization studies

Ueno, Akira

New Journal of Physics (Internet), 19(1), p.015004_1 - 015004_15, 2017/01

 Times Cited Count:12 Percentile:64.28(Physics, Multidisciplinary)

In order to satisfy the increasing intensity requirements of high-energy and high-intensity proton accelerators for an H$$_{-}$$ ion beam with small transverse normalized rms emittances of around 0.25 $$pi$$mm$$cdot$$mrad, diverse parameters possibly reducing the emittances were optimised. Such as the plasma electrode shape and temperature, the radio-frequency (RF) matching network for the igniter plasma, the filter-field strength and distribution, the strength of the axial magnetic field around the beam extraction hole, the cesiasion procedure and the cesium (Cs) density, impurity elements, and so on, were optimized with H$$_{-}$$ ion sources for the Japan Proton Accelerator Research Complex (J-PARC). By optimizing each parameter step by step, the J-PARC cesiated RF-driven H$$_{-}$$ ion source successfully produced the world brightest class beam with 95% beam transverse normalized rms emittances of 0.24 $$pi$$mm$$cdot$$mrad and an intensity of 66 mA.

Journal Articles

Development of ion exchange ligands with high separation performance and colorimetric analysis using gold nanoparticles decorated with the functional ligands

Shimojo, Kojiro

Nihon Ion Kokan Gakkai-Shi, 28(1), p.1 - 10, 2017/01

Development of metal separating reagents with high selectivity is necessary for efficient separation and recovery of valuable metals contained in industrial wastes, and removal and detection of toxic metals. We have developed novel metal separating ligands with a diglycolamic acid (DGAA) framework. The ligands have a tridentate coordination structure consisting of an amide group and a carboxy group connected by an ether chain and provide a metal separation ability superior to that of commercial ligands. Since the ligands can be synthesized simply in one step, this helps to reduce the production costs of the ligands. In the present review article, we report the extraction characteristics of DGAA-type ligand for 56 kinds of metal ions, extraction separation of rare-earth metal ions, and removal of toxic metal ions. Furthermore, a one-pot biological approach to fabricate DGAA-decorated gold nanoparticles has been developed using the DGAA-type ligand fused to the N-terminus of a gold-binding peptide. It was found that the DGAA-decorated gold nanoparticles can act as a high-sensitive colorimetric sensor for detecting toxic metal ions with color change.

Journal Articles

Development of simple estimation method for the influence of parameter uncertainty of probability distributions against evaluation result of probabilistic fracture mechanics

Okajima, Satoshi; Takaya, Shigeru; Asayama, Tai

Nihon Kikai Gakkai Rombunshu (Internet), 83(845), p.16-00434_1 - 16-00434_13, 2017/01

no abstracts in English

Journal Articles

Systematic measurement of double-differential neutron production cross sections for deuteron-induced reactions at an incident energy of 102 MeV

Araki, Shohei*; Watanabe, Yukinobu*; Kitajima, Mizuki*; Sadamatsu, Hiroki*; Nakano, Keita*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.

Nuclear Instruments and Methods in Physics Research A, 842, p.62 - 70, 2017/01

 Times Cited Count:12 Percentile:75.51(Instruments & Instrumentation)

Recently, deuteron incident reaction is expected to be used as a neutron source for study of radiation damage in fusion materials, boron neutron capture therapy, and so on. However, experimental data to validate the model is very few. In this work, double-differential neutron production cross sections (DDXs) for deuteron-induced reactions on $$^{nat}$$Li, $$^{9}$$Be, $$^{nat}$$C, $$^{27}$$Al, $$^{nat}$$Cu, and $$^{93}$$Nb at 102 MeV were measured at forward angles $$leq$$ 25$$^{circ}$$ by means of a time of flight (TOF) method with NE213 liquid organic scintillators at the Research Center of Nuclear Physics (RCNP), Osaka University. The experimental DDXs and energy-integrated cross sections were compared with TENDL-2015 data and PHITS calculation. The PHITS calculation showed better agreement with the experimental results than TENDL-2015 for all target nuclei, although the shape of the broad peak around 50 MeV was not satisfactorily reproduced by the PHITS calculation.

Journal Articles

Development of spin-wave-like dispersive excitations below the pseudogap temperature in the high-temperature superconductor La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$

Matsuura, Masato*; Kawamura, Sho*; Fujita, Masaki*; Kajimoto, Ryoichi; Yamada, Kazuyoshi*

Physical Review B, 95(2), p.024504_1 - 024504_6, 2017/01

 Times Cited Count:10 Percentile:45.87(Materials Science, Multidisciplinary)

Journal Articles

Excited configurations of hydrogen in the BaTiO$$_{3-x}$$H$$_x$$ perovskite lattice associated with hydrogen exchange and transport

Ito, Takashi; Koda, Akihiro*; Shimomura, Koichiro*; Higemoto, Wataru; Matsuzaki, Teiichiro*; Kobayashi, Yoji*; Kageyama, Hiroshi*

Physical Review B, 95(2), p.020301_1 - 020301_5, 2017/01

 Times Cited Count:11 Percentile:48.83(Materials Science, Multidisciplinary)

Journal Articles

Search for the $$0^{--}$$ Glueball in $$Upsilon(1S)$$ and $$Upsilon(2S)$$ decays

Jia, S.*; Tanida, Kiyoshi; Belle Collaboration*; 170 of others*

Physical Review D, 95(1), p.012001_1 - 012001_13, 2017/01

AA2016-0474.pdf:1.26MB

 Times Cited Count:20 Percentile:68.68(Astronomy & Astrophysics)

Journal Articles

Theoretical elucidation of space charge effects on the coupled-bunch instability at the 3 GeV Rapid Cycling Synchrotron at the Japan Proton Accelerator Research Complex

Shobuda, Yoshihiro; Chin, Y. H.*; Saha, P. K.; Hotchi, Hideaki; Harada, Hiroyuki; Irie, Yoshiro*; Tamura, Fumihiko; Tani, Norio; Toyama, Takeshi*; Watanabe, Yasuhiro; et al.

Progress of Theoretical and Experimental Physics (Internet), 2017(1), p.013G01_1 - 013G01_39, 2017/01

AA2016-0375.pdf:3.07MB

 Times Cited Count:14 Percentile:68.14(Physics, Multidisciplinary)

The Rapid Cycling Synchrotron (RCS), whose beam energy ranges from 400 MeV to 3 GeV and which is located in the Japan Proton Accelerator Research Complex, is a kicker-impedance dominant machine, which violates the impedance budget from a classical viewpoint. Contrary to conventional understanding, we have succeeded to accelerate a 1-MW equivalent beam. The machine has some interesting features: for instance, the beam tends to be unstable for the smaller transverse beam size, the beam is stabilized by increasing the peak current ${it etc}$. Space charge effects play an important role in the beam instability at the RCS. In this study, a new theory has been developed to calculate the beam growth rate with the head-tail and coupled-bunch modes ($$m,mu$$) while taking space charge effects into account. The theory sufficiently explains the distinctive features of the beam instabilities at the RCS.

Journal Articles

Effect of storage environment on hydrogen generation by the reaction of Al with water

Wang, Y.-Q.*; Gai, W.-Z.*; Zhang, X.-Y.*; Pan, H.-Y.*; Cheng, Z.-X.*; Xu, P. G.; Deng, Z.-Y.*

RSC Advances (Internet), 7(4), p.2103 - 2109, 2017/01

AA2016-0521.pdf:1.55MB

 Times Cited Count:25 Percentile:64.07(Chemistry, Multidisciplinary)

Journal Articles

Classification of radioactive waste drums using random forests for their $$gamma$$-ray spectra

Hata, Haruhi; Ishimori, Yuu

Radioisotopes, 66(1), p.1 - 10, 2017/01

The feasibility of Random Forests, one of machine learning methods was examined for the classification of radioactive waste drums. It was carried out using 954 $$gamma$$-ray spectra of drums which were already classified to natural or reprocessed uranium. After 300 spectra were selected at random to reassemble training datasets, the percentages of correct classification by Random Forests were evaluated with another 654 spectra. When the counts of spectra were reprocessed as the difference of their logarithm, Random Forests accurately classified 654 drums.

Journal Articles

What can we measure by radiation measurement instruments?

Takeyasu, Masanori

Tomioka Hoshasen Joho Matome Saito (Internet), 2 Pages, 2017/01

Some radiation measurement instruments are lent out to the residents in Tomioka-machi, Fukushima. In this paper, it is explained that the kinds of those instruments, their purposes, the attention points on their uses and the interpretation of the measurement results by those instruments.

Journal Articles

Estimation of corrosion mechanisms from the data obtained by the reproduced experiments considering the actual environments; Maritime structures and nuclear facilities

Yamamoto, Masahiro

Zairyo To Kankyo, 66(1), p.3 - 12, 2017/01

The laboratory simulation tests which could be reproduced the corrosion reactions propagating in the actual environments were utilized to analyze the mechanism of corrosion phenomena. In this report, some results are introduced in the cases of maritime structures and nuclear facilities. Experimental apparatus was originally designed to obtain the data in high radioactive condition simulating actual plants. One is a result showing the effect of Np ion to the corrosion of stainless steel in nuclear fuel reprocessing plant. Corrosion mechanism was revealed that Np$$^{6+}$$ ion is reduced to Np$$^{5+}$$ ion by a corrosion reaction of stainless steel and then re-oxidized to Np$$^{6+}$$ ion in the bulk solution. And repetition of this cycle accelerated corrosion of stainless steel by a little amounts of Np addition in nitric acid solution. Another result is introduced that an effect of H$$_{2}$$O$$_{2}$$ created by radiolysis of cooling water at high radioactive environment in light water reactor.

