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Journal Articles

Superfluid signatures in a dissipative quantum point contact

Huang, M.-Z.*; Mohan, J.*; Visuri, A.-M.*; Fabritius, P.*; Talebi, M.*; Wili, S.*; Uchino, Shun; Giamarchi, T.*; Esslinger, T.*

Physical Review Letters, 130(20), p.200404_1 - 200404_8, 2023/05

 Times Cited Count:4 Percentile:88.42(Physics, Multidisciplinary)

We measure superfluid transport of strongly-interacting fermionic lithium atoms through a quantum point contact with local, spin-dependent particle loss. We observe that the characteristic non-Ohmic superfluid transport enabled by high-order multiple Andreev reflections transitions into an excess Ohmic current as the dissipation strength exceeds the superfluid gap. We develop a model with mean-field reservoirs connected via tunneling to a dissipative site. Our calculations in the Keldysh formalism reproduce the observed non-equilibrium particle current, yet do not fully explain the observed loss rate or spin current.

Journal Articles

Post fission time evolution calculation by FIFRELIN coupled with PHITS and DCHAIN

Ogawa, Tatsuhiko; Litaize, O.*; Mancusi, D.*; Chebboubi, A.*; Serot, O.*

European Physical Journal A, 58(8), p.153_1 - 153_9, 2022/08

 Times Cited Count:1 Percentile:33.4(Physics, Nuclear)

The Monte-Carlo code FIFRELIN was originally developed for the simulation of first chance fission of fissile nuclei. It can predict fission observables such as fragment yields and neutron yields accurately by using experimental data and databases. However, FIFRELIN cannot calculate remnant dose and decay heat considering delayed decay of fission fragments. Moreover, FIFRELIN can predict the energy spectra of neutrons and gammas but further transport calculation required generation of heavy external files. In this study, FIFRELIN was interfaced to radiation transport code PHITS to perform burn up calculation and particle transport calculation. Owing to the burn up calculation, decay heat and remnant dose were calculated for given irradiation condition and cooling period. Interface of particle transport calculation by PHITS and FIFRELIN can perform particle transport simulation based on the source term calculated by FIFRELIN.

Journal Articles

Effect of particle size on the colonization of biofilms and the potential of biofilm-covered microplastics as metal carriers

Wu, C.*; Tanaka, Kazuya; Tani, Yukinori*; Bi, X.*; Liu, J.*; Yu, Q.*

Science of the Total Environment, 821, p.153265_1 - 153265_9, 2022/05

 Times Cited Count:21 Percentile:94.35(Environmental Sciences)

Microplastics (MPs) with different particle sizes were co-cultured with a model freshwater fungus, ${it Acremonium strictum}$ strain KR21-2, to form biofilms on their surface. We also determined the changes in surface physicochemical properties of the biofilm-covered MPs (BMPs) and the heavy metal adsorption capacity of the original MPs and BMPs. The results revealed that the biofilms improve the adsorption of heavy metals on MPs, and the particle size of MPs plays a crucial role in biofilm colonization and adsorption of heavy metals by BMPs.

Journal Articles

A Comparative CFD exercise on bubble hydrodynamics using Euler-Euler and interface tracking approaches

Dehbi, A.*; Cheng, X.*; Liao, Y.*; Okagaki, Yuria; Pellegrini, M.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 15 Pages, 2022/03

Journal Articles

Integration of pool scrubbing research to enhance source-term calculations (IPRESCA) project

Gupta, S.*; Herranz, L. E.*; Lebel, L. S.*; Sonnenkalb, M.*; Pellegrini, M.*; Marchetto, C.*; Maruyama, Yu; Dehbi, A.*; Suckow, D.*; K$"a$rkel$"a$, T.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

Journal Articles

Study of charged particle activation analysis, 2; Determination of boron concentration in human blood samples

Ikebe, Yurie*; Oshima, Masumi*; Bamba, Shigeru*; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi*; Bi, C.*; Seto, Hirofumi*; Amano, Hikaru*; et al.

