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Journal Articles

JAEA-JRC collaborative development of delayed gamma-ray spectroscopy for nuclear safeguards nuclear material accountancy

Rodriguez, D.; Abbas, K.*; Bertolotti, D.*; Bonaldi, C.*; Fontana, C.*; Fujimoto, Masami*; Geerts, W.*; Koizumi, Mitsuo; Macias, M.*; Nonneman, S.*; et al.

Proceedings of INMM & ESARDA Joint Annual Meeting 2023 (Internet), 8 Pages, 2023/05

Journal Articles

The Joint evaluated fission and fusion nuclear data library, JEFF-3.3

Plompen, A. J. M.*; Cabellos, O.*; De Saint Jean, C.*; Fleming, M.*; Algora, A.*; Angelone, M.*; Archier, P.*; Bauge, E.*; Bersillon, O.*; Blokhin, A.*; et al.

European Physical Journal A, 56(7), p.181_1 - 181_108, 2020/07

 Times Cited Count:234 Percentile:99.41(Physics, Nuclear)

The Joint Evaluated Fission and Fusion nuclear data library 3.3 is described. New evaluations for neutron-induced interactions with the major actinides $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu, on $$^{241}$$Am and $$^{23}$$Na, $$^{59}$$Ni, Cr, Cu, Zr, Cd, Hf, W, Au, Pb and Bi are presented. It includes new fission yileds, prompt fission neutron spectra and average number of neutrons per fission. In addition, new data for radioactive decay, thermal neutron scattering, gamma-ray emission, neutron activation, delayed neutrons and displacement damage are presented. JEFF-3.3 was complemented by files from the TENDL project. The libraries for photon, proton, deuteron, triton, helion and alpha-particle induced reactions are from TENDL-2017. The demands for uncertainty quantification in modeling led to many new covariance data. A comparison between results from model calculations using the JEFF-3.3 library and those from benchmark experiments for criticality, delayed neutron yields, shielding and decay heat, reveals that JEFF-3.3 is excellent for a wide range of nuclear technology applications, in particular nuclear energy.

Journal Articles

Non-destructive analysis of samples with a complex geometry by NRTA

Ma, F.; Kopecky, S.*; Alaerts, G.*; Harada, Hideo; Heyse, J.*; Kitatani, Fumito; Noguere, G.*; Paradela, C.*; $v{S}$alamon, L.*; Schillebeeckx, P.*; et al.

Journal of Analytical Atomic Spectrometry, 35(3), p.478 - 488, 2020/03

AA2019-0356.pdf:2.54MB

 Times Cited Count:2 Percentile:22.6(Chemistry, Analytical)

Journal Articles

Sample shape effect on nuclear material quantification with neutron resonance transmission analysis

Tsuchiya, Harufumi; Ma, F.; Kitatani, Fumito; Paradella, C.*; Heyse, J.*; Kopecky, S.*; Schillebeeckx, P.*

Proceedings of 41st ESARDA Annual Meeting (Internet), p.374 - 377, 2019/05

Journal Articles

Neutron resonance transmission analysis for measurement of nuclear materials in nuclear fuel

Tsuchiya, Harufumi; Kitatani, Fumito; Toh, Yosuke; Paradela, C.*; Heyse, J.*; Kopecky, S.*; Schillebeeckx, P.*

Proceedings of INMM 59th Annual Meeting (Internet), 6 Pages, 2018/07

Journal Articles

Development of active neutron NDA system for nuclear materials

Toh, Yosuke; Ozu, Akira; Tsuchiya, Harufumi; Furutaka, Kazuyoshi; Kitatani, Fumito; Komeda, Masao; Maeda, Makoto; Koizumi, Mitsuo; Heyse, J.*; Paradela, C.*; et al.