Journal Articles

Numerical simulation of surface energy and water balances over a semiarid grassland ecosystem in the West African Savanna

Quansah, E.*; Katata, Genki; Mauder, M.*; Annor, T.*; Amekudzi, L. K.*; Bliefernicht, J.*; Heinzeller, D.*; Balogun, A.*; Kunstmann, H.*

Advances in Meteorology, 2017, p.6258180_1 - 6258180_11, 2017/00

AA2016-0147.pdf:2.3MB

 Times Cited Count:3 Percentile:9.47(Meteorology & Atmospheric Sciences)

An accurate prediction in the energy partitioning of the net solar radiation into latent and sensible heat fluxes over arid and semiarid regions is one of the challenges in land surface study in weather and climate simulations. Numerical simulations of surface energy and water balances were carried out using a one-dimensional multi-layer atmosphere-SOil-VEGetation (SOLVEG) model for selected days of the dry and rainy seasons over a savanna grassland ecosystem in Sumbrungu in the Upper East region of Ghana. The results for the investigated period between both seasons showed that the model overall reproduced the diurnal changes in the observed net radiation, sensible heat flux, latent heat flux, and ground heat flux. The statistics for the above variables as the correlation coefficient, root mean square error, and normalized standard deviation between the observations and calculations in the dry and wet periods suggest that the model was able to simulate the observed energy fluxes, soil evaporation, and transpiration in savanna grassland ecosystems.

Journal Articles

Structural engineering studies on reinforced concrete structure using neutron diffraction

Suzuki, Hiroshi; Kusunoki, Koichi*; Kanematsu, Manabu*; Mukai, Tomohisa*; Harjo, S.

Materials Research Proceedings, Vol.2, p.25 - 30, 2017/00

 Times Cited Count:3 Percentile:70.51(Metallurgy & Metallurgical Engineering)

It has been demonstrated in our past studies that neutron diffraction can be an alternative method to conventional strain gauge for measuring the stress distribution along rebar embedded in concrete. The current study investigated the possibility of the bond stress evaluation using neutron diffraction in order to find further capability of neutron diffraction for the structural engineering study on the reinforced concrete structure. Several peaks appeared in the bond stress distribution measured by neutron diffraction, showing the inhomogeneous bond variation along the embedded rebar. This result suggests that the neutron diffraction technique with high spacial resolution makes it possible to catch local bond resistance caused by the transverse ribs. The bond stress distribution measured by the neutron diffraction technique is expected to bring detailed understanding of the bond mechanism between rebar and concrete for the reinforced concrete structure.

Journal Articles

Effect of interaction of embedded crack and free surface on remaining fatigue life

Katsumata, Genshichiro*; Lacroix, V.*; Li, Y.

AIMS Materials Science, 3(4), p.1748 - 1758, 2016/12

Journal Articles

Determination of $$^{107}$$Pd in Pd recovered by laser-induced photoreduction with inductively coupled plasma mass spectrometry

Asai, Shiho; Yomogida, Takumi; Saeki, Morihisa*; Oba, Hironori*; Hanzawa, Yukiko; Horita, Takuma; Kitatsuji, Yoshihiro

Analytical Chemistry, 88(24), p.12227 - 12233, 2016/12

 Times Cited Count:16 Percentile:53.58(Chemistry, Analytical)

Safety evaluation of a radioactive waste repository requires credible activity estimates confirmed by actual measurements. A long-lived radionuclide, $$^{107}$$Pd, which can be found in radioactive wastes, is one of the difficult-to-measure nuclides and results in a deficit in experimentally determined contents. In this study, a precipitation-based separation method has been developed for the determination of $$^{107}$$Pd with ICP-MS. The photoreduction induced by laser irradiation at 355 nm provides short-time and one-step recovery of Pd. The proposed method was verified by applying it to a spent nuclear fuel sample. In order to efficiently recover Pd, a natural Pd standard was employed as the Pd carrier. The chemical yield of Pd was about 90% with virtually no impurities, allowing accurate quantification of $$^{107}$$Pd.

Journal Articles

Gamma radiation resistance of spin Seebeck devices

Yagmur, A.*; Uchida, Kenichi*; Ihara, Kazuki*; Ioka, Ikuo; Kikkawa, Takashi*; Ono, Madoka*; Endo, Junichi*; Kashiwagi, Kimiaki*; Nakashima, Tetsuya*; Kirihara, Akihiro*; et al.

Applied Physics Letters, 109(24), p.243902_1 - 243902_4, 2016/12

 Times Cited Count:3 Percentile:14.94(Physics, Applied)

Thermoelectric devices based on the spin Seebeck effect (SSE) were irradiated with gamma ($$gamma$$) rays with the total dose of around 3$$times$$10$$^{5}$$ Gy in order to investigate the $$gamma$$-radiation resistance of the devices. To demonstrate this, Pt/Ni$$_{0.2}$$Zn$$_{0.3}$$Fe$$_{2.5}$$O$$_{4}$$/Glass and Pt/Bi$$_{0.1}$$Y$$_{2.9}$$Fe$$_{5}$$O$$_{12}$$/Gd$$_{3}$$Ga$$_{5}$$O$$_{12}$$ SSE devices were used. We confirmed that the thermoelectric, magnetic, and structural properties of the SSE devices are not affected by the $$gamma$$-ray irradiation. This result demonstrates that SSE devices are applicable to thermoelectric generation even in high radiation environments.

Journal Articles

Temporal variation of dose rate distribution around the Fukushima Daiichi Nuclear Power Station using unmanned helicopter

Sanada, Yukihisa; Orita, Tadashi; Torii, Tatsuo

Applied Radiation and Isotopes, 118, p.308 - 316, 2016/12

 Times Cited Count:28 Percentile:93.3(Chemistry, Inorganic & Nuclear)

An unmanned helicopter monitoring system (UHMS) was developed to survey the environmental effect of radioactive cesium scattered as a result of the Fukushima Daiichi Nuclear Power Station accident. The UHMS was mainly used to monitor the area surrounding the Fukushima Daiichi Nuclear Power Station six times from 2012 to 2015. Quantitative changes in the radioactivity distribution trend were revealed from the results of these monitorings runs.

Journal Articles

A Trajectory generation method for mobile robot based on iterative extension-like process

Kawabata, Kuniaki

Artificial Life and Robotics, 21(4), p.500 - 509, 2016/12

In this paper, we propose a trajectory generation method for mobile robot based on iterative extension-like process. Due to use mobile robots in the real world, trajectory generation must be done depending on the faced situation on each occasion. Proposed method enables online iterative trajectory extension process based on a low-order polynomial curve named as trajectory segment. The waypoints on the existing trajectory segment and a waypoint designated every fixed interval are the constraints to trigger the trajectory extension. For maintaining the smooth continuity of the trajectory, the velocity state must be sustained at the connecting point. Resultantly, the trajectory segments are organized into a single smooth trajectory.

Journal Articles

Retention of rare earth elements, thorium and uranium in sedimentary rocks; A Case study in the Horonobe area of Hokkaido, Japan

Murakami, Takuma; Sasamoto, Hiroshi; Mizuno, Takashi

Chikyu Kagaku, 50(4), p.299 - 317, 2016/12

Development of techniques for investigating the long-term migration of elements in deep underground is important with respect to safety assessment for the geological disposal of high-level radioactive waste. As one study of the migration of elements in deep underground, the distribution of REE, Th and U in sedimentary rock of Horonobe area in Hokkaido was investigated, and discussed whether the difference of hydrogeological structure and lithofacies influences on the distributions. As the results, it was considered that REE and Th were mainly retained in minerals originating from terrigenous clastic and secondary mineral occurred in early diagenesis, and their distributions were relatively homogenous in both the Koetoi and Wakkanai formations. Uranium was indicated to be maintained in the sedimentary rock until now after depositing in deep-sea sediment. It was considered that the U deposition was occurred by adsorption on organic matter and reductive precipitation with decomposition of organic matter. In addition, it was confirmed that the distributions of these elements were not influenced by the difference of hydrogeological and lithofacies.

Journal Articles

Erratum; Effects of OH$$^{-}$$ activity and temperature on the dissolution rate of compacted montmorillonite under highly alkaline conditions [Clay Minerals, vol.51, p.275 (2016), Corrected Fig. 7.]

Sawaguchi, Takuma; Tsukada, Manabu; Yamaguchi, Tetsuji; Mukai, Masayuki

Clay Minerals, 51(5), P. 815, 2016/12

ERRATUM; Effects of OH$$^{-}$$ activity and temperature on the dissolution rate of compacted montmorillonite under highly alkaline conditions [Clay Minerals, vol.51, p.275 (2016), Corrected Fig. 7.]

Journal Articles

Chemical properties of rutherfordium (Rf) and dubnium (Db) in the aqueous phase

Nagame, Yuichiro; Kratz, J. V.*; Sch$"a$del, M.*

EPJ Web of Conferences, 131, p.07007_1 - 07007_8, 2016/12

BB2016-0022.pdf:0.96MB

 Times Cited Count:3 Percentile:72.98(Chemistry, Inorganic & Nuclear)

Journal Articles

First ionization potential of the heaviest actinide lawrencium, element 103

Sato, Tetsuya; Asai, Masato; Borschevsky, A.*; Stora, T.*; Sato, Nozomi*; Kaneya, Yusuke; Tsukada, Kazuaki; D$"u$llmann, C. E.*; Eberhardt, K.*; Eliav, E.*; et al.

EPJ Web of Conferences, 131, p.05001_1 - 05001_6, 2016/12

 Times Cited Count:0 Percentile:0.9(Chemistry, Inorganic & Nuclear)

Ionization efficiency in a surface ionization process depends on the first ionization potential of the atom. Based on the dependence, the ionization potential of the atom can be determined. We measured ionization efficiencies of fermium, einsteinium, mendelevium, and lawrencium by using a newly developed gas-jet coupled surface ion-source. The ionization potential of the elements have not been determined so far due to their low production rates and/or their short half-lives. Based on a relationship between the ionization efficiency and the ionization potential obtained via measurements of short-lived lanthanide isotopes, the ionization potentials of these actinide elements have been successfully determined.

