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Pb and 
Bi in proton-induced reactions near 100 MeVIwamoto, Hiroki; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Ishi, Yoshihiro*; Uesugi, Tomonori*; Yashima, Hiroshi*; Nishio, Katsuhisa; Sugihara, Kenta*; 
elik, Y.*; et al.
Nuclear Instruments and Methods in Physics Research B, 544, p.165107_1 - 165107_15, 2023/11
Times Cited Count：0 Percentile：0.02(Instruments & Instrumentation)The lack of double-differential cross-section (DDX) data for neutron production below the incident proton energy of 200 MeV hinders the validation of spallation models in technical applications, such as research and development of accelerator-driven systems (ADSs). The present study aims to obtain experimental DDX data for ADS spallation target materials in this energy region and identify issues related to the spallation models by comparing them with the analytical predictions. The DDXs for the (
) reactions of Pb and Bi in the 100-MeV region were measured over an angular range of 30
to 150 using the time-of-flight method. The measurements were conducted at Kyoto University utilizing the FFAG accelerator. The DDXs obtained were compared with calculation results from Monte Carlo-based spallation models and the evaluated nuclear data library, JENDL-5. Comparison between the measured DDX and analytical values based on the spallation models and evaluated nuclear data library indicated that, in general, the CEM03.03 model demonstrated the closest match to the experimental values. Additionally, the comparison highlighted several issues that need to be addressed in order to improve the reproducibility of the proton-induced neutron-production DDX in the 100 MeV region by these spallation models and evaluated nuclear data library.
Pb(p,x)
Hg and Bi(p,x)Hg excitation functions in the energy range 0.04 - 2.6 GeVTitarenko, Yu. E.*; Batyaev, V. F.*; Pavlov, K. V.*; Titarenko, A. Yu.*; Malinovskiy, S. V.*; Rogov, V. I.*; Zhivun, V. M.*; Kulevoy, T. V.*; Chauzova, M. V.*; Khalikov, R. S.*; et al.
Nuclear Instruments and Methods in Physics Research A, 1026, p.166151_1 - 166151_9, 2022/03
Times Cited Count：1 Percentile：33.4(Instruments & Instrumentation)The paper presents the Hg production cross-sections measured by the direct gamma-spectrometry technique in the samples of lead enriched with isotopes 206, 207 and 208, as well as in the samples of natural lead and bismuth, irradiated by protons of 11 energies in the range from 0.04 to 2.6 GeV. The obtained experimental results are compared with the previous measurements, with the TENDL-2019 data-library evaluations and the simulated data by means of the high-energy transport codes MCNP6.1 (CEM03.03), PHITS (INCL4.6/GEM), Geant4 (INCL++/ABLA) and the nuclear reaction code TALYS.
Pb(p,x)
Bi and Bi(p,x)Bi excitation functions in the energy range of 0.04 - 2.6 GeVTitarenko, Yu. E.*; Batyaev, V. F.*; Pavlov, K. V.*; Titarenko, A. Yu.*; Malinovskiy, S. V.*; Rogov, V. I.*; Zhivun, V. M.*; Kulevoy, T. V.*; Chauzova, M. V.*; Lushin, S. V.*; et al.
Nuclear Instruments and Methods in Physics Research A, 984, p.164635_1 - 164635_8, 2020/12
Times Cited Count：3 Percentile：36.4(Instruments & Instrumentation)The paper presents the Bi production cross-sections measured by the direct gamma-spectrometry technique in the samples of lead enriched with isotopes 208, 207 and 206, as well as in the samples of natural lead and bismuth, irradiated by protons of 11 energies in the range from 0.04 to 2.6 GeV. The obtained experimental results are compared with the previous measurements, with the TENDL-2019 data-library evaluations and the simulated data by means of the high-energy transport codes MCNP6.1 (CEM03.03), PHITS (INCL4.6/GEM), and Geant4 (INCL++/ABLA). The observed discrepancies between model predictions and experimental data are discussed.
Dupont, E.*; Bossant, M.*; Capote, R.*; Carlson, A. D.*; Danon, Y.*; Fleming, M.*; Ge, Z.*; Harada, Hideo; Iwamoto, Osamu; Iwamoto, Nobuyuki; et al.
EPJ Web of Conferences, 239, p.15005_1 - 15005_4, 2020/09
Times Cited Count：13 Percentile：99.69(Nuclear Science & Technology)Plompen, A. J. M.*; Cabellos, O.*; De Saint Jean, C.*; Fleming, M.*; Algora, A.*; Angelone, M.*; Archier, P.*; Bauge, E.*; Bersillon, O.*; Blokhin, A.*; et al.
European Physical Journal A, 56(7), p.181_1 - 181_108, 2020/07
Times Cited Count：321 Percentile：99.41(Physics, Nuclear)The Joint Evaluated Fission and Fusion nuclear data library 3.3 is described. New evaluations for neutron-induced interactions with the major actinides 
U, 
U and 
Pu, on 
Am and 
Na, 
Ni, Cr, Cu, Zr, Cd, Hf, W, Au, Pb and Bi are presented. It includes new fission yileds, prompt fission neutron spectra and average number of neutrons per fission. In addition, new data for radioactive decay, thermal neutron scattering, gamma-ray emission, neutron activation, delayed neutrons and displacement damage are presented. JEFF-3.3 was complemented by files from the TENDL project. The libraries for photon, proton, deuteron, triton, helion and alpha-particle induced reactions are from TENDL-2017. The demands for uncertainty quantification in modeling led to many new covariance data. A comparison between results from model calculations using the JEFF-3.3 library and those from benchmark experiments for criticality, delayed neutron yields, shielding and decay heat, reveals that JEFF-3.3 is excellent for a wide range of nuclear technology applications, in particular nuclear energy.