Proceedings of INMM 59th Annual Meeting (Internet), 9 Pages, 2018/07

Journal Articles

CIELO collaboration summary results; International evaluations of neutron reactions on uranium, plutonium, iron, oxygen and hydrogen

Chadwick, M. B.*; Capote, R.*; Trkov, A.*; Herman, M. W.*; Brown, D. A.*; Hale, G. M.*; Kahler, A. C.*; Talou, P.*; Plompen, A. J.*; Schillebeeckx, P.*; et al.

Nuclear Data Sheets, 148, p.189 - 213, 2018/02

 Times Cited Count:61 Percentile:98.12(Physics, Nuclear)

The CIELO collaboration has studied neutron cross sections on nuclides that significantly impact criticality in nuclear facilities - $$^{235}$$U, $$^{238}$$U, $$^{239}$$Pu, $$^{56}$$Fe, $$^{16}$$O and $$^{1}$$H - with the aim of improving the accuracy of the data and resolving previous discrepancies in our understanding. This multi-laboratory pilot project, coordinated via the OECD/NEA Working Party on Evaluation Cooperation (WPEC) Subgroup 40 with support also from the IAEA, has motivated experimental and theoretical work and led to suites of new evaluated libraries that accurately reflect measured data and also perform well in integral simulations of criticality. This report summarizes our results and outlines plans for the next phase of this collaboration.

Journal Articles

Systematic effects on cross section data derived from reaction rates in reactor spectra and a re-analysis of $$^{241}$$Am reactor activation measurements

$v{Z}$erovnik, G.*; Schillebeeckx, P.*; Becker, B.*; Fiorito, L.*; Harada, Hideo; Kopecky, S.*; Radulovic, V.*; Sano, Tadafumi*

Nuclear Instruments and Methods in Physics Research A, 877, p.300 - 313, 2018/01

 Times Cited Count:3 Percentile:46.53(Instruments & Instrumentation)

Methodologies to derive cross section data from spectrum integrated reaction rates were studied. The Westcott convention and some of its approximations were considered. The accuracy of the results strongly depends on the assumptions that are made about the neutron energy distribution, which is mostly parameterised as a sum of a thermal and an epi-thermal component. Resonance integrals derived from such data can be strongly biased. When the energy dependence of the cross section is known and information about the neutron energy distribution is available, a method to correct for a bias on the cross section at thermal energy is proposed. Reactor activation measurements to determine the thermal $$^{241}$$Am(n, $$gamma$$) cross section reported in the literature were reviewed, where the results were corrected to account for possible biases. These data combined with results of time-of-flight measurements give a capture cross section 720 (14) b for $$^{241}$$Am(n, $$gamma$$) at thermal energy.

Journal Articles

Improving nuclear data accuracy of $$^{241}$$ Am and $$^{237}$$ Np capture cross sections

$v{Z}$erovnik, G.*; Schillebeeckx, P.*; Cano-Ott, D.*; Jandel, M.*; Hori, Junichi*; Kimura, Atsushi; Rossbach, M.*; Letourneau, A.*; Noguere, G.*; Leconte, P.*; et al.

EPJ Web of Conferences, 146, p.11035_1 - 11035_4, 2017/09

 Times Cited Count:3 Percentile:86.61

Journal Articles

Delayed $$gamma$$-ray spectroscopy combined with active neutron interrogation for nuclear security and safeguards

Koizumi, Mitsuo; Rossi, F.; Rodriguez, D.; Takamine, Jun; Seya, Michio; Bogucarska, T.*; Crochemore, J.-M.*; Varasano, G.*; Abbas, K.*; Pedersen, B.*; et al.