Journal Articles

Dating of crush zones associated with plastic deformation of biotite; Constraints by fission-track thermochronometry

Sueoka, Shigeru; Shimada, Koji; Ishimaru, Tsuneari; Niwa, Masakazu; Yasue, Kenichi; Umeda, Koji*; Danhara, Toru*; Iwano, Hideki*

Fisshion, Torakku Nyusureta, (29), p.5 - 7, 2016/12

no abstracts in English

Journal Articles

Thermochronological contribution to the Crustal Dynamics Project

Tagami, Takahiro*; Sueoka, Shigeru; Kohn, B. P.*; Fukuda, Shoma*

Fisshion, Torakku Nyusureta, (29), p.1 - 2, 2016/12

no abstracts in English

Journal Articles

Report on the International Conference on Thermochronology 2016 in Maresias, Brazil

Sueoka, Shigeru; Tagami, Takahiro*

Fisshion, Torakku Nyusureta, (29), p.26 - 28, 2016/12

no abstracts in English

Journal Articles

Report on 40th Annual Meeting of Fission Track Research Group in Japan

Sueoka, Shigeru

Fisshion, Torakku Nyusureta, (29), p.29 - 34, 2016/12

no abstracts in English

Journal Articles

Measurement of atomic radii

Kaneko, Masashi

Gendai Kagaku, (549), P. 11, 2016/12

This article was made to explain the paper stating that atomic size was measured by computational method (R. Hoffmann, et al., Chem. Eur. J., 22, doi: 10.1002/chem.201602949) for student majoring chemistry. The estimation of atomic size was performed by means relativistic density functional theory. The atomic radii of noble gas and d-block elements were discussed.

Journal Articles

Characteristics of micro transfer paths and diffusion phenomena in the matrix of deep crystalline rock

Ishibashi, Masayuki; Sasao, Eiji; Hama, Katsuhiro

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 23(2), p.121 - 130, 2016/12

Matrix diffusion is one of the important phenomena for safety assessment of radioactive waste disposal because it has an effect of retarding the mass transport in crystalline rocks. Although there is not enough knowledge on the matrix diffusion in unaltered (intact) rocks around fractures. Intact granitic rocks around fractures are affected by primary alteration related to hydrothermal fluid resulting from crystallization of granitic magma. Therefore, detailed observations were carried out to clarify the effects of primary alteration focused on the intact granite around fractures sampled from the MIU, central Japan. The results of observation provide that the micropores are formed in plagioclases affected by primary alteration and have the potential of acting as matrix diffusion paths. This is indicating the possibility that intact granitic rock around fractures in an orogenic belt such as Japan have also the retardation functions due to matrix diffusion.

Journal Articles

Symposium on "Science of nuclear fuel cycle and backend; Research and education" with a memory of Professor Joonhong Ahn, the University of California, Berkeley

Nakayama, Shinichi; Okumura, Masahiko*; Nagasaki, Shinya*; Enokida, Yoichi*; Umeki, Hiroyuki*; Takase, Hiroyasu*; Kawasaki, Daisuke*; Hasegawa, Shuichi*; Furuta, Kazuo*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 23(2), p.131 - 148, 2016/12

A symposium "Science of nuclear fuel cycle and backend - Research and education -" was held at the Univer-sity of Tokyo in June 25, 2016. This aimed at developing the research on nuclear fuel cycle and backend. The time and the number of participants of the symposium were limited, but the active discussion was conducted, and the common perception for the future was shared among the experienced participants in those fields. This paper provides the discussions made in the symposium, and also, as a memory to Professor Ahn, the University of California, Berkeley, his prominent achievements in academic research and education.

Journal Articles

Additional information to report on site tour of the Fukushima Daiichi Nuclear Power Station

Suto, Toshiyuki

Genshiryoku, hoshasen Bukaiho (Internet), (19), P. 15, 2016/12

The Tritiated Water Task Force under METI's Committee on Countermeasures for Contaminated Water Treatment for Fukushima Daiichi Nuclear Power Plant (1F) reported that the option of post-dilution offshore release could dispose the tritiated water at a smallest cost in the shortest amount of time. The amount of tritium in the contaminated water at 1F was compared with ones released from nuclear power plants and reprocessing plants as some help for grasping its level of magnitude.

Journal Articles

One-year measurements of $$gamma$$-ray background using a high-purity germanium detector

Sakoda, Akihiro; Tanaka, Hiroshi; Ishimori, Yuu

Hoken Butsuri, 51(4), p.245 - 250, 2016/12

In the present work, the natural $$gamma$$-ray background was thoroughly measured using a high-purity germanium detector in a year (283.5 days in total, $$n$$ = 271). The data was first discussed in relation to radon concentrations in the laboratory. No correlations were found between the $$gamma$$-ray count rates from $$^{214}$$Pb and $$^{214}$$Bi and radon concentrations, meaning that radon just around the germanium detector was reduced to the negligible level by the introduction of nitrogen gas. Also, the count rates of major nuclides appeared to fluctuate with the coefficient of variance of a few up to several tens of percent, without seasonal variations. Furthermore, summing of all $$gamma$$-ray spectra allowed us to see neutron-induced peaks that cannot be detected in usual short-term measurements. All data obtained here would be the knowledge useful for the practice of $$gamma$$-ray measurements.

Journal Articles

Report on the Workshop "Radiation Research Based on Computer Simulation" held at the 59th Annual Meeting of the Japanese Radiation Research Society

Sato, Tatsuhiko; Hamada, Nobuyuki*

Hoshasen Seibutsu Kenkyu, 51(4), p.397 - 401, 2016/12

A workshop entitled "Radiation Research Based on Computer Simulation" was held at the 59th annual meeting of the Japanese Radiation Research Society. Approximately 50 participants attended the workshop, and six speakers gave a talk about their computational radiation biology studies. The title of the presentations are "Research on DNA damage and track structure simulation", "Study of cellular response based on stochastic model for simulating irradiated and non-irradiated cells", "Effectiveness of mathematical model for low-dose radiation effect", "Research on particle therapy based on cell surviving fraction model", "Development of model for natural induction of cataract", and "Mathematical model for carcinogenesis considering the differences of temporal and spatial doses". In the workshop, possible future collaborations were intensively discussed. This report briefly summarizes the outline of the workshop.

Journal Articles

Formation of carbon alloys by low-energy ion doping and its application for adsorptive desulfurization

Shimoyama, Iwao

Hoshasen To Sangyo, (141), p.7 - 11, 2016/12

Desulfurization is an indispensable process on hydrogen formation from fossil fuel. Adsorptive desulfurization, alternative to conventional hydrogenation desulfurization, requires development of stable activated carbon adsorbents with high performance. I study dopant dependence on thiophene adsorption for carbon alloys prepared by heteroatom doping using low-energy ion beam. I doped nitrogen and phosphorus as dopants of group 15 elements in graphite surfaces, and clarified that phosphorus is superior in thiophene adsorption to nitrogen, and that the effect of phosphorus is higher with room temperature doping than with high temperature doping by about 10 times. X-ray absorption spectroscopy indicated that local structures around phosphorus sites were different between them. I attribute the high adsorption property to formation of curved phosphorus sites prepared by room temperature doping. Above results suggest that the property of carbon alloy can be controlled by low-energy ion beam.

Journal Articles

Simultaneous recovery and separation of rare earth elements in ferromanganese nodules by using ${{it Shewanella putrefaciens}}$

Fujimoto, Jun*; Tanaka, Kazuya; Watanabe, Naoko*; Takahashi, Yoshio*

Hydrometallurgy, 166, p.80 - 86, 2016/12

 Times Cited Count:6 Percentile:31.51(Metallurgy & Metallurgical Engineering)

We examined recovery of REEs in Fe-Mn nodules by using ${{it Shewanella putrefaciens}}$ (Fe-reducing bacterium). In this method, Fe-Mn nodule decomposition and REE recovery were achieved simultaneously in a single solution system. Fe-Mn nodules were reductively decomposed in NaCl solution under anaerobic conditions with daily addition of sodium lactate as an electron donor. During the decomposition of Fe-Mn nodule, REEs released from the Fe-Mn nodule were adsorbed on bacterial cells. Of the conditions studied here, the best REE adsorption rates were obtained with 0.5M NaCl solution at pH7 with daily addition of 1 mmol sodium lactate.

Journal Articles

Local fields at nonmagnetic impurity sites in a perovskite $${rm La_{0.7}Ca_{0.3}MnO_3}$$

Sato, Wataru*; Komatsuda, Sayaka*; Osa, Akihiko; Sato, Tetsuya; Okubo, Yoshitaka*

Hyperfine Interactions, 237(1), p.113_1 - 113_6, 2016/12

 Times Cited Count:2 Percentile:61.78(Physics, Atomic, Molecular & Chemical)

The magnetic hyperfine field and electric field gradient at the$$^{111}$$Cd($$leftarrow$$ $$^{rm 111m}$$Cd) and $$^{rm 111}$$Cd($$leftarrow$$$$^{rm 111}$$In) probe nuclei introduced in a perovskite manganese oxide $${rm La_{0.7}Ca_{0.3}MnO_{3}}$$ ($$T_C$$ $$sim$$ 250 K) were measured for the study of the local magnetism and structure by means of time-differential perturbed angular correlation spectroscopy. In the ferromagnetic phase at 77 K, a very slight supertransferred magnetic hyperfine field (SMHF) ($$<$$ 0.014 T) combined with a well-defined electric field gradient was observed at the nonmagnetic $$^{111}$$Cd nucleus on the La/Ca A site. This observation suggests that the large magnetic hyperfine field ($$B_{hf}$$ = 6.9 T) measured, in our previous work, at the $$^{140}$$Ce probe nucleus on the A site originates from the contribution of a 4$$f$$ spin oriented by the SMHF from adjacent Mn ions.