Applied Radiation and Isotopes, 164, p.109106_1 - 109106_7, 2020/10

 Times Cited Count:2 Percentile:24.28(Chemistry, Inorganic & Nuclear)

Boron Neutron Capture Therapy (BNCT) is a radiotherapy for the treatment of intractable cancer. In BNCT precise determination of $$^{10}$$B concentration in whole blood sample before neutron irradiation is crucial for control of the neutron irradiation time and the neutron dosimetry. We have applied the Charged Particle Activation Analysis (CPAA) to non-destructive and accurate determination of $$^{10}$$B concentration in whole blood sample. The experiment was performed at JAEA Tandem Accelerator using an 8 MeV proton beam. The 478 keV $$gamma$$ ray of $$^{7}$$Be produced in the $$^{10}$$B(p,$$alpha$$)$$^{7}$$Be reaction was used to quantify the $$^{10}$$B, and $$gamma$$ rays of $$^{56}$$Co originating from the reaction with Fe in blood was used to normalize the $$gamma$$-ray intensity. The results demonstrated that the present CPAA method can be applied to the determination of the $$^{10}$$B concentration in the blood sample.

Journal Articles

The Joint evaluated fission and fusion nuclear data library, JEFF-3.3

Plompen, A. J. M.*; Cabellos, O.*; De Saint Jean, C.*; Fleming, M.*; Algora, A.*; Angelone, M.*; Archier, P.*; Bauge, E.*; Bersillon, O.*; Blokhin, A.*; et al.

European Physical Journal A, 56(7), p.181_1 - 181_108, 2020/07

 Times Cited Count:321 Percentile:99.41(Physics, Nuclear)

The Joint Evaluated Fission and Fusion nuclear data library 3.3 is described. New evaluations for neutron-induced interactions with the major actinides $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu, on $$^{241}$$Am and $$^{23}$$Na, $$^{59}$$Ni, Cr, Cu, Zr, Cd, Hf, W, Au, Pb and Bi are presented. It includes new fission yileds, prompt fission neutron spectra and average number of neutrons per fission. In addition, new data for radioactive decay, thermal neutron scattering, gamma-ray emission, neutron activation, delayed neutrons and displacement damage are presented. JEFF-3.3 was complemented by files from the TENDL project. The libraries for photon, proton, deuteron, triton, helion and alpha-particle induced reactions are from TENDL-2017. The demands for uncertainty quantification in modeling led to many new covariance data. A comparison between results from model calculations using the JEFF-3.3 library and those from benchmark experiments for criticality, delayed neutron yields, shielding and decay heat, reveals that JEFF-3.3 is excellent for a wide range of nuclear technology applications, in particular nuclear energy.

Journal Articles

Sensitivity of charged particle activation analysis for long-lived radioactive nuclide determination

Oshima, Masumi*; Yamaguchi, Yurie*; Asai, Masato; Tsukada, Kazuaki; Goto, Jun*; Bamba, Shigeru*; Bi, C.*; Morimoto, Takao*

Journal of Nuclear Science and Technology, 56(9-10), p.866 - 872, 2019/09

 Times Cited Count:1 Percentile:11.15(Nuclear Science & Technology)

Sensitivity of charged particle activation analysis with 8 MeV proton beam was studied for determination of 35 long-lived radioactive nuclides. Reaction cross sections for those nuclides were estimated with ALICE-91 code and isomer yield ratios were estimated from those of neighboring isotopes by taking into account their spins and parities. It was found that the proposed charged particle activation analysis should show high sensitivity for the determination of several hardly measurable nuclides with long half-lives such as $$^{135}$$Cs, $$^{244}$$Pu, $$^{129}$$I, $$^{126}$$Sn, $$^{93}$$Mo, $$^{107}$$Pd, $$^{236}$$U, $$^{248}$$Cm, and $$^{237}$$Np.