EPJ Web of Conferences, 146, p.09018_1 - 09018_4, 2017/09

 Times Cited Count:3 Percentile:86.61

Journal Articles

Neutron resonance analysis for nuclear safeguards and security applications

Paradela, C.*; Heyse, J.*; Kopecky, S.*; Schillebeeckx, P.*; Harada, Hideo; Kitatani, Fumito; Koizumi, Mitsuo; Tsuchiya, Harufumi

EPJ Web of Conferences, 146, p.09002_1 - 09002_4, 2017/09

 Times Cited Count:7 Percentile:97.4

Journal Articles

The CIELO collaboration; Progress in international evaluations of neutron reactions on Oxygen, Iron, Uranium and Plutonium

Chadwick, M. B.*; Capote, R.*; Trkov, A.*; Kahler, A. C.*; Herman, M. W.*; Brown, D. A.*; Hale, G. M.*; Pigni, M.*; Dunn, M.*; Leal, L.*; et al.

EPJ Web of Conferences, 146, p.02001_1 - 02001_9, 2017/09

 Times Cited Count:6 Percentile:95.25

The CIELO collaboration has studied neutron cross sections on nuclides ($$^{16}$$O, $$^{56}$$Fe, $$^{235,238}$$U and $$^{239}$$Pu) that significantly impact criticality in nuclear technologies with the aim of improving the accuracy of the data and resolving previous discrepancies in our understanding. This multi-laboratory pilot project, coordinated via the OECD/NEA Working Party on Evaluation Cooperation (WPEC) Subgroup 40 with support also from the IAEA, has motivated experimental and theoretical work and led to suites of new evaluated libraries that accurately reflect measured data and also perform well in integral simulations of criticality.

Journal Articles

Development of active neutron NDA techniques for nuclear nonproliferation and nuclear security

Toh, Yosuke; Ozu, Akira; Tsuchiya, Harufumi; Furutaka, Kazuyoshi; Kitatani, Fumito; Komeda, Masao; Maeda, Makoto; Kureta, Masatoshi; Koizumi, Mitsuo; Seya, Michio; et al.

EUR-28795-EN (Internet), p.684 - 693, 2017/00

Journal Articles

Delayed gamma-ray analysis for characterization of fissile nuclear materials

Koizumi, Mitsuo; Rossi, F.; Rodriguez, D.; Takamine, Jun; Seya, Michio; Bogucarska, T.*; Crochemore, J.-M.*; Varasano, G.*; Abbas, K.*; Pedersen, B.*; et al.

EUR-28795-EN (Internet), p.868 - 872, 2017/00

Journal Articles

LaBr$$_3$$ $$gamma$$-ray spectrometer for detecting $$^{10}$$B in debris of melted nuclear fuel

Koizumi, Mitsuo; Tsuchiya, Harufumi; Kitatani, Fumito; Harada, Hideo; Heyse, J.*; Kopecky, S.*; Mondelaers, W.*; Paradela, C.*; Schillebeeckx, P.*

Nuclear Instruments and Methods in Physics Research A, 837, p.153 - 160, 2016/11

 Times Cited Count:1 Percentile:19.85(Instruments & Instrumentation)

Journal Articles

Journal Articles

Characteristics of neutron resonance densitometry, 2; Neutron resonance capture analysis

Tsuchiya, Harufumi; Harada, Hideo; Koizumi, Mitsuo; Kitatani, Fumito; Kureta, Masatoshi; Becker, B.*; Kopecky, S.*; Heyse, J.*; Paradela, C.*; Mondelaers, W.*; et al.

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-36-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2015/12

Neutron Resonance Densitometry (NRD) was developed as a non-destructive assay to quantify U and Pu isotopes in particle-like debris. NRD is composed of neutron resonance transmission analysis (NRTA) and Neutron Resonance Capture Analysis (NRCA) or Prompt Gamma-ray Analysis (PGA). NRCA/PGA in NRD plays a role of identifying impurities in debris under the high-radiation field primarily caused by $$^{137}$$Cs. For this purpose, a novel LaBr$$_3$$ $$gamma$$-ray detector employing specific shields has been newly developed. With the developed $$gamma$$-ray detector, a demonstration NRCA experiment was performed at a neutron time of flight facility GELINA (Belgium). As a result, samples (Hf, Gd, Ni) placed in a black box that is completely sealed by third party were successfully identified by the experiment. This presentation explains the design concept of the $$gamma$$ ray detector including its detection principle and details of the demonstration NRCA experiment.