Journal Articles

Solvent extraction and synergistic effect using an ionic liquid

Okamura, Hiroyuki; Shimojo, Kojiro

Ion Ekitai Kenkyu Saizensen To Shakai Jisso, p.220 - 227, 2016/12

Solvent extraction is a separation method based on the difference in the distribution of solutes between two immiscible liquid phases. Recently, ionic liquids have been widely investigated as novel extraction media. Solvent properties of an ionic liquid can be adjusted by combination of a cationic and an anionic component. It is, therefore, possible to provide an attractive reaction field as an extraction medium. In this article, specific extraction phenomena observed in the ionic liquid extraction system for metal ions were introduced.

Journal Articles

Contrast variation by dynamic nuclear polarization and time-of-flight small-angle neutron scattering, 1; Application to industrial multi-component nanocomposites

Noda, Yohei*; Koizumi, Satoshi*; Masui, Tomomi*; Mashita, Ryo*; Kishimoto, Hiromichi*; Yamaguchi, Daisuke; Kumada, Takayuki; Takata, Shinichi; Oishi, Kazuki*; Suzuki, Junichi*

Journal of Applied Crystallography, 49(6), p.2036 - 2045, 2016/12

 Times Cited Count:19 Percentile:78.58(Chemistry, Multidisciplinary)

Journal Articles

The Effect of oxidation-and-quenching process during a LOCA on the behavior of the oxidation and embrittlement of Zircaloy-4 cladding under reheating transients

Miwa, Hideki; Amaya, Masaki

Journal of Nuclear Science and Technology, 53(12), p.2090 - 2097, 2016/12

 Times Cited Count:6 Percentile:49.29(Nuclear Science & Technology)

Two-sided oxidation tests, ring compression tests and semi-integral quench tests on Zircaloy-4 cladding specimens were conducted under the temperature transient conditions simulating a post-quench reheat transient in order to evaluate the effect of high temperature oxidation and quenching during a LOCA on the behavior of the oxidation and embrittlement of the cladding under a loss of long-term-core-cooling condition. Test specimens prepared from non-irradiated Zircaloy-4 cladding tube were oxidized at a temperature between 1173 and 1473 K in steam flow and quenched by soaking the specimen in room temperature water. By using the test specimens, re-heating tests were performed in steam flow at a temperature between 1173 and 1473 K. The suppression of oxide layer growth and weight gain was observed under certain reheating-after-quenching conditions. Nevertheless, it seemed that the temperature transients including quenching-and-reheating process did not significantly affect the embrittlement of cladding. It was found that the embrittlement behavior of cladding during the temperature transients including quenching-and-reheating process could be dealt with on the basis of the ECR based on Baker-Just correlation.

Journal Articles

Phase transitions and polymerization of C$$_{6}$$H$$_{6}$$-C$$_{6}$$F$$_{6}$$ cocrystal under extreme conditions

Wang, Y.*; Wang, L.*; Zheng, H.*; Li, K.*; Andrzejewski, M.*; Hattori, Takanori; Sano, Asami; Katrusiak, A.*; Meng, Y.*; Liao, F.*; et al.

Journal of Physical Chemistry C, 120(51), p.29510 - 29519, 2016/12

 Times Cited Count:23 Percentile:62.07(Chemistry, Physical)

Pressure-induced polymerization (PIP) of aromatic molecules can generate saturated carbon nanostructures. As a strongly interacted $$pi$$-$$pi$$ stacking unit, the C$$_{6}$$H$$_{6}$$-C$$_{6}$$F$$_{6}$$ adduct is widely applied in supramolecular chemistry, and it provides a good preorganization for the PIP. Here we investigated the structural variation of C$$_{6}$$H$$_{6}$$-C$$_{6}$$F$$_{6}$$ cocrystal and the subsequent PIP process under high pressure. Four new molecular-complex phases V, VI, VII, and VIII have been identified and characterized by the in situ Raman, IR, synchrotron X-ray, and neutron diffraction. The phase V is different from the phases observed at low temperature, which has a tilted column structure. Phases VI and VII have a structure similar to phase V. Phase VIII polymerizes irreversibly upon compression above 25 GPa without any catalyst, producing sp$$^{3}$$(CH/F)$$_{n}$$ materials. The $$pi$$-$$pi$$ interaction is still dominant below 0.5 GPa but is most likely to be overstepped under further compression, which is important for discussing the supramolecular phase transition and the polymerization process.

Journal Articles

The Welded joint strength reduction factors of modified 9Cr-1Mo Steel for the advanced loop-type sodium cooled fast reactor

Yamashita, Takuya; Wakai, Takashi; Onizawa, Takashi; Sato, Kenichiro*; Yamamoto, Kenji*

Journal of Pressure Vessel Technology, 138(6), p.061407_1 - 061407_6, 2016/12

 Times Cited Count:0 Percentile:0(Engineering, Mechanical)

Journal Articles

Determination of optimal vapor pressure data by the second and third law methods

Nakajima, Kunihisa

Mass Spectrometry (Internet), 5(2), p.S0055_1 - S0055_6, 2016/12

Though equilibrium vapor pressures are utilized to determine thermodynamic properties of not only gaseous species but also condensed phases, the obtained data often disagree by a factor of 100 and more. A new data analysis method is proposed using the so-called second and third law procedures to improve accuracy of vapor pressure measurements. It was found from examination of vapor pressures of cesium metaborate and silver that the analysis of the difference between the second and third law values can result in determination of an optimal data set. Since the new thermodynamic method does not require special techniques and or experiences in dealing with measured data, it is reliable and versatile to improve the accuracy of vapor pressure evaluation.

Journal Articles

Development of inspection and repair techniques in reactor vessel of experimental fast reactor "Joyo"; Retrieval of the bent test subassembly

Ashida, Takashi; Ito, Hideaki; Miyamoto, Kazuyuki*; Nakamura, Toshiyuki; Koga, Kazuhiro*; Ohara, Norikazu*; Ino, Hiroichi*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 15(4), p.210 - 222, 2016/12

In the experimental fast reactor Joyo, it was confirmed that the top of the irradiation test sub-assembly of material testing rig named "MARICO-2" had been broken and bent onto the in-vessel storage rack as an obstacle and had damaged the upper core structure (UCS). As the result, for Joyo restart, it was necessary to replace the damaged UCS and to retrieve the bent sub-assembly. This paper describes in-vessel repair techniques performed in the retrieval work of the obstacle inside of the reactor vessel. The devices which were prepared for this work demonstrated expected performance under the environmental conditions of an SFR such as high temperature and radiation dose, and the work was completed in 2014. The successful operation of this retrieval work of the damaged component inside of a reactor vessel will contribute to the development of in-service inspections and repair technics in an SFR.

Journal Articles

Effect of seawater on heat transfer without boiling in internally heated annulus

Uesawa, Shinichiro; Liu, W.; Jiao, L.; Nagatake, Taku; Takase, Kazuyuki; Shibata, Mitsuhiko; Yoshida, Hiroyuki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 15(4), p.183 - 191, 2016/12

no abstracts in English

Journal Articles

Creep-fatigue evaluation method for weld joint of Mod.9Cr-1Mo steel, 2; Plate bending test and proposal of a simplified evaluation method

Ando, Masanori; Takaya, Shigeru

Nuclear Engineering and Design, 310, p.217 - 230, 2016/12

AA2016-0318.pdf:2.62MB

 Times Cited Count:1 Percentile:10.71(Nuclear Science & Technology)

In the present study, to develop an evaluation procedure and design rules for Mod.9Cr-1Mo steel weld joints, a method for creep-fatigue life evaluation of Mod.9Cr-1Mo steel weld joints was proposed based on the finite element analysis (FEA) results with a series of cyclic plate bending tests of the longitudinal and horizontal seamed plates. The strain concentration and redistribution behaviors were evaluated and failure cycles were estimated using FEA by considering the test conditions and metallurgical discontinuities in the weld joints. The elastic follow-up factors calculated from a comparison of the elastic and inelastic FEA results were determined to be less than 1.5. Based on the estimated elastic follow-up factors obtained via inelastic FEA, a simplified technique using elastic FEA was proposed for evaluating the creep-fatigue life in Mod.9Cr-1Mo steel weld joints.

Journal Articles

Effect of thermo-mechanical treatments on nano-structure of 9Cr-ODS steel

Oka, Hiroshi; Tanno, Takashi; Otsuka, Satoshi; Yano, Yasuhide; Uwaba, Tomoyuki; Kaito, Takeji; Onuma, Masato*

Nuclear Materials and Energy (Internet), 9, p.346 - 352, 2016/12

 Times Cited Count:21 Percentile:88.83(Nuclear Science & Technology)

Journal Articles

Dissolution behavior of lithium compounds in ethanol

Furukawa, Tomohiro; Hirakawa, Yasushi; Kondo, Hiroo; Kanemura, Takuji

Nuclear Materials and Energy (Internet), 9, p.286 - 291, 2016/12

BB2015-1402.pdf:3.16MB

 Times Cited Count:5 Percentile:36.53(Nuclear Science & Technology)

In order to exchange the components which received irradiation damage during the operation at the International Fusion Materials Irradiation Facility, the adhered lithium, which is partially converted to lithium compounds such as lithium oxide and lithium hydroxide, should be removed from the components. In this study, the dissolution experiments of lithium compounds (lithium nitride, lithium hydroxide, and lithium oxide) were performed in a candidate solvent, allowing the clarification of time and temperature dependence. Based on the results, a cleaning procedure for adhered lithium on the inner surface of the components was proposed.