Journal Articles

ETSON-MITHYGENE benchmark on simulations of upward flame propagation experiment in the ENACCEF2 experimental facility

Bentaib, A.*; Chaumeix, N.*; Grosseuvres, R.*; Bleyer, A.*; Gastaldo, L.*; Maas, L.*; Jallais, S.*; Vyazmina, E.*; Kudriakov, S.*; Studer, E.*; et al.

Proceedings of 12th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation and Safety (NUTHOS-12) (USB Flash Drive), 11 Pages, 2018/10

Journal Articles

$$^{12}$$C + p resonant elastic scattering in the Maya active target

Sambi, S.*; Raabe, R.*; Borge, M. J. G.*; Caamano, M.*; Damoy, S.*; Fern$'a$ndez-Dom$'i$nguez, B.*; Flavigny, F.*; Fynbo, H.*; Gibelin, J.*; Grinyer, G. F.*; et al.

European Physical Journal A, 51(3), p.25_1 - 25_7, 2015/03

 Times Cited Count:6 Percentile:42.02(Physics, Nuclear)

Journal Articles

Unravelling the role of steps in Cu$$_{2}$$O formation via hyperthermal O$$_{2}$$ adsorption at Cu(410)

Okada, Michio*; Vattuone, L.*; Gerbi, A.*; Savio, L.*; Rocca, M.*; Moritani, Kosuke*; Teraoka, Yuden; Kasai, Toshio*

Journal of Physical Chemistry C, 111(46), p.17340 - 17345, 2007/11

 Times Cited Count:18 Percentile:50.99(Chemistry, Physical)

We report a study on the oxidation process of Cu(410) using high-resolution electron energy loss spectroscopy and X-ray photoemission spectroscopy using synchrotron radiation. We demonstrate that a hyperthermal O$$_{2}$$ molecular beam (HOMB) is an efficient tool to fabricate Cu$$_{2}$$O thin film also at room temperature. The efficiency of the Cu$$_{2}$$O formation in the initial stages depends on the angle of incidence of HOMB. Step roughening, acting as a source of mobile precursor Cu adatoms and opening channels for bulk diffusion of the O atoms, is a key feature in determining the Cu$$_{2}$$O formation rate.

Oral presentation

Role of steps in Cu$$_{2}$$O formation on Cu(410) using a hyperthermal O$$_{2}$$ molecular beam

Okada, Michio*; Vattuone, L.*; Moritani, Kosuke*; Gerbi, A.*; Savio, L.*; Yoshigoe, Akitaka; Teraoka, Yuden; Rocca, M.*; Kasai, Toshio*

no journal, , 

Herein we report the results of our detailed studies on the initial oxidation process, especially the Cu$$_{2}$$O formation, on Cu(410). From the high-resolution electron energy-loss spectroscopy (HREELS), the Cu$$_{2}$$O formation is verified at a high temperature for the thermal O$$_{2}$$ exposure. However, from the X-ray photoemission spectroscopy (XPS) measurements in conjunction with synchrotron radiation (SR), the efficiency of Cu$$_{2}$$O formation is quite low for the thermal O$$_{2}$$ exposure. On the other hand, it was found on Cu(410) that hyperthermal O$$_{2}$$ molecular beams (HOMB) at 2.2eV is an efficient tool for the fabrication of Cu$$_{2}$$O even at room temperature or at lower temperatures. The O-1s and valence-band XPS spectra clearly demonstrate the characteristic features of Cu$$_{2}$$O formation induced by HOMB. Furthermore, such Cu$$_{2}$$O formation depends strongly on the azimuthal direction of the incident HOMB, impinging dominantly on a terrace or on a step.

