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Journal Articles

Incorporation of boron into metakaolin-based geopolymers for radionuclide immobilisation and neutron capture potential

Niu, X.*; Elakneswaran, Y.*; Li, A.*; Seralathan, S.*; Kikuchi, Ryosuke*; Hiraki, Yoshihisa; Sato, Junya; Osugi, Takeshi; Walkley, B.*

Cement and Concrete Research, 190, p.107814_1 - 107814_17, 2025/04

 Times Cited Count:0 Percentile:0.00(Construction & Building Technology)

Journal Articles

Robustness of ferromagnetism in van der Waals magnet Fe$$_3$$GeTe$$_2$$ to hydrostatic pressure

Wang, Y.*; Zeng, X.-T.*; Li, B.*; Su, C.*; Hattori, Takanori; Sheng, X.-L.*; Jin, W.*

Chinese Physics B, 34(4), p.046203_1 - 046203_6, 2025/03

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Two-dimensional van der Waals ferromagnet Fe$$_3$$GeTe$$_2$$ (FGT) holds a great potential for applications in spintronic devices, due to its high Curie temperature, easy tunability, and excellent structural stability in air. In this study, we have performed high-pressure neutron powder diffraction (NPD) up to 5 GPa, to investigate the evolution of its structural and magnetic properties with hydrostatic pressure. The NPD data clearly reveal the robustness of the ferromagnetism in FGT, despite of an apparent suppression by hydrostatic pressure. As the pressure increases from 0 to 5 GPa, the Curie temperature is found to decrease monotonically from 225(5) K to 175(5) K, together with a dramatically suppressed ordered moment of Fe, which is well supported by the first-principles calculations. Although no pressure-driven structural phase transition is observed up to 5 GPa, quantitative analysis on the changes of bond lengths and bond angles indicate a significant modification of the exchange interactions, which accounts for the pressure-induced suppression of the ferromagnetism in FGT.

Journal Articles

Remote alpha/beta measurement system with support vector machine algorithm

Morishita, Yuki; Miyamura, Hiroko; Sato, Yuki; Matsubara, Jun*; Sumali, B.*; Mitsukura, Yasue*

Nuclear Instruments and Methods in Physics Research A, p.170368_1 - 170368_16, 2025/03

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Decommissioning nuclear reactor sites presents challenges due to the presence of various radionuclides, including alpha emitters (e.g., Pu, Am, Cm) and beta emitters (e.g., $$^{137}$$Cs, $$^{90}$$Sr-$$^{90}$$Y), which pose significant internal exposure risks to workers. Traditional measurement methods require multiple instruments and are time-consuming, particularly in high gamma-ray environments. To address these issues, we developed a remote alpha and beta discrimination measurement system that integrates a stilbene scintillator detector with a silicon photomultiplier, enabling simultaneous detection of both alpha and beta particles. This study further incorporates machine learning techniques, specifically Support Vector Machines (SVM), for automatic discrimination, eliminating the need for user-defined thresholds and ensuring consistent operational conditions. The system was tested with known radiation sources, demonstrating over 96% classification accuracy for alpha and beta particles. Measurements conducted in motion effectively identified contamination sources, confirming the system's capability for real-time analysis. This innovative approach enhances radiation safety and efficiency in nuclear decommissioning operations, making it particularly beneficial in environments where human access is limited.

Journal Articles

Uncertainty quantification for severe-accident reactor modelling; Results and conclusions of the MUSA reactor applications work package

Brumm, S.*; Gabrielli, F.*; Sanchez Espinoza, V.*; Stakhanova, A.*; Groudev, P.*; Petrova, P.*; Vryashkova, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; et al.

Annals of Nuclear Energy, 211, p.110962_1 - 110962_16, 2025/02

 Times Cited Count:6 Percentile:93.24(Nuclear Science & Technology)

Journal Articles

Strong low-energy rattling modes enabled liquid-like ultralow thermal conductivity in a well-ordered solid

Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; Kofu, Maiko*; Nirei, Masami; Xu, J.*; Yin, W.*; Wang, F.*; et al.