Journal Articles

Effect of dissolved gas on mechanical property of sheath material of mineral insulated cables under high temperature and pressure water

Takeuchi, Tomoaki; Nakano, Hiroko; Uehara, Toshiaki; Tsuchiya, Kunihiko

Nuclear Materials and Energy (Internet), 9, p.451 - 454, 2016/12

 Times Cited Count:1 Percentile:10.71(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Tensile properties and hardness of two types of 11Cr-ferritic/martensitic steel after aging up to 45,000 h

Yano, Yasuhide; Tanno, Takashi; Sekio, Yoshihiro; Oka, Hiroshi; Otsuka, Satoshi; Uwaba, Tomoyuki; Kaito, Takeji

Nuclear Materials and Energy (Internet), 9, p.324 - 330, 2016/12

BB2015-1728.pdf:1.04MB

 Times Cited Count:14 Percentile:79.24(Nuclear Science & Technology)

Journal Articles

Strength anisotropy of rolled 11Cr-ODS steel

Tanno, Takashi; Yano, Yasuhide; Oka, Hiroshi; Otsuka, Satoshi; Uwaba, Tomoyuki; Kaito, Takeji

Nuclear Materials and Energy (Internet), 9, p.353 - 359, 2016/12

BB2015-1727.pdf:6.74MB

 Times Cited Count:9 Percentile:64.88(Nuclear Science & Technology)

Materials for core components of fusion reactors and fast reactors, such as blankets and fuel cladding tubes, must be excellent in high temperature strength and irradiation resistance because they will be exposed to high heat flux and heavy neutron irradiation. Oxide dispersion strengthened (ODS) steels have been developing as the candidate material. Japan Atomic Energy Agency (JAEA) have been developing 9 and 11 Chromium (Cr) ODS steels for advanced fast reactor cladding tubes. The JAEA 11Cr-ODS steels were rolled in order to evaluate their anisotropy. Tensile tests and creep tests of them were carried out at 700 $$^{circ}$$C in longitudinal and transverse orientation. The anisotropy of tensile strength was negligible, though that of creep strength was distinct. The observation results and chemical composition analysis suggested that the cause of the anisotropy in creep strength was prior powder boundary including Ti-rich precipitates.

Journal Articles

Overview and outcomes of the OECD/NEA benchmark study of the accident at the Fukushima Daiichi Nuclear Power Station

Nagase, Fumihisa; Gauntt, R. O.*; Naito, Masanori*

Nuclear Technology, 196(3), p.499 - 510, 2016/12

 Times Cited Count:19 Percentile:86.84(Nuclear Science & Technology)

The OECD/NEA Benchmark Study of the Accident at the Fukushima Daiichi Nuclear Power Station (BSAF) project was established in November 2012. The primary objectives of this benchmark study are to estimate accident progression and status inside the nuclear reactors, including fuel debris distribution, and consequently to contribute to the decommissioning activity at the Fukushima Daiichi Nuclear Power Plant. Fifteen organizations of eight countries calculated thermo-hydraulic behavior inside the three reactors for the time span of about six days from the occurrence of the earthquake with their severe accident integral codes. The submitted results were compared on coolant level change, hydrogen generation, initiation and progression of melt in fuel bundle and control blade, failure of reactor pressure vessel, distribution and composition of molten and solidified materials, and progression of molten core concrete interaction. This issue summarizes the results of the comparison and discussion with still remaining uncertainties and data needs as the output from the project.

Journal Articles

The Reaction mechanism of polyalcohol dehydration in hot pressurized water

Ruiz-Barragan, S.*; Ribas Ari$~n$o, J.*; Shiga, Motoyuki

Physical Chemistry Chemical Physics, 18(47), p.32438 - 32447, 2016/12

 Times Cited Count:8 Percentile:32.26(Chemistry, Physical)

The use of high-temperature liquid water (HTW) as a reaction medium is a very promising technology in the field of green chemistry. In order to fully exploit this technology, it is crucial to unravel the reaction mechanisms of the processes carried out in HTW. In this work, the reaction mechanism of 2,5-hexanediol dehydration in HTW has been studied by means of three different ab initio simulations: string method, metadynamics and molecular dynamics in real time. It is found that the whole reaction involving the protonation, bond exchange and the deprotonation occurs in a single step without a stable intermediate. The hydrogen bonded network of surrounding water has a vital role in assisting an efficient proton relay at the beginning and at the end of the reaction. It is confirmed that the reaction is energetically most favorable in the SN2 pathway with an estimated barrier of 36 kcal/mol, which explains the high stereo selectivity and the reaction rate observed in experiment.

Journal Articles

Superconductivity in repulsively interacting fermions on a diamond chain; Flat-band-induced pairing

Kobayashi, Keita*; Okumura, Masahiko; Yamada, Susumu; Machida, Masahiko; Aoki, Hideo*

Physical Review B, 94(21), p.214501_1 - 214501_7, 2016/12

 Times Cited Count:56 Percentile:89.32(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Azimuthally anisotropic emission of low-momentum direct photons in Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Hasegawa, Shoichi; Imai, Kenichi; Nagamiya, Shoji; Sako, Hiroyuki; Sato, Susumu; Tanida, Kiyoshi; PHENIX Collaboration*; 545 of others*

Physical Review C, 94(6), p.064901_1 - 064901_14, 2016/12

AA2016-0473.pdf:0.66MB

 Times Cited Count:74 Percentile:97.96(Physics, Nuclear)

Journal Articles

Measurements of double-helicity asymmetries in inclusive $$J/psi$$ production in longitudinally polarized $$p+p$$ collisions at $$sqrt{s}=510$$ GeV

Adare, A.*; Imai, Kenichi; Hasegawa, Shoichi; Nagamiya, Shoji; Sako, Hiroyuki; Sato, Susumu; Tanida, Kiyoshi; PHENIX Collaboration*; 328 of others*

Physical Review D, 94(11), p.112008_1 - 112008_10, 2016/12

AA2016-0475.pdf:0.51MB

 Times Cited Count:9 Percentile:42.39(Astronomy & Astrophysics)

Journal Articles

Characterization of the insoluble sludge from the dissolution of irradiated fast breeder reactor fuel

Aihara, Haruka; Arai, Yoichi; Shibata, Atsuhiro; Nomura, Kazunori; Takeuchi, Masayuki

Procedia Chemistry, 21, p.279 - 284, 2016/12

BB2015-3214.pdf:0.31MB

 Times Cited Count:5 Percentile:94.32(Chemistry, Inorganic & Nuclear)

Journal Articles

Flow-sheet study of MA recovery by extraction chromatography for SmART cycle project

Watanabe, So; Nomura, Kazunori; Kitawaki, Shinichi; Shibata, Atsuhiro; Kofuji, Hirohide; Sano, Yuichi; Takeuchi, Masayuki

Procedia Chemistry, 21, p.101 - 108, 2016/12

BB2015-3215.pdf:0.34MB

 Times Cited Count:14 Percentile:99.14(Chemistry, Inorganic & Nuclear)

Journal Articles

Effect of sludge behavior on performance of centrifugal contactor

Sakamoto, Atsushi; Sano, Yuichi; Takeuchi, Masayuki

Procedia Chemistry, 21, p.495 - 502, 2016/12

BB2016-0040.pdf:0.51MB

 Times Cited Count:2 Percentile:81.17(Chemistry, Inorganic & Nuclear)

Journal Articles

Uranium and plutonium extraction by ${it N,N}$-dialkylamides using multistage mixer-settler extractors

Ban, Yasutoshi; Hotoku, Shinobu; Tsutsui, Nao; Suzuki, Asuka; Tsubata, Yasuhiro; Matsumura, Tatsuro

Procedia Chemistry, 21, p.156 - 161, 2016/12

 Times Cited Count:5 Percentile:94.32(Chemistry, Inorganic & Nuclear)

A continuous counter-current experiment was carried out to demonstrate the validity of a process using ${it N,N}$-dialkylamides for recovering U and Pu. This process consisted of two cycles, and the 1st cycle and the 2nd cycle employed ${it N,N}$-di(2-ethylhexyl)-2,2-dimethylpropanamide and ${it N,N}$-di(2-ethylhexyl)butanamide as extractants, respectively. The feed solution for the 1st cycle was 5.1 mol/dm$$^{3}$$ (M) nitric acid containing 0.92 M U, 1.6 mM Pu, and 0.6 mM Np. The raffinate collected in the 1st cycle was used as the feed for the 2nd cycle. The ratios of U recovered in the U fraction and U-Pu fraction were 99.1% and 0.8%, respectively. The ratio of Pu recovered in the U-Pu fraction was 99.7%. The concentration ratio of U with respect to Pu in the U-Pu fraction was 9, and this indicated that Pu was not isolated. The decontamination factor of U with respect to Pu in the U fraction was obtained as 4.5$$times$$10$$^{5}$$. These results supported the validity of the proposed process.

Journal Articles

On the structure observed in the in-flight $$^{3}$$He($$K^{-}, Lambda p)n$$ reaction at J-PARC

Sekihara, Takayasu; Oset, E.*; Ramos, A.*

Progress of Theoretical and Experimental Physics (Internet), 2016(12), p.123D03_1 - 123D03_27, 2016/12

AA2016-0237.pdf:1.53MB

 Times Cited Count:37 Percentile:85.97(Physics, Multidisciplinary)

Journal Articles

Dynamics in condensed matter by 4SEASONS

Kajimoto, Ryoichi

Radioisotopes, 65(12), p.523 - 534, 2016/12

no abstracts in English

Journal Articles

Computational science simulations of laser coating processes using a metal powder direct injection system

Muramatsu, Toshiharu

Reza Kenkyu, 44(12), p.799 - 803, 2016/12

no abstracts in English

Journal Articles

Forest type effects on the retention of radiocesium in organic layers of forest ecosystems affected by the Fukushima nuclear accident

Koarashi, Jun; Atarashi-Andoh, Mariko; Matsunaga, Takeshi; Sanada, Yukihisa

Scientific Reports (Internet), 6, p.38591_1 - 38591_11, 2016/12

 Times Cited Count:46 Percentile:81.79(Multidisciplinary Sciences)

Forest-floor organic layers play a key role in controlling the overall bioavailability of $$^{137}$$Cs in forest ecosystems; however, there is still an insufficient understanding of how forest types influence the retention capability of $$^{137}$$Cs in organic layers in Japanese forest ecosystems. Here we conducted plot-scale investigations on the retention of $$^{137}$$Cs in organic layers at two contrasting forest sites in Fukushima. In a deciduous broad-leaved forest, approximately 80% of the deposited $$^{137}$$Cs migrated to mineral soil located below the organic layers within two years after the accident, with an ecological half-life of approximately one year. Conversely, in an evergreen coniferous forest, more than half of the deposited $$^{137}$$Cs remained in the organic layers, with an ecological half-life of 2.1 years. The observed retention behavior can be well explained by the tree phenology and accumulation of $$^{137}$$Cs associated with litter materials with different degrees of degradation in the organic layers.