for MYRRHA using a Monte Carlo techniqueIwamoto, Hiroki; Stankovskiy, A.*; Fiorito, L.*; Van den Eynde, G.*
EPJ Nuclear Sciences & Technologies (Internet), 4, p.42_1 - 42_7, 2018/11
This paper presents a nuclear data sensitivity and uncertainty analysis of the effective delayed neutron fraction for critical and subcritical cores of the MYRRHA reactor using the continuous-energy Monte Carlo transport code MCNP. The sensitivities are calculated by the modified 
-ratio method proposed by Chiba. Comparing the sensitivities obtained with different scaling factors 
introduced by Chiba shows that a value of 
is the most suitable for the uncertainty quantification of . Using the calculated sensitivities and the JENDL-4.0u covariance data, the uncertainties for the critical and subcritical cores are determined to be 2.2 
0.2% and 2.0 0.2%, respectively, which are dominated by delayed neutron yield of Pu and U.
Stankovskiy, A.*; Iwamoto, Hiroki; elik, Y.*; Van den Eynde, G.*
Annals of Nuclear Energy, 120, p.207 - 218, 2018/10
Times Cited Count：8 Percentile：62.99(Nuclear Science & Technology)Propagation of high-energy (above 20-MeV) nuclear data uncertainties on the safety related neutronic responses in accelerator driven systems has been assessed. The total core power and production of radionuclides contributing to radiation source terms were focused on. The article features a method based on the Monte Carlo sampling of random nuclear data files from the covariance matrices generated from the sets of reaction cross sections obtained with model calculations of high-energy particle interactions with matter or picked up from already existing nuclear data libraries. It has been demonstrated that nuclear data uncertainties do not need to be propagated through particle transport calculations to obtain uncertainties on the responses. This advantage allowed to investigate the convergence of the sample average to the best estimate. The number of random nuclear data file sets needed to obtain reliable uncertainty on the total core power is around 300 that results in the uncertainty of 14%. The uncertainties on the concentrations of nuclides most important for the safety assessment that are accumulated in lead-bismuth eutectic during irradiation, range from 5 to 60%. Concentrations of some nuclides exemplified by Tritium converge much slower than neutron multiplicities so that several thousands of samples are needed to ensure reliable uncertainty estimates.
Iwamoto, Hiroki; Stankovskiy, A.*; Fiorito, L.*; Van den Eynde, G.*
Journal of Nuclear Science and Technology, 55(5), p.539 - 547, 2018/05
Times Cited Count：9 Percentile：67.52(Nuclear Science & Technology)The applicability of Monte Carlo techniques, namely the Monte Carlo sensitivity method and the random-sampling method, for uncertainty quantification of the effective delayed neutron fraction is investigated using the continuous-energy Monte Carlo transport code, MCNP, from the perspective of statistical convergence issues. This study focuses on the nuclear data as one of the major sources of uncertainty. For validation of the calculated , a critical configuration of the VENUS-F zero-power reactor was used. It is demonstrated that Chiba's modified -ratio method is superior to Bretscher's prompt -ratio method in terms of reducing the statistical uncertainty in calculating not only but also its sensitivities and the uncertainty due to nuclear data. From this result and a comparison of uncertainties obtained by the Monte Carlo sensitivity method and the random-sampling method, it is shown that the Monte Carlo sensitivity method using Chiba's modified -ratio method is the most practical for uncertainty quantification of . Finally, total uncertainty due to nuclear data for the VENUS-F critical configuration is determined to be approximately 2.7% with JENDL-4.0u, which is dominated by the delayed neutron yield of U.
Iwamoto, Hiroki; Stankovskiy, A.*; Uyttenhove, W.*
Energy Procedia, 71, p.33 - 41, 2015/05
Times Cited Count：1 Percentile：69.64(Energy & Fuels)Sugawara, Takanori; Sarotto, M.*; Stankovskiy, A.*; Van den Eynde, G.*
Annals of Nuclear Energy, 38(5), p.1098 - 1108, 2011/03
Times Cited Count：12 Percentile：66.82(Nuclear Science & Technology)The XT-ADS, an accelerator-driven system for an experimental demonstration, has been investigated in the framework of IP EUROTRANS FP6 project. In this study, the sensitivity and uncertainty analyses were performed to comprehend the reliability of the XT-ADS neutronic design. For the sensitivity analysis, it was found that the sensitivity coefficients were significantly different by changing the geometry models and calculation codes. For the uncertainty analysis, it was confirmed that the uncertainties deduced from the covariance data varied significantly by changing them. The uncertainties deduced from the covariance data for the XT-ADS criticality were 0.94%, 1.9% and 1.1% by the SCALE 44-group, TENDL-2009 and JENDL-3.3 data, respectively. When the target accuracy of 0.3%dk for the criticality was considered, the uncertainties did not satisfy it. To achieve this accuracy, the uncertainties should be improved by experiments under an adequate condition.
Sugawara, Takanori; Stankovskiy, A.*; Sarotto, M.*; Van den Eynde, G.*
NEA/NSC/DOC(2011)4, p.27 - 35, 2011/00
A flexible fast spectrum research reactor MYRRHA able to operate in subcritical (driven by a proton accelerator) and critical modes is being developed in SCK
CEN. In the framework of IP EUROTRANS programme the XT-ADS model has been investigated for MYRRHA. In this study, the sensitivity and uncertainty analysis was performed to comprehend the reliability of the XT-ADS neutronics design. The calculated sensitivity coefficients for neutronics parameters varied significantly between calculation models. The uncertainties deduced from the covariance data strongly depend on the original covariance data. The calculated nuclear data uncertainties could not meet the target accuracy. To improve uncertainties, the integral experiments in adequate conditions are expedient.