National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12

 Times Cited Count:12 Percentile:91.22(Multidisciplinary Sciences)

Journal Articles

$$mu$$SR study on the noncentrosymmetric superconductor NbGe$$_2$$

Jiao, J. C.*; Chen, K. W.*; Hillier, A. D.*; Ito, Takashi; Higemoto, Wataru; Li, Z.*; Lv, B.*; Xu, Z.-A.*; Shu, L.*

Physical Review B, 110(21), p.214516_1 - 214516_9, 2024/12

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

Journal Articles

The LINACs simulation framework

Yee-Rendon, B.; Jameson, R. A.*; Okamura, Masahiro*; Li, C.*; Jiang, P.*; Maus, J. M.*

Proceedings of 32nd Linear Accelerator Conference (LINAC 2024) (Internet), p.492 - 495, 2024/10

LINACs is a simulation framework for designing optics and beam dynamics of charged particles in particle accelerators. LINACs is an open-source software that enables the user complete control over all design and simulation parameters of RFQs. This includes beam-driven design, fully 3D simulation using precise quadrupolar symmetry, and rigorous Poisson solution for external and space charge fields. The code can handle simultaneous particle beams with analytical input distributions and allows input beam scans. The software offers a relatively short running time and provides extensive analysis techniques. This work provides a historical overview of the code, presents results from RFQ models, and discusses future developments.

Journal Articles

Brightening triplet excitons enable high-performance white-light emission in organic small molecules via integrating n-$$pi^*/pi$$-$$pi^*$$ transitions

Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.

Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09

 Times Cited Count:9 Percentile:88.46(Multidisciplinary Sciences)

Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n-$$pi^*/pi$$-$$pi^*$$ transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.

Journal Articles

Antiferromagnetism and phase stability of CrMnFeCoNi high-entropy alloy

Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*

Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09

 Times Cited Count:1 Percentile:48.32(Physics, Multidisciplinary)

Journal Articles

Application of neutron characterization techniques to metallic structural materials

Wang, Y.*; Gong, W.; Su, Y. H.; Li, B.*

Acta Metallurgica Sinica, 60(8), p.1001 - 1016, 2024/08

 Times Cited Count:1 Percentile:41.92(Metallurgy & Metallurgical Engineering)

Journal Articles

Reevaluation of structures in $$^{70}$$Se from combined conversion-electron and $$gamma$$-ray spectroscopy

Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Muir, D.*; Pr$'o$chniak, L.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; et al.

Physical Review C, 110(2), p.024318_1 - 024318_16, 2024/08

 Times Cited Count:1 Percentile:0.00(Physics, Nuclear)

Journal Articles

Giant barocaloric effects in sodium hexafluorophosphate and hexafluoroarsenate

Zhang, Z.*; Hattori, Takanori; Song, R.*; Yu, D.*; Mole, R.*; Chen, J.*; He, L.*; Zhang, Z.*; Li, B.*

Journal of Applied Physics, 136(3), p.035105_1 - 035105_8, 2024/07

 Times Cited Count:2 Percentile:40.97(Physics, Applied)

Solid-state refrigeration using barocaloric materials is environmentally friendly and highly efficient, making it a subject of global interest over the past decade. Here, we report giant barocaloric effects in sodium hexafluorophosphate (NaPF$$_6$$) and sodium hexafluoroarsenate (NaAsF$$_6$$) that both undergo a cubic-to-rhombohedral phase transition near room temperature. We have determined that the low-temperature phase structure of NaPF$$_6$$ is a rhombohedral structure with space group R$=3 by neutron powder diffraction. There are three Raman active vibration modes in NaPF$_6$$ and NaAsF$$_6$$, i.e., F$$_{2g}$$, E$$_g$$, and A$$_{1g}$$. The phase transition temperature varies with pressure at a rate of dT$$_t$$/dP = 250 and 310 K/GPa for NaPF$$_6$$ and NaAsF$$_6$$. The pressure-induced entropy changes of NaPF$$_6$$ and NaAsF$$_6$$ are determined to be around 45.2 and 35.6J kg$$^{-1}$$K$$^{-1}$$, respectively. The saturation driving pressure is about 40 MPa. The pressure-dependent neutron powder diffraction suggests that the barocaloric effects are related to the pressure-induced cubic-to-rhombohedral phase transitions.

Journal Articles

Phase transformation and equation of state in Ti-45Al alloy under high pressure

Li, X.*; Zhu, R.*; Xin, J.*; Luo, M.*; Shang, S.-L.*; Liu, Z.-K.*; Yin, C.*; Funakoshi, Kenichi*; Dippenaar, R. J.*; Higo, Yuji*; et al.

CALPHAD; Computer Coupling of Phase Diagrams and Thermochemistry, 84, p.102641_1 - 102641_6, 2024/03

 Times Cited Count:0 Percentile:0.00(Thermodynamics)

Journal Articles

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

 Times Cited Count:2 Percentile:58.81(Physics, Nuclear)

no abstracts in English

Journal Articles

Cooling mechanism by barocaloric effect in plastic crystal

Li, B.*; Kawakita, Yukinobu

Kakushinteki Reikyaku Gijutsu; Mekanizumu Kara Soshi, Shisutemu Kaihatsu Made, p.19 - 28, 2024/01

no abstracts in English

Journal Articles

Grain size independence of cryogenic strain recovery behavior in high-Zr $$beta$$-Ti alloy

Zhang, B.*; Xin, S.*; Huang, M.*; Mao, W.; Jia, W.*; Li, Q.*; Li, S.*; Zhang, S.*; Mao, C.*

Materials Science & Engineering A, 890, p.145898_1 - 145898_7, 2024/01

 Times Cited Count:0 Percentile:0.00(Nanoscience & Nanotechnology)

A significant increase in the recovery strain of a high-Zr $$beta$$-Ti alloy from 2.25 % to 5.5 % when decreasing the deformation temperature from 300 K to 77 K is reported in this study. It is found that the super-elasticity of this alloy is independent of the $$beta$$-grain size at 77 K. The results reveal that a coarse-grained specimen exhibited approximately the same super-elasticity as its ultra-fine grain counterpart at 77 K. The relative easiness of deformation-induced martensitic transformation and dislocation slip was substantially changed at 77 K, with a strong suppression of dislocation slip, which overshadowed the effect of grain refinement on the super-elasticity.

Journal Articles

ICRU Report 98, Stochastic nature of radiation interactions; Microdosimetry

Braby, L. A.*; Conte, V.*; Dingfelder, M.*; Goodhead, D. T.*; Pinsky, L. S.*; Rosenfeld, A. B.*; Sato, Tatsuhiko; Waker, A. J.*; Guatelli, S.*; Magrin, G.*; et al.

Journal of ICRU, 23(1), p.1 - 168, 2023/12

This report provides a comprehensive description of the basic concepts and theories, computational and experimental procedures, and applications of microdosimetry.

Journal Articles

Colossal barocaloric plastic crystals

Lloveras, P.*; Zhang, Z.*; Zeng, M.*; Barrio, M.*; Kawakita, Yukinobu; Yu, D.*; Lin, S.*; Li, K.*; Moya, X.*; Tamarit, J.-L.*; et al.

Barocaloric Effects in the Solid State; Materials and methods, p.7_1 - 7_30, 2023/10

 Times Cited Count:232 Percentile:99.37(Multidisciplinary Sciences)

As Chapter 1 of the ebook entitled as "Barocaloric Effects in the Solid State", various plastic crystals (PC) showing colossal barocaloric (BC) effect are introduced. A method to determine the BC response in PCs, thermodynamic origin of BC effects, spectroscopic insights from quasi-elastic neutron scattering and application of PCs are explained.

Journal Articles

PANDORA Project for the study of photonuclear reactions below $$A=60$$

Tamii, Atsushi*; Pellegri, L.*; S$"o$derstr$"o$m, P.-A.*; Allard, D.*; Goriely, S.*; Inakura, Tsunenori*; Khan, E.*; Kido, Eiji*; Kimura, Masaaki*; Litvinova, E.*; et al.

European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09

 Times Cited Count:7 Percentile:76.15(Physics, Nuclear)

no abstracts in English

Journal Articles

Direct observation of topological magnon polarons in a multiferroic material

Bao, S.*; Gu, Z.-L.*; Shangguan, Y.*; Huang, Z.*; Liao, J.*; Zhao, X.*; Zhang, B.*; Dong, Z.-Y.*; Wang, W.*; Kajimoto, Ryoichi; et al.

Nature Communications (Internet), 14, p.6093_1 - 6093_9, 2023/09

 Times Cited Count:18 Percentile:92.93(Multidisciplinary Sciences)

183 (Records 1-20 displayed on this page)