Journal Articles

$$^{14}$$C ages and calendar years of Japanese swords measured with accelerator mass spectrometry

Nagata, Kazahiro*; Matsubara, Akihiro*; Kokubu, Yoko; Nakamura, Toshio*

Tetsu To Hagane, 102(12), p.736 - 741, 2016/12

 Times Cited Count:2 Percentile:12.27(Metallurgy & Metallurgical Engineering)

Steel of Japanese swords has been produced with Tatara process from iron sand and charcoal. Carbon dissolved in steel was absorbed from wooden charcoal fuel at the production of the steel. From the decay of $$^{14}$$C activity in the steel, the $$^{14}$$C age of Japanese sword can be determined. The $$^{14}$$C ages of 4 Japanese swords were calibrated to a few calendar years. There are several generations of the same names of sword masters. The year of production of each sword was determined from the calendar year and the sword master's name cut in the grip of his sword after taking the age of charcoal into account. The oldest calendar year with high probability agreed with the age of sword master.

Journal Articles

Efforts in the "Fugen"; The History of up to termination of operation and Efforts of decommissioning measures

Morishita, Yoshitsugu

Denki Hyoron, 101(11), p.24 - 29, 2016/11

no abstracts in English

Journal Articles

Development of a prediction system for radionuclide dispersion in Fukushima coast

Kamidaira, Yuki; Kawamura, Hideyuki; Kobayashi, Takuya; Uchiyama, Yusuke*

Doboku Gakkai Rombunshu, B2 (Kaigan Kogaku) (Internet), 72(2), p.I_451 - I_456, 2016/11

no abstracts in English

Journal Articles

Impact of mesoscale recirculation of the Kuroshio on asymmetric oceanic structure around Okinawa Island

Uchiyama, Yusuke*; Odani, Sachika*; Yamanishi, Takafumi*; Kamidaira, Yuki; Mitarai, Satoshi*

Doboku Gakkai Rombunshu, B2 (Kaigan Kogaku) (Internet), 72(2), p.I_481 - I_486, 2016/11

no abstracts in English

Journal Articles

Experiments EAGLE project for fast reactor safety; A Joint-research program with the Republic of Kazakhstan (NNC/RK)

Kamiyama, Kenji; Sato, Ikken; Kubo, Shigenobu

Enerugi Rebyu, 36(11), p.46 - 49, 2016/11

no abstracts in English

Journal Articles

Synthesis and characteristics of ternary Be-Ti-V beryllide pebbles as advanced neutron multipliers

Kim, Jae-Hwan; Nakamichi, Masaru

Fusion Engineering and Design, 109-111(Part B), p.1764 - 1768, 2016/11

 Times Cited Count:13 Percentile:77.16(Nuclear Science & Technology)

Journal Articles

Report on site tour of the Fukushima Nuclear Power Station

Suto, Toshiyuki

Gijutsushi, 28(11), p.8 - 11, 2016/11

Five years have passed since the accident of the Fukushima Daiichi Nuclear Power Station. The Nuclear and Radiation section of the Institute of Professional Engineers hosted a site tour of the plant to make themselves sure what is going on in it and to disseminate information about it. The conditions of landscape during traveling between the gathering place and the plant, each reactor, contaminated water treatment, site, and work environment improvement will be reported.

Journal Articles

Novel neutron scattering techniques using neutron transmission spectra

Oba, Yojiro*; Morooka, Satoshi; Sato, Hirotaka*; Sato, Nobuhiro*; Inoue, Rintaro*; Sugiyama, Masaaki*

Hamon, 26(4), p.170 - 173, 2016/11

Journal Articles

Journal Articles

Evaluation of DNA damage induced by Auger electrons from $$^{137}$$Cs

Watanabe, Ritsuko; Hattori, Yuya; Kai, Takeshi

International Journal of Radiation Biology, 92(11), p.660 - 664, 2016/11

 Times Cited Count:2 Percentile:19.71(Biology)

To understand the effect of internal exposure of $$^{137}$$Cs, we focus on estimation of microscopic energy deposition pattern and DNA damage induced by directly emitted electrons (beta-rays, internal conversion electrons, Auger electrons) from $$^{137}$$Cs. Monte Carlo track simulation method was used to calculate the microscopic energy deposition pattern. To simulate the energy deposition by directly emitted electrons, we considered the multiple ejections of electrons after internal conversion. Induction process of DNA strand breaks and base lesions was modeled and simulated using Monte Carlo methods for cell mimetic condition. The yield and spatial distribution of simple and complex DNA damage were calculated for the cases of $$gamma$$-rays and electrons from $$^{137}$$Cs. The simulation showed that significant difference of DNA damage spectrum was not caused by the difference between secondary electron spectrum by $$gamma$$-rays and directly ejected electron spectrum. The result support that the existing evaluation that internal exposure and external exposure are almost equivalent.

Journal Articles

Deceleration processes of secondary electrons produced by a high-energy Auger electron in a biological context

Kai, Takeshi; Yokoya, Akinari; Ukai, Masatoshi; Fujii, Kentaro; Watanabe, Ritsuko

International Journal of Radiation Biology, 92(11), p.654 - 659, 2016/11

 Times Cited Count:10 Percentile:68.36(Biology)

Journal Articles

Review of the microdosimetric studies for high-energy charged particle beams using a tissue-equivalent proportional counter

Tsuda, Shuichi; Sato, Tatsuhiko; Ogawa, Tatsuhiko; Sasaki, Shinichi*

JPS Conference Proceedings (Internet), 11, p.060004_1 - 060004_6, 2016/11

Track structure and energy deposition around charged particle beams in microscopic site of a living cell is important information for understanding of biological effects of energetic heavy ion beams. In this work, measurements of lineal energy ($$y$$) distributions for various kinds of ion beams have been performed for the verification of the microdosimetric function that incorporated in the PHITS code. In the international symposium focused on radiation detectors, the wall-less tissue equivalent proportional counter that developed in this study to measure $$y$$ distributions will be introduced, together with a series of data.

Journal Articles

Evaluation of neutron response of criticality accident alarm system detector to quasi-monoenergetic 24 keV neutrons

Tsujimura, Norio; Yoshida, Tadayoshi; Yashima, Hiroshi*

JPS Conference Proceedings (Internet), 11, p.050005_1 - 050005_6, 2016/11

Journal Articles

Performance of Panasonic ZP-1460 electronic personal dosemeter under exposure conditions likely to be found at Fukushima Daiichi Nuclear Power Plant

Tsujimura, Norio; Yoshida, Tadayoshi; Hoshi, Katsuya; Momose, Takumaro

JPS Conference Proceedings (Internet), 11, p.070008_1 - 070008_6, 2016/11

Journal Articles

Development of micro-structured fluorescent plates for high-resolution imaging

Sakai, Takuro; Yasuda, Ryo; Iikura, Hiroshi; Matsubayashi, Masahito

JPS Conference Proceedings (Internet), 11, p.020005_1 - 020005_6, 2016/11

Journal Articles

The Evaluation of the 0.07 mm and 3 mm dose equivalent with a portable beta spectrometer

Hoshi, Katsuya; Yoshida, Tadayoshi; Tsujimura, Norio; Okada, Kazuhiko

JPS Conference Proceedings (Internet), 11, p.070009_1 - 070009_6, 2016/11

Beta spectra of various nuclide species were measured by commercially available compact spectrometer. The shape of spectra obtained from the spectrometer approximately agreed with that of theoretical spectra. The beta dose equivalent at any depths has been able to be obtained as a product of measured pulse height spectra and appropriate conversion coefficients of ICRP Publ. 74. The dose rates evaluated from the spectra were comparable to the reference dose rates of standard beta calibration sources. And, we were able to determine the dose equivalent with relative error of indication of 10% without the complicated correction.

Journal Articles

Measurement of radioactive contamination on work clothing of workers engaged in decontamination operations

Tsujimura, Norio; Yoshida, Tadayoshi; Hoshi, Katsuya

JPS Conference Proceedings (Internet), 11, p.070003_1 - 070003_7, 2016/11

Journal Articles

Influence of temperature histories during reactor startup periods on microstructural evolution and mechanical properties of austenitic stainless steel irradiated with neutrons

Kasahara, Shigeki; Kitsunai, Yuji*; Chimi, Yasuhiro; Chatani, Kazuhiro*; Koshiishi, Masato*; Nishiyama, Yutaka

Journal of Nuclear Materials, 480, p.386 - 392, 2016/11

 Times Cited Count:0 Percentile:0.01(Materials Science, Multidisciplinary)

This paper addresses influence of two different temperature profiles during startup periods in the Japan Materials Testing Reactor and a boiling water reactor upon microstructural evolution and mechanical properties of austenitic stainless steel irradiated with neutrons to about 1 dpa and 3 dpa. Tensile tests at 290$$^{circ}$$C and Vickers hardness tests at room temperature were carried out, and their microstructures were observed by FEG-TEM. Influence of difference in the temperature profiles was observed obviously in interstitial cluster formation, in particular, growth of Frank loops. The influence was also found certainly in loss of strain hardening capacity and ductility, although the influence on the yield strength and the Vickers hardness was not clearly observed. As a result, Frank loops, which were observed in austenitic stainless steel irradiated at doses of 1 dpa or more, were considered to contribute to deformation of the austenitic stainless steel.

