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Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.
Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05
Fang, Y.*; Kong, L.*; Wang, R.*; Zhang, Z.*; Li, Z.*; Wu, Y.*; Bu, K.*; Liu, X.*; Yan, S.*; Hattori, Takanori; et al.
Materials Today Physics (Internet), 34, p.101083_1 - 101083_7, 2023/05
Times Cited Count:1 Percentile:0(Materials Science, Multidisciplinary)The layered van der Waals halides are particularly sensitive to external pressure, suggesting a feasible route to pinpoint their structure with extraordinary behavior. However, a very sensitive pressure response usually lead to a detrimental phase transition and/or lattice distortion, making the approach of materials manipulation in a continuous manner remain challenging. Here, the extremely weak interlayer coupling and high tunability of layered RhI crystals are observed. A pressure-driven phase transition occurs at a moderate pressure of 5 GPa, interlinking to a change of layer stack mode. Strikingly, such a phase transition does not affect the tendency of quasi-linear bandgap narrowing, and a metallization with an ultra-broad tunability of 1.3 eV redshift is observed at higher pressures. Moreover, the carrier concentration increases by 4 orders of magnitude at 30 GPa, and the photocurrent enhances by 5 orders of magnitude at 7.8 GPa. These findings create new opportunities for exploring, tuning, and understanding the van der Waals halides by harnessing their unusual feature of a layered structure, which is promising for future devices based on materials-by-design that are atomically thin.
Sato, Yosuke*; Sekiyama, Tsuyoshi*; Fang, S.*; Kajino, Mizuo*; Qurel, A.*; Qulo, D.*; Kondo, Hiroaki*; Terada, Hiroaki; Kadowaki, Masanao; Takigawa, Masayuki*; et al.
Atmospheric Environment; X (Internet), 7, p.100086_1 - 100086_12, 2020/10
The third model intercomparison project for investigating the atmospheric behavior of Cs emitted during the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident (FDNPP-MIP) was conducted. A finer horizontal grid spacing (1 km) was used than in the previous FDNPP-MIP. Nine of the models used in the previous FDNPP-MIP were also used, and all models used identical source terms and meteorological fields. Our analyses indicated that most of the observed high atmospheric Cs concentrations were well simulated, and the good performance of some models improved the performance of the multi-model ensemble. The analyses also confirmed that the use of a finer grid resolution resulted in the meteorological field near FDNPP being better reproduced. The good representation of the wind field resulted in the reasonable simulation of the narrow distribution of high deposition amount to the northwest of FDNPP and the reduction of the overestimation over the area to the south of FDNPP. In contrast, the performance of the models in simulating plumes observed over the Nakadori area, the northern part of Gunma, and the Tokyo metropolitan area was slightly worse.
Wang, Y.*; Dong, X.*; Tang, X.*; Zheng, H.*; Li, K.*; Lin, X.*; Fang, L.*; Sun, G.*; Chen, X.*; Xie, L.*; et al.
Angewandte Chemie; International Edition, 58(5), p.1468 - 1473, 2019/01
Times Cited Count:35 Percentile:80.07(Chemistry, Multidisciplinary)Pressure-induced polymerization (PIP) of aromatics is a novel method to construct sp-carbon frameworks, and nanothreads with diamond-like structures were synthesized by compressing benzene and its derivatives. Here by compressing benzene-hexafluorobenzene cocrystal(CHCF), we identified H-F-substituted graphane with a layered structure in the PIP product. Based on the crystal structure determined from the in situ neutron diffraction and the intermediate products identified by the gas chromatography-mass spectrum, we found that at 20 GPa CHCF forms tilted columns with benzene and hexafluorobenzene stacked alternatively, which leads to a [4+2] polymer, and then transfers to short-range ordered hydrogenated-fluorinated graphane. The reaction process contains [4+2] Diels-Alder, retro-Diels-Alder, and 1-1' coupling, and the former is the key reaction in the PIP. Our studies confirmed the elemental reactions of the CHCF for the first time, which provides a novel insight into the PIP of aromatics.
Sato, Yosuke*; Takigawa, Masayuki*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Terada, Hiroaki; Nagai, Haruyasu; Kondo, Hiroaki*; Uchida, Junya*; Goto, Daisuke*; Qulo, D.*; et al.