Oral presentation

Role of steps in Cu$$_{2}$$O formation on Cu(410) using a hyperthermal O$$_{2}$$ molecular beam

Okada, Michio*; Vattuone, L.*; Moritani, Kosuke*; Gerbi, A.*; Savio, L.*; Yoshigoe, Akitaka; Teraoka, Yuden; Rocca, M.*; Kasai, Toshio*

no journal, , 

It is important to make clear oxidation processes of Cu from an industrial view point because cupper oxides are candidates of high-Tc super conductor and solar cells. However, the details of the chemical reaction dynamics for the Cu oxidation processes have not been understood yet. We have already studied initial oxidation processes of Cu(100) and Cu(110) surfaces by using supersonic oxygen molecular beams. In this research, effects of surface defects for the surface oxidation are investigated by using the Cu(410) surface with large step density. It was found that oxidation rate of the Cu(410) surface was larger than Cu(100) surface, but, smaller than Cu(110) surface in the oxygen coverage range larger than 0.5 monolayer, from which formation of Cu$$_{2}$$O was observed. The phenomenon can be understood from the fact that the (410) surface consists of (100) terraces and (110) steps.

Oral presentation

Sureface-temperature dependence of oxide formation on Cu(410) using a hyperthermal O$$_{2}$$ molecular beam

Okada, Michio*; Vattuone, L.*; Moritani, Kosuke*; Gerbi, A.*; Savio, L.*; Yoshigoe, Akitaka; Teraoka, Yuden; Rocca, M.*; Kasai, Toshio*

no journal, , 

Initial oxidation processes at Cu(100) and Cu(410) surfaces by hyperthermal oxygen molecular beams (HOMB) have been investigated. In order to make clear effects of surface temperature, oxidation behaviour of steps at the Cu(410) surface, which had a moderate oxidation rate, was studied by high energy-resolution X-ray photoemission spectroscopy at the BL23SU in the SPring-8. Consequently, formation of Cu$$_{2}$$O was observed at room temperature by using HOMB of about 2 eV. And metastable CuO was formed at 100 K. These facts indicate that interest surface layers can be formed by controlling incident energy of oxygen molecular beams and surface temperature.

Oral presentation

Extension of fission reaction model FIFRELIN for wider reaction conditions and post processing

Ogawa, Tatsuhiko; Litaize, O.*; Mancusi, D.*; Chebboubi, A.*; Serot, O.*

no journal, , 

The Monte-Carlo code FIFRELIN was originally developed for the simulation of first chance fissions of fissile nuclei. In case of neutron-induced fissions, the compound nucleus always fissioned from an exited state whose excitation energy is sum of the incoming neutron energy and the neutron binding energy. While in the new version, with the multi-chance fission algorithm, the fissioning nuclei can start from higher exited states considering the competition of fission reactions, neutron emission, and gamma emission. When fission is selected in the competition, the partitioning of mass, charge, excitation energy, and angular momentum to the two fission fragments is determined either by the FIFRELIN native algorithm or by GEF. In fission reactions induced by energetic neutrons, pre-fission particle emission reduces the excitation energy of the compound nucleus before fission, leading to a noticeable difference of the final observables such as neutron multiplicity and fission product mass distribution. The other updated feature is the interface to codes handling the post-reaction processes. The energy spectra of neutrons, electrons and photons from fission reactions are output in a format compatible with PHITS, a general-purpose particle transport code. By using this functionality, one can simulate the transport and reactions of particles based on the cross section data and reaction models of PHITS, and the spectra calculated by FIFRELIN. Finally, the other interface developed in this study is nuclide yield output in a format compatible with DCHAIN-SP2014, a burn-up calculation code. This interface is necessary to consider the build-up, which depends on the time structure of the incoming neutron beam as well as the decay during the cooling period.

Oral presentation

Coupling of fission event generator FIFRELIN to radiation transport code PHITS

Ogawa, Tatsuhiko; Litaize, O.*; Mancusi, D.*; Chebboubi, A.*; Serot, O.*

no journal, , 

The Monte-Carlo code FIFRELIN was originally developed for the simulation of first chance fissions of fissile nuclei. In this study, its interfaces to codes handling the post-reaction processes were developed. The energy spectra of neutrons, electrons and photons from fission reactions are output in a format compatible with PHITS, a general-purpose particle transport code. By using this functionality, one can simulate the transport and reactions of particles based on the cross section data and reaction models of PHITS, and the source spectra calculated by FIFRELIN. The other interface developed in this study outputs nuclide yield output in a format compatible with DCHAIN-PHITS, a burn-up calculation code. This interface is necessary to consider the build-up, which depends on the time structure of the incoming neutron beam as well as the decay during the cooling period.