Journal Articles

Effect of hydrocarbons on the efficiency of catalytic reactor of detritiation system in an event of fire

Edao, Yuki; Sato, Katsumi; Iwai, Yasunori; Hayashi, Takumi

Journal of Nuclear Science and Technology, 53(11), p.1831 - 1838, 2016/11

 Times Cited Count:8 Percentile:60.26(Nuclear Science & Technology)

Journal Articles

Nanoscopic structural investigation of physically cross-linked nanogels formed from self-associating polymers

Sekine, Yurina; Endo, Hitoshi*; Iwase, Hiroki*; Takeda, Shigeo*; Mukai, Sadaatsu*; Fukazawa, Hiroshi; Littrell, K. C.*; Sasaki, Yoshihiro*; Akiyoshi, Kazunari*

Journal of Physical Chemistry B, 120(46), p.11996 - 12002, 2016/11

 Times Cited Count:10 Percentile:26.96(Chemistry, Physical)

The detailed structure of a nanogel formed by self-association of cholesterol-bearing pullulans (CHP) was determined by contrast variation small-angle neutron scattering. The decomposition of scattering intensities into partial scattering functions of each CHP nanogel component, i.e., pullulan, cholesterol, and the cross-term between the pullulan and the cholesterol allows us to investigate the internal structure of the nanogel. The effective spherical radius of the skeleton formed by pullulan chains was found to be about 8.1 nm. In the CHP nanogel, there are about 19 cross-linking points where a cross-linking point is formed by aggregation of trimer cholesterol molecules with the spatially inhomogeneous distribution of the mass fractal dimension of 2.6. The average radius of the partial chains can also be determined to be 1.7 nm. As the result, the complex structure of the nanogels is coherently revealed at the nanoscopical level.

Journal Articles

Year-round variations in the fluvial transport load of particulate $$^{137}$$Cs in a forested catchment affected by the Fukushima Daiichi Nuclear Power Plant accident

Matsunaga, Takeshi; Nakanishi, Takahiro; Atarashi-Andoh, Mariko; Takeuchi, Erina; Muto, Kotomi; Tsuzuki, Katsunori; Nishimura, Shusaku; Koarashi, Jun; Otosaka, Shigeyoshi; Sato, Tsutomu*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 310(2), p.679 - 693, 2016/11

AA2015-0821.pdf:3.78MB

 Times Cited Count:6 Percentile:49.29(Chemistry, Analytical)

Particulate $$^{137}$$Cs in stream water was collected continuously for two years in order to assess the long-term trend of the $$^{137}$$Cs discharge from the forest environment. Sampling was conducted from December 2011 to December 2013 in a mountainous stream, which received the $$^{137}$$Cs from the Fukushima Daiichi Nuclear Power Plant accident. A seasonal increase in fluvial transport load of particulate $$^{137}$$Cs associated with suspended solids (SS) was observed in August and September when rainfall was abundant. The particulate $$^{137}$$Cs concentration decreased at a faster rate than the rate due to radioactive decay. This decrease might be resulted from redistribution of the easily eroded and polluted soil surface due to heavy rain events such as typhoons. These findings indicate that the particulate $$^{137}$$Cs load was subject to the inter-annual variations in rainfalls, and decreased gradually over a long period of time due to a decrease in $$^{137}$$Cs concentration in SS.

Journal Articles

Texture measurement of A1050 aluminum alloy using neutron diffraction

Xu, P. G.; Harjo, S.; Onuki, Yusuke*

Kako To Netsushori Niyoru Yusen Hoi Seigyo, p.1 - 6, 2016/11

no abstracts in English

Journal Articles

Assessment of radiation doses to the public and its management in the areas contaminated by a nuclear accident

Takahara, Shogo

Kankyo Eisei Kogaku Kenkyu, 30(4), p.12 - 30, 2016/11

no abstracts in English

Journal Articles

Survey and countermeasures on radiocesium inflow into a laboratory building for radioactivity analysis

Kurita, Yoshiyuki; Saegusa, Jun; Maeda, Satoshi

Nihon Hoshasen Anzen Kanri Gakkai-Shi, 15(2), p.180 - 185, 2016/11

In 2012, JAEA has established a laboratory in Fukushima-city to implement radioactivity analysis of environmental samples. Key nuclides measured in this laboratory are $$^{134}$$Cs and $$^{137}$$Cs (radiocesium). For the purpose, situation of radiocesium inflow into the laboratory building and its effects were investigated based on high-resolution gamma-spectrometry with germanium detectors. As a result, the surface density of radiocesium in the laboratory was found to be far below the minimum detectable activities of survey instruments routinely used for radiation control purposes.

Journal Articles

Flux pinning properties in YBCO films with growth-controlled nano-dots and heavy-ion irradiation defects

Sueyoshi, Tetsuro*; Kotaki, Tetsuya*; Uraguchi, Yusei*; Suenaga, Momotaro*; Makihara, Takahiro*; Fujiyoshi, Takanori*; Ishikawa, Norito

Physica C, 530, p.72 - 75, 2016/11

 Times Cited Count:9 Percentile:41.22(Physics, Applied)

In order to clarify the influence of size and spatial distribution of three-dimensional pinning centers (3D-PCs) on hybrid flux pinning, columnar defects (CDs) were installed by using 200 MeV Xe ions along the $$c$$-axis direction into quasi-multilayered films consisting of YBa$$_{2}$$Cu$$_{3}$$Oy layers and pseudo layers of BaSnO$$_{3}$$. The positive effect of the BaSnO$$_{3}$$ doping on the hybrid flux pinning stands out for the critical current density $$J_{rm c}$$ around $$B parallel c$$ in high magnetic field and/or inclined magnetic field off the $$c$$-axis, whereas there is little difference in the $$J_{rm c}$$ at $$B parallel c$$ among the same growth temperature samples for low magnetic field. In the case of the in-plane distributed BaSnO$$_{3}$$ nano-dots, the Jc around $$B parallel ab$$ is remarkably enhanced, whereas there is a detrimental effect on the Jc around $$B parallel c$$. These imply that the tuning of 3D-PCs is one of the keys to improve the $$J_{rm c}$$ at all magnetic field orientations for the hybrid flux pinning.

Journal Articles

Spin transport in half-metallic ferromagnets

Onuma, Yuichi; Matsuo, Mamoru; Maekawa, Sadamichi

Physical Review B, 94(18), p.184405_1 - 184405_5, 2016/11

 Times Cited Count:23 Percentile:67.71(Materials Science, Multidisciplinary)

We theoretically investigate spin transport in half-metallic ferromagnets at finite temperatures. The side-jump and skew-scattering contributions to spin Hall conductivity are derived using the Kubo formula. The electron-magnon interaction causes a finite density of states in the energy gap of the minority-spin band and induces spin Hall conductivity. We show that spin Hall conductivity is proportional to $$T^{3/2}$$, with $$T$$ being temperature and is sensitive to $$T$$. We propose that spin Hall conductivity may be a tool to study the minority-spin state.

Journal Articles

Measurements of directed, elliptic, and triangular flow in Cu+Au collisions at $$sqrt{s_{NN}}$$=200 GeV

Adare, A.*; Hasegawa, Shoichi; Imai, Kenichi; Nagamiya, Shoji; Sako, Hiroyuki; Sato, Susumu; Tanida, Kiyoshi; PHENIX Collaboration*; 397 of others*

Physical Review C, 94(5), p.054910_1 - 054910_18, 2016/11

AA2016-0472.pdf:0.98MB

 Times Cited Count:24 Percentile:84.18(Physics, Nuclear)

Journal Articles

Nitrogen hot trap design and manufactures for lithium test loop in IFMIF/EVEDA project

Wakai, Eiichi; Watanabe, Kazuyoshi*; Ito, Yuzuru*; Suzuki, Akihiro*; Terai, Takayuki*; Yagi, Juro*; Kondo, Hiroo; Kanemura, Takuji; Furukawa, Tomohiro; Hirakawa, Yasushi; et al.

Plasma and Fusion Research (Internet), 11, p.2405112_1 - 2405112_4, 2016/11

BB2015-1982.pdf:2.03MB

Journal Articles

Improvement of ex-vessel molten core behavior models for the JASMINE code

Matsumoto, Toshinori; Kawabe, Ryuhei; Sugiyama, Tomoyuki; Maruyama, Yu

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 9 Pages, 2016/11

During severe accident at nuclear power stations, molten core material jet could be discharged from the reactor pressure vessel into the water pool formed at the pedestal or cavity in the containment vessel. To improve the JASMINE code, The method for determining particle diameters which follow the Rosin-Rammler distribution was implemented. The jet breakup experiments, DEFOR-A conducted by KTH (Royal Institute of Technology, Sweden) were analyzed with the code. The influence of the experimental conditions, such as water subcooling, melt jet diameter and superheat were discussed. A crust layer formation model was also implemented in the code. The analyses using the model were carried out for the melt spreading experiments, PULiMS conducted by KTH. The spreading area was overestimated. Further improvement of the melt spreading model were discussed to close the gaps by introducing additional models such as heat conduction in the substrate materials, void formed inside the melt and so on.

Journal Articles

CFD simulation of a CIGMA experiment CC-PL-04 on the containment thermal hydraulics affected by the outer surface cooling

Ishigaki, Masahiro; Abe, Satoshi; Shibamoto, Yasuteru; Yonomoto, Taisuke

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 10 Pages, 2016/11

no abstracts in English

Journal Articles

Development of air cooling performance evaluation method for fuel debris on retrieval of Fukushima Daiichi NPS by dry method, 2; Outline of numerical method and preliminary analysis of free convection around fuel debris

Yamashita, Susumu; Uesawa, Shinichiro; Yoshida, Hiroyuki

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

In fuel debris retrieval in decommissioning of the Fukushima Daiichi NPS, dry method is under consideration. Investigation of the cooling performance of fuel debris in the dry method will be very important problem to realize the method. However, there are uncertainties in the shape and surface temperature of fuel debris. In order to evaluate the cooling performance, the investigation of the cooling performance by free convection is required. We have been developing the numerical simulation method, which can evaluate the cooling performance of the fuel debris by free convection, using the JUPITER code in JAEA. In this paper, we show the evaluation result of the thermal conductivity by the free convection from fuel debris to the atmosphere in the simplified system.