Journal of Geophysical Research; Atmospheres, 123(20), p.11748 - 11765, 2018/10
Times Cited Count:40 Percentile:85.28(Meteorology & Atmospheric Sciences)A model intercomparison of the atmospheric dispersion of Cs emitted following the Fukushima Daiichi Nuclear Power Plant accident was conducted by 12 models to understand the behavior of Cs in the atmosphere. The same meteorological data, horizontal grid resolution, and an emission inventory were applied to all the models to focus on the model variability originating from the processes included in each model. The multi-model ensemble captured 40% of the observed Cs events, and the figure-of-merit in space for the total deposition of Cs exceeded 80. Our analyses indicated that the meteorological data were most critical for reproducing the Cs events. The results also revealed that the differences among the models were originated from the deposition and diffusion processes when the meteorological field was simulated well. However, the models with strong diffusion tended to overestimate the Cs concentrations.
Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; Tsunoda, Yusuke*; Otsuka, T.*; Nishimura, Shunji*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; et al.
Physics Letters B, 765, p.328 - 333, 2017/02
Times Cited Count:34 Percentile:91.97(Astronomy & Astrophysics)Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; Nishimura, Shunji*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; Lorusso, G.*; Patel, Z.*; et al.
Physical Review C, 93(3), p.034328_1 - 034328_14, 2016/03
Times Cited Count:25 Percentile:85.25(Physics, Nuclear)Benzoni, G.*; Morales, A. I.*; Watanabe, H.*; Nishimura, Shunji*; Coraggio, L.*; Itaco, N.*; Gargano, A.*; Browne, F.*; Daido, R.*; Doornenbal, P.*; et al.
Physics Letters B, 751, p.107 - 112, 2015/12
Times Cited Count:20 Percentile:78.02(Astronomy & Astrophysics)Li, G. S.*; Liu, M. L.*; Zhou, X. H.*; Zhang, Y. H.*; Liu, Y. X.*; Zhang, N. T.*; Hua, W.*; Zheng, Y. D.*; Fang, Y. D.*; Guo, S.*; et al.
Physical Review C, 89(5), p.054303_1 - 054303_9, 2014/05
Times Cited Count:5 Percentile:38.03(Physics, Nuclear)High-spin states of Pt have been reinvestigated using the Yb(O, 4) reaction at a beam energy of 88 MeV. The previously known positive parity band associated with the ( being or ) configuration has been revised and extended significantly. A new negative parity band has been established and proposed to be based on the configuration. Possible structure evolution of the yrast line from predominantly vibrational to rotational with increasing spin is discussed with the help of E over spin curves. Additionally, calculations of Total Routhian surfaces have been performed to investigate the band properties.
Walsh, M.*; Andrew, P.*; Barnsley, R.*; Bertalot, L.*; Boivin, R.*; Bora, D.*; Bouhamou, R.*; Ciattaglia, S.*; Costley, A. E.*; Counsell, G.*; et al.
Proceedings of 23rd IAEA Fusion Energy Conference (FEC 2010) (CD-ROM), 8 Pages, 2011/03
Zhang, Y. H.*; Zhou, X. H.*; He, J. J.*; Liu, Z.*; Fang, Y. D.*; Guo, W. T.*; Lei, X. G.*; Guo, Y. X.*; Ndontchueng, M. M.*; Ma, L.*; et al.
International Journal of Modern Physics E, 15(7), p.1437 - 1445, 2006/10
Times Cited Count:3 Percentile:28.19(Physics, Nuclear)Search for low-spin signature inversion in the bands in odd-odd Au have been made through in-beam -ray spectroscopy techniques. The bands in the three nuclei have been identified and extended up to high-spin states. In particlular, the interband connection between the band and the ground-state band in Au have been established, leading to a firm spin-and-parity assignment for the band. The low-spin signature inversion is found in the bands in Au.
Liang, N.*; Chiang, P.-N.*; Wang, Y.*; Teramoto, Munemasa*; Takagi, Kentaro*; Kondo, Toshiaki*; Koarashi, Jun; Zhang, Y.*; Li, S.*; Fang, J.*; et al.
no journal, ,
Sato, Yosuke*; Takigawa, Masayuki*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Terada, Hiroaki; Nagai, Haruyasu; Kondo, Hiroaki*; Uchida, Junya*; Goto, Daisuke*; Qulo, D.*; et al.
no journal, ,
no abstracts in English
Yamazawa, Hiromi*; Sato, Yosuke*; Adachi, Shinichiro*; Takigawa, Masayuki*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Terada, Hiroaki; Kondo, Hiroaki*; Uchida, Junya*; Goto, Daisuke*; et al.
no journal, ,
Cs-137 released from the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident was conducted by 12 models. The present study focuses on differences in the model results of atmospheric Cs-137 concentration of Plume 2, which traveled southward in the morning of 15 March, 2011, in the area 100 to 200 km downwind from FDNPP by using the concentration data recently evaluated from gamma radiation spectral data at monitoring stations (MS data) and those measured from the suspended particulate matter filters (SPM data). Comparison was made from the following aspects: (1) plume arrival time, (2) concentration level, (3) cross-wind surface concentration profile, (4) vertical concentration profile and (5) mass balance of Cs-137 activity including deposition processes. Additional analyses were made also for Plume 4, which traveled over the same area on 16 March under rainy condition.