Oral presentation

New results in the modeling of fission and radiative neutron capture with FIFRELIN

Litaize, O.*; Piau, V.*; Chalil, A.*; Ogawa, Tatsuhiko; Chebboubi, A.*; Gook, A.*; Gunsing, F.*; Kessedjian, G.*; Lhuillier, D.*; Mancusi, D.*; et al.

no journal, , 

The Monte-Carlo code FIFRELIN was originally developed for the simulation of first chance fission of fissile nuclei. In this study, its interfaces to radiation transport code PHITS, extension for neutron capture reactions, and a function to calculate neutrinos from fission fragments were developed. In order to extend FIFRELIN for neutron capture reactions, accurate gamma-ray yield was obtained by tuning the level density considering the nuclide species and excitation energy. Accurate neutrino yield was obtained by adopting up-to-date database on the thermal neutron capture state. JAEA developed an interface of FIFRELIN to PHITS to perform new FIFRELIN benchmark using FIFRELIN-DCHAIN joint calculation.

Oral presentation

Development of multi-chance fission module for fission event generator FIFRELIN

Ogawa, Tatsuhiko; Litaize, O.*; Mancusi, D.*; Chebboubi, A.*; Serot, O.*

no journal, , 

The Monte-Carlo code FIFRELIN was originally developed for the simulation of first chance fissions of fissile nuclei and spontaneous fissions. In this study, a reaction module for multi-chance fission was developed. Multi-chance fission reaction are fission reactions preceded by neutron emission owing to the incident neutron energy higher than the fission barrier. For this development, an algorithm to calculate the excitation energy, spin and parity of the compound nucleus was implemented. In addition, a fission width and neutron emission width were calculated by Bohr-Wheeler formula and Hauser-Feshbach formula, respectively. If neutron emission reaction is sampled and the excitation energy reaches below the fission barrier, fission reaction is prohibited and the nucleus is deexcited by evaporation. The prompt fission probability of $$^{240}$$U(n,fission) calculated with these new algorithms, qualitatively agreed with experimental data. By improving the neutron transmission coefficient and level density formalism used in the Hauser-Feshbach calculation to calculate multi-chance fission calculation more accurately.

Oral presentation

Investigation of the structure of $$^{235}$$U(n$$_{th}$$,fission) prompt gamma energy spectrum by FIFRELIN

Ogawa, Tatsuhiko; Litaize, O.*; Mancusi, D.*; Chebboubi, A.*; Serot, O.*

no journal, , 

Thermal fission of U-235 is fundamental for nuclear energy engineering, whose details were observed through neutrons and gamma-rays. Among them, gamma-rays above 8 MeV, which come from immediate gamma deexcitation of fission fragments, were recently measured as a probe to observe fission more directly. The energy spectrum measured by a theoretical model CoH3 (Coupled-Channels Hauser-Feshbach Code) reproduced a peak around 4 MeV and a shoulder from 6 to 8 MeV, however, underestimated the components above 14 MeV. In this study, we used FIFRELIN developed by the French Atomic Energy, Alternative Energy Commission (CEA) to reproduce the gamma-ray energy spectrum. In addition to the peak around 4 MeV and a shoulder from 6 to 8 MeV, gamma spectrum up to 20 MeV was reproduced. This calculation also discovered that the level-density model for fission fragments plays the critical role. It was thus illustrated that FIFRELIN is useful to reproduce the spectra of gamma-ray from fission and investigate the reaction processes responsible for gamma-ray spectrum.

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