Journal Articles

Analysis with CFD code for THAI test on thermal-hydraulics during PAR activation

Sato, Masatoshi; Matsumoto, Toshinori; Sugiyama, Tomoyuki; Maruyama, Yu

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 10 Pages, 2016/11

Journal Articles

Water experiments on thermal striping in reactor vessel of advanced sodium-cooled fast reactor; Influence of flow collector of backup CR guide tube

Kobayashi, Jun; Ezure, Toshiki; Tanaka, Masaaki; Kamide, Hideki

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 5 Pages, 2016/11

JAEA has been conducting a design study for an advanced large-scale sodium-cooled fast reactor (SFR). Hot sodium from the fuel subassembly can mix with the cold sodium from the control rod (CR) channel at the bottom of Upper Internal Structure (UIS). Temperature fluctuation due to the fluid mixing at the core outlet may cause high cycle thermal fatigue at the bottom of UIS. JAEA had performed a water experiment to examine countermeasures for the significant temperature fluctuation generated at the bottom of SFRs UIS. Meanwhile, a self-actuated shutdown system (SASS) is equipped in a backup control rod (BCR) channel to ensure reactor shutdown. The BCR guide tubes have a flow guide structure "flow-collector" to provide reliable operation of SASS. Flow-collector may affect the thermal mixing behavior at the bottom of the UIS. This study has investigated the influence of the flow- collector on characteristics of the temperature fluctuation around the BCR channels.

Journal Articles

Event sequence analyses of a forest fire heat effect on a sodium-cooled fast reactor for an external hazard PRA methodology development

Okano, Yasushi; Yamano, Hidemasa

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 9 Pages, 2016/11

This paper deals with an event sequence by forest fire heat effect on a decay heat removal function of a sodium-cooled fast reactor. Related to the potential vulnerability, an event scenario was developed using conservative assumptions. An event tree was developed with an initiating event of the loss of off-site power, and the headings are related to "external diesel fuel tanks", "emergency diesel generator and its auxiliary system", "alternative cooling system and its power source", and "decay heat air cooler". A failure probability on each heading was given from a fragility curve as a function of reaction intensity or by assumptions based on conservative models. A core damage frequency, under the conditional of the loss of off-site power, was conservatively evaluated around 10$$^{-7}$$/year. A key heading in the event tree with large effect on the frequency is the intactness of the external diesel fuel tanks.

Journal Articles

Development of extreme rainfall PRA methodology for sodium-cooled fast reactor

Nishino, Hiroyuki; Kurisaka, Kenichi; Yamano, Hidemasa

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 10 Pages, 2016/11

Journal Articles

Event sequence analysis of core disruptive accident in a metal-fueled sodium-cooled fast reactor

Yamano, Hidemasa; Tobita, Yoshiharu; Kubo, Shigenobu; Ueda, Nobuyuki*

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 10 Pages, 2016/11

In this study, the event sequence analysis of CDA in a large metal-fueled SFR has been performed in order to investigate reactivity progression and molten fuel relocation behavior in the metal-fueled SFR. The initiating phase analysis during the CDA initiated by unprotected loss-of-flow accidents has been conducted using the CANIS code, which showed a small power peak. Using the initial conditions based on the initiating phase analysis, the SIMMER-III code was applied to a whole-core scale analyses to clarify the event sequence including the reactivity progression and molten fuel relocation. As a result, recriticality in the whole core analysis resulted in a very mild energy release. The mild energy release in the metal-fueled core can be attributed to the small specific heat of metal fuel and the large prompt negative reactivity feedback mechanism.

Journal Articles

Development of air cooling performance evaluation method for fuel debris on retrieval of Fukushima Daiichi NPS by dry method, 3; Heat transfer and flow visualization experiment of free convection adjacent to upward facing horizontal surface

Uesawa, Shinichiro; Shibata, Mitsuhiko; Yamashita, Susumu; Yoshida, Hiroyuki

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

Journal Articles

In-vessel retention of unprotected accident in a fast reactor; Assessment of material-relocation and heat-removal behavior in ULOF

Sogabe, Joji; Suzuki, Toru; Wada, Yusaku; Tobita, Yoshiharu

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

Journal Articles

Improvements to the simmer code model for steel wall failure based on EAGLE-1 test results

Toyooka, Junichi; Kamiyama, Kenji; Tobita, Yoshiharu; Suzuki, Toru

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

Journal Articles

Experimental database for bed formation behaviors of solid particles

Sheikh, M. A. R.*; Son, E.*; Kamiyama, Motoki*; Morioka, Toru*; Matsumoto, Tatsuya*; Morita, Koji*; Matsuba, Kenichi; Kamiyama, Kenji; Suzuki, Toru

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 10 Pages, 2016/11

During the material relocation phase of core disruptive accidents in sodium-cooled fast reactors, the sedimentation behavior of fragmented debris leading to the formation of debris beds is crucial for in-vessel retention by debris bed cooling. In this study, a series of experiments using simulant materials was performed to develop an experimental database of bed formation behavior by gravity driven discharge of solid particles from a nozzle into a quiescent cylindrical water pool. The bed height as well as the bed shape was measured. Three types of spherical and non-spherical particles, namely Al$$_{2}$$O$$_{3}$$, ZrO$$_{2}$$ and stainless steel with different size were employed to study the effect of key experimental parameter on debris bed mound shape. Based on the experimental results, an empirical correlation as experimental database was proposed to predict the particle bed height. The proposed correlation reasonably reproduces the experimental trend of the bed height variation on the crucial factors. This result demonstrates a wide applicability of the proposed empirical model to predict the bed height in terms of all crucial factors with reasonable accuracy.

Journal Articles

A Recent experimental program to evidence in-vessel retention by controlled material relocation during core disruptive accidents of sodium-cooled fast reactors

Matsuba, Kenichi; Kamiyama, Kenji; Toyooka, Junichi; Zuev, V. A.*; Ganovichev, D. A.*; Kolodeshnikov, A. A.*

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 5 Pages, 2016/11

Molten fuel discharge through control rod guide tubes (CRGTs) is a key process that dominates the termination of core disruptive accidents of sodium-cooled fast reactors, since fuel dispersion from the core contributes to the achievement of both deeper subcriticality in the degraded core and formation of coolable debris bed. Within a framework of a collaborative research program between Japan Atomic Energy Agency and National Nuclear Center of the Republic of Kazakhstan, called EAGLE program, a new experimental program has been started with out-of-pile experiments to clarify the fuel discharge through CRGTs. This paper presents the status of the new program, including experimental results obtained so far.

Journal Articles

Production of droplets during liquid jet impingement onto a flat plate

Yi, Z.*; Oya, Naoki*; Enoki, Koji*; Okawa, Tomio*; Ohno, Shuji; Aoyagi, Mitsuhiro; Takata, Takashi

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

It is important to set the amount of sodium droplet mechanistically for appropriate numerical evaluations of sodium leak and fire behavior in a sodium-cooled fast reactor plant. In the present work, fundamental experiments were performed to measure the splash ratio during the vertical water jet impact onto a horizontal wall. It was shown that the splash ratio can be correlated well as a function of the impact Weber number, the Strouhal number and the Ohnesorge number of the droplets impinging the liquid film.

Journal Articles

Identification of important phenomena under sodium fire accidents based on PIRT process with factor analysis in sodium-cooled fast reactor

Aoyagi, Mitsuhiro; Uchibori, Akihiro; Kikuchi, Shin; Takata, Takashi; Ohno, Shuji; Ohshima, Hiroyuki

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 10 Pages, 2016/11

The present PIRT process was aimed to identify key phenomena involved in sodium fire accidents that involve complex phenomena in sodium-cooled fast reactor plants. In this PIRT process, the figures of merit (FOMs) were specified through factor analysis. Associated phenomena were identified through the element- and sequence-based phenomena analyses. Importance of each associated phenomenon was evaluated by considering the sequence-based analysis of associated phenomena correlated with the FOMs. Then, we complete the ranking table through the factor and phenomenon analyses.

Journal Articles

Development of air cooling performance evaluation method for fuel debris on retrieval of Fukushima Daiichi NPS by dry method, 1; Outline of research project

Yoshida, Hiroyuki; Uesawa, Shinichiro; Yamashita, Susumu; Nagase, Fumihisa

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

Journal Articles

Study on spray cooling capability for spent fuel pool at coolant loss accident, 1; Research plan

Liu, W.; Nagatake, Taku; Shibata, Mitsuhiko; Koizumi, Yasuo; Yoshida, Hiroyuki; Nemoto, Yoshiyuki; Kaji, Yoshiyuki

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 4 Pages, 2016/11

The Fukushima Daiichi NPP accident asks that the accident management of the LOCA in the SFPs must be considered to avoid occurrences of severe accident in the SFPs. To prevent the failure of the spent fuel assemblies at the LOCA, transportable spray systems are expected to be put into use to discharge water into fuel assemblies to moderate the temperature increase. To apply the spray system as a countermeasure for the LOCA of the SFP, the capability of the spray cooling system must be evaluated to keep the spent fuel rods safety. JAEA has started the research project to investigate the spray cooling capability for the SFP. In this research project, we aim to construct a numerical simulation method for evaluating the capability of the spray cooling. To develop the method, the basic key phenomena that affect the cooling performance must be clarified and the validation data required for the code development. To clarify the basic key phenomena that affect the cooling performance, that is, the CCFL and the drop size effect on the CCFL, and to obtain the code validation data, we are planning to carry out 2 experiments with two test sections, the spray visualization experiment and the spray cooling experiment. The spray visualization test section aims to get CCFL data in air-water two-phase flow and to understand the two-phase flow behavior over the upper tie plate. The spray cooling test section aims to get the CCFL data in steam-water two-phase flow and to obtain the validation data. This paper focus on the outline of the research plan for the whole research project.

Journal Articles

Development of evaluation method for hydraulic behavior in venturi scrubber for filtered venting

Horiguchi, Naoki; Yoshida, Hiroyuki; Nakao, Yasuhiro*; Kaneko, Akiko*; Abe, Yutaka*

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

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