Liang, N.*; Zhang, Y.*; Chiang, P.-N.*; Lai, D.*; Teramoto, Munemasa*; Takagi, Kentaro*; Kondo, Toshiaki*; Koarashi, Jun; Wang, Y.*; Li, S.*; et al.
no journal, ,
Yamazawa, Hiromi*; Sato, Yosuke*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Goto, Daisuke*; Morino, Yu*; Kondo, Hiroaki*; Qurel, A.*; Fang, S.*; Takigawa, Masayuki*; et al.
no journal, ,
Following the previous atmospheric transport model intercomparison project (MIP2), a new model intercomparison (MIP3) has been conducted in which, out of 12 models in MIP2, 9 models are participating. The main aim of MIP3 is to examine the effects of using a refined meteorological data with a finer horizontal resolution of 1 km. The horizontal distribution Cs-137 deposition in the eastern part of Honshu Island calculated by the models were compared with the aerial survey results to find that the simple ensemble average of the 9 models was a little worse than that of the 12-model ensemble in MIP2 statistically. However, in the sector in the northwestern direction from the accidental site, the deposition pattern by the MIP3 ensemble is more consistent with the survey result compared with that of MIP2. As for the atmospheric concentrations, although the model performance for the plumes that traveled over wider areas was slightly poorer for MIP3 than MIP2, the MIP3 ensemble generally showed better performance for the plumes that affected the near area in the Hamadori area. This better performance can be attributed to the better representation of topography in the meteorological simulation.
Sato, Yosuke*; Takigawa, Masayuki*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Terada, Hiroaki; Nagai, Haruyasu; Kadowaki, Masanao; Kondo, Hiroaki*; Uchida, Junya*; Goto, Daisuke*; et al.
no journal, ,
Two Model Intercomparison of Projects (MIPs) of atmospheric dispersion model targeting on Cs released from Fukushima Daiichi Nuclear Power Plant (FDNPP) on March 2011 were conducted. Both MIPs were conducted using an identical source term of Cs, identical meteorological data, and the same horizontal grid resolution (3 km and 1 km) to exclude the uncertainties of the model originated from them. Our analyses indicated that most of the model well simulated the atmospheric Cs obtained from the operational aerosol sampling of the national suspended particle matter network. Our analyses also indicated that meteorological data were most critical for reproducing the atmospheric Cs events, and the extent of the horizontal diffusion and the deposition were critical if the meteorological field was reasonably simulated. The comparison of the results between the two MIPs elucidated that the fine grid resolution is required to simulate atmospheric Cs in the vicinity of FDNPP, but the use of the fine grid resolution does not always improve the performance of the models especially for areas distant from the FDNPP. The results of both MIPs elucidated that the good performance of some models improved the performance of the multimodel, highlighting the advantage of using a multimodel ensemble.
Yamazawa, Hiromi*; Sato, Yosuke*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Fang, S.*; Qurel, A.*; Qulo, D.*; Kondo, Hiroaki*; Terada, Hiroaki; Kadowaki, Masanao; et al.
no journal, ,
The 3rd model intercomparison project (MIP) of atmospheric dispersion model targeting on Cs emitted from Fukushima Daiichi Nuclear Power Plant (FDNPP) in March 2011 were conducted. All participated 9 models used the identical source term and meteorological data as in the previous MIP (2nd MIP), but finer horizontal grid resolution (1 km) than that of 2nd MIP (3 km) was used for understanding the behavior of atmospheric Cs in the vicinity of FDNPP. Results of the models elucidated that most of the observed high atmospheric Cs concentrations were well simulated, and the good performance of some models cancelled bad performance of some models when used as an ensemble, which highlights the advantage of multimodel ensemble. The analyses also indicated that the use of the finer grid resolution improved the meteorological field in the vicinity of FNDPP and the atmospheric Cs measured near FDNPP was more reasonably reproduced in 3rd MIP than 2nd MIP. As well as the evaluation of the performance of the model, we examined usefulness of the results of atmospheric dispersion simulation in an emergency. The analyses reported that the multimodel ensemble missed only 3% of the observed plumes, even if the absolute value of the simulated Cs in each model was different in the range of factor 3-6. The analyses also indicated that from six to eight models are required for making most of advantages of the multimodel ensemble.