Journal Articles

Characteristics of neutron resonance densitometry, 1; Neutron resonance transmission analysis

Kitatani, Fumito; Harada, Hideo; Koizumi, Mitsuo; Tsuchiya, Harufumi; Kureta, Masatoshi; Becker, B.*; Kopecky, S.*; Heyse, J.*; Paradela, C.*; Mondelaers, W.*; et al.

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-36-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2015/12

From 2012 to 2014, Neutron Resonance Densitometry (NRD) is being developed as a non-destructive assay to quantify U and Pu isotopes. NRD is composed of neutron resonance transmission analysis (NRTA) and Neutron Resonance Capture Analysis (NRCA)/Prompt Gamma-ray Analysis (PGA). NRTA in NRD plays a role of quantifying the amounts of the isotopes of a nuclear fuel material (U, Pu) in molten fuel debris. Therefore, the neutron absorption measurement using Time-of-Flight (TOF) method is carried out. A demonstration NRTA experiment was performed at a neutron time of flight facility GELINA (Belgium). Consequently, we succeeded in iquantifying the randomly selected sample from Au, W, Rh, Nb, Cu. Co, Mn, B contained in a black box. In this presentation, we describe the principle of measurement of the developed NRTA and explain details of the demonstration experiment.

Journal Articles

Active neutron NDA techniques for nuclear non-proliferation applications, 4; Development of delayed gamma-ray spectroscopy; Experimental research plan

Koizumi, Mitsuo; Heyse, J.*; Mondelaers, W.*; Paradela, C.*; Pedersen, B.*; Schillebeeckx, P.*; Seya, Michio; Rodriguez, D.; Takamine, Jun

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-36-Kai Nenji Taikai Rombunshu (Internet), 6 Pages, 2015/12

The fission-product yield distributions are unique for each fissionable nuclide and interrogating neutron energy. Ratios of fissile materials (e.g. $$^{235}$$U, $$^{239}$$Pu, and $$^{241}$$Pu), therefore, could be deduced from differences in the observed neutron-induced Delayed Gamma-ray (DG) spectra characterized by the difference of these yields. This DG Spectroscopy (DGS) project includes research and development of a measurement system along with confirming and improving nuclear data. Experiments will be held at multiple facilities, including ITU/Ispra (Italy), IRMM/Geel (Belgium), and KURRI/Kumatori (Japan), using a wide range of neutron sources and nuclear material sample targets. The experimental efforts of this DGS project are described in this presentation.

Journal Articles

Systematic effects on cross-section data derived from reaction rates at a cold neutron beam

$v{Z}$erovnik, G.*; Becker, B.*; Belgya, T.*; Genreith, C.*; Harada, Hideo; Kopecky, S.*; Radulovi$'c$, V.*; Sano, Tadafumi*; Schillebeeckx, P.*; Trkov, A.*

Nuclear Instruments and Methods in Physics Research A, 799, p.29 - 36, 2015/11

 Times Cited Count:4 Percentile:33.51(Instruments & Instrumentation)

The methodology to derive cross section data from measurements in a cold neutron beam was studied. Mostly, capture cross sections at thermal energy are derived relative to a standard cross section, and proportionality between the standard and the measured cross section is often assumed. Due to this assumption the derived capture cross section at thermal energy can be biased by more than 10%. Evidently the bias depends on how much the energy dependence of the cross section deviates from a direct proportionality with the inverse of the neutron speed. The effect is reduced in case the cross section is not derived at thermal energy but at an energy close to the average energy of the cold neutron beam. Nevertheless, it is demonstrated that the bias can only be avoided in case the energy dependence of the cross section is known and proper correction factors are applied. In some cases the results can also be biased when the attenuation of the neutron beam within the sample is neglected in the analysis. Some of the cross section data reported in the literature suffer from such bias effects.

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