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Journal Articles

Resonant X-ray scattering study of NpRhGa$$_5$$ and NpCoGa$$_5$$

Detlefs, B.*; Wilkins, S. B.*; Caciuffo, R.*; Paix$~a$o, J. A.*; Kaneko, Koji; Honda, Fuminori*; Metoki, Naoto; Bernhoeft, N.*; Rebizant, J.*; Lander, G. H.*

Physical Review B, 77(2), p.024425_1 - 024425_10, 2008/01

 Times Cited Count:17 Percentile:58.3(Materials Science, Multidisciplinary)

We report a resonant X-ray scattering study of the antiferromagnetic neptunium compounds NpCoGa$$_5$$ and NpRhGa$$_5$$. Large resonant signals of magnetic dipole character are observed below the N$'e$el temperatures. The signals at the Np edges confirm the behavior determined previously from neutron diffraction. On application of a magnetic field of 9 T along the [010] direction in NpRhGa$$_5$$, we observe a change in the population of different [110]-type domains. We also observe a magnetic dipole signal at the Ga $$K$$ edge, similarly to the reported UGa$$_3$$ case, that can be interpreted within a semilocalized model as an orbital polarization of the Ga 4$$p$$ states induced via strong hybridization with the Np 5$$f$$ valence band. Quantitative analysis of the signal shows that the Ga dipole on the two different Ga sites follows closely the Np magnetic moment reorientation in NpRhGa$$_5$$. The ratios of the signals on the two inequivalent Ga sites are not the same for the different compounds.

Journal Articles

Probing the Coulomb interaction of PuCoGa$$_5$$ by phonon spectroscopy

Raymond, S.*; Piekarz, P.*; Sanchez, J. P.*; Serrano, J.*; Kirsch, M.*; Detlefs, B.*; Rebizant, J.*; Metoki, Naoto; Kaneko, Koji; Jochym, P. T.*; et al.

Journal of Alloys and Compounds, 444-445, p.104 - 108, 2007/10

 Times Cited Count:2 Percentile:21.49(Chemistry, Physical)

The phonon dispersion curves of the unconventional superconductor PuCoGa$$_5$$ were studied by inelastic X-ray scattering at room temperature. The experimental data agree well with ab initio lattice dynamics calculations. An accurate theoretical description of the phonon spectrum is obtained only when a local Coulomb repulsion $$U{approx}$$3 eV among 5f electrons is taken into account. This implies partial localization of the 5f electrons in this compound. A comparison made with the phonon spectrum of UCoGa$$_5$$ suggests that the latter compound is better described with a fully itinerant f electrons model.

Journal Articles

Probing the coulomb interaction of the unconventional superconductor PuCoGa$$_5$$ by phonon spectroscopy

Raymond, S.*; Piekarz, P.*; Sanchez, J. P.*; Serrano, J.*; Kirsch, M.*; Janousova, B.*; Rebizant, J.*; Metoki, Naoto; Kaneko, Koji; Jochym, P. T.*; et al.

Physical Review Letters, 96(23), p.237003_1 - 237003_4, 2006/06

 Times Cited Count:26 Percentile:74.49(Physics, Multidisciplinary)

The phonon dispersion curves of the superconductor PuCoGa$$_{5}$$ were studied by inelastic X-ray scattering at room temperature. The experimental data agree well with ${it ab initio}$ lattice dynamics calculations. An accurate description of the phonon spectrum is obtained only when a local Coulomb repulsion U$${simeq}$$ 3 eV among 5$$f$$ electrons is taken into account.

Journal Articles

Magnetic structure and metamagnetism in single crystals of NpCoGa$$_{5}$$

Metoki, Naoto; Kaneko, Koji; Colineau, E.*; Javorsk$'y$, P.*; Aoki, Dai*; Homma, Yoshiya*; Boulet, P.*; Wastin, F.*; Shiokawa, Yoshinobu; Bernhoeft, N.*; et al.

Physical Review B, 72(1), p.014460_1 - 014460_8, 2005/07

 Times Cited Count:50 Percentile:83.68(Materials Science, Multidisciplinary)

no abstracts in English

Oral presentation

Phonon in ATGa$$_{5}$$(A:U, Pu)

Metoki, Naoto; Kaneko, Koji; Ikeda, Shugo; Matsuda, Tatsuma; Haga, Yoshinori; Onuki, Yoshichika; Raymond, S.*; Piekarz, P.*; Sanchez, J. P.*; Serrano, J.*; et al.

no journal, , 

no abstracts in English

5 (Records 1-5 displayed on this